Generation of ultrashort coherent vacuum ultraviolet pulses using electron storage rings: a new bright light source for experiments

We demonstrate for the first time that seeded harmonic generation on electron storage rings can produce coherent optical pulses in the vacuum ultraviolet spectral range. The experiment is performed at Elettra, where coherent pulses are generated at 132 nm, with a duration of about 100 fs. The light source has a repetition rate of 1 kHz and adjustable polarization; it is very bright, with a peak power several orders of magnitude above that of spontaneous synchrotron radiation. Owing to high stability, the source is used in a test photoemission electron microscopy experiment. We anticipate that seeded harmonic generation on storage rings can lead to unprecedented developments in time-resolved femtosecond spectroscopy and microscopy.     

Coherent harmonic generation on UVSOR-II storage ring

Among the attractive coherent light sources resulting from the interaction between femtosecond lasers and relativistic electron beams, simultaneous Coherent Synchrotron Radiation (CSR) in the THz region, slicing and UV-VUV Coherent Harmonic Generation (CHG) can be achieved on synchrotron radiation facilities. Recently, a Ti:Sa laser at high repetition rate (1 kHz) has been seeded in the optical klystron of the Free Electron Laser at UVSOR-II (Okazaki, Japan). In this paper, the experimental set-up allowing delivery of sub picosecond UV pulses from CHG, and TeraHertz radiation from CSR is described. We further focus on the third coherent harmonic (266 nm) generated. The expected typical characteristics of this radiation, predicted by both numerical and analytical models recalled here, are experimentally verified and several studies of the influence of the seed laser on the output CHG intensity are reported. Such experiment enables UVSOR-II facility to produce in parallel short pulses at two different colors, synchronized at high repetition rate with one single infrared laser: a unique set-up of great interest for the facility users.     

用ICCD作光开关测量储存环中光学速调管谐波超辐射

 用高通断比ICCD作为快速光开关,在中国科学技术大学的800MeV电子储存环上建造了一套光学速调管谐波超辐射测量系统,从每隔106个自发辐射脉冲1个谐波超辐射脉冲所形成的脉冲链里选出超辐射脉冲,测量谐波辐射的相干增强因子和谱宽。     

Single-pass high-harmonic generation at 20.8 MHz repetition rate

We report on single-pass high-harmonic generation (HHG) with amplified driving laser pulses at a repetition rate of 20.8?MHz. An Yb:YAG Innoslab amplifier system provides 35?fs pulses with 20?W average power at 1030?nm after external pulse compression. Following tight focusing into a xenon gas jet, we observe the generation of high-harmonic radiation of up to the seventeenth order. Our results show that state-of-the-art amplifier systems have become a promising alternative to cavity-assisted HHG for applications that require high repetition rates, such as frequency comb spectroscopy in the extreme UV.     

Picosecond pulse laser ablation of yttria-stabilized zirconia from kilohertz to megahertz repetition rates

Thin films of yttria stabilized zirconia were deposited onto silicon substrates using high repetition rate picosecond pulse lasers. The applied lasers covered the repetition rate range from 10 kHz to 4 MHz. We found that the laser pulse overlapping which results from increased repetition rates led to considerable changes in the ablation process. Defect formation and local heating lead to lower ablation thresholds and, with sufficiently high repetition rates, to melting of the target and even to thermal evaporation. We found that yttria-stabilized zirconia (YSZ) films deposited with picosecond pulses at 1064 nm wavelength below repetition rates of 2 MHz have rough, nanostructured morphology and the same atomic ratio of yttrium and zirconium as the target. Films deposited with 2 MHz and higher repetition rates with high number of overlapping pulses are very smooth, but are yttrium deficient, providing evidence of the importance of the thermal processes.     

Ultrafast thin-disk Yb:KY(WO4)2 regenerative amplifier with a 200-kHz repetition rate

We report an Yb:KYW thin-disk amplifier system that provides ultrashort pulses in the 10-microJ energy range at high repetition rates. The thin-disk concept uses large laser beam cross sections to avoid high peak intensities. Without using a traditional diffraction-grating stretcher, pulse energies of approximately 9 microJ with pulse durations of 280 fs at repetition rates of 200 kHz were generated.     

A simulation study of Tsinghua Thomson scattering X-ray source

Thomson scattering X-ray sources are compact and affordable facilities that produce short duration, high brightness X-ray pulses enabling new experimental capacities in ultra-fast science studies, and also medical and industrial applications. Such a facility has been built at the Accelerator Laboratory of Tsinghua University, and upgrade is in progress. In this paper, we present a proposed layout of the upgrade with design parameters by simulation, aiming at high X-ray pulses flux and brightness, and also enabling advanced dynamics studies and applications of the electron beam. Design and construction status of main subsystems are also presented.     

Passive coherent combination of two ultrafast rod type fiber chirped pulse amplifiers

Using passive coherent beam combining of two ultrafast fiber amplifiers, we demonstrate the generation of high temporal quality 300 fs and 650 μJ pulses corresponding to 60 W of average power at a repetition rate of 92 kHz. Furthermore, at 2 MHz of repetition rate record coherent combining average powers of 135 W before and 105 W after compression are measured. A combining efficiency higher than 90% is maintained over the whole range of output powers and repetition rates investigated demonstrating the efficiency and robustness of the passive combining technique. The measured pulse-to-pulse relative power fluctuation at high energy is 2%, indicating that the system is essentially immune to environmental phase noise. We believe the passive combining method to be an attractive approach for compact multi-GW peak power femtosecond fiber-based sources.     

Yb:YAG Innoslab amplifier: efficient high repetition rate subpicosecond pumping system for optical parametric chirped pulse amplification

We report on a Yb:YAG Innoslab laser amplifier system for generation of subpicsecond high energy pump pulses for optical parametric chirped pulse amplification (OPCPA) at high repetition rates. Pulse energies of up to 20 mJ (at 12.5 kHz) and repetition rates of up to 100 kHz were attained with pulse durations of 830 fs and average power in excess of 200 W. We further investigate the possibility to use subpicosecond pulses to derive a stable continuum in a YAG crystal for OPCPA seeding.     

Fully coherent hard X-ray generation by two-stage phase-merging enhanced harmonic generation

Cascading stages of seeded free electron lasers (FELs) is a promising way to produce fully coherent X-ray radiation. We study a new approach to produce coherent hard X-rays by cascading the recently proposed phase-merging enhanced harmonic generation (PEHG) The scheme consists of one dogleg and two PEHG configurations, and may be one of the leading candidates for the extracted undulator branch in future X-ray FEL facilities. FEL physics studies show that such a scheme is feasible within the present technology and can provide high brightness X-ray radiation pulses with narrow bandwidth and full coherence The radiated peak power at 1 Å wavelength converted from an initial 200 nm seed laser is over 2 GW.     

A simulation study of Tsinghua Thomson scattering X-ray source

Thomson scattering X-ray sources are compact and a?ordable facilities that produce short duration, high brightness X-ray pulses enabling new experimental capacities in ultra-fast science studies, and also medical and industrial applications. Such a facility has been built at the Accelerator Laboratory of Tsinghua University, and upgrade is in progress. In this paper, we present a proposed layout of the upgrade with design parameters by simulation, aiming at high X-ray pulses flux and brightness, and also enabling advanced dynamics studies and applications of the electron beam. Design and construction status of main subsystems are also presented.     

Regenerative amplification of femtosecond laser pulses in Ti:sapphire at multikilohertz repetition rates

We have generated and applied noncoherent x-ray radiation in an all-solid-state laser system operating at repetition rates up to 20 kHz. Based on a model that takes into account the strong thermal loading of the Ti:sapphire rod, a laser cavity with low sensitivity to thermal lensing was chosen. With a maximum pump power of 80 W, an output power as high as 27 W was obtained in gain-switched operation, and, with a seeding from a femtosecond oscillator, 60-fs, 0.8-mJ (8-W) pulses at 10 kHz and 0.32-mJ (6.5-W) pulses at 20 kHz were generated. High power femtosecond output was used to generate x-ray continuum radiation up to 5 keV from a liquid-gallium jet target.     

Experiment of X-ray Generations Using Laser-Compton Scattering at LINAC of SINAP

Laser Compton scattering(LCS) can generate X-rays or y-rays with high brightness and easy controlled polarization by applying high-peak-power laser pulses to relativistic electron bunches.One of the most promising approaches to short pulsed X-ray sources is the laser synchrotron source.It is based on LCS between picoseconds relativistic electron bunches and picoseconds laser pulses.A project of Shanghai laser electron gamma source with LCS method has been proposed on Shanghai synchrotron radiation facility.Before that,a prototype has been developed in the beamline of the linear accelerator at the Shanghai Institute of Applied Physics,Chinese Academy of Sciences.The LCS experiment was carried out by using the 107 MeV,5 Hz,1 ns,0.1 nC electron bunches from the linear accelerator and the 18 ns,10 MW peak power,Nd:YAG laser pulses.In this communication,we describe the details and report the first results of this experiment.     

A multi‐MHz single‐shot data acquisition scheme with high dynamic range: pump–probe X‐ray experiments at synchrotrons

The technical implementation of a multi‐MHz data acquisition scheme for laser–X‐ray pump–probe experiments with pulse limited temporal resolution (100 ps) is presented. Such techniques are very attractive to benefit from the high‐repetition rates of X‐ray pulses delivered from advanced synchrotron radiation sources. Exploiting a synchronized 3.9 MHz laser excitation source, experiments in 60‐bunch mode (7.8 MHz) at beamline P01 of the PETRA III storage ring are performed. Hereby molecular systems in liquid solutions are excited by the pulsed laser source and the total X‐ray fluorescence yield (TFY) from the sample is recorded using silicon avalanche photodiode detectors (APDs). The subsequent digitizer card samples the APD signal traces in 0.5 ns steps with 12‐bit resolution. These traces are then processed to deliver an integrated value for each recorded single X‐ray pulse intensity and sorted into bins according to whether the laser excited the sample or not. For each subgroup the recorded single‐shot values are averaged over ～10⁷ pulses to deliver a mean TFY value with its standard error for each data point, e.g. at a given X‐ray probe energy. The sensitivity reaches down to the shot‐noise limit, and signal‐to‐noise ratios approaching 1000 are achievable in only a few seconds collection time per data point. The dynamic range covers 100 photons pulse^?1 and is only technically limited by the utilized APD.     

Surface-emitted THz generation using a compact ultrashort pulse fiber amplifier at 1060 nm

Generation of InAs-surface-emitted terahertz radiation by application of an ultrashort pulse 1060 nm parabolic fiber amplifier source is reported for the first time. The fiber amplifier delivers 100 fs pulses at a repetition rate of 75 MHz and an average power of maximum 12 W. This new excitation laser for surface-emitters generates high brightness broadband THz radiation ranging from 100 GHz to over 2.5 THz. THz detection is demonstrated based on two-photon absorption at low-temperature-grown GaAs dipole receivers.     

Generation of 8-fs pulses at 390 nm

We demonstrated the generation of pulses as short as approximately 8 fs at 390 nm, with an average power of 80 mW by frequency-doubling the output of a sub-10-fs, 1.2-MW Ti:sapphire oscillator. Cross-correlation technique was employed to measure the pulse duration. To our knowledge, these are the shortest pulses produced in the violet-blue spectral range at high repetition rates so far.     

One way only to synchrotron light sources upgrade?

The last decade has seen a renaissance of machine‐physics studies and technological advancements that aim to upgrade at least 15 synchrotron light sources worldwide to diffraction‐limited storage rings. This is expected to improve the average spectral brightness and transversally coherent fraction of photons by several orders of magnitude in the soft‐ and hard‐X‐ray wavelength range, at the expense of pulse durations longer than ～80 ps FWHM. This paper discusses the compatibility of schemes for the generation of sub‐picosecond photon‐pulse durations in synchrotron light sources with standard multi‐bunch user operation and, in particular, diffraction‐limited electron optics design. The question of this compatibility is answered taking into consideration the storage ring beam energy and the constraint of existing synchrotrons' infrastructure. An alternative scheme for the upgrade of medium‐energy synchrotron light sources to diffraction‐limited storage rings and the simultaneous production of picosecond‐long photon pulses in a high‐gain free‐electron laser scheme are illustrated.     

X radiation sources based on accelerators

Light sources based on accelerators aim at producing very high brilliance coherent radiation, tuneable from the infrared to X-ray range, with picosecond or femtosecond light pulses.The first synchrotron light sources were built around storage rings in which a large number of relativistic electrons produce “synchrotron radiation” when their trajectory is subjected to a magnetic field, either in bending magnets or in specific insertion devices (undulators), made of an alternating series of magnets, allowing the number of curvatures to be increased and the radiation to be reinforced.These “synchrotron radiation” storage rings are now used worldwide (there are more than thirty), and they simultaneously distribute their radiation to several tens of users around the storage ring.The most effective installations in term of brilliance are the so-called 3rd generation synchrotron radiation light sources. The radiation produced presents pulse durations of the order of a few tens of ps, at a high rate (of the order of MHz); it is tuneable over a large range, depending on the magnetic field and the electron beam energy and its polarisation is adjustable (in the VUV-soft-X range). Generally, a very precise spectral selection is made by the users with a monochromator.The single pass linear accelerators can produce very short electron bunches (). The beam of very high electronic density is sent into successive undulator modules, reinforcing the radiation's longitudinal coherence, produced according to a Free Electron Laser (FEL) scheme by the interaction between the electron bunch and a light wave. The very high peak brilliance justifies their designation as 4th generation sources. The number of users is smaller because an electron pulse produces a radiation burst towards only one beamline. Energy Recovery Linacs (ERL) let the beam pass several times in the accelerator structures either to recover the energy or to accelerate the electrons during several turns, and thus provide subpicosecond beams for a greater number of users.A state-of-the-art of X sources using conventional (and not laser plasma based) accelerators is given here, underlying the performance already reached or forecast and the essential challenges. To cite this article: M.-E. Couprie, J.-M. Filhol, C. R. Physique 9 (2008).