Fluorescence measurements in a Low-pressure Kr/F2 medium

The time-resolved measurement of the sidelight fluorescence of KrF* formed by a short electron-beam pumping pulse (20 ns FWHM, 19 kA, 860 kV) was performed as a function of both the total pressure ranging from 100 Torr to 400 Torr and the partial F₂ concentration (0.1–1.0%). We have estimated the fluorescence yields (FY) for various laser-gas conditions experimentally and the results were compared with numerical predictions. This study indicates a superior amplification performance for a single ultrashort pulse in a low-pressure medium because of the higher FY for KrF*.     

Auto-prepulse operation of a long-pulse XeCl laser

A standard corona preionized XeCl laser prototype has been excited by a very simple L-C circuit consisting of a large storage capacitance charged at relatively low voltage (12 kV) and discharged via a switch on the electrodes, tightly coupled with the peaking capacitors. The resulting overvoltage following the switch closure behaves as an effective and automatic prepulse, providing a homogeneous discharge lasting up to 400 ns. Energy output levels of the order of 150 mJ at 1.4% overall efficiency have been achieved.     

Efficient low-voltage operation of a reverse-biased autoprepulse XeCl laser

An improved version of the auto-prepulse excitation scheme for long-pulse operation of the XeCl excimer laser is reported. A pulsed reverse bias on the small peaking capacitance allows efficient (1.7%) operation at 100 mJ output level with a charge voltage limited to 5–7 kV. Analogies and differences with other long-pulse operation schemes are also discussed.     

Direct generation of sub-nanosecond pulses in a high-pressure miniature excimer laser

Direct generation of subnanosecond pulses in a 9.0 cm discharge-length high-pressure XeCl laser is reported. The shortest pulse obtained was 670 ps (FWHM) with an energy of 1.2 mJ corresponding to 1.8 MW peak power.     

Influence of circuit and UV prioniser parameters on the performance of a discharge pumped KrF laser

The influence of the preioniser and main discharge circuit parameters on the performance of a high pressure UV preionised KrF laser using NF₃ as the fluorine donor has been investigated. Output laser energy densities of 1.7J·1⁻¹ based on the mode volume have been obtained under optimised conditions.     

Theoretical study of the feasibility of dual-band multiline operation of a TEA CO2 laser with intracavity fabry-perot etalons

It is shown that dual-band multiline operation of a TEA CO₂ laser can be conveniently achieved with the use of either one or two intracavity etalons of judiciously selected finesse and optical lengths.     

Continuous-wave high-power multi-pass pumped thin-disc Nd:GdVO4 laser

A thin-disc Nd:GdVO₄ laser in multi-pass pumping scheme was developed. Continuous-wave output power of 13.9 W at 1.06 μm for an absorbed power at 808 nm of 22 W was demonstrated from a 250-μm thick, 0.5-at.% Nd:GdVO₄ in a 4-pass pumping; the slope efficiency in absorbed power was 0.65, or 0.47 in input power. Output performances were also investigated under diode laser pumping at 879 nm, directly into the emitting ⁴F_3/2 level: maximum power of 3.6 W was obtained at 6.2 W of absorbed power with 0.69 slope efficiency. Compared with pumping at 808 nm, into the highly absorbing ⁴F_5/2 level, improvements of laser parameter in absorbed power (increase of slope efficiency, decrease of threshold) were obtained, showing the advantages of the pumping into the emitting level. However, the laser performances expressed vs. the incident power were modest owing to the low absorption efficiency at 879 nm. Thus, increased number of passes of the medium would be necessary in order to match the performances in input power obtained under 808-nm pumping.     

Discharge pumped C1F laser at 285 nm

This paper reports on experiments carried out in order to improve the performance of the TEA discharge pumped C1F uv laser at 285 nm. Factors which influence the gas degradation with increasing operating time, resulting in a decrease of laser output power, were investigated, aiming at a better understanding of the relevant mechanisms. By optimizing several parameters, laser pulse energies beyond 25 mJ were obtained in a high-pressure discharge laser chamber. C1F lasing has also been demonstrated in a commercially available multigas TEA laser system.As a byproduct of our C1F experiments, laser action on the correspondingDA transition of Cl₂ at 258 nm has also been achieved for the first time in a discharge laser chamber.     

Two-wavelength operation of a tunable KrF excimer laser — A promising technique for combustion diagnostics

A KrF excimer laser was operated on two independently tunable lines. This was achieved by a double-resonator configuration with two gratings. Tuning range and gain competition were investigated. The narrow line width (<1 cm^–1) and the independent tunability make this laser ideal for simultaneous spectroscopic detection of two species and temperature measurements in combustion processes.     

Peculiarities of KrF excimer vibrational relaxation in low-pressure Kr/F2 mixtures excited by a short pulse

The importance of excimer vibrational relaxation is manifested once again by the example of the low-pressure Kr/F₂ gain medium excited by a short pulse. The pressure is determined at which a sharp fall of the population efficiency of low KrF(B) vibrational levels should appear. Time peculiarities of the gain are investigated analytically for short-pulse excitation operation.     

Formation of diffraction-free beams by laser generation of conical radiation in a Kerr medium

Received: 16 June 1998     

A study of the electron quenching of excimers in a KrF* laser excited by a coaxial electron beam

Measurements of the output energy, the optical pulse length and the build-up time of the laser pulse, obtained with a coaxially e-beam pumped KrF^* laser, were performed varying the total gas fill pressure, the F₂ content and the e-beam current from 1–5 bar, 0.1–0.8% and 13.3–26.6 kA, respectively. The maximum specific extraction energy amounts to 64 J/l. The large range of measurements, especially at low F₂ concentrations, reveals the necessity to extend the kinetics of the F₂ chain in the usual computer model. With the introduction of electron quenching of KrF^* and ArF^* by dissociative attachment the predictions are also for low F₂ concentration in agreement with experiments.     

Highly efficient synchronous amplification of a picosecond dye laser at a kHz repetition rate

A short pulse, high energy, high repetition rate dye amplifier with superior conversion efficiency is reported. The dye amplifier is composed of three single-pass dye cells, longitudinally pumped by a frequency doubled 1 kHz Nd: YLF regenerative amplifier. The dye amplifier yields 3.5 ps, 150 J pulses at 595 nm, corresponding to a 12% conversion efficiency. The ASE is 1% or less, and the transverse mode quality is near-Gaussian.In absentia from the Department of Chemistry, Princeton University, Princeton, NJ 08544, USA     

Efficient amplification of sub-picosecond pulses of a non-CW dye laser

Efficient amplification in a dye laser amplifier is investigated theoretically and experimentally. A five-level rate equation approach is considered including rotational relaxation of the dye molecules. The effects of the pump pulse duration and of the parameters of the input pulse are discussed. The results are compared with experimental data for 0.5 ps pulses of a pulsed dye laser. Conversion efficiencies >10% are achieved for a single pass amplifier using Nd:YAG pump pulses of 2 ns while an effective fluorescence lifetime of 1.7±0.2 ns is determined for the gain medium rhodamine 6G. The triple pass amplifier stage of the laser system achieves an energy conversion of 4% with 40 J output pulses.     

Theoretical study of a new energy extraction scheme of a chemically pumped pulsed iodine laser amplifier

A new energy extraction scheme of a chemically pumped pulsed large-scale iodine laser based on a high-pressure pulsed singlet oxygen generator is proposed. In previous investigations only low-pressure oxygen generators have been considered. Since they require a high iodine density for an efficient amplifier operation, the lifetime of the stored energy is correspondingly small and thus only small-sized iodine amplifiers appear to be technically feasible. We found, however, that when the singlet oxygen is generated at high-pressure, the iodine density required can be considerably reduced so that the lifetime of the stored energy becomes sufficiently long to fill up large amplifier cells. A numerical model is developed and the extractable energy is theoretically estimated. It is shown that 0.2J/1·pass can be extracted when an input pulse of 20 ns duration (FWHM) and 1 J/cm² fluence is fed into the amplifying medium.     

Continuous-wave operation of a room-temperature Ho:YAP laser pumped by a Tm:YAP laser

We reported the Ho:YAP laser pumped by the Tm:YAP laser. The Ho:YAP laser maximum output power was 4.91 W when the incident power was 10.1 W with the threshold of 2.63 W. The slope efficiency was 63.7%, corresponding to an optical-to-optical efficiency of 48.6%. The Ho:YAP output wavelength was centered at 2118.2 nm with bandwidth of about 1 nm. We estimate the beam quality to be M² = 1.29.     

Tunable and high-energy Q-switched operation of an alexandrite slave ring laser

Narrow bandwith tunable Q-switched operation of an alexandrite oscillator was used for injection-locking of a high-energy alexandrite slave ring laser. Pulses with up to 600 mJ in energy over a 600 cm^–1 tuning range were obtained.     

Gain and saturation measurements in a discharge excited F2 laser using an oscillator amplifier configuration

The small-signal gain coefficient and the saturation intensity of a F₂ pulsed discharge molecular laser at 157 nm have been measured using two discharge devices in an oscillator-amplifier configuration. The small signal gain coefficient was measured to be 5.2±0.4% cm^–1 at 3 atm total pressure and 1.5 cm electrode spacing and 4.1±0.4% cm^–1 at 2 atm total pressure and 2 cm electrode spacing while the values of the saturation intensity were 5 MW/cm² and 4.6 MW/cm², respectively.     

Specialty Yb fiber amplifier for microchip Nd laser: Towards ∼1-mJ/1-ns output at kHz-range repetition rate

We demonstrate and optimize, for a mJ/ns release at the wavelength 1.064 μm, the operation of a compact laser system designed in the form of a hybrid, active-passive, Q-switched Nd³⁺:YAG/Cr⁴⁺:YAG microchip laser seeding an Yb-doped specialty multi-port fiber amplifier. As the result of the amplifier optimization, ∼1 mJ, ∼1 ns, almost single-mode pulses at a 1-10-kHz repetition rate are achieved, given by a gain factor of ∼19 dB for an 11-μJ input from the microchip laser. Meanwhile, a lower pulse energy, ∼120 μJ, but a much higher gain (∼25 dB) are eligible for the less powerful (0.35 μJ) input pulses.     

Thomson-scattering diagnostics of Kr/Ne and Kr/He plasmas using a picosecond laser

Thomson scattering from plasmas in high-pressure discharges for rare-gas-halide excimer-laser pumping was observed using a frequency-doubled 300 ps Nd: YAG laser. A temporal resolution of 1 ns was realized for the Thomson-scattering measurement, and detailed temporal changes of the electron density and temperature were measured in Kr/Ne and Kr/He plasmas. Calculations using a computer simulation showed good agreement with the experimental results, implying that the plasma dynamics is properly treated in the simulation.