Ultrasonic detection of resonant cavitation bubbles in a flow tube by their second-harmonic emissions

During low-power exposures, biophysical effects of ultrasonic cavitation are induced primarily by resonant bubbles, and there is a need for a new method of detecting these small bubbles. Bubble pulsation theory indicates that second-harmonic emissions emanate from resonant bubbles even at low amplitudes. A device was constructed to detect resonant bubbles passing through it in a flowing liquid by monitoring second-harmonic responses to a low amplitude, 1.64 MHz ultrasonic field. During testing, 4.2 μm diameter resonant bubbles produced signals 40 times larger than 500 μm diameter bubbles, and this technique was much better than a first-harmonic scattering technique for counting resonant bubbles.     

Numerical 3D flow simulation of ultrasonic horns with attached cavitation structures and assessment of flow aggressiveness and cavitation erosion sensitive wall zones

As a contribution to a better understanding of cavitation erosion mechanisms, a compressible inviscid finite volume flow solver with barotropic homogeneous liquid–vapor mixture cavitation model is applied to ultrasonic horn set-ups with and without stationary specimen, that exhibit attached cavitation at the horn tip. Void collapses and shock waves, which are closely related to cavitation erosion, are resolved. The computational results are compared to hydrophone, shadowgraphy and erosion test data. At the horn tip, vapor volume and topology, subharmonic oscillation frequency as well as the amplitude of propagating pressure waves are in good agreement with experimental data. For the evaluation of flow aggressiveness and the assessment of erosion sensitive wall zones, statistical analyses of wall loads and of the multiplicity of distinct collapses in wall-adjacent flow regions are applied to the horn tip and the stationary specimen. An a posteriori projection of load collectives, i.e. cumulative collapse rate vs. collapse pressure, onto a reference grid eliminates the grid dependency effectively for attached cavitation at the horn tip, whereas a significant grid dependency remains at the stationary specimen. The load collectives show an exponential decrease towards higher collapse pressures. Erosion sensitive wall zones are well predicted for both, horn tip and stationary specimen, and load profiles are in good qualitative agreement with measured topography profiles of eroded duplex stainless steel samples after long-term runs. For the considered amplitude and gap width according to ASTM G32-10 standard, the analysis of load collectives reveals that the distinctive erosive ring shape at the horn tip can be attributed to frequent breakdown and re-development of a small portion of the tip-attached cavity. This partial breakdown of the attached cavity repeats at each driving cycle and is associated with relatively moderate collapse peak pressures, whereas the stationary specimen is rather unfrequently stressed at the end of each subharmonic oscillation cycle by the violent collapse of the complete cavity.     

Respective contribution of cavitation and convective flow to local stirring in sonoreactors

The knowledge of respective parts of convection and cavitation to the stirring induced by ultrasound at one exact position into a sonoreactor is useful for all processes implementing surfaces exposed to sonication. PIV measurement allows real fluid motion determination, whereas the electrochemical technique gives an equivalent flow velocity considered as the sum of all stirring contributions to the electrode. Thus, by a simple subtraction between real fluid velocity and equivalent flow velocity, it is possible to identify the contribution of each phenomenon. Applied to low frequency reactors, it had been observed that cavitation is the preponderant phenomenon, with a contribution of stirring close to the electrode always more than 90%. High frequency reactors, frequently known to produce less cavitation, have shown that at the focal zone, if it concerns HIFU, cavitation becomes preponderant and reaches similar values to those close to the ultrasonic horn in low frequency sonoreactors.     

Luminescence intensity of vortex cavitation in a Venturi tube changing with cavitation number

Hydrodynamic cavitation in a Venturi tube produces luminescence, and the luminescence intensity reaches a maximum at a certain cavitation number, which is defined by upstream pressure, downstream pressure, and vapor pressure. The luminescence intensity of hydrodynamic cavitation can be enhanced by optimizing the downstream pressure at a constant upstream pressure condition. However, the reason why the luminescence intensity increases and then decreases with an increase in the downstream pressure remains unclear. In the present study, to clarify the mechanism of the change in the luminescence intensity with cavitation number, the luminescence produced by the hydrodynamic cavitation in a Venturi tube was measured, and the hydrodynamic cavitation was precisely observed using high-speed photography. The sound velocity in the cavitating flow field, which affects the aggressive intensity of the cavitation, was evaluated. The collapse of vortex cavitation was found to be closely related to the luminescence intensity of the hydrodynamic cavitation. A method to estimate the luminescence intensity of the hydrodynamic cavitation considering the sound velocity was developed, and it was demonstrated that the estimated luminescence intensity agrees well with the measured luminescence intensity.     

Experimental study of the cavitation noise and vibration induced by the choked flow in a Venturi reactor

In this paper, the cavitation performance and corresponding pressure pulsation, noise and vibration induced by the choked cavitating flow in a Venturi reactor are investigated experimentally under different cavitation conditions by using high-speed camera and high frequency sensors. Based on the instantaneous continuous cavitation images, the Proper Orthogonal Decomposition (POD), a tool to analyze the large-scale cavitation flow structure, is applied to investigate the choked cavitating flow dynamics. The POD results show that two mechanisms, re-entrant jet flow mechanism and shock wave mechanism, govern the shedding and collapse of cavitation cloud at different pressure ratios. These mechanisms contribute to the variation of pressure pulsation, noise and vibration at different pressure ratios. The pressure pulsation spectrum behaves differently in various cavitation regions induced by the choked cavitating flow. Due to the existence of low pressure in re-entrant region, the influence of high frequency fluctuation on pressure pulsation caused by re-entrant flow is small. Moreover, with the increase of pressure ratio, the induced noise and vibration intensity decreases gradually, then increases and reaches a maximum value. Finally, it drops to a low and stable level. Despite different inlet pressures, the intensity of cavitation noise and vibration reaches the maximum value at the same pressure ratio. Specifically, the FFT analysis of noise and vibration signals indicates that low frequency component prevails at small pressure ratio owing to the re-entrant jet mechanism, while high frequency component prevails at large pressure ratio owing to the shock wave mechanism. The relationship between the choked cavitation dynamics and the induced pressure pulsation, noise and vibration in the Venturi reactor is highlighted. The results can provide guidance for the optimal operation condition of the Venturi reactor for cavitation applications such as water treatment.     

Effect of fluid flow on cavitation erosion of materials under exposure to vibrations from a hydrodynamic generator

The results of investigation of cavitation erosion of lead in various places of a hydrodynamic-generator submerged jet are presented. Features of erosion caused by the effect of flow are established. It can both strengthen the erosion intensity and weaken it in dependence on the angle of incidence. The stratification of air bubbles under the action of pressure waves is possible in the flow under the interaction with the surface of objects. The flow can change the number of air bubbles participating in the cavitation near the surface. It can also influence the mechanical effect on the surface of the tested materials inducing their nonuniform deformation. All the factors listed affect the cavitation erosion complicating considerably the physics of the process.     

Waveform analysis of cavitation in a globe valve

Cavitation is a dynamic phenomenon occurring in fluid flows, where the local static pressure is lower than the saturated vapor pressure at working temperature. The growth and collapse of cavitation bubbles leads to corrosion and pitting of metal surfaces. Considering the fact that erosion by cavitation is still one of the current problems, it is important to detect the initiation, fully developed point of cavitation and to analyze its characteristics. In this research, an attempt is made to study acoustic waveform of cavitation in the globe valve. The waveform is transformed by Fast Fourier Transform and its important parameters such as amplitude, energy, frequency and so on are analyzed.     

Quantitative observations of cavitation activity in a viscoelastic medium

Quantitative experimental observations of single-bubble cavitation in viscoelastic media that would enable validation of existing models are presently lacking. In the present work, single bubble cavitation is induced in an agar gel using a 1.15 MHz high intensity focused ultrasound transducer, and observed using a focused single-element passive cavitation detection (PCD) transducer. To enable quantitative observations, a full receive calibration is carried out of a spherically focused PCD system by a bistatic scattering substitution technique that uses an embedded spherical scatterer and a hydrophone. Adjusting the simulated pressure received by the PCD by the transfer function on receive and the frequency-dependent attenuation of agar gel enables direct comparison of the measured acoustic emissions with those predicted by numerical modeling of single-bubble cavitation using a modified Keller-Miksis approach that accounts for viscoelasticity of the surrounding medium. At an incident peak rarefactional pressure near the cavitation threshold, period multiplying is observed in both experiment and numerical model. By comparing the two sets of results, an estimate of the equilibrium bubble radius in the experimental observations can be made, with potential for extension to material parameter estimation. Use of these estimates yields good agreement between model and experiment.     

The dynamics of cavitation bubbles in a sealed vessel

A model of cavitation bubbles is derived in liquid confined in an elastic sealed vessel driven by ultrasound. In this model, an assumption that the pressure acting on the sealed vessel due to bubble pulsations is proportional to total volume change of bubbles is made. Numerical simulations are carried out for a single bubble and for bubbles. The results show that the pulsation of a single bubble can be suppressed to a large extent in sealed vessel, and that of two matched bubbles with same ambient radius can be further suppressed. However, when two mismatched bubbles have the same ambient radii, an interesting breathing phenomenon takes place, where one bubble pulsates inversely with the other one. Due to this breathing phenomenon the suppression effect becomes weak, so the maximum radii of two mismatched bubbles can be larger than that of a single bubble or that of two matched bubbles in sealed vessel. Besides that, for two mismatched bubbles with different ambient radii, the small one in sealed vessel under some certain parameters can pulsate as strong as or even stronger than that of a single bubble in an open vessel.     

Investigation of acoustic cavitation energy in a large-scale sonoreactor

Acoustic cavitation energy distributions were investigated for various frequencies such as 35, 72, 110 and 170 kHz in a large-scale sonoreactor. The energy analyses were conducted in three-dimensions and the highest and most stable cavitation energy distribution was obtained not in 35 kHz but in 72 kHz. However, the half-cavitation-energy distance was larger in the case of 35 kHz ultrasound than in the case of 72 kHz, demonstrating that cavitation energy for one cycle was higher for a lower frequency. This discrepancy was due to the large surface area of the cavitation-energy-meter probe. In addition, 110 and 170 kHz ultrasound showed a very low and poor cavitation energy distribution. Therefore larger input power was required to optimize the use of higher frequency ultrasound in the sonoreactor with long-irradiation distance. The relationship between cavitation energy and sonochemical efficiency using potassium iodide (KI) dosimetry was best fitted quadratically. From 7.77 × 10^?10 to 4.42 × 10^?9 mol/J of sonochemical efficiency was evaluated for the cavitation energy from 31.76 to 103. 67 W. In addition, the cavitation energy attenuation was estimated under the assumption that cavitation energy measured in this study would be equivalent to sound intensity, resulting in 0.10, 0.18 and 2.44 m^?1 of the attenuation coefficient (α) for 35, 72 and 110 kHz, respectively. Furthermore, α/(frequency)² was not constant, as some previous studies have suggested.     

Dynamics of a cavitation bubble near a solid wall

The cavitation bubble dynamics, the variation of pressure and velocity fields of the surrounding liquid in the process of the bubble axisymmetric compression near a planar solid wall are considered. It is assumed that the liquid is at rest at the initial moment of time, and the bubble has a spheroidal shape. The liquid is assumed inviscid and incompressible, its motion being potential. The bubble surface deformation and the liquid velocity on the surface are computed by the Euler scheme using the boundary element method until the moment of the collision of some parts of the bubble surface with one another. The influence of the distance of the bubble from the wall and its initial nonsphericity on the liquid pressure and velocity fields, the bubble shape, and the pressure inside the bubble at the end of the time interval under consideration are studied. The maximum pressure in liquid is shown to realize at the bottom of the cumulative jet arising at the bubble collapse with direction to the wall. In the upper part of this jet, the velocity and pressure are practically constant, and the pressure in the jet is approximately equal to the pressure in the bubble.     

Activation of mononuclear bone marrow cells treated in vitro with a complex homeopathic medication

Canova is a Brazilian homeopathic medication with immunomodulatory properties, recommended for patients where the immune system is depressed. Previous studies demonstrated that Canova induces up-regulation in numbers of leukocytes. The bone marrow microenvironment is composed of growth factors, stromal cells, extracellular matrix and progenitor cells that differentiate into mature blood cells. We now report the effect of in vitro administration of the medication on the mononuclear differentiation of the bone marrow cell. Swiss mice femurs were dissected cleaned and the cells of the marrow were flushed. The cells were plated, treated or not, incubated for different times and processed for light, transmission and scanning electron, and confocal microscopy analysis. Bone marrow cells showed an enhanced proliferation in vitro in response to Canova medication and Canova plus M-CSF and an increase was also observed in the numbers of the cell niches and ring-shaped nuclei cells. Confocal and transmission and scanning electron microscopy showed the stages of monocyte maturation, with resting and activated cells. With Canova treatment there was a marked increase in cell size, which is mainly attributable to the augmented cytoplasm, an increase in the number of mitochondria, expansion of the RER and an enlarged Golgi. The response to Canova treatment indicates that it influences mononuclear differentiation and activation of bone marrow progenitor and stromal cells.     

混响场中脉冲超声空化效应的研究

本文实验研究了不同脉冲宽度的８２０ｋＨｚ超声波的空化效应，结果得出，空化致自基产量随脉冲宽度及声强呈现规律性变化，尤其观察到了“脉冲空化峰”现象，本文从液面受迫振动角度出混响场中“脉冲空化峰”现象的机制。     

Acoustic cavitation mechanism: a nonlinear model

During acoustic cavitation process, bubbles appear when acoustic pressure reaches a threshold value in the liquid. The ultrasonic field is then submitted to the action of the bubbles. In this paper we develop a model to analyze the cavitation phenomenon in one-dimensional standing waves, based on the nonlinear code SNOW-BL. Bubbles are produced where the minimum rarefaction pressure peak exceeds the cavitation threshold. We show that cavitation bubbles appear at high amplitude and drastically affect (dissipation, dispersion, and nonlinearity) the ultrasonic field. This paper constitutes the first work that associates the nonlinear ultrasonic field to a bubble generation process.     

Noise as an indicator of cavitation in a centrifugal pump

One of the sources of instability in a centrifugal pump is cavitation within the pump. Cavitation of a centrifugal pump is the result of insufficient net positive suction head (NPSH) and can occur within the entire range of operating conditions. Cavitation may cause three different and undesirable effects: (1) a drop in head-capacity and efficiency curves, (2) damage to the impeller by pitting and erosion, and (3) structure vibration and resulting noise. Therefore, the cavitation process must be prevented by all means. To prevent the onset of cavitation we have to detect the beginning of the cavitation process in the pump. To detect the beginning of the cavitation process, the emitted noise can be used, among other possibilities. Specifically, a noise spectra structure can be used to detect the beginning of cavitation and its development. Experiments have shown that there is a discrete frequency tone, at 147 Hz, which is strongly dependent on the cavitation process and its development. Therefore, noise spectra can also be used to determine the NPSH required or the critical value, representing the upper limit of the permissible pump operation without cavitation.     

Surface damage as a result of cavitation erosion

Erosion is regarded as a result of the periodic loading of a surface with spherical waves generated at the sites of the collapse of cavitation bubbles. One feature of cavitation loading is the formation of a zone of intense failure at the center of the contact surface. Damage appears a consequence of the formation of longitudinal cleavage cracks under the contact zone, which comprise a system of small annular cracks coaxial to a deep channel crack. The damage zone (blister) occupies a small fraction of the crater surface (the contact zone with the shock wave). The depth of the longitudinal cracks is an order of magnitude smaller than the thickness of the hardened layer. The hardening and erosion processes occur simultaneously. Zh. Tekh. Fiz. 68, 110–114 (September 1998)     

Simulations of a full sonoreactor accounting for cavitation

In spite of the increasing interest in ultrasound processing applications, industrial scale-up remains limited, in particular by the unavailability of predictive computer tools. In this study, using a previously published model of cavitating liquids implementable as a non-linear Helmholtz equation, it is shown that a full sonoreactor can be modelled and simulated. The model includes the full transducer and the vibrations of the vessel walls, using the physics of elastic solids and piezo-electricity. The control-loop used by the generator to set the optimal frequency is also accounted for. Apart from the geometry, the unique input of the model is the current feeding the transducer whereas the dissipated electrical power, transducer complex impedance and working frequency are available as outputs. The model is put to the test against experiments realized in different geometries, varying either the input current or the transducer immersion depth. Despite the overestimation of the power dissipated in the liquid, the evolution of the acoustic load in both cases is reasonably well reproduced by simulation, which partially validates the method used.