Simplified approach to double jumps for fluorescing dipole-dipole interacting atoms

A simplified scheme for the investigation of cooperative effects in the quantum jump statistics of small numbers of fluorescing atoms and ions in a trap is presented. It allows the analytic treatment of three dipole-dipole interacting four-level systems which model the relevant level scheme of Ba⁺ ions. For the latter, a huge rate of double and triple jumps was reported in a former experiment and the huge rate was attributed to the dipole-dipole interaction. Our theoretical results show that the effect of the dipole-dipole interaction on these rates is at most 5% and that for the parameter values of the experiment there is practically no effect. Consequently it seems that the dipole-dipole interaction can be ruled out as a possible explanation for the huge rates reported in the experiment.     

Superradiant laser: First-order phase transition and non-stationary regime

We solve the superradiant laser model in two limiting cases. First the stationary low-pumping regime is considered where a first-order phase transition in the semiclassical solution occurs. This discontinuity is smeared out in the quantum regime. Second, we solve the model in the non-stationary regime where we find a temporally periodic solution. For a certain parameter range well-separated pulses may occur. Received: 19 June 1998 / Accepted: 19 October 1998     

Photon statistics of a bad-cavity laser near threshold

A simple model of a bad-cavity laser is presented based on Haken's master equation for N pumped two-level atoms in a cavity. Via adiabatic elimination of fast variables the whole photon statistics is solved analytically near threshold. It is shown that the second order coherence function g ⁽²⁾ (0) has a very different behavior near threshold for a bad-cavity laser compared to a good-cavity laser. The power spectrum illustrates nicely the different time scales involved in the dynamics. Received: 13 November 1998 / Revised: 19 May 1998 / Accepted: 6 July 1998     

Frequency dependence of the photonic noise spectrum in an absorbing or amplifying diffusive medium

A theory is presented for the frequency dependence of the power spectrum of photon current fluctuations originating from a disordered medium. Both the cases of an absorbing medium (“grey body”) and of an amplifying medium (“random laser”) are considered in a waveguide geometry. The semiclassical approach (based on a Boltzmann-Langevin equation) is shown to be in complete agreement with a fully quantum mechanical theory, provided that the effects of wave localization can be neglected. The width of the peak in the power spectrum around zero frequency is much smaller than the inverse coherence time, characteristic for black-body radiation. Simple expressions for the shape of this peak are obtained, in the absorbing case, for waveguide lengths large compared to the absorption length, and, in the amplifying case, close to the laser threshold. Received 8 August 2000     

3d D lifetime in laser cooled Ca : Influence of cooling laser power

We have measured the lifetime of the metastable 3D _5/2 level in Ca⁺ using the “quantum jump" technique on a single stored and laser cooled ion in a linear Paul trap. We found a linear dependence of the measured decay rate on the power of the laser which repumps the ions from the long lived 3D _3/2 level. This can be explained by off-resonant depletion of the 3D _5/2 level. The proper lifetime of this level is obtained by a linear extrapolation of the measured lifetime to zero laser power. We obtain 1100(18) ms in agreement with theoretical calculations. The observed systematic change of the decay rate resolves discrepancies between earlier experiments in which this effect had not been considered. Measurements on a linear chain of 10 laser cooled ions showed unexpected frequent coincidences of quantum jumps within our observation time of 20 ms. This indicates a so far unexplained correlation between the ions in the chain at large distances. Received 3 March 1999     

Retrieval of spatial shot-noise in the full dynamic range of calibrated CCD cameras

The pixel by pixel calibration of a scientific CCD camera allows Poissonian statistics of the spatial fluctuations of an uniform enlightening to be retrieved in the full range of the camera dynamic. The procedure works efficiently for thermal as well as for laser sources, provided that the wavelength and the coherence properties of the source are chosen in order to avoid the formation of equal thickness fringes in the chip (etaloning effect). Calibration allows also the comparison at the shot noise level of images recorded at different places on the chip. Received 9 September 2002 / Received in final form 16 October 2002 Published online 21 January 2003     

Absorption and dispersion by a multiple driven two-level atom

We investigate the absorption and dispersion properties of a two-level atom driven by a polychromatic field. The driving field is composed of a strong resonant (carrier) frequency component and a large number of symmetrically detuned sideband fields (modulators). A rapid increase in the absorption at the central frequency and the collapse of the response of the system from multiple frequencies to a single frequency are predicted to occur when the Rabi frequency of the modulating fields is equal to the Rabi frequency of the carrier field. These are manifestations of the undressing or a disentanglement of the atomic and driving field states, that leads to a collapse of the atom to its ground state. Our calculation permits consideration of the question of the undressing of the driven atom by a multiple-modulated field and the predicted spectra offer a method of observing undressing. Moreover, we find that the absorption and dispersion spectra split into multiplets whose structures depend on the Rabi frequency of the modulating fields. The spectral features can jump between different resonance frequencies by changing the Rabi frequency of the modulating fields or their initial phases, which can have potential applications as a quantum frequency filter. Received 23 October 2001 and Received in final form 31 January 2002     

Manipulating the phase of a single-mode micromaser by polarized three-level atoms

We investigate the phase probability distribution (PPD) of a single-mode micromaser pumped by atoms injected in the most general case, i.e. in the superposition of the upper, intermediate and lower states by the Monte Carlo wave function approach. The phase properties of the cavity mode are greatly influenced by the relative phases and the amplitudes of the polarized atoms, and the detunings between the atom and cavity. The cavity field has a single preferred phase if the cavity is pumped by the atoms in the superposition of the upper and intermediate states or of the intermediate and lower states. However, a double-peak feature appears in the PPD of the cavity field when the cavity is pumped by the atoms in the superposition of the upper and lower states. With appropriate detunings, the double peaks become narrower and more remarkable, which shows the better defined phase of the cavity field, as compared to the resonant case. The PPD displays complicated characteristics when the cavity is pumped by the atoms in the superposition of the upper, intermediate and lower states. The phase distribution changes from a single peak to double peaks and to another single peak when we modulate the phase of the intermediate state, which has been explained in the semi-classical radiation theory.     

Ultimate quantum limits for resolution of beam displacements

We compare two high sensitivity techniques which are used to measure very small displacements of physical objects by optical techniques: the interferometric devices, measuring longitudinal phase shifts, and the devices used to monitor transverse displacement of light beams. We detail the differences and the similarities for the quantum limits on the resolution of both systems. In both cases squeezed light can be used to resolve beyond the standard quantum limit and number correlated states allow us to reach the “Heisenberg” limit. Received 12 September 2002 Published online 21 January 2003     

Dependence on crystal parameters of the correlation time between signal and idler beams in parametric down conversion calculated in the Wigner representation

The theory of parametric down conversion within the framework of the Wigner representation has been treated recently in a series of papers using the standard model Hamiltonian. Here we take a more fundamental point of view studying the mechanism, inside the crystal, for the production of the signal and idler beams. We begin from the evolution equations for the quantum field operators, pass to the Wigner function and solve the resulting (Maxwell) equations with the use of the Green's function method. We derive the time dependence of the coincidence detection probability as a function of the parameters of the nonlinear crystal (in particular the length) the radius of the pumping beam, and the bandwidth of the filters in front of the detectors. Received 24 January 2000 and Received in final form 24 March 2000     

Modelling the diffraction of laser-cooled atoms from magnetic gratings

The diffraction of laser-cooled atoms from a spatially-periodic potential is modelled using rigorous coupled-wave analysis. This numerical technique, normally applied to light-diffraction, is adapted for use with atomic de Broglie waves incident on a reflecting diffraction grating. The technique approximates the potential by a large number of constant layers and successively solves the complex eigenvalue problem in each layer, propagating the solution up to the surface of the grating. The method enables the diffraction efficiencies to be calculated for any periodic potential. The results from the numerical model are compared with the thin phase-grating approximation formulae for evanescent light-wave diffraction gratings and idealised magnetic diffraction gratings. The model is applied to the problem of diffracting Rb atoms from a grating made from an array of permanent magnets. Received 13 June 2000 and Received in final form 15 December 2000     

Spectrum of the parametric down converted radiation calculated in the Wigner function formalism

We continue the study of parametric down conversion within the framework of the Wigner representation, by using a Maxwellian approach developed in a recent paper [A. Casado et al., Eur. Phys. J. D 11, 465 (2000)]. This gives a mechanism, inside the crystal, for the production of the down-converted radiation. We obtain the electric field to second order in the coupling constant by using the Green's function method, and compare our treatment with the standard Hamiltonian approach. The spectrum of the down-converted radiation is calculated as a function of the parameters of the nonlinear crystal (in particular the length) and the radius of the pumping beam. Received 15 May 2000     

Noiseless amplification of images in a confocal cavity

We study the noiseless amplification of an optical image by means of a confocal cavity containing a parametric medium. We demonstrate, in the ideal situation, the possibility of preserving the signal-to-noise ratio while amplifying uniformly the entire image. Some specific effects, which may degrade the performances of the scheme, are taken into account. Received 23 March 2000     

Quantum phase transition in the generalized single-mode superradiant model

In this paper we reveal a zero-temperature quantum phase transition for the single-mode superradiant model with the form A² from the normal to superradiant phase by mean of the Holstein-Primakoff transformation. In the thermodynamic limit, in which the numbers of atoms becomes infinite, the ground state energy and corresponding wavefunctions of both the normal and superradiant phases are obtained and therefore the scaling behavior near the critical transition point is derived.     

Effective quantum efficiency in the pulsed homodyne detection of a n-photon state

Homodyne detection can be used to perform measurements on various quantum states of the light, such as conditional single photon states produced by parametric fluorescence processes. In the pulsed regime, the time and frequency overlap between the single photon wave packet and the local oscillator field plays a crucial role. We show in this paper that this overlap can be characterized by an effective quantum efficiency, which is explicitly calculated in various situations of experimental interest. Received 27 July 2000 and Received in final form 29 November 2000     

Quantum chemical construction of a reduced reaction Hamiltonian and T 1 -relaxation and pure T 2 -dephasing rates for the proton transfer in 3-chlorotropolone

Separating multidimensional problems into that of a relevant system which is coupled to a bath of harmonic oscillators is a common concept in condensed phase theory. Focusing on the specific problem of intramolecular proton transfer in an isolated tropolone derivative, we consider the reactive proton moving in the plane of the molecule as the system and the remaining substrate normal modes as the bath. An all-Cartesian system-plus-substrate Hamiltonian is constructed employing density functional theory. It is then used to determine the temperature-dependent effective reduced reaction Hamiltonian and the state-to-state dissipation rates induced via the system-substrate coupling up to the bi-quadratic order. The important substrate modes for the T₁-relaxation and the pure T₂-dephasing rates, which are either intra- or inter-well in nature, are identified numerically and analyzed physically with molecular details. Received 19 November 2001 and Received in final form 19 February 2002     

General theory of population transfer by adiabatic rapid passage with intense, chirped laser pulses

We present a general theory of adiabatic rapid passage (ARP) with intense, linearly chirped laser pulses. For pulses with a Gaussian profile and a fixed bandwidth, we derive a rigorous formula for the maximum temporal chirp rate that can be sustained by the pulse. A modified Landau-Zener formula displays clearly the relationships among the pulse parameters. This formula is used to derive the optimal conditions for efficient, robust population transfer. As illustrations of the theory, we present results for two- and four-level systems, and selective vibronic excitation in the I₂ molecule. We demonstrate that population transfer with chirped pulses is more robust and more selective than population transfer with transform-limited pulses. Received 6 September 2000 and Received in final form 25 September 2000     

Relationships between a microscopic parameter and the stochastic equations for interface's evolution of two growth models

The relationship between a microscopic parameter p, that is related to the probability of choosing a mechanism of deposition, and the stochastic equation for the interface's evolution is studied for two different models. It is found that in one model, that is similar to ballistic deposition, the corresponding stochastic equation can be represented by a Kardar-Parisi-Zhang (KPZ) equation where both λ and ν depend on p in the following way: ν(p) = νp and λ(p) = λp ^3/2. Furthermore, in the other studied model, which is similar to random deposition with relaxation, the stochastic equation can be represented by an Edwards-Wilkinson (EW) equation where ν depends on p according to ν(p) = νp ². It is expected that these results will help to find a framework for the development of stochastic equations starting from microscopic details of growth models. Received 26 August 2002 / Received in final form 20 November 2002 Published online 6 March 2003 RID="a" ID="a"e-mail: ealbano@inifta.unlp.edu.ar     

Autocorrelation function of microcavity-emitting field in the linear regime

We study the photon statistics of the field emitted from a semiconductor microcavity containing a quantum well. We present an analytical expression of the autocorrelation function in non-resonant pumping. A dynamical behavior of the autocorrelation function depending of the detuning between exciton and cavity frequencies is discussed.