On the valency of uranium in aegirine and on behavior of isotopes<Superscript>234</Superscript>U and<Superscript>238</Superscript>U at dissolving the mineral

An attempt has been undertaken to find a correlation between the valency forms of uranium and the isotopic ratio (AR=²³⁴U/²³⁸U) following the incongruent dissolving of the mineral aegirine. The low values of AR (≈0.7) observed for hematite are assumed to be connected with the existence of considerable fraction of U(V) form in the original mineral. The discussion is given on the origin of the values of AR≈1 and on its connection with different stabilities of U(IV) and U(VI).     

Preliminary results of calculations for heavy-water nuclear-power-plant reactors employing <Superscript>235</Superscript>U, <Superscript>233</Superscript>U,and <Superscript>232</Superscript>Th as a fuel and meeting requirements of a nonproliferation of nuclear weapons

A physical design is developed for a gas-cooled heavy-water nuclear reactor intended for a project of a nuclear power plant. As a fuel, the reactor would employ thorium with a small admixture of enriched uranium that contains not more than 20% of ²³⁵U. It operates in the open-cycle mode involving ²³³U production from thorium and its subsequent burnup. The reactor meets the conditions of a nonproliferation of nuclear weapons: the content of fissionable isotopes in uranium at all stages of the process, including the final one, is below the threshold for constructing an atomic bomb, the amount of product plutonium being extremely small.     

Rare Earth Centered Hybrid Materials: Tb<Superscript>3+</Superscript> Covalently Bonded with La<Superscript>3+</Superscript>, Gd<Superscript>3+</Superscript>, Y<Superscript>3+</Superscript> Through Sulfonamide Bridge and Luminescence Enhancement

The organic ligand 5-sulfosalicylic acid (SSA) is grafted by (3-aminopropyl) triethoxysilane (APTES) to achieve functionalized sulfonamide bridge (SSA-Si) which can both coordinate to Ln³⁺ to form luminescent center and link inorganic Si-O network through hydrolysis and condensation reaction with tetraethoxysilane (TEOS). Thus the organic–inorganic hybrid is obtained with sol-gel method. The organic polymer poly-methyl methacrylate (PMMA) acts as another precursor is prepared through the direct addition polymerization of MMA monomer in the presence of the initiator BPO (benzoyl peroxide). The two kinds of precursors are coordinated to the Ln³⁺ simultaneously to form organic–inorganic-polymeric hybrids which contain both inorganic Si-O-Si net and organic periodic C–C chains. In these complicated compounds we intercalate different ratios of Tb³⁺ and inert lanthanide ion (La³⁺, Gd³⁺, Y³⁺) and find that the introduction of the inert lanthanide ions can enhance the luminescence intensity. This enhancement phenomenon is called co-luminescence effect which is studied by emission spectra in this paper.     

On the momentum correlations in the fragmentation of <Superscript>197</Superscript>Au + <Superscript>197</Superscript>Au reactions

We aim to present the formation of fragments using static as well as momentum-dependent interactions and larger nucleonic cross-sections. We shall also examine, in detail, the role of momentum correlations in these situations which are close to the fire-ball as well as to the spectator matter decay. The role of momentum correlations will be studied by imposing an additional cut in the momentum space. A clear need of a momentum cut is demonstrated in both fire-ball as well as spectator matter physics. The momentum-dependent interactions and larger cross-sections play a drastic role in peripheral reactions, whereas the role of momentum cut remains the same in these situations.     

Isotopomer selective optimization of <Superscript>39</Superscript>K<Superscript>85</Superscript>Rb<Superscript>+</Superscript> and <Superscript>41</Superscript>K<Superscript>87</Superscript>Rb<Superscript>+</Superscript> using optimal control

We report on isotope selective three-photon ionization of two isotopomers of KRb by applying evolution strategies. The particularity of this experiment is based on the high resolution phase and amplitude modulation of the fs-laser pulses provided by a 2 × 640 pixel pulse shaper. The optimization in a closed feedback loop performed with spectrally broad pulses centered at 840 nm shows high enhancements of one isotopomer at the expense of the other isotopomer and vice versa. From the optimal laser field we aim to gain details about the selective ionization sequence and the wavepacket evolution on the involved vibrational states.     

Description of elastic scattering in the <Superscript>16</Superscript>O + <Superscript>16</Superscript>O and <Superscript>16</Superscript>O + <Superscript>12</Superscript>C systems

The objective of the present study was to describe more precisely experimental data on elastic scattering in the ¹⁶O + ¹⁶O system at E _lab = 124, 145, 250, 350, and 480 MeV and in the ¹⁶O + ¹²C system at E _lab = 132, 170, 181, 200, 230, 260, and 281 MeV. The role of exchange interaction in the region of backward angles is investigated. The coefficient of incompressibility of nuclear matter is estimated at K = 205 MeV ± 15%.     

Comparison of halo of <Superscript>11</Superscript>Be, <Superscript>15</Superscript>C,and <Superscript>19</Superscript>C

We have compared the halo of ¹¹Be, ¹⁵C, and ¹⁹C nuclei by analyzing the one-neutron stripping reaction data on the Be target at 60-, 54-, and 57-MeV/A beam energies, respectively, within the framework of the eikonal approximation approach. The determination of effective range through the comparison of the total cross section data and prediction has revealed that the halo of ¹⁹C is the well developed, while that of ¹⁵C is the least and that of ¹¹Be lies in between these two. The longitudinal momentum distribution data also strengthen these observations. The text was submitted by the authors in English.     

Momentum distributions of <Superscript>4</Superscript>He nuclei from the <Superscript>6</Superscript>He and <Superscript>6</Superscript>Li breakup

Experimental data on the momentum distributions of ⁴He nuclei originating from ⁶He and ⁶Li breakup on various targets are presented over a wide beam energy range. The experiment with ⁶He was performed at the DRIBs accelerator complex for radioactive beams at the Joint Institute for Nuclear Research (JINR, Dubna). The intensity of the ⁶He beam used was 5 × 10⁶ particles per second and its energy was 10 MeV per nucleon. The momentum distributions of breakup products were measured by means of the MSP-144 magnetic spectrometer. The distribution width was shown to be virtually independent of the target mass. A small value of this width, σ ～ 28 MeV/c, confirms the presence of a halo in ⁶He. The measurements performed with ⁶Li beams of energy 18 and 46 MeV per nucleon at the U-400M accelerator yielded a width value of σ ～ 50 MeV/c for the momentum distributions of ⁴He nuclei, which is intermediate between that for ⁶He and those for stable nuclei. A compilation of the widths of the momentum distributions of fragments originating from the breakup of various nuclei is presented versus the binding energy of one or two neutrons in these nuclei, the target mass and the projectile energy.     

Band interaction in <Superscript>162</Superscript>Dy, <Superscript>168</Superscript>Er,and <Superscript>172</Superscript>Yb

Coriolis interaction between levels of two rotational bands in ¹⁷²Yb with K ^π = 2⁺ and 3⁺ and in ¹⁶⁸Er between levels with K ^π = 0^?, 1^?, and 2^? is studied. The values of the interaction parameters are obtained. The mutual influence of two bands in ¹⁶²Dy with ΔK = 2, K _i ^π = 0 ₂ ⁺ and 2 ₁ ⁺ due to Coriolis interaction is demonstrated.     

<Superscript>123</Superscript>I → <Superscript>123</Superscript>Te β decay

The β decay of ¹²³I has been calculated within the dynamic collective model developed by the authors earlier. The expression for the reduced matrix element of the weak-interaction Hamiltonian has been used for the partial β decay. The influence of the vacuum fluctuations and creation or annihilation of one or two phonons on the reduced β-decay probabilities is taken into account.     

High-lying excited states in <Superscript>10</Superscript>Be from the <Superscript>9</Superscript>Be(<Superscript>9</Superscript>Be,<Superscript>10</Superscript>Be)<Superscript>8</Superscript>Be reaction

A transfer-reaction experiment of ⁹Be(⁹Be, ¹⁰Be)⁸Be was performed at a beam energy of 45 MeV. Excited states in ¹⁰Be up to 18.80 MeV are produced using missing mass and invariant mass methods. Most of the observed high-lying resonant states, reconstructed from the α + ⁶He and t + ⁷Li decay channels, agree with the previously reported results. In addition, two new resonances at 15.6 and 18.8 MeV are identified from the present measurement. The 18.55 MeV state is found to decay into both the t + ⁷Li_g.s. and t + ⁷Li* (0.478 MeV) channels, with a relative branching ratio of 0.93 ± 0.33. Further theoretical investigations are encouraged to interpret this new information on cluster structure in neutron-rich light nuclei.     

Effect of high doses of N<Superscript>+</Superscript>, N<Superscript>+</Superscript> + Ni<Superscript>+</Superscript>, and Mo<Superscript>+</Superscript> + W<Superscript>+</Superscript> ions on the physicomechanical properties of TiNi

The surface layer of an equiatomic TiNi alloy, which exhibits the shape memory effect in the martensitic state, is modified with high-dose implantation of 65-keV N⁺ ions (the implantation dose is varied from 10¹⁷ to 10¹⁸ ions/cm²). TiNi samples are implanted by N⁺, Ni⁺-N⁺, and Mo⁺-W⁺ ions at a dose of 10¹⁷–10¹⁸ cm⁻² and studied by Rutherford backscattering, scanning electron microscopy, energy dispersive spectroscopy, X-ray diffraction (glancing geometry), and by measuring the nanohardness and the elastic modulus. A Ni⁺ concentration peak is detected between two maxima in the depth profile of the N⁺ ion concentration. X-ray diffraction (glancing geometry) of TiNi samples implanted by Ni⁺ and N⁺ ions shows the formation of the TiNi (B2), TiN, and Ni₃N phases. In the initial state, the elastic modulus of the samples is E = 56 GPa at a hardness of H = 2.13 ± 0.30 GPa (at a depth of 150 nm). After double implantation by Ni⁺-N⁺ and W⁺-Mo⁺ ions, the hardness of the TiNi samples is ∼2.78 ± 0.95 GPa at a depth of 150 nm and 4.95 ± 2.25 GPa at a depth of 50 nm; the elastic modulus is 59 GPa. Annealing of the samples at 550°C leads to an increase in the hardness to 4.44 ± 1.45 GPa and a sharp increase in the elastic modulus to 236 ± 39 GPa. A correlation between the elemental composition, microstructure, shape memory effect, and mechanical properties of the near-surface layer in TiNi is found.     

Nonlinear-laser effects in χ(<Superscript>3</Superscript>)-and χ(<Superscript>2</Superscript>)-active organic single crystals

The process of stimulated Raman scattering (SRS) allows one to convert laser emission wavelength of crystals, providing suitable molecular or lattice modes which contribute to third-order nonlinear optical susceptibility. Renewed interest in this field emerged because of the discovery of SRS in crystals that contain molecular units exhibiting Raman active modes. Particularly, organic nonlinear optical crystals used so far for frequency doubling and third harmonic generation seem to have a great potential for SRS application. This review paper reported same results on efficient SRS lasing effects that were discovered recently in organic crystals.     

A single laser system for ground-state cooling of <Superscript>25</Superscript>Mg<Superscript>+</Superscript>

We present a single solid-state laser system to cool, coherently manipulate and detect ²⁵Mg⁺ ions. Coherent manipulation is accomplished by coupling two hyperfine ground state levels using a pair of far-detuned Raman laser beams. Resonant light for Doppler cooling and detection is derived from the same laser source by means of an electro-optic modulator, generating a sideband which is resonant with the atomic transition. We demonstrate ground-state cooling of one of the vibrational modes of the ion in the trap using resolved-sideband cooling. The cooling performance is studied and discussed by observing the temporal evolution of Raman-stimulated sideband transitions. The setup is a major simplification over existing state-of-the-art systems, typically involving up to three separate laser sources.     

Effect of projectile structure in incomplete fusion in <Superscript>24</Superscript>Mg + <Superscript>59</Superscript>Co reaction

Integrated cross-section data for proton-proton bremsstrahlung including the points with the phase-space singularity, which occurs close to the maximum non-coplanarity angle, are presented. A numerical integration of theoretical cross-sections is performed over the non-coplanarity angle to integrate out this singularity. Furthermore, a comparison is made between measured cross-sections and predictions of two soft-photon models. All features observed for the data far from the singularity, including the overestimation of the cross-section by 30% by the theoretical calculations, emerge as well for the data close to and including the singularity.     

Analysis of <Superscript>4</Superscript>He+<Superscript>40</Superscript>Ca and <Superscript>4</Superscript>He+<Superscript>44</Superscript>Ti scattering using different optical model potentials

Elastic scattering of ⁴He+⁴⁰Ca and ⁴He+⁴⁴Ti reactions at backward angles has been analyzed using two differentmodels, microscopic and semimicroscopic folding potentials. The derived real potentials supplemented with phenomenological Woods–Saxon imaginary potentials, provide good agreement with the experimental data at energy E_c.m. = 21.8 MeV without need to renormalize the potentials. Coupledchannels calculations are used to extract the inelastic scattering cross section to the low-lying state 2+ (1.083 MeV) of ⁴⁴Ti. The deformation length is obtained and compared with the electromagnetic measurement values as well as those obtained from previous studies.     

High-precision mass measurements of hydrogen-like <Superscript>24</Superscript>Mg<Superscript>11+</Superscript> and <Superscript>26</Superscript>Mg<Superscript>11+</Superscript> ions in a Penning trap

For the determination of the bound-electron g factor in hydrogen-like heavy ions the mass of the ion is needed at a relative uncertainty of at least 1 ppb. With the SMILETRAP Penning trap mass spectrometer at the Manne Siegbahn Laboratory in Stockholm several mass measurements of ions with even-even nuclei at this level of precision have been performed so far, exploiting the fact that the mass precision increases linearly with the ion charge. Measurements of masses of the hydrogen-like ions of the two Mg-isotopes ²⁴Mg and ²⁶Mg are reported. The masses of the hydrogen-like ions are 23.979011054(14) u and 25.976562354(34) u, corresponding to the atomic masses 23.985041690(14) u and 25.982592986(34) u, respectively. The possibility to use these two isotopes for the first observation of an isotope effect in the bound-electron g factor in hydrogen-like heavy ions is discussed.     

<Superscript>6</Superscript>He + <Superscript>6</Superscript>He Clustering of <Superscript>12</Superscript>Be in a Microscopic Algebraic Approach

The norm kernel of the A=12 system composed of two ⁶He clusters, and the L=0 basis functions (in the SU(3) and angular momentum-coupled schemes) are analytically obtained in the Fock-Bargmann space. The norm kernel has a diagonal form in the former basis, but the asymptotic conditions are naturally defined in the latter one. The system is a good illustration for the method of projection of the norm kernel to the basis functions in the presence of SU(3) degeneracy that was proposed by the authors. The coupled-channel problem is considered in the algebraic version of the resonating-group method, with the multiple decay thresholds being properly accounted for. The structure of the ground state of ¹²Be obtained in the approximation of zero-range nuclear force is compared with the shell-model predictions. In the continuum part of the spectrum, the S-matrix is constructed, the asymptotic normalization coefficients are deduced and their energy dependence is analyzed.