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1.
The important feature of the alkali-metal-doped C60 is that the intramolecular high, frequency vibration modes arising from the covalent interaction and the intermolecular lowfrequency vibration modes arising from the weak Van der Wads interaction both play important roles in the properties of superconductivity. We propose a two-peak form for the phonon density of states. By solving the Eliashberg equations we get the formula for the reduced gap 2Δ0/kBTc and the transition temperature Tc whidh are all in accordance with the experimental values.  相似文献   

2.
This paper gives methods to calculate the pairing temperature T*,at which a pseudogap is opened,and the superconducting temperature Tc,at which superconductivity appears,in the high-Tc cuprates,and demonstrates directly that at Tc < T < T* the pseudogap is the gap of Cooper pair without long-range phase coherence,and at T < Tc there is long-range phase coherence between Cooper pairs.Based on the above clear physical picture on the pseudogap state and our mechanism for the ac Josephson effect,this paper proposes that there should be a novel oscillatory current in P-I-P junction,induced by a constant bias on the junction.Here,P represents the high-Tc curates in the pseudogap state,where Cooper pairs do not have long-range phase coherence,and I represents the thin insulating barrier.This paper conjectures that there is a possible high-temperature superconductivity in the heavily underdoped high-Tc cuprates.  相似文献   

3.
For both BiSrCaCuO and TlBaCaCuO samples, internal frictions (Q-1) in the kHz range reveal a plateau (Q-1p) above Tc and a rapid drop below Tc with the turning points located just at Tc for various samples with different Tc. This anomaly cannot be observed in non-superconducting samples. The ultrasonic attenuation (α) in TlBaCaCuO displays similar results to the internal friction. Moreover, it is discovered that the Q-1p is nearly proportional to the carrier density for Y(Pr)BaCuO and Gd(Pr)BaCuO with different Pr contents. These results show that the drop of Q-1 and a below Tc is closely related to superconducting condensation. The Q-1p and αp can be explained using coupling-model of carriers with local dynamic distortion because high Tc superconductors are strong-correlation systems. Furthermore, by taking account of the smearing of superconducting gap structure resulting from the recombination of quasi-particles and by modifying the BCS relative jump rate as S(E, E', Γ) = Re{1-Δ2/[(E-iΓ)(E'-iΓ)]}, the calculated results of internal friction and ultrasonic attenuation below Tc are in good agreement with the experimental data. The superconducting gap Δ and the damping rate Γ for both BiSrCaCuO and TlBaCaCuO have also been obtained, they are in accordance with those got by tunneling spectrum and NMR methods, etc.  相似文献   

4.
In the framework of the weak coupling theory of superconductivity, we have proved that spin and charge fluctuations in the high-Tc superconductors can pro-duce respectively, pair-breaking and pair-forming effects on the superconductivity resulting from the "generalized BCS mechanism". With the coupling constant for spin fluctuations larger than that for charge fluctuations, they combine to produce a temperature-dependent effective pair-breaking effect, which makes Tc decrease more rapidly than Δ(0), the superconducting gap at T=0, and therefore, enhances the ratio 2Δ(0)/Tc. This provides a reasonable physical interpretation for the relevant experimental results.  相似文献   

5.
董晓莉  金魁  袁洁  周放  张广铭  赵忠贤 《物理学报》2018,67(20):207410-207410
FeSe基超导体的超导临界温度可大范围调控,物理现象丰富,是非常规超导机理研究的热点.由于较高的超导临界参数及易于加工等特点,FeSe基超导体在超导应用开发方面也日益受到重视.大尺寸高质量的单晶和薄膜形态的FeSe基超导材料,对于相关基础科学研究和应用开发都极为重要.作者近年来先后开发和发明了水热离子交换(ion-exchange)、离子脱插(ion-deintercalation)、基底辅助水热外延生长方法,成功解决了二元FeSe和插层(Li,Fe)OHFeSe超导体高质量单晶和薄膜的生长和物性调控难题.进而在相关物理问题的研究中取得新进展,包括发现二元FeSe中自旋向列序与超导电性密切相关,观测到(Li,Fe)OHFeSe中的电子相分离现象.此外,(Li,Fe)OHFeSe超导薄膜呈现很高的超导临界电流密度和上临界磁场,其应用前景值得关注.  相似文献   

6.
In this paper, the preparation process of the tetragonal LaBaCaCu3O7-x (LBCCO) superconductor with Tc=84 K is repored. The superconductivity and structure of the LBCCO superconducting phase are investigated by means of X-ray diffraction (XRD), transmission electron microscope(TEM) and superconductivity measurements, The results indicate that the superconducting phase with Tc=82K in the LBCCO system has a tetragonal structure with a=0.3966nm, c=l.1838nm and space group P4/mmm. About 50% of the Ca and La atoms are located in 1d sites (i.e. Y site in the YBCO structure). It is confirmed that there is in fact no orthorhombic to tetragonal transition in this material. The relationship between the oxygen content and Tc is also presented.  相似文献   

7.
熊光成  尹道乐 《物理学报》1982,31(9):1176-1182
本文研究了C-15结构化合物(Zr0.5Hf0.5-xTax)V2(x≤0.2)和(Hf0.5Zr0.5-xNbx)V2(x≤0.2)的超导转变温度Tc及其压力效应?Tc/?P。报道了实验方法与结果。与(Hf1-xTax)V2和(Zr1-xTax)V2的情况不同,在(Zr0.5Hf0.5-xTax)V2中Ta的引入使常压下的Tc下降,然而(?)Tc/(?)P却大为提高。因此高压下Zr0.5Hf0.45Ta0.05V2的Tc反而比Hf0.5Zr0.5V2更高。导出了一个基于角动量分波表象能带论方法的描述压力效应的新关系式。它指出导带电子波函数中的高角动量成分变化对Tc的压力效应影响比较重要。这个公式有助于理解上述复杂的实验现象,并能合理地解释某些元素(如Cs,Ba,La等)的Tc随压力剧增的事实。 关键词:  相似文献   

8.
丁发柱  古宏伟  张腾  王洪艳  屈飞  彭星煜  周微微 《物理学报》2013,62(13):137401-137401
本文通过在前驱液中添加过量钇盐和铈的有机盐,采用三氟乙酸盐-金属有机沉积法(TFA-MOD) 在铝酸镧单晶基体上制备了含有纳米氧化钇和纳米铈酸钡的YBCO薄膜. 与纯YBCO薄膜相比,掺杂Y2O3/BaCeO3的YBCO膜的临界转变温度几乎保持不变,为91 K左右. 而掺杂Y2O3/BaCeO3的YBCO膜的临界电流密度达到5.0 MA/cm2 (77 K, 0T), 是纯YBCO膜临界电流密度的1.5倍.薄膜中的Y2O3和BaCeO3可能在YBCO内部起到了 有效的钉扎磁通作用. 关键词: 钇钡铜氧薄膜 2O3和纳米BaCeO3')" href="#">纳米Y2O3和纳米BaCeO3 磁通钉扎 三氟乙酸盐-金属有机沉积  相似文献   

9.
杨桦  冯中沛  林泽丰  胡卫  秦明阳  朱北沂  袁洁  金魁 《物理学报》2018,67(20):207416-207416
在铁基超导体中,FeSe具有最简单的晶体结构和化学组成,而且其超导转变温度具有较大的调控空间,因此适合作为超导机理研究和应用的载体.高质量样品的研制是物性研究和器件应用的前提,本文系统地研究了利用激光脉冲沉积技术制备FeSe薄膜的工艺条件,在多种衬底上成功地制备出高质量的β-FeSe薄膜,并首次实现了超导临界转变温度从小于2 K到14 K的连续调控,这为FeSe超导机理研究提供了样品支持.为探究FeSe薄膜超导电性变化的起因,从β-FeSe超导电性与晶格常数c正相关出发,基于简单的费米面填充假设,第一性原理计算可以很好地解释晶格常数c的变化规律,但该假设并不能完全符合角分辨光电子能谱实验给出的电子结构演变过程.因此β-FeSe薄膜的超导电性、晶格结构和电子结构三者之间的关系还有待澄清,该问题的解决将为FeSe超导机理研究提供重要的线索,而上述系列高质量的β-FeSe薄膜样品恰好能为该问题的研究提供理想的载体.本文根据实验和已有的相关研究结果,详细介绍了FeSe薄膜的脉冲激光沉积制备及其优化,以期为后续的薄膜研究应用提供参考.  相似文献   

10.
The gap equation at finite temperature in the top-quark condensate scheme of electroweak symmetry breaking is proven to have the identical form in both the imaginary and real time formalisms of thermal field theory. By means of the gap equation, combined with the basic relation to define the vacuum expectation value v of the effective Higgs field, we analyze the dependence on temperature T and chemical potential p of the dynamical top-quark mass as the order parameter characteristic of symmetry breaking, and obtain the p-T criticality curve for symmetry restoration. We find out that the critical temperature Tc = 2υ for μ = 0 and the critical chemical potential μc = 2 π υ / √3 for T = 0. When μ = 0, the top-quark mass near Tc has the leading (Tc2 - T2)1/2 behavior with an extra factor dependent on temperature T and the momentum cutoff Λ. However, it is generally argued that the symmetry restoration at T ≥ Tc is still a second-order phase transition.  相似文献   

11.
We describe the molecular ferromagnet decamethylchromocenium tetracyanoethanide [CrCp2*] [TCNE] by a quasi-one-dimensional alternating-spin model with ferromagnetic exchange interaction. The spin-wave theory is used to discuss the magnetic excitation of the molecular ferromagnet. We obtain the magnetizations corresponding to different external magnetic fields without interchain exchange interaction which is consistent with the experimental results. The formula of the Curie temperature Tc is obtained by using the thermodynamic Green's function method. It is found to be related to the spin of donors, to the intrachain exchange interaction and to the spatial anisotropic parameter. The result obtained by this Tc formula is consistent with the experimental result Tc = 3.6 K for [CrCp2*][TCNE].  相似文献   

12.
董晓莉  袁洁  黄裕龙  冯中沛  倪顺利  田金朋  周放  金魁  赵忠贤 《物理学报》2018,67(12):127403-127403
单晶薄膜形态的高温超导材料对于相关基础科学研究和应用开发都极为重要.多带的铁基高温超导体往往呈现丰富的物理现象,并具有较高的超导临界参数.特别是近年发现的插层(Li,Fe)OHFeSe超导体,无论对高温超导机理还是应用研究而言,都日益受到重视,已成为铁基家族中重要的典型材料.但是,该化合物含有OH键,加热易分解.因此,现有的常规高温成膜技术均不适用于生长该薄膜材料.为解决这一生长难题,我们最近发明了基体辅助水热外延生长法,实现了超导薄膜制备技术上的突破.本文简要介绍用此软化学成膜技术首次成功制备出(Li,Fe)OHFeSe单晶薄膜.该薄膜材料具有优良的结晶质量和较高的超导临界参数,特别是其高的临界电流密度和上临界场对应用开发有实际价值.因此,(Li,Fe)OHFeSe超导单晶薄膜的成功合成,为机理研究和应用开发分别提供了重要的实验载体和备选材料.另外,该薄膜技术也有望应用于其他功能材料的探索与合成,尤其是对常规手段难以获取的材料更具重大价值.  相似文献   

13.
The two-dimensional plasmonic mechanism of superconductivity has been studied by solving the momentum-and frequency-dependent Tc eigenvalue equation containing vertex and self-energy corrections. Our result shows the failure of appearing superconductivity in one-component electron system. The Coulomb interaction including plasmon effects in the electron gas is estimated to yield net repulsive values of μ between 0.24 and 0.6 for rs between 1 and 10.  相似文献   

14.
Based on the mechanism of charge fluctuation, the effective Hamiltonian is, derived to discuss the superconductivity for the non-cuprate compound BaPb1-xBixO3. The desired Tc versus δ curve is obtained. It is shown that the explanation of superconductivity for non-cuprate superconductors is the same as that of cuprate ones. Furthermore, that the non-cuprate superconductors have no ferromagnetism and anti-ferromagnetism can be explained, and the superconductivity windaw is due to the Cooper pairirtg in coordinate space.  相似文献   

15.
《中国物理 B》2021,30(7):76301-076301
Based on density functional first-principles calculations and anisotropic Eliashberg equations, we have investigated the electronic structure, lattice dynamics, and phonon-mediated superconductivity in newly synthesized layered compound Sr BC under pressure. Different from Li BC and Mg B2, our calculations surprisingly reveal that Sr BC is isotropic in compressibility, due to the accumulation of substantial electrons in the interstitial region. We find that the Sr phonons strongly couple with B-2 pz orbital and the interstitial states, giving rise to a two-gap superconductivity in Sr BC, whose transition temperature shows an inverted V-shaped dependence on pressure. The maximal transition temperature is about 22 K at50 GPa. On both sides of 50 GPa, the transition temperature exhibits quasi-linear variation with positive and negative slopes, respectively. Such a variation of transition temperature is infrequent among phonon-mediated superconductors. The competition between enhanced electron–phonon matrix element and hardened phonons plays an essential role in governing the behavior of the critical temperature.  相似文献   

16.
Superconducting transition temperature Tc and normal-state electrical resistivities ρ of the Tm1-xPrxBa2Cu3O7-δ system have been measured. The results indicate that Tc remains constant for x = 0 to 0.08 before it drops steadily with higher x. Following the Abrikosov-Gor'kov model, a total suppression of superconductivity occurs at a critical Pr concentration xcr≈0.56. It is found for the first time, as far as we know, that the logarithmic resistivity at 270 K increases linearly with increasing x, yielding ρ= ρ0eax. Judging from the relation between dρ/dT and x, a metal to insulator transition occurs just beyond xcr.  相似文献   

17.
刘敏霞  何林  张耿  叶海  黄晓园  徐永钊 《物理学报》2016,65(3):37401-037401
非中心对称超导体LaNiC_2是传统BCS超导体还是能隙存在节点又或是两带超导体,目前仍然存在争议.基于此,文章用两带Ginzburg-Landau理论分析了超导体LaNiC_2的上临界磁场随温度的变化关系,计算结果与实验结果在整个温度区间内符合得很好,说明LaNiC_2是两带超导体,和陈健等人的观点一致.文章还分析了两个不同能带对上临界磁场的影响,发现相对较小的相干长度对LaNiC_2的上临界磁场影响较大.  相似文献   

18.
Using microscopic theory of superconductivity, we find a universal relationship between Tc and hole content in p-type cuprate superconductors, which is consistent with the empirical ones given by Zhang and Sato. This paper predicts that there is also a universal relationship between energy gap and hole content.  相似文献   

19.
通过对FeSe进行化学插层可以将其超导转变温度(Tc)从约8 K提高到40 K以上,实现高温超导电性.最近,我们对两种插层FeSe高温超导材料(Li0.84Fe0.16)OHFe0.98Se和Li0.36(NH3yFe2Se2开展了高压调控研究,发现压力会首先抑制高温超导相(称为SC-I相),然后在临界压力Pc以上诱导出第二个高温超导相(称为SC-Ⅱ相),呈现出双拱形T-P超导相图.这两个体系的Pc分别约为5和2 GPa,两个体系SC-Ⅱ相的最高Tc分别可以达到约52和55 K,比相应SC-I相的初始Tc提高了10 K.对(Li0.84Fe0.16)OHFe0.98Se的正常态电输运性质分析表明,SC-I和SC-Ⅱ相的正常态分别具有费米液体和非费米液体行为,意味着这两个超导相可能存在显著差异.此外,还发现这两个体系的SC-Ⅱ相的Tc与霍尔系数倒数1/RH(∝载流子浓度ne)具有很好的线性依赖关系.对(Li0.84Fe0.16)OHFe0.98Se的高压X射线衍射测量排除了其在10 GPa以内发生结构相变的可能,因此Pc以上SC-Ⅱ相的出现和载流子浓度的增加很可能起源于压力导致的费米面重构.  相似文献   

20.
The determination of Tc in dilute alloys is examined. As an example, magnetization vs field data in a Pd0.95Gd0.05 alloy are presented. For this alloy, it was not possible to determine a value of Tc using Arrott-Belov-Kouvel (ABK) plots; the conditions for the applicability of ABK plots were not satisfied. Results of very-low-field ac and dc magnetization vs T, which depend mainly on the demagnetization factor, yield a more precise measure of Tc. We conclude that the latter procedures are more useful than ABK plots for determination of Tc in dilute alloys.  相似文献   

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