Electro-optic spectral tuning in a continuous-wave, asymmetric-duty-cycle, periodically poled LiNbO(3) optical parametric oscillator

We demonstrate electro-optic spectral tuning in a continuous-wave periodically poled LiNbO(3) (PPLN) optical parametric oscillator (OPO). We achieve 8.91 cm(-1) of rapid spectral tuning, with a linear tuning rate of 2.89 cm(-1) /(kV/mm), by applying electric fields up to +/-1.5 kV/mm across the crystal while it is operating within the OPO. Intentionally poling the PPLN crystal with an asymmetric domain structure enables tuning, and numerical predictions closely match the experimental observations. The tuning is considerably larger than the typical operational bandwidth of the OPO, indicating that we are in fact shifting the gain curve of the PPLN crystal.     

飞秒光参量振荡器中非线性晶体的空间啁啾与角色散

对飞秒光参量振荡器的空间啁啾和角色散进行了理论计算和分析.给出了在非线性晶体中的空间啁啾表达式，以及在BBO晶体Ⅰ类非共线相位匹配情况下，在角度调谐过程中非线性晶体包括角色散在内的二阶、三阶色散的解析表达式，并精确计算了角色散对其二阶、三阶色散的影响. 关键词： 飞秒光参量振荡器 空间啁啾 角色散 二阶、三阶色散     

Optical parametric oscillation in quasi-phase-matched GaAs

We demonstrate an optical parametric oscillator (OPO) based on GaAs. The OPO utilizes an all-epitaxially-grown orientation-patterned GaAs crystal that is 0.5 mm thick, 5 mm wide, and 11 mm long, with a domain reversal period of 61.2 microm. Tuning either the near-IR pump wavelength between 1.8 and 2 microm or the temperature of the GaAs crystal allows the mid-IR output to be tuned between 2.28 and 9.14 microm, which is limited only by the spectral range of the OPO mirrors. The pump threshold of the singly resonant OPO is 16 microJ for the 6-ns pump pulses, and the photon conversion slope efficiency reaches 54%. We also show experimentally the possibility of pump-polarization-independent frequency conversion in GaAs.     

Spatial chirp and angular dispersion of the nonlinear crystal for a femtosecond OPO

In this paper spatial chirp and angular dispersion are calculated theoretically and analyzed for a four-mirror, standing-wave cavity femtosecond OPO. The analytical expression of spatial chirp in the nonlinear crystal is deduced. The analytical expressions of second- and third-order dispersion including angular dispersion of the nonlinear crystal are presented, for the noncollinear type-I phase-matched Fs BBO OPO using angle tuning. Moreover, variations of GDD and TOD with cavity parameters are calculated exactly. The analysis method and the obtained result also are efficacious for a same type Fs OPO.     

磷锗锌光学参量振荡器技术研究

 报道了一台高重复频率2 mm光学参量振荡器泵浦的磷锗锌光学参量振荡器。磷锗锌晶体(ZnGeP₂,简称ZGP)采用Ⅰ类相位匹配方式,切割角度q为55°,f为0°,尺寸5.5 mm×6 mm×18 mm,在4.0 kHz重复频率下,当注入5.2 W的2 mm圆偏振光时,获得310 mW中红外输出,p偏振态2 mm到3～5 mm光-光转换效率12%。通过调节晶体的角度,实验获得ZGP光学参量振荡器的波长调谐曲线,在误差范围内与理论变化规律相符。     

Self‐phase‐locked degenerate femtosecond optical parametric oscillator based on BiB3O6

A self‐phase‐locked degenerate femtosecond optical parametric oscillator (OPO) based on the birefringent nonlinear material, bismuth triborate, BiB₃O₆, synchronously‐pumped by a Kerr‐lens‐mode‐locked Ti:sapphire laser at 800 nm is described. By exploiting versatile phase‐matching properties of BiB₃O₆, including large spectral and angular acceptance for parametric generation and low group velocity dispersion in the optical xz plane, stable self‐phase‐locked degenerate OPO operation centered at 1600 nm is demonstrated using collinear type I (e → oo) interaction in a 1.5‐mm crystal at room temperature. The degenerate OPO output spectrum extends over 46 nm (∼5.4 THz) with 190 fs pulse duration for input pump pulses of 155 fs with a bandwidth of 7 nm. Phase coherence between the pump and degenerate output is verified using f‐2f interferometry, and discrete frequency beats caused by different carrier‐envelope‐offset frequencies are measured using radio frequency measurements. Photo shows a 1.5‐mm BiB₃O₆ crystal used as a nonlinear gain medium in a degenerate self‐phase‐locked femtosecond OPO operating at room temperature. The green beam is the result of non‐phase‐matched sum‐frequency mixing between the pump light and the sub‐harmonic OPO field at degeneracy.     

Widely and continuously tunable optical parametric oscillator based on a cylindrical periodically poled KTiOPO(4) crystal

We report on what is to our knowledge the first realization of a quasi-phase-matched optical parametric oscillator (OPO) based on a crystal with a cylindrical shape. The main reason for interest in this device is its broad, continuous tuning. In experiments with a 1064-nm pump, the signal tuning range was equal to 525 nm (1515-2040 nm), and the corresponding idler was continuously tuned over 1340 nm (2220-3560 nm). The angular tuning was 26 degrees , with only a minor variation of the OPO threshold over the entire tuning range.     

Nanosecond optical parametric oscillator based on large-aperture periodically poled RbTiOAsO(4)

We report on optical parametric oscillators (OPO's) based on periodically poled RbTiOAsO(4) (PP RTA), which are pumped by Q -switched solid-state lasers. With a diode-pumped Nd:YVO(4) laser (pulse energy, 800microJ ; pulse duration, 5.5 ns; repetition rate, 1 kHz) the PP RTA OPO generated 1.58-microm signal and 3.26-microm idler radiation with a signal pulse energy of 45microJ . The large aperture of 3 mmx3 mm of the PP RTA crystal also permitted OPO operation with pump pulse energies as high as 65 mJ, provided by a flash-lamp-pumped Q -switched Nd:YAG laser (pulse duration, 20 ns; repetition rate, 10 Hz). With this pump source the OPO generated signal pulse energies as high as 17 mJ, corresponding to an efficiency of 26%. The performance of this OPO shows that large-aperture PP RTA crystals are well suited for pulsed nanosecond OPO operation with pump pulse energies of tens of millijoules.     

Mid-infrared optical parametric oscillator based on ZnGeP2 pumped by 2-μm laser

We present a 3 5 μ m optical parametric oscillator (OPO) based on ZGP pumped by KTP OPO 2.1-μ m laser. The tuning curves of ZGP OPO are calculated. The 8 ×6 ×18 (mm) ZGP crystal, whose end faces are antireflection coated at 2.1 and 3.7 4.6 μ m, is cut as θ =53.5°, φ =0°. When the pump power of 2.1-μ m polarized laser is 15 W at 8 kHz, 5.7-W output power and 46.6% slope efficiency are obtained with a ZGP type I phase match. Central wavelengths of the signal and idler lasers are 4.10 and 4.32 μ m, respectively. Pulse duration is about 27 ns. Beam quality factor M 2 is better than 1.8. The tunability of 3 5 μ m can be achieved by changing the angle of the ZGP crystal.     

Comparative studies of eye-safe intracavity and extracavity optical parametric oscillators with an unstable telescopic cavity

We have experimentally studied the lasing characteristics of an eye-safe optical parametric oscillator (OPO) with an unstable telescopic cavity when it is placed inside (intracavity OPO) and outside (extracavity OPO) the plane-parallel cavity of a pulsed, nearly single-mode KGW:Nd pump laser. We used a KTP crystal as the nonlinear medium for the OPO. We have shown that the intracavity OPO has the higher lasing efficiency. We have observed that the distribution of nonlinear losses introduced by the intracavity OPO, nonuniform over the cavity cross section, leads to an increase in the diameter and divergence of the radiation beam from the pump laser and a dependence of its temporal lasing dynamics on the transverse beam coordinate. We propose a physical model qualitatively explaining the spatial and temporal lasing dynamics of a radiation source with an intracavity OPO. Both OPO versions generate beams of radiation with about the same divergence. When the KGW:Nd laser has an electrical pumping energy of 7.3 J and a cavity length of 77 cm, the intracavity OPO and the extracavity OPO emit pulses with energies of 14.5 mJ and 12.0 mJ and duration 18 nsec and 13 nsec respectively. The divergence of the eye-safe radiation (λ = 1.578 μm) at 86.5% of the total pulse energy is no greater than 5.5 mrad for an OPO output beam diameter of = 2 mm. __________ Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 73, No. 4, pp. 535–543, July–August, 2006.     

Beam divergence effects on high power optical parametric oscillation

The beam divergence effects of the input pump laser on a high power nanosecond optical parametric oscillator （OPO） have been numerically simulated. The OPO conversion efficiency is affected due to the angular deviation of real laser beams from ideal phase matching conditions. Our theoretical model is based on the decomposition of the Gaussian beam and assumes each component has a single deviation angle and thus a particular wave vector mismatch. We take into account the variable intensity profile in the spatial and temporal domains of the Gaussian beam, the pump depletion effects for large-signal processes as well as the oscillatory effects of the three waves. Two nonlinear crystals β-BaB2O4 （BBO） and LiB305 （LBO） have been investigated in detail. The results indicate that the degree of beam divergence strongly influences the maximum pump intensity, optimum crystal length and OPO conversion efficiency. The impact of beam divergence is much more severe in the case of critical phase-matching for BBO than in the case of non-critical phase-matching for LBO. The results provide a way to choose the optimum parameters for a high power ns OPO such as the nonlinear material, the crystal length and the pump intensity, etc. Good agreement is obtained with our experimental results.     

Electro-optic tuning of a periodically poled LiNbO3 optical parametric oscillator and mixing its output waves to generate mid-IR tunable from 9.4 to 10.5 μm

We demonstrate electro-optic spectral tuning in a pulsed periodically poled LiNbO₃ (PPLN) optical parametric oscillator (OPO) in ns regime. A 3-cm-long LiNbO₃ crystal is segmented in three equal sections; the outer sections are periodically poled. The center segment is of single domain whose refractive index is changed by electro-optic effect. Applying voltage from 0 to −5000 V, the OPO signal and idler waves are tuned from 1.932 to 1.912 μm and 2.368 to 2.40 μm, respectively. The signal and idler waves obtained are difference-frequency-mixed in a 10 mm long AgGaS₂ crystal to produce mid-IR tunable from ∼10.5 to ∼9.4 μm, which matches the tuning range of a CO₂ laser.     

Broadband, rapidly tunable Ti:sapphire-pumped BiB₃O₆ femtosecond optical parametric oscillator

We report a femtosecond optical parametric oscillator (OPO) based on the nonlinear material BiB?O? (BIBO) pumped directly by a Kerr lens mode-locked Ti:sapphire laser. Using a 1.5 mm long BIBO crystal cut at θ=11.4° for collinear type I (e→o+o) phase matching in the xz optical plane, femtosecond signal pulses across 1.4-1.6 μm, and idler pulses across 1.6-1.87 μm spectral range are generated, limited by the reflectivity bandwidth of the OPO mirrors. The high nonlinear gain and large spectral acceptance for type I interaction in the xz plane of BIBO permit rapid and continuous tuning across the entire range by simple fine adjustment of OPO cavity delay or through small changes in the pump wavelength, without varying any other parameters. Additionally, owing to the near-zero group velocity mismatch and dispersion, the OPO supports broad spectrum as wide as 33 nm, which results in self-compressed signal pulses. For 150 fs pump pulses, signal pulses with durations down to 106 fs with a time-bandwidth product of 0.48 are obtained without the need for intracavity dispersion compensation.     

Spectral properties and numerical modelling of a critically phase-matched nanosecond LiB3O5 Optical Parametric Oscillator

We report on the spectral properties and numerical modelling of a singly resonant Optical Parametric Oscillator (OPO) of Lithium-triBOrate (LBO). The OPO is pumped by the second, third or fourth harmonic of an injection-seeded,Q-switched Nd:YAG laser. The measured OPO parameters are the tuning range, the threshold, the spectral linewidth, the efficiency and the output power. For the LBO-OPO critical type-I phase-matching (xy-plane) provides a wide tuning range and optimum values of the effective nonlinear coefficient. Pumped, for example, by the 355nm third harmonic the spectral range extends from 414 nm to 2.47 µm. With a 15 mm long crystal the OPO generates a total output-pulse energy of 77 mJ with an efficiency of 45%. For 266 nm pump radiation the signal wave is in the near ultraviolet at 307–325 nm. If pumped at 532 nm the OPO generates simultaneously two pairs of signal and idler waves in the infrared (0.707–2.15 µm). The pulse-energy fluctuations of the two pairs are correlated. If, however, the OPO is injection-seeded at one of the signal waves the two wavelength pairs are anti-correlated. The observed wavelength tuning as well as the measured spectral line-widths, threshold energies and efficiencies are in agreement with the values predicted by computer simulation.     

Experimental investigation and numerical simulation of the spatio-temporal dynamics of the light-pulses in nanosecond optical parametric oscillators

This paper reports on the experimental investigation and the numerical simulation of the spatio-temporal dynamics of the pulse formation in nanosecond optical parametric oscillators. The temporal evolution of the spatial intensity distribution is measured with a fast two-dimensional CCD-camera. The measurements are performed for a signal-resonant nanosecond pulsed optical-parametric-oscillator (OPO) which consists of a 12 mm long, critically phase-matched beta-barium-borate (BBO)-crystal in a 40 mm long cavity of two plane mirrors. The OPO was pumped by the third harmonic of a flashlamp-pumped Nd:YAG-Laser at a repetition rate of 10 Hz. At pump energies close to the OPO threshold the emitted OPO-radiation has an almost gaussian intensity distribution throughout the entire pulse. The beam quality factor M² remains below 2.2. At high pump energies the OPO oscillation also starts with an almost gaussian beam-profile. During the build-up and parametric amplification of the pulse the fields experience, however, a spatially inhomogeneous gain, caused by walk-off in the birefringent crystal, pump-depletion, and back-conversion. The spatial intensity distribution thus becomes asymmetric and the M² value increases. The measurements are compared with the results of detailed numerical calculations. The model takes the amplification of the OPO-radiation in the nonlinear crystal, and the properties of the OPO cavity as well as the diffraction of the beams during propagation into account. The spatio-temporal dynamics of the pulse formation predicted by the numerical model are in good agreement with the experimental results. PACS 42.65.Sf; 42.65.Yj     

Comparative investigation of long-wave infrared generation based on ZnGeP2 and CdSe optical parametric oscillators

Long-wave infrared(IR) generation based on type-II(o→e+o) phase matching ZnGeP 2(ZGP) and CdSe optical parametric oscillators(OPOs) pumped by a 2.05 μm Tm,Ho:GdVO 4 laser is reported.The comparisons of the birefringent walk-off effect and the oscillation threshold between ZGP and CdSe OPOs are performed theoretically and experimentally.For the ZGP OPO,up to 419 mW output at 8.04 μm is obtained at the 8 kHz pump pulse repetition frequency(PRF) with a slope efficiency of 7.6%.This ZGP OPO can be continuously tuned from 7.8 to 8.5 μm.For the CdSe OPO,we demonstrate a 64 mW output at 8.9 μm with a single crystal 28 mm in length.     

High average power 2 μm generation using an intracavity PPMgLN optical parametric oscillator

An intracavity quasi-phase-matched optical parametric oscillator (OPO) has been developed for the purpose of generating radiation with high average power and high repetition rate in the 2 μm regime. The device is a degenerate OPO based on a 3 mm thick MgO-doped periodically poled LiNbO(3) (PPMgLN) crystal, which is pumped in turn within the cavity by a diode side-pumped, Q-switched 1 μm Nd:YAG laser operating at 10 kHz. Up to 20 W broadband 2 μm radiation can be generated with a compact configuration under the crystal temperature of 115 °C. The beam profile is close to circularly symmetric with M(2) ~ 10.     

High-power, continuous-wave, singly resonant optical parametric oscillator based on MgO:sPPLT

We report a high-power, widely tunable, cw singly resonant optical parametric oscillator (OPO) based on MgO:sPPLT. The OPO is pumped in the green by a cw diode-pumped Nd:YVO(4) laser at 532 nm and can provide continuously tunable output across 848-1430 nm. Using a 30 mm crystal and double-pass pumping, an oscillation threshold of 2.88 W has been obtained, and single-pass idler powers in excess of 1.51 W have been generated over 1104-1430 nm for 6W of pump power at an extraction efficiency of 25.2% and photon conversion efficiency of 56.7%.     

Performance evaluation of ZnGeP2 optical parametric oscillator pumped by a Q-switched Tm,Ho:GdVO4 laser

A doubly resonant ZnGeP2 （ZGP） optical parametric oscillator （OPO） pumped by a novel Tm,Ho：GdVO4 laser was demonstrated. Cryogenic Tin（5 at.-%）, Ho（0.5 at.-%）：GdVO4 laser with high pulse repetition frequency （PRF） of 10 kHz at 2.05 μm was employed as pumping source of ZGP OPO. The 15-mm-long ZGP crystal, 55° cut for I-type phase-matching with low absorption coefficient less than 0.05 cm^-1 at 2 μm, was placed in a piano-piano cavity with resonator length of 30 mm. The ZGP OPO generated a total combined output power of 1.2 W at 3.75 and 4.52 μm under pumping power of 5.3 W, corresponding to slope efficiency of 40% from incident 2μm laser power to midinfrared （Mid-IR） output. A widely tunable range from 3.0 to 6.5 μm was achieved by changing the crystal angle only 3.5°.     

Comparative investigation of long-wave infrared generation based on ZnGeP2 and CdSe optical parametric oscillators

Long-wave infrared (IR) generation based on type-II (o→e+o) phase matching ZnGeP₂ (ZGP) and CdSe optical parametric oscillators (OPOs) pumped by a 2.05 μm Tm,Ho:GdVO₄ laser is reported. The comparisons of the birefringent walk-off effect and the oscillation threshold between ZGP and CdSe OPOs are performed theoretically and experimentally. For the ZGP OPO, up to 419 mW output at 8.04 μm is obtained at the 8 kHz pump pulse repetition frequency (PRF) with a slope efficiency of 7.6%. This ZGP OPO can be continuously tuned from 7.8 to 8.5 μm. For the CdSe OPO, we demonstrate a 64 mW output at 8.9 μm with a single crystal 28 mm in length.