Magnetooptical images of inhomogeneous magnetic fields in metallic films with in-plane anisotropy

The magnetooptical (MO) images of the inhomogeneous field created by permanent magnets in magnetic metallic films with in-plane anisotropy are experimentally studied. The MO images recorded using the longitudinal Kerr effect are the superposition of two pictures, namely, a polar-sensitivity MO image and a longitudinal-sensitivity MO image. An analysis of these images after separation shows that the polar-sensitivity MO image reflects the distribution of the inhomogeneous field component that is normal to the surface of an indicator film in an analog manner. The longitudinal-sensitivity MO image reflects the angular distribution of the in-plane component of a stray field in an analog manner. The coincidence of the experimental and corresponding simulated MO images makes it possible to interpret the experimental images. In particular, it is shown that the specific features detected in the topological characteristics of the inhomogeneous field correspond to experimental singular points. Hidden magnetic images (magnetic bar codes) are shown to be visualized with metallic CoFe films. As an example, the stray field of a magnetic system made of cylindrical magnets is mapped.     

Magneto-optical visualization of three spatial components of inhomogeneous stray fields

The article deals with the physical principles of magneto-optical visualization (MO) of three spatial components of inhomogeneous stray fields with the help of FeCo metal indicator films in the longitudinal Kerr effect geometry. The inhomogeneous field is created by permanent magnets. Both p- and s-polarization light is used for obtaining MO images with their subsequent summing, subtracting and digitizing. As a result, the MO images and corresponding intensity coordinate dependences reflecting the distributions of the horizontal and vertical magnetization components in pure form have been obtained. Modeling of both the magnetization distribution in the indicator film and the corresponding MO images shows that corresponding to polar sensitivity the intensity is proportional to the normal field component, which permits normal field component mapping. Corresponding to longitudinal sensitivity, the intensity of the MO images reflects the angular distribution of the planar field component. MO images have singular points in which the planar component is zero and their movement under an externally homogeneous planar field permits obtaining of additional information on the two planar components of the field under study. The intensity distribution character in the vicinity of sources and sinks (singular points) remains the same under different orientations of the light incidence plane. The change of incident plane orientation by π/2 alters the distribution pattern in the vicinity of the saddle points.     

ESR study of magnetic structures in La0.7Ca0.3MnO3

Comprehensive measurements of electron spin resonance (ESR) and magnetization of La_0.7Ca_0.3MnO₃ in the ferromagnetic as well as paramagnetic phases were carried out. Quantitative evidences for the inhomogeneous magnetic structure, consisting of ferromagnetic microregions embedded in the antiferromagnetic surrounding near T_c, were found. It is suggested that the microscopic local magnetic structures above and below T_c are qualitatively similar except that the phase below T_c carries long range order between the ferromagnetic microregions whose sizes grow with decreasing temperature.     

Fe-doping induced Griffiths-like phase in La0.7Ba0.3CoO3

The effect of Fe-doping on the magnetic properties of the ABO3-type perovskite cobaltites La0.7Ba0.3Co1 yFeyO3 (0 ≤ y ≤ 0.80) is reported.With no apparent structural change in any doped sample,the Curie temperature (TC) and the magnetization (M) are greatly suppressed for y ≤ 0.30 samples,while a distinct increase in TC for the y = 0.40 sample is observed.With the further increase of Fe concentration,TC increases monotonically.Griffiths-like phases in 0.40 ≤ y ≤ 0.60 samples are confirmed.The formation of the Griffiths-like phase is ascribed to B-site disordering induced isolation of ferromagnetic (FM) clusters above TC.     

Collective volume plasmons in manganites with nanoscale phase separation: simulation of the measured infrared spectra of La(0.7)Ca(0.3)MnO3

Optical characteristics of manganites with nanoscale electronic phase separation are simulated using an exact renormalization group transformation in Kirchhoff's equations. The local electric field is found to be highly inhomogeneous, exceeding the incident-wave field by orders of magnitude when the permittivities of the phases have opposite signs and plasmons are excited. The spatial scale of the field fluctuations suggests the collective character of the plasmon modes. The results of the simulation explain the optical anomalies of La(0.7)Ca(0.3)MnO(3) single crystals and films in the infrared frequency range in a natural way.     

Cr掺杂对Nd0.7Sr0.3MnO3电磁性质的影响

我们对多晶样品Nd0.7Sr0.3Mn1-xCrxO3(x≤0.30)进行了X射线衍射谱、电阻温度关系和磁化强度测量.实验发现:随Cr掺杂量的增加,样品的电阻率变大,电阻峰温度和居里温度降低,这是由Cr的介入弱化了双交换作用所致;在x=0.10附近,电阻出现了双峰现象,在其M~T上没有发现与低温峰对应的磁性异常;在锰位磁矩与Cr含量的关系中发现,Cr掺杂对样品的磁性几乎无贡献;通过分析,我们用相分离的图象解释了有关的现象.     

Magnetic and photomagnetic studies in Nd0.7Sr0.3CoO3

We report magnetic and photomagnetic studies on polycrystalline Nd_0.7Sr_0.3CoO₃. Strong irreversibility in field cooled and zero field cooled data is observed. The hysteresis plot exhibits a very high coercivity at low temperatures. On photon irradiation, a decrease in the coercivity and an irreversible magnetization enhancement are observed. The analysis of all these data suggest that microscopic phase separation of competing ferromagnetism and antiferromagnetism and/or light-induced spin conversion processes among low, intermediate and high spin states of cobalt ions are responsible for all the properties.     

Fano factor reduction on the 0.7 conductance structure of a ballistic one-dimensional wire

We have measured the nonequilibrium current noise in a ballistic one-dimensional wire which exhibits an additional conductance plateau at 0.7x2e(2)/h. The Fano factor shows a clear reduction on the 0.7 structure, and eventually vanishes upon applying a strong parallel magnetic field. These results provide experimental evidence that the 0.7 structure is associated with two conduction channels that have different transmission probabilities.     

Micromagnetic imaging to determine the nature of the ferromagnetic phase transition in La(0.7)Ca(0.3)MnO3

There is considerable controversy surrounding the nature of the paramagnetic to ferromagnetic phase transition in La(0.7)Ca(0.3)MnO3. We have used transmission electron microscopy to determine whether the phase transition is first or second order. On warming through the transition point, the ferromagnetic phase retreats from the sample surface as it is replaced by the paramagnetic phase. This coexistence of ferromagnetic and paramagnetic phases indicates a primarily first order transition. However, there is also continuous loss of magnetization which precedes the phase transition. We compare this with the phase transition in nickel, an archetypal second order ferromagnet.     

Magnetization and susceptibility studies of LaCu4.3Mn0.7

AC-susceptibility and magnetization measurements of LaCu_4.3Mn_0.7 below 60 K are reported. The susceptibility resembles an ordering of ferromagnetic-type to occur at 49 K. The magnetization shows that only 1% of the total manganese moment participates in this ordering.     

Resonant microwave conductivity response to ac current in La0.7Pb0.3MnO3 crystals

An experimental study of the effect of low-frequency transport current on the microwave conductivity of single-crystal La_0.7Pb_0.3MnO₃ is reported. In the absence of an external magnetic field, the microwave conductivity response to a current follows a relaxation behavior. In a nonzero external magnetic field, the response spectrum exhibits a peak of resonant amplitude enhancement. The resonant response has a nonlinear nature. The temperature and field dependences of the main parameters of the microwave response correlate directly with the behavior of the magnetoresistance. The results obtained are analyzed within the oscillator approximation. Electronic phase separation is proposed as a possible mechanism for the current action. Fiz. Tverd. Tela (St. Petersburg) 41, 2187–2192 (December 1999)     

A comparative study of magnetic and dielectric behaviors for La(1-x)Bi(x)Mn(1-y)Fe(y)O3 series (with x = 0.5, 0.7 and y = 0.3, 0.7)

We have carried out an extensive investigation into the effect of doping on both the A- and B-sites for the multiferroic La(0.5)Bi(0.5)Mn(0.5)Fe(0.5)O(3) in relation to its physical properties. The temperature dependent magnetization and dielectric response are determined for different percentages of Bi- and Fe-substitutions. For La(0.5)Bi(0.5)Mn(0.7)Fe(0.3)O(3), there is a prominent ferromagnetic transition T(C) around 110 K, whereas the other La(0.5)Bi(0.5)Mn(0.3)Fe(0.7)O(3) and La(0.3)Bi(0.7)Mn(0.3)Fe(0.7)O(3) phases fail to exhibit any clear transition. On the other hand, for the Fe-rich phases, the coercive field increases to 2450 Oe compared to 1720 Oe (for the Mn-rich phase). All the compositions exhibit coexistence of ferromagnetic and antiferromagnetic phases at low temperatures. The temperature dependent dielectric constant of the investigated samples varies from 32,000 to 500 at room temperature and the data has been analyzed using the universal dielectric response model.     

Inhomogeneous fluctuations in liquids and gases

The coupled inhomogeneous density and temperature oscillations in liquids and gases are described with the help of dynamical equations of motion for fluctuations. It is proved that stationary points are asymptotically stable when the preset temperature distribution is inhomogeneous. It is shown that the temperature setting in a gas is a result of the competition between viscosity and heat conduction mechanisms. The phase trajectories in the T-ρ plane are constructed in the inhomogeneous case by numerically solving the derived equations.     

Magnetotransport characteristics of strained La<Subscript>0.7</Subscript>Sr<Subscript>0.3</Subscript>MnO<Subscript>3</Subscript> epitaxial manganite films

The electrical and magnetic characteristics of La_0.7Sr_0.3MnO₃ (LSMO) epitaxial manganite films are investigated by different methods under conditions when the crystal structure is strongly strained as a result of mismatch between the lattice parameters of the LSMO crystal and the substrate. Substrates with lattice parameters larger and smaller than the nominal lattice parameter of the LSMO crystal are used in experiments. It is shown that the behavior of the temperature dependence of the electrical resistance for the films in the low-temperature range does not depend on the strain of the film and agrees well with the results obtained from the calculations with allowance made for the interaction of electrons with magnetic excitations in the framework of the double-exchange model for systems with strongly correlated electronic states. Investigations of the magneto- optical Kerr effect have revealed that an insignificant (0.3%) orthorhombic distortion of the cubic lattice in the plane of the NdGaO₃(110) substrate leads to uniaxial anisotropy of the magnetization of the film, with the easy-magnetization axis lying in the substrate plane. However, LSMO films on substrates (((LaAlO₃)_0.3+(Sr₂AlTaO₆)_0.7)(001)) ensuring minimum strain of the films exhibit a biaxial anisotropy typical of cubic crystals. The study of the ferromagnetic resonance lines at a frequency of 9.76 GHz confirms the results of magnetooptical investigations and indicates that the ferromagnetic phase in the LSMO films is weakly inhomogeneous.     

Multiferroic magnetoelectric coupling and relaxor ferroelectric behavior in 0.7BiFeO3-0.3BaTiO3 nanocrystals

The structural, microstructural, polarization, magnetization, dielectric constant, and relaxor characteristics of 0.7BiFeO₃-0.3BaTiO₃ (BF-BT) nanocrystals have been studied. BF-BT nanocrystals were prepared by a chemical route using polyvinyl alcohol as surfactant. The phase structure is confirmed by X-ray diffraction and average particle size by transmission and scanning electron microscopy. The magnetoelectric coupling is studied by polarization hysteresis loops under the influence of applied magnetic field and the phase transition anomaly. The diffuse phase transition is studied by modified Curie-Weiss law and relaxor characteristics by Vogel-Fulcher relation.     

Structure, spin reorientation and M(o)ssbauer effect studies of Tb0.3Dy0.7(Fe1-xAlx)1.95 alloys

The effect of Al substitution for Fe on crystal structure, magnetostriction and spontaneous magnetostriction, anisotropy and spin reorientation of a series of polycrystalline Tb0.3Dy0.7(Fe1-xAlx)1.95 alloys (x = 0, 0.05, 0.1, 0.15, 0.20, 0.25, 0.30, 0.35) at room temperature and 77 K was investigated systematically. It was found that the primary phase of Tb0.3Dy0.7(Fe1-xAlx)1.95 is the MgCu2-type cubic Laves phase structure when x < 0.4 and the lattice constant a of Tb0.3Dy0.7(Fe1-xAlx)1.95 increases approximately and monotonically with the increase of x. The substitution of Al leads to the fact that the magnetostriction ( inceases slightly in a low magnetic field (H ≤ 40 kA/m), but decreases sharply and is easily close to saturation in a high applied field as x increases, showing that a small amount of Al substitution is beneficial to a decrease in the magnetocrystalline anisotropy. It was also found that the spontaneous magnetostriction (ζ)111 decreases greatly with x increasing. The analysis of the M(o)ssbauer spectra indicated that the easy magnetization direction in the {110} plane deviates slightly from the main axis of symmetry with the changes of composition and temperature, namely spin reorientation. A small amount of non-magnetic phase exists for x = 0.15 in Tb0.3Dy0.7(Fe1-xAlx)1.95 alloys and the alloys become paramagnetic for x > 0.15 at room temperture, but at 77 K the alloys still remain magnetic phase even for x = 0.2. At room temperature and 77 K, the hyperfine field decreases and the isomer shifts increase with Al concentration increasing.     

Anomalous Hall effect in La0.7Sr0.3MnO3/SrTiO3 superlattices: hopping transport and a probe of dimensionality

The anomalous Hall effect (AHE) in La0.7Sr0.3MnO3/SrTiO3 (LSMO/STO) superlattices was analyzed using theories of the Berry phase effect. The temperature-dependent anomalous Hall coefficient Rs is found to be expressed by -Rs = Rs0 exp[(T/T0)1.5], where Rs0 is a prefactor and T0 is in units of kelvin, and is explained by the carrier-hopping mechanism. In addition, a scaling analysis for the Hall resistivity as a function of magnetization supports the scenario of the Berry phase effects. Furthermore, a shifting extremum of Hall resistivity in LSMO/STO superlattices is observed and regarded as a probe of dimensionality in quasi-two-dimensional systems.     

Magneto-transport and magnetic properties of (1-x)La0.7Ca0.3MnO3+xAl2O3 composites

We report magneto-transport and magnetic properties of (1-x)La_0.7Ca_0.3MnO₃+xAl₂O₃ composites synthesized through a solid-state reaction method combined with a high energy milling method. Most interestingly, the effective magnetic anisotropy is found to decrease with increase in the non-magnetic insulating Al₂O₃ phase fraction in the composites. In addition, we observed that the magnitude of low-field magnetoresistance arising from spin-polarized tunneling of conduction electrons, as well as that of high-field magnetoresistance, displays a Curie-Weiss law-like behavior. Finally, we found that the temperature dependence of low and high-field magnetoresistance is controlled predominantly by the nature of temperature response of surface magnetization of the particles.     

A structural, magnetostrictive and M(o)ssbauer study of Tb0.3Dy0.7(Fe0.9T0.1)1.95 alloys

The effect of ⅢA metal and transition metal T substitution for Fe on crystal structure, magnetostriction and spontaneous magnetostriction, anisotropy and spin reorientation of a series of polycrystalline Tb0.3Dy0.7(Fe0.9T0.1)1.95 (T = Mn, Fe, Co, B, Al, Ga) alloys at room temperature were investigated systematically. It was found that the primary phase of the Tb0.3Dy0.7(Fe0.9T0.1)1.95 alloys is the MgCu2-type cubic Laves phase structure for different substitution. The magnetostriction λs decrases greatly for the substitution of IIIA metal B, Al and Ga, but is saturated more easily for Al and Ga substitution, showing that the Al and Ga substitution is beneficial to a decrease in the magnetocrystalline anisotropy of Tb0.3Dy0.7(Fe0.9T0.1)1.95 alloys. However, the substitution of transition metal Mn and Co decreases slightly the magnetostriction λs. It was also found that the effect of different substitutions on the spontaneous magnetostriction λ111 is distinct. The analysis of the Mossbauer spectra indicates that the easy magnetization direction in the {110} plane deviates slightly from the main axis of symmetry for Al and Ga substitution, namely spin reorientation, but it does not change evidently for B, Mn and Co substitution.