非对称条形纳磁体的铁磁共振频率和自旋波模式

通过建立微波激励下的非对称条形多铁纳磁体的微磁模型,研究了倾斜角和缺陷角对该形纳磁体的铁磁共振谱和自旋波模式的影响.通过对微磁仿真得到的动态磁化数据进行分析发现,非对称条形纳磁体倾斜角度增加,铁磁共振频率随之增加,而这一现象与纳磁体的缺陷角度无关.倾斜角不变,非对称条形纳磁体的铁磁共振频率与缺陷角度呈单调递增关系,并且不同缺陷角度纳磁体的自旋波模式显示出极大的差异.非对称条形纳磁体与矩形纳磁体相比,它的自旋波模式局部化,具体为非对称条形纳磁体的自旋波模式不对称且高进动区域存在于边缘,表现为非对称边缘模式.倾斜角改变导致纳磁体内部退磁场变化,引起纳磁体边缘模式的移动,而中心模式对倾斜角的变化并不敏感.最后,对建立的模型在高频微波磁场激励下的磁损耗进行了分析,验证了模型的可靠性.这些结论说明缺陷角和倾斜角可用于纳磁体自旋波模式和铁磁共振频率的调谐,所得结果为可调纳磁微波器件的设计提供了重要的理论依据和思路.     

Electrical manipulation of nanomagnets

We demonstrate that it is possible to manipulate the magnetic coupling between two nanomagnets by means of an ac electric field. In the scheme suggested, the magnetic coupling is mediated by a magnetic particle that is in contact with both nanomagnets via tunnel barriers. The time-dependent electric field is applied so that the height of first one barrier then the other is suppressed in an alternating fashion. We show that the result is a pumping of magnetization from one nanomagnet to the other through the mediating particle. The dynamics of the magnetization of the mediating particle allows the coupling to be switched between being ferromagnetic and being antiferromagnetic.     

基于倾斜纳磁体翻转倾向性的与(或)逻辑门应力模型

纳米磁性逻辑器件具有高抗辐射性、低功率、天然非易失性等优势,应用前景广阔.倾斜放置的纳磁体具有翻转倾向性,在控制时钟撤去后倾斜纳磁体倾向于翻转至长轴的一端.利用倾斜纳磁体的翻转倾向性,提出了一种应力调控的与(或)磁逻辑门,并建立了其动态磁化的数学模型.使用微磁学方法对逻辑门进行了仿真,结果验证了预期逻辑门功能.与现有的逻辑门相比,基于倾斜纳磁体的与(或)门结构具有能耗更低、可靠性更高和制造工艺更简单等优点.     

Films of Mn12-acetate by pulsed laser evaporation

Films of the molecular nanomagnet, Mn₁₂-acetate, have been deposited using pulsed laser deposition and its novel variant, matrix assisted pulsed laser evaporation. The films have been characterized by X-ray photoelectron spectroscopy, mass spectrometry and magnetic hysteresis. The results indicate that an increase in laser energy and/or pulse frequency leads to fragmentation of Mn₁₂-acetate, whereas its chemical and magnetic integrity is preserved at low laser energy (200 mJ). This technique allows for the fabrication of patterned thin films of molecular nanomagnets for fundamental and applied experiments.     

磁性量子元胞自动机逻辑电路的转换特性研究

本文研究了磁性量子元胞自动机反相器和择多逻辑门等基本逻辑电路在不同纳磁体厚度和间距下的转换特性.采用单畴近似LLG方程对纳磁体以及电路进行了建模和仿真,结果表明更厚的纳磁体需要更大的转换磁脉冲,大厚度纳磁体逻辑电路表现出较慢的转换;相同厚度和间距下,择多逻辑门比反相器的转换时间略长.此外,模拟结果还表明纳磁体间距对反相器的转换过程影响明显,而对择多逻辑门则影响较小. 关键词： 磁性量子元胞自动机 转换特性 厚度和间距 逻辑电路     

Micromagnetic simulations of 200-nm-diameter cobalt nanorings using a Reuleaux triangular geometry

Using micromagnetic simulations, we investigated the magnetic states and switching processes of Co nanorings with lateral dimensions of 200 nm. We propose a special geometry of nanorings that adopts different Reuleaux triangular shapes. Reuleaux's triangles (RT) combine both the equilateral triangle and circular geometries. We studied the magnetic spin configurations of individual nanorings by varying the thickness and geometry of the nanomagnets. Our results demonstrated that in most nanomagnets exhibiting a thickness of less than 4 nm, there exists an onion-type state, which precedes either a twisted, double twisted, or cardioid state, when studying the magnetization reversal process. The hysteresis loops and magnetic states found in these RTs are compared with circular nanorings.     

Optimal design of nanomagnets for targeted hyperthermia

We have numerically simulated the dynamic response of single-domain nanomagnets to alternating magnetic fields and discuss nanometer-sized thermal seeds suitable for selectively targeted magnetic hyperthermia. When we assign priority to the easy delivery and biological safety of these fields, the maximum heating power is obtained by the irradiation of a weak field at a medium frequency (∼1 MHz) on almost spherical magnetite nanomagnets with a diameter of approximately 20 nm. On the other hand, the irradiation of the amplified field at a low frequency (∼100 kHz) is more effective if the neural stimulation is allowable.     

Magnetic properties and relaxation dynamics of a frustrated Ni? molecular nanomagnet

The Ni? nanomagnet represents an ideal model system for investigating the effects of geometrical frustration in magnetic interactions. The Ni ions in the magnetic core are arranged on two corner-sharing tetrahedra and interact through antiferromagnetic exchange couplings. We show that the high degree of frustration leads to a magnetic energy spectrum with large degeneracies which result in unusual static and dynamical magnetic properties. In particular, the relaxation dynamics of the magnetization is characterized by several distinct characteristic times. We also discuss the possible interest of Ni? for magnetocaloric refrigeration.     

Exploring the thermodynamic limits of computation in integrated systems: magnetic memory, nanomagnetic logic, and the Landauer limit

Nanomagnetic memory and logic circuits are attractive integrated platforms for studying the fundamental thermodynamic limits of computation. Using the stochastic Landau-Lifshitz-Gilbert equation, we show by direct calculation that the amount of energy dissipated during nanomagnet erasure approaches Landauer's thermodynamic limit of kTln(2) with high precision when the external magnetic fields are applied slowly. In addition, we find that nanomagnet systems behave according to generalized formulations of Landauer's principle that hold for small systems and generic logic operations. In all cases, the results are independent of the anisotropy energy of the nanomagnet. Lastly, we apply our computational approach to a nanomagnet majority logic gate, where we find that dissipationless, reversible computation can be achieved when the magnetic fields are applied in the appropriate order.     

Magnetization patterns simulations of Fe,Ni, Co,and permalloy individual nanomagnets

Hysteresis loop behaviours are studied in circular, triangular and Reuleaux's triangle (RT) of Fe, Co, Ni, and permalloy nanomagnets using micromagnetic simulations. The size and morphology of the nanomagnets are analyzed for three different thickness (10, 20, and 40 nm). For the triangle and RT shapes, our results reveal that for all magnetic material considered and in the low thickness (10 nm) the hysteresis prefer to be open, showing important coercive fields and remanence. However, when the thickness is increased (40 nm) almost all hysteresis loops are closed. Finally, the different mechanism of the magnetization reversal are investigated by monitoring the spin configuration as a function of the applied magnetic field.     

基于多铁纳磁体的择多逻辑门三维磁化动态特性研究

建立了多铁纳磁体择多逻辑门的三维磁化动态模型,并施加应变时钟(应力或电压)对多铁择多逻辑门的择多计算功能进行了动态仿真,同时分析了应变时钟工作机制以及它与择多逻辑门可靠转换之间的关系.仿真结果表明所建三维动态模型准确地描述了择多逻辑门的工作机制,在30 MPa应力作用下,择多逻辑门接受新输入实现了正确的择多计算功能.研究还发现对中心纳磁体和输出纳磁体依次撤去应变时钟时,提前撤去输出纳磁体上的应力会降低择多逻辑门的正确计算概率,而延迟撤去输出纳磁体上的应力会降低择多逻辑门的工作频率.研究结果深化了人们对多铁择多逻辑门动态特性的认识,可为多铁逻辑电路的设计提供重要指导.     

Heavy and light monopoles in magnetic reversion in artificial spin ice

This work makes a theoretical study of the dynamics of emergent elemental excitations in artificial spin ice systems with hexagonal geometry during the magnetic reversion of the system. The magnetic and physical parameters of the nanoislands that form the array are considered as variables in the study. The parameters considered are: the energy barrier for the inversion of each nanoisland, the magnetic moment of the nanomagnets and the possible disorder in the sample. Our results show that the reversion dynamic presents two distinct mechanisms of magnetic reversion, with different elemental excitations for each mechanism. The first mechanism presents a reversion with the appearance of magnetic monopoles that do not move in the samples (heavy monopoles) and the absence of Dirac chains. In the other mechanism elemental magnetic excitations (light monopoles) appear that move great distances in the sample, giving rise to extensive Dirac chains during the magnetic reversion.     

Switching field modulation of a nanomagnet by resonant microwave spin torque

We report on the effect of a low amplitude microwave current on the switching field of magnetic layers in a 40 nm diameter pseudo-spin valve grown by template synthesis. We show a frequency dependence at room temperature reflecting the dynamic behavior of the switching process. This is confirmed by numerical calculation of the Landau-Lifschitz-Gilbert equation including Slonczewski Spin Transfer Torque term within a macrospin approximation. The possibility to modulate the switching fields of a nanomagnet with microwave currents offers an alternative to the magnetic switching assisted by microwave magnetic field.     

Single-electron transport in electrically tunable nanomagnets

We study a single-electron transistor (SET) based upon a II-VI semiconductor quantum dot doped with a single-Mn ion. We present evidence that this system behaves like a quantum nanomagnet whose total spin and magnetic anisotropy depend dramatically both on the number of carriers and their orbital nature. Thereby, the magnetic properties of the nanomagnet can be controlled electrically. Conversely, the electrical properties of this SET depend on the quantum state of the Mn spin, giving rise to spin-dependent charging energies and hysteresis in the Coulomb blockade oscillations of the linear conductance.     

Superradiance from crystals of molecular nanomagnets

We show that crystals of molecular nanomagnets can exhibit giant magnetic relaxation due to the Dicke superradiance of electromagnetic waves. Rigorous theory is presented that combines superradiance with the Landau-Zener effect.     

Effective-medium approach for surface-localized magnetic polaritons in magnetic (ferromagnetic and antiferromagnetic) superlattices

The general effective-medium dispersion relations are derived for surface-localized magnetic polaritons which propagate parallel to the surface between a superlattice and semi-infinite bulk material, as applied to ferromagnetic and antiferromagnetic superlattices, in the situation when a static magnetic field is applied in the plane of the layers and parallel to the magnetization. The dependence of the energy of the surface waves on the volume fraction of the ferromagnetic superlattice component and the influence of the external magnetic field on the spectrum of the surface magnetic polaritons for the antiferromagnetic superlattice are investigated. The spectrum of the surface-localized magnetic polaritons which appear at the junction of the magnetic (ferromagnetic and antiferromagnetic) superlattice with the magnetic material are more complex, in contrast to the cases of semi-infinite magnetic material or semi-infinite magnetic SL. It is essential that in all cases in the presence of the external magnetic field the spectrum of the magnetic polaritons are non-reciprocal. The properties of surface polaritons are discussed in detail for the system ferromagnetic superlattice (YIG/non magnet)/YAG and the antiferromagnetic superlattice (MnF₂/ZnF₂)/FeF₂.     

A new manganese-based single-molecule magnet with a record-high antiferromagnetic phase transition temperature

We perform both dc and ac magnetic measurements on the single crystal of Mn30（Et-sao）3（C104）（MeOH）3 single- molecule magnet （SMM） when the sample is preserved in air for different durations. We find that, during the oxidation process, the sample develops into another SMM with a smaller anisotropy energy barrier and a stronger antiferromagnetic intermolecular exchange interaction. The antiferromagnetic transition temperature observed at 6.65 K in the new SMM is record-high for the antiferromagnetic phase transition in all the known SMMs. Compared to the original SMM, the only apparent change for the new SMM is that each molecule has lost three methyl groups as revealed by four-circle x-ray diffraction （XRD）, which is thought to be the origin of the stronger antiferromagnetic intermolecular exchange interaction.     

Analytical treatment of synchronization of spin-torque oscillators by microwave magnetic fields

An analytical approach is presented for the study of synchronization effects in spin-transfer-driven nanomagnets subjected to radio-frequency magnetic fields. The conditions are derived and discussed under which the current-induced magnetization precession is synchronized by the radio-frequency field. Exact analytical results are obtained for the case when the problem exhibits uniaxial symmetry around the axis perpendicular to the device plane. It is demonstrated that the magnetization dynamics under nonzero current and nonzero rf field is identical in structure to that under zero current. On this basis, analytical predictions are obtained for: the existence of phase-locking between current-induced magnetization precession and rf field oscillations; the frequency pulling effect in proximity of phase locking; the occurrence of hysteresis effects in phase-locking as a function of the spin-polarized current. The proposed approach is valid for arbitrary rf field amplitude and current intensity.     

Tailoring interacting magnetic nanodots via dimensionality variation of mediating electrons

Nature produces ferromagnetic materials based on nearest neighbor exchange interaction between atomic spins. For artificially fabricated nanomagnets, it is those “small” magnetic energies, e.g. anisotropy, dipolar interaction and indirect exchange interaction that play crucial roles against the thermal fluctuation. We have developed strong capabilities to grow nanodot assemblies in ultrahigh vacuum with controllable size and density on/in both metallic and insulating templates. Based on our novel synthesis capability, we have studied artificial nanomagnets with tunable coupling strength via dimensionality control of the mediating electrons in one-dimensional (1-D), 2-D, and 3-D. We show that such kind of dimensional confinement provides a unique way to induce novel magnetic properties and to gain control of them. The research outlined in this work provides the science base to understand, modify, and manipulate the magnetic properties through dimensional confinement.