共查询到19条相似文献,搜索用时 973 毫秒
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在多电子态模型下,利用二阶劈裂传播子算法计算了H2^+在强激光场中的离散行为。结果发现在高频场时分子的多光子离散碎片是近对称的,而对于低频场,在所考虑的激光强度下H2^+是被隧道离散的,因而其离散碎片H^+分布是反对称的,另外,文中还探讨了三脉冲形状对分子离解几率、离解碎片动力学行为的影响。 相似文献
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超短脉冲强激光与团簇的相互作用已被证明能够产生能量高达MeV量级的高能离子和中子以及非常强的X射线辐射。广阔好原子团簇在超短脉冲强激光场的作用下的加热、电离和膨胀等机制,对这种相互作用的深入研究可能会对激光核聚变和X射线激光等应用领域产生重大影响。 相似文献
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采用三维粒子动力学模拟方法研究了甲烷团簇在超短强激光脉冲激励下的爆炸动力学行为,重点讨论了几种典型的内电离机理对团簇爆炸过程中离子的价态和动能的影响.研究表明,在激光脉冲强度比较小的情况下,团簇中的原子主要是在光场作用下通过隧道电离的方式发生电离.当激光场进一步增强时,势垒压低电离是电离的主要方式.在相同的较高激光强度下,团簇更容易通过势垒压低电离达到高的电离价态.团簇发生电离后,其内部库仑电场的点火电离效应和内部滞留自由电子的碰撞电离效应也将增强团簇的再次电离过程.
关键词:
超短强激光脉冲
甲烷团簇
内电离 相似文献
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Autler-Townes Splitting in Photoelectron Spectrum of Three-Level Li2 Molecule in Ultrashort Pulse Laser Fields
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The Autler-Townes (AT) splitting in femtosecond photoelectron spectrum of three-level Li2 molecules is theoretically investigated using time-dependent quantum wave packet method. With proper femtosecond laser pulses, three peaks of the AT splitting can be observed in the photoelectron spectrum. The AT splitting stems from rapid Rabi oscillation caused by intense ultrashort laser pluses. The effects of laser parameters on the molecular ionization dynamics are also discussed. 相似文献
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Numerical simulations of ionization and dissociation processes of hydrogen molecular ion H2+ interacting with two-color intense ( 1014W/cm2-1015W/cm2) ultrashort (the duration ≈ 22fs) laser pulse are made. The result shows that the ionization and dissociation processes are strongly dependent upon the relative phase between the two color fields. It means that, in the case of ultrashort pulse, the phase coherence control of ionization and dissociation processes can be realized. 相似文献
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S.?Borbély K.?T?kési L.?Nagy 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2010,59(3):337-348
The ionization of the water molecule by intense ultrashort half-cycle electric pulses is studied theoretically. The formation
of the electron wave packets in the continuum was investigated by calculating ionization probability densities using classical
and quantum mechanical models. Single active electron and frozen core calculations were performed within the hydrogenic approximation.
Electrons from the highest occupied molecular orbital 1b11b_1 were considered. We found good agreement between the classical and quantum mechanical calculation at high intensities, where
the over-the-barrier ionization mechanism is dominant. 相似文献
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We present quantum mechanical calculations of the electron and ion momentum distributions following double ionization of a one-dimensional helium atom by ultrashort laser pulses (780 nm) at various intensities. The two-electron momentum distributions exhibit a clear transition from nonsequential to sequential double ionization. We provide strong evidence that rescattering is responsible for nonsequential ionization by calculating the momentum spectrum of the He2+ recoil ions-which we find in excellent agreement with recent experiments-and by analyzing the electronic center-of-mass motion via Wigner transforms. 相似文献
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Double ionization of helium interacting with elliptically polarized laser pulse by classical ensemble simulations
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This paper uses the classical ensemble method to study the
double ionization of a 2-dimensional (2D) model helium atom
interacting with an elliptically polarized laser pulse. The classical
ensemble calculation demonstrates that the ratio of double to single
ionization decreases with the increasing ellipticity of the driving
field. The classical scenario shows that there are hardly any e--e
recollisions with the circularly polarized laser pulse. The double
ionization probability is studied for linearly and circularly
polarized laser pulses. The classical numerical results are
consistent with the semiclassical rescattering mechanism and in
agreement with the experimental results and the quantum calculations
qualitatively. 相似文献
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Control of electron localization in the dissociation of H2+ and its isotopes with a THz pulse
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The molecular dissociation with a two-laser-pulse scheme is theoretically investigated for the hydrogen molecular ion(H+2)and its isotopes(HD+and HT+).The terahertz pulse is used to steer the electron motion after it has been excited by an ultrashort ultraviolet laser pulse and an unprecedented electron localization ratio can be achieved.With the coupled equations,the mass effect of the nuclei on the effective time of the electron localization control is discussed. 相似文献
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Dynamic Interference Photoelectron Spectra in Double Ionization:Numerical Simulation of 1D Helium
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《中国物理快报》2016,(12)
We report our numerical simulation on the dynamic interference photoelectron spectra for a one-dimensional(1D) He model exposed to intense ultrashort extreme ultraviolet(XUV) laser pulses.The results demonstrate an unambiguous interference feature in the photoelectron spectra,and the interference is unveiled to originate from the dynamic Stark effect.The interference photoelectron spectra are prompted for intense sub-femtosecond XUV laser pulses in double ionization.The stationary phase picture is corroborated qualitatively in the two-electron system.The ability of probing the dynamic Stark effect by the photoelectron spectra in a pragmatic experiment of single-photon double ionization of He may shed light on further investigation on multi-electron atoms and molecules. 相似文献
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Analytical expressions and numerical results describing ionization of atoms by intense linearly polarized ultrashort laser pulses are obtained in the frame of the Keldysh approach. Photoelectron spectra and total ionization probabilities are presented for several analytical models of a single-cycle laser pulse. In particular, strong left-right asymmetry of the spectra is shown for the case of odd pulses. 相似文献
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Generation of XUV attosecond pulses in the process of atomic ionization by few-cycle laser radiation
Ionization of a model two-electron atom in the presence of a strong field of ultrashort laser pulses is investigated using the numerical integration of the nonstationary Schrödinger equation, which describes the dynamics of a quantum system in the presence of an electromagnetic wave. The features of two-electron ionization in the presence of one-and two-cycle pulses are analyzed. The suppression of double ionization in the presence of ultrashort laser pulses related to a finite-time interelectron energy exchange upon the laser action is demonstrated. The features of the generation of high-order harmonics and single XUV attosecond pulses are studied for the atomic ionization by few-cycle laser pulses. The parameters of the laser pulse are optimized for the effective generation of a single XUV attosecond pulse. 相似文献