强激光场中真空极化效应

 通过求解狄拉克方程,对强激光场下真空极化问题进行了研究。理论计算结果表明：在仅随时间变化的电场下,要激发狄拉克海中负能级的电子,需要两个阈值条件,即激光场的电场强度大于等于10¹⁶ V/cm和激光场的持续时间大于等于10^-21 s。前者主要保证负能态电子有足够的能量跃迁到正能态,后者主要是保证电子在跃迁过程中动量亏损得以补偿。     

强激光场中真空极化效应

通过求解狄拉克方程,对强激光场下真空极化问题进行了研究。理论计算结果表明：在仅随时间变化的电场下,要激发狄拉克海中负能级的电子,需要两个阈值条件,即激光场的电场强度大于等于1016 V/cm和激光场的持续时间大于等于10-21 s。前者主要保证负能态电子有足够的能量跃迁到正能态,后者主要是保证电子在跃迁过程中动量亏损得以补偿。     

Nonsequential double recombination in intense laser fields

A second plateau in the harmonic spectra of laser-driven two-electron atoms is observed both in the numerical solution of a low-dimensional model helium atom and using an extended strong field approximation. It is shown that the harmonics well beyond the usual cutoff are due to the simultaneous recombination of the two electrons, which were emitted during different, previous half-cycles. The new cutoff is explained in terms of classical trajectories. Classical predictions and the time-frequency analysis of the ab initio quantum results are in excellent agreement. The mechanism corresponds to the inverse single photon double ionization process in the presence of a (low frequency) laser field.     

Xenon clusters in intense VUV laser fields

A simple model is developed that quantitatively describes intense interactions of a vacuum ultraviolet (VUV) laser pulse with a xenon cluster. We find good agreement with a recent experiment [Nature (London) 420, 482 (2002)]]. In particular, the large number of VUV photons absorbed per atom, at intensities significantly below 10(16) W/cm(2), is now understood.     

Saturated ionization of fullerenes in intense laser fields

We investigate the ionization of icosahedral fullerenes (C20, C60, C80, and C180) in an intense laser pulse using the S-matrix theory. The results obtained are in excellent agreement with the recent observations of unexpectedly high saturation intensities of the Buckminster fullerene and its multiply charged ions. Our analysis strongly suggests that the related phenomenon of suppressed ionization of these complex fullerenes is due to the finite cage size and the "multislit" interference effect between partial waves emitted from the different nuclei rather than to a dynamical multielectron polarization effect.     

Dissociative ionization of molecules in intense laser fields

Accurate and efficient grid based techniques for the solution of the time-dependent Schrödinger equation for few-electron diatomic molecules irradiated by intense, ultrashort laser pulses are described. These are based on hybrid finite-difference, Lagrange mesh techniques. The methods are applied in three scenarios, namely H₂ ⁺ with fixed internuclear separation, H₂ ⁺ with vibrating nuclei and H₂ with fixed internuclear separation and illustrative results presented.Received: 19 November 2002, Published online: 24 April 2003PACS: 02.60.Cb Numerical simulation; solution of equations - 02.70.Bf Finite-difference methods - 33.80.Rv Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states) - 33.80.-b Photon interactions with molecules     

Photoemission mechanisms of methane in intense laser fields

The visible and near-UV emission spectroscopy of methane(CH4) induced by a femtosecond intense laser field(800 nm, 40 fs, 1014W∕cm2) is studied. By measuring the decay profiles of the neutral fragment product CH(A2Δ→ X2Π), two reaction pathways, i.e., the electron-ion recombination through e-t CHt4 and the direct disintegration of CHt4 are found to be responsible for populating the electronic excited states of the neutral fragment product CH, which gives rise to the photoemissions. Our results provide complementary information on previous understanding of the strong-field-induced photoemission mechanism of CH4 through neutral dissociation of superexcited states.     

Stabilization of hydrogen atom in intense laser fields

The stabilization of real hydrogen atom rather than the model under the influence of high frequency superstrong laser pulse is investigated by numerical integration of time-dependent Schrödinger equation. The target wavefunctions are expanded in terms of a discrete L² basis. The evidence of stabilization as found by Su et al. for 1D model atom using the split operator technique has been confirmed for the hydrogen atom using L² technique.     

Energy-gap distortion in solids under intense laser fields

We discuss, within the framework of the nearly-free electron model, the influence of an intense laser field on the motion of an electron in the effective lattice potential. It is shown that, for moderately intense fields, the band gap decreases linearly with increasing laser intensity.     

Photoemission from solid surfaces in intense laser fields

We present a Floquet analysis of photoemission of electrons from a solid surface due to its interaction with a laser beam. The method we use is based on a three-dimensional quasifree electron model. The model takes account of the changes in the effective mass of the electron inside and outside the solid and in the reflected and refracted beams due to the presence of the surface. It is shown that the photoemission of electrons from the solid surface may take place not only with no absorption of photons but also along with the emission of extra photons.     

高频强激光场中H-电离特性理论研究

高频强激光场中高价负离子（比如H-,H2-,He-,He2-等等）的稳定存在虽然在理论上早已得到得到证明,但在实验上至今没有被直接验证。为了探索可行的实验验证方案,通过以高频强场中的负一价氢离子H-为例,采用相空间平均法,详细研究了其在外加激光场中的电离率及光电子角分布情况。研究发现 的电离率比氢原子高,并且不存在氢原子在较强激光场中的电离抑制现象。另外随着激光场强度的增大和激光频率的减小,电子角分布与H-在高频场直接卸载后电子角分布的差别也增大。这些结果为将来在实验上验证高频强场中高价负离子的存在性提供了很好的理论依据。     

Charging dynamics of metal clusters in intense laser fields

Clusters of heavy metal atoms in strong femtosecond laser-light fields undergo multi-ionization with the loss of hundreds of electrons. The cross section largely exceeds that of corresponding isolated atoms, which leads in the case of Pb_N to a complete ionization of the 4f shell with a light intensity of 1.2×10¹⁵ W/cm². Experimental investigations on Pb and Pt clusters with variable pulse widths and, for the first time, with the pump&probe technique give insight into the dynamics of the coupling of electromagnetic radiation into the clusters. Both approaches support the picture according to which, after an initial charging, the clusters expand due to Coulomb forces. This expansion is accompanied by a reduction of the electron density and at the same time by an increase of the optical sensitivity. Once the plasmon energy of the diluted nanoplasma approaches the photon energy, the charging efficiency increases significantly. The experimental observations are confirmed by random-phase approximation (RPA) calculations of the optical response, including molecular-dynamics simulations of the expanding systems. Received: 11 November 1999 / Published online: 13 July 2000     

Classical study of and collisions in intense laser fields

In this paper, ion-atom and ion-ion collisions in the presence of intense laser fields are qualitatively studied by Classical Trajectory Monte Carlo (CTMC) simulations. It is found that in contrast to the field-free collisions, the colliding ion and the target nucleus could absorb energy from the applied laser fields when the electrons escape from the collision system. This result is explained in terms of Coulomb explosion induced by the enhanced ionization at the so-called critical internuclear distance. Also, the corresponding energy gain cross-sections are evaluated. Received: 7 October 1998 / Received in final form: 28 January 1999     

Microscopic analysis of large-cluster explosion in intense laser fields

We present a three dimensional microscopic particle in cell code. The code models nanoplasmas in intense laser fields, taking account of all relevant microscopic interactions. Our simulation reveals the physical processes determining the laser induced explosion of large clusters with several 10,000 atoms.     

Optical properties of semiconductors under intense laser fields

Recent progress is reviewed in the investigation of optical responses from highly photo-excited semiconductor plasma. The theoretical interpretation of the spectroscopy data is outlined on the basis of the coupling of the usual scattering theory with Zubarev's non-equilibrium statistical operator method. Connection with appropriate extension to the non-equilibrium state of the thermodynamic double-time Green functions is also presented.     

Atomic and molecular ions in intense ultra-fast laser fields

The interaction of a 60 fs 790 nm laser pulse with beams of Ar⁺, C⁺, H₂ ⁺, HD⁺ and D₂ ⁺ are discussed. Intensities up to 10¹⁶ Wcm^-2 are employed. An experimental z-scanning technique is used to resolve the intensity dependent processes in the confocal volume.Received: 6 January 2003, Published online: 15 July 2003PACS: 32.80.Fb Photoionization of atoms and ions - 33.80.Rv Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states) - 42.50.Hz Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift     

超快强激光驱动的原子分子电离

强场电离是超快强激光与物质相互作用时发生的基本物理过程。强场驱动原子分子的电离电子动力学过程发生在一个光学振荡周期以内,是在阿秒时间尺度上研究电子超快动力学的典范。不仅如此,强场驱动下的超短电子束还为探测原子分子的结构及其超快动力学提供了重要的技术手段。文章首先简要阐述了超快强光场中原子分子电离的基本物理图像,在此基础上,介绍了近年来基于强场电离电子开展的超快过程研究的几个例子,最后简要讨论了强场电离研究的未来可能发展方向。     

Energy distribution of photoelectrons generated from highly charged ions in a circularly polarized intense laser field

We observed the energy distribution of the photoelectrons generated from the highly charged ions in the tunneling regime by using a circularly polarized Ti:Sapphire laser (745 nm, 100 fs). The peaks for each successive charge state up to Ar³⁺, Kr⁴⁺, and Xe⁵⁺ were clearly resolved, and the peaks due to higher charge states were flattened in the high-energy region and deviated from those predicted by the quasistatic model. This deviation is explained by pondero-motive acceleration in the strong field gradient. In Xe, Xe⁸⁺ was generated at a peak intensity of 2.0 × 10¹⁶ W/cm².