Interactions of slow neutrons with the chromium isotopes

Neutron transmission experiments and determinations of coherent scattering lengths were performed on natural chromium and enriched samples of⁵⁰Cr,⁵²Cr,⁵³Cr and⁵⁴Cr. By means of the Christiansen-filter-technique we obtained new values for the scattering lengths of the bound atoms:b(^natCr)=3.635±0.007 fm,b(⁵⁰Cr)=?4.50±0.05 fm,b(⁵²Cr)=4.914±0.015 fm,b(53Cr)=?4.20±0.03 fm, andb(⁵⁴Cr)=4.55±0.10 fm. The transmission experiments with neutrons of 510 ΜeV, 1.26 eV and 5.19 eV energy resulted in data for the absorption cross sectionσ _a (^natCr) =3.05±0.08 b and for the scattering cross section at “zero energy”:σ ₀ (^natCr)=3.381±0.010 b. Data for incoherent and spin-state scattering and for the potential-scattering radius of the nuclei could be deduced from these results.     

Interaction of neutrons with zinc and its isotopes

Coherent neutron scattering lengths and total cross sections have been measured for elemental Zn,Zn-compounds and on isotopicly enriched samples for neutron energies from 0.5 meV up to 143 keV using different techniques. From the experimental data the following quantities were obtained:

the coherent scattering lengths (b in fm) of Zn (5.689±0.014);⁶⁴Zn (5.23±0.04);⁶⁶Zn (5.98±0.05);⁶⁷Zn (7.58±0.08;b ₊=9.4±0.5/5.8±0.5;b _?=5.0±0.7/10.1±0.7);⁶⁸Zn (6.04 ±0.03);

the potential scattering radii (R′ in fm) of Zn (6.2±0.2),⁶⁴Zn (6.0±0.3) and⁶⁶Zn (6.2 ±0.3);

the absorption cross sections (σ _γ at 0.025 eV in barn) of Zn (1.11±0.02);⁶⁴Zn (1.1 ±0.1) and⁶⁶Zn (0.62±0.06).

Derived quantities are the “zero energy” scattering cross sections (σ ₀ in barn) for Zn (4.128±0.010) and⁶⁷Zn (7.8±0.3) and the incoherent bound cross sections of Zn (0.061 ±0.023) and⁶⁷Zn (0.6±0.4). In the epithermal region the Zn-cross section can be described by introduction of two strong bound levels of⁶⁷Zn+n for which estimated parameters are given.     

Interaction of low-energy neutrons with Nd isotopes

Low-energy neutron data for even-even isotopes 1^142–150Nd are considered. It is shown that the diffuseness parameter noticeably changes in going from one isotope to another (from a = 0.55 fm for ¹⁴²Nd to a = 0.75 fm for ¹⁵⁰Nd), which agrees with the theoretical indications of a decrease in the skin thickness for nuclei with closed shells. The analysis points to the possible existence of the semimagic number Z = 58.     

Interaction of slow neutrons with natural terbium,holmium and erbium and its isotopes

Coherent neutron scattering lengths and total cross sections have been measured on samples of ordinary Tb, Ho and Er and on isotopically enriched Er-compounds. From the experiment the following data were obtained:

• - the coherent scattering lengths (in fm) of the bound atoms ¹⁵⁹Tb(7.34 ± 0.02), ¹⁶⁵Ho(8.44 ± 0.03), ^ordEr(7.79 ± 0.02), ¹⁶²Er(9.01 ± 0.11), ¹⁶⁴Er(7.95 ± 0.14), ¹⁶⁶Er(10.51 ± 0.19), ¹⁶⁷Er(3.06 ± 0.05), ¹⁶⁸Er(7.43 ± 0.08), and ¹⁷⁰Er(9.61 ± 0.06)
• - the thermal absorption cross sections (in b) ¹⁴¹Pr(12.7 ± 0.6), ^ordNd(58 ± 1), ¹⁵⁹Tb(30 ± 2), ¹⁶⁵Ho (65 ± 2), ^ordEr (145 ± 2), ¹⁶⁶Er (18 ± 2), ¹⁶⁷Er(568 ± 9), ¹⁶⁸Er(2.3 ± 0.3), and ¹⁷⁰Er(15 ± 1). In combination with the resonance parameters, the measured coherent scattering lengths allowed the determination of potential scattering radii R′ which are of particular interest for the optical model theory.

     

Interactions of fast neutrons with45Sc

The surface resistance of lead was measured in a coaxial cavity at frequencies between 375 and 5000 MHz and temperatures between 4.2 and 1.5 °K. The residual resistance was determined from these data.     

Interaction of slow neutrons with the isotopes of molybdenum

Coherent neutron scattering lengths and total cross sections were measured on samples of ordinary Mo and isotopically enriched samples. From the experiments with neutrons of 0.57 meV and 1.26 eV the following values have been obtained:

1. the coherent scattering lengths (in fm) of the bound atoms of Mo (6.715±0.020) and for the isotopes with the mass numbers 92 (6.93±0.08), 94 (6.82±0.07), 95 (6.93±0.06), 96 (6.22±0.06), 97 (7.26±0.08), 98 (6.60±0.07) and 100 (6.75±0.07);
2. the incoherent scattering cross section at zero-energy for ordinary Mo: σ_i=0.02 ± 0.02 barn;
3. the absorption cross sections (in barn) for Mo (2.48 ± 0.04) and for the isotopes with the mass numbers 95(13.4 ± 0.3), 97(2.5 ± 0.2) and 100(0.4 ± 0.2). The relation of the present results to the resonance parameters of the neutron — Mo interaction has been discussed.

     

Scattering of slow neutrons by arsenic and selenium isotopes

Coherent neutron scattering lengths and free cross sections were measured for arsenic, for ordinary selenium and its isolated isotopes. By means of the Cristiansen filter technique the following scattering lengths for the bound atoms were obtained (in fm):b(As) =6.58(1) [b ₊=6.04(5) andb _?=7.47(8)],b(Se)=7.970(9),b(⁷⁶Se)=12.2(1),b(⁷⁷Se) =08.25(8),b(⁷⁸Se)=8.24(9),b(⁸⁰Se)=7.48(3) andb(⁸²Se)=6.34(8). Transmission measurements with neutrons of 1.26 eV and 5.19 eV resulted in an energy independent free scattering cross section for arsenic ofσ _{s, t}=5.40(3)b (in the eV-region). For ordinary selenium energy dependent free cross sections ofσ _{s, t}(1.26 eV)=7.9(1)b andσ _{s, t} (5.19 eV)=7.55(3)b were found. The results were compared with the resonance parameters of the nuclei and with different sets of potential scattering radii. Thus it could be concluded that there is no evidence for a bound state of the neutron-nucleus compound⁷⁵As+n but a clear evidence for strong bound levels of⁷⁶Se+n and⁷⁷Se+n.     

Interactions of slow neutrons with nuclides of antimony,tellurium and iodine

Coherent neutron scattering lengths and total cross sections have been measured on samples of ordinary Sb, Te, I and on isotopically enriched compounds. From the experimental data for neutron energies of 0.57 meV, 1.26 eV and 5.2 eV the following data were obtained: the coherent scattering lengths (in fm) of the bound atoms Sb (5.57±0.03);¹²¹Sb(5.71±0.06),¹²³Sb(5.38±0.07); Te(5.80±0.03) and for its isotopes of the mass number 122(3.8±0.2); 123(?0.05±0.25?i·0.100); 124(7.95±0.10); 125(5.01±0.08); 126(5.55±0.07); 128 (5.88±0.07); 130(6.01±0.07). the thermal absorption cross sections (in barn) for Sb(4.91±0.05);¹²¹Sb(5.77±0.12);¹²³Sb(3.8±0.2); Te(4.05±0.05) and I(6.15±0.06). The combination of the measured values of scattering lengths and -cross sections resulted in data for coherent and incoherent cross sections. Taking account of resonance data a complete set of spin state- and reconance scattering lengths has been obtained and discussed.     

Hyperfine anomaly measurements in francium isotopes and the radial distribution of neutrons

We have performed precision measurements in a magneto-optical trap of the 7P_1/2 hyperfine structure of the isotopes ^209-210Fr. The ratio of these hyperfine constants to the previously measured 7S_1/2 ground state values reveals a significant hyperfine anomaly. This anomaly results from the different radial dependence of the electron density in the two atomic levels. The measurements are sensitive to changes in the radial distribution of the neutron magnetism. This revised version was published online in August 2006 with corrections to the Cover Date.     

Scattering and resonance properties of the interaction of slow neutrons with the isotopes of silicon and sulfur

In¹¹⁷Te,¹¹⁹Te and¹²¹Te isomeric states withJ ^π=5/2⁺, 5/2⁺ and 7/2⁺ and half-lives of 19.1(9)ns, 2.2(2) ns and 86(6) ns, respectively, have been identified at low excitation energies using (α, 2n) reactions on enriched^115–119Sn targets. Positive parityΔJ=1 bands built on these isomeric states have been observed up to 17/2⁺. The states are interpreted as members of rotational bands built on deformation driving 5/2⁺ [402] and 7/2⁺ [404] Nilsson orbitals which overcome theN=64 subshell gap. The irregular level spacings and electromagnetic properties of the bands are well explained in Coriolis calculations. The moment of inertia parameter as function of collective angular momentum has been derived from the doubly even Te cores. The hindrance of the band head deexcitation may be caused by shape fluctuations of these transitional nuclei.     

Shell structure of even-even nickel isotopes containing twenty to forty neutrons

Shell parameters of even-even nickel isotopes involving twenty to forty neutrons are analyzed, and the results of this analysis are presented. A detailed comparison of the results obtained by calculating, on the basis of the mean-field model with the Koura-Yamada potential and the dispersive optical potential, single-particle energies of proton and neutron subshells with experimental data on the isotopes ^{56,58,60,62,64,68}Ni and with evaluated data on the neutron-deficient isotopes ^48,50,52,54Ni is performed.     

Interactions of neutrons with239Pu in the energy range between 1.5 and 5.5 MeV

Neutron scattering angular distributions of²³⁹Pu were measured at seven primary neutron energies between 1.5 and 5.5 MeV. Absolute differential scattering cross-section results are plotted and tabulated. Cross section calculations using a central optical model were made and the results were compared with the experimental values. Moreover, nuclear temperatures of the fission and the inelastic neutron evaporation processes were extracted from the measured spectra.     

Interactions between hydrogen isotopes and carbon monoxide on rhenium

The rate of absorption by a clean rhenium filament of carbon monoxide and deuterium from a mixture of the two gases was little different in the early stages from that of the two gases individually. However, continued exposure of the deuterium-covered filament to carbon monoxide led to ready replacement, the sticking probability of carbon monoxide being about 80% of its value on a clean filament. A similar experiment with a hydrogen deuteride-covered filament led to a gas phase hydrogen isotope composition consistent with dissociative adsorption of hydrogen deuteride.     

Interaction of slow neutrons with natural Rutenium,Rhodium, Cadmium and Thallium and some of their isotopes

By means of Christiansen filter technique the following bound coherent neutron scattering lengths were obtained:^natRu:b=7.02 ± 0.02 fm¹⁰⁸Cd:b=5.31 ± 0.24 fm¹⁰³Rh:b=5.90 ± 0.04 fm¹¹⁰Cd:b=5.78 ± 0.08 fm^natTl:b=8.773 ± 0.015 fm¹¹¹Cd:b=6.47 ± 0.08 fm²⁰³Tl:b=8.51 ± 0.08 fm¹¹²Cd:b=6.34 ± 0.06 fm²⁰⁵Tl:b=8.87 ± 0.07 fm¹¹⁴Cd:b=7.48 ± 0.05 fm¹¹⁶Cd:b=6.26 ± 0.09 fm In combination with some total cross section measurements with neutrons in the eV-energy range and with the compiled resonance parameters we deduced consistent sets of spin state scattering lengths and potential radii.     

Variation of electron concentration in gallium arsenide due to irradiation by fast neutrons

The effects of irradiation by fast neutrons on gallium arsenide crystals with different degrees of initial perfection is investigated. It is shown that for relatively perfect, specially non-doped n-type crystals the degree of damage K is weakly dependent on the integrated radiative flux up to some critical flux determined by the initial current carrier concentration. The decrease in the rate of carrier removal in crystals with an elevated concentration of residual defects is due to the participation of the latter in the kinetics of defect formation. The initial rates of carrier removal are obtained in crystals grown by different methods.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 1, pp. 47–51, January, 1973.     

Production of neutron-rich isotopes in fission of uranium induced by neutrons of 20 MeV average energy

In the context of a parameter study conducted by several laboratories for future European radioactive beam facilities based on fast-neutron induced fission, in particular for the SPIRAL-II project at GANIL, we have measured the yields of neutron-rich isotopes in the mass range of 88 to 144. These nuclei were obtained as fission products of natural uranium bombarded by neutrons of 20 MeV average energy emitted by a thick carbon target irradiated by 50 MeV deuterons. Yields have been measured using on-line mass separation with the ion-guide method. Compared with proton-induced fission at 25 MeV the magnitude of cross-sections, except for the symmetric region, is similar. Z-distributions of isobars have the same width, 0.7 charge units, but their maxima are shifted by about 0.8 charge units, favouring production of the neutron-richer isobars. Our data allow calculations of absolute cross-sections for fission of natural uranium induced by neutrons of about 20 MeV. Received: 10 July 2000 / Accepted: 27 October 2000