Theory of 2×2 switch based on electro-optic and piezoelectric effects in photorefractive LiNbO3 crystal

Based on the electro-optic and piezoelectric effects, the principle of a 2×2 bypass-exchange switch in photorefractive LiNbO₃ crystal is discussed. In photorefractive volume grating, the Bragg condition can be changed by applying a field during readout. That is, by applying a specific field E_s or zero, the diffraction efficiency will be 0 or 1, respectively and this property can be used to realize the bypass or exchange operation of the switch. In this paper, considering both the piezoelectric and electro-optic effects caused by the applied electric field, we analyzed relations of both the specific field and the incident intensity ratio with respect to the writing angles and polarizations of writing beams.     

光折变晶体LiNbO_3:Fe中的特殊散射现象

用柱面透镜把经针孔滤波器扩束的激光束沿某一个方向聚焦成细丝状(或长条状),细丝状光束垂直入射到LiNbO_3:Fe晶体上,在远场位置观察散射光.我们发现光散射的方向与晶体的c轴方向不一致,不仅沿着晶体的c轴方向有散射光出现,沿光束的条形方向也出现很强的散射光.     

Ultraviolet photorefractive effect in Mg-doped near-stoichiometric LiNbO3

The ultraviolet photorefractive effect of Mg-doped near-stoichiometric LiNbO₃ crystals prepared by vapor transport equilibration (VTE) technique was studied at 351 nm. It was found in the near-stoichiometric LiNbO₃ crystals that the ultraviolet photorefractive effect could be enhanced greatly with the increase of Mg concentration. Based on the activation energy of dark decay of the photorefractive grating, possible centers responsible for the ultraviolet photorefractive effect were also discussed.     

Holographic angle multiplexing combined with peristrophic multiplexing in a photorefractive LiNbO3 crystal

We have investigated angle multiplexing combined with peristrophic (rotational) multiplexing in a photorefractive LiNbO₃ crystal of cylindrical shape. The peristrophic multiplexing was achieved by rotating the recording medium while the angle multiplexing, by varying the incident angle of the reference beam. Angle multiplexing in synchronization with rotation of the sample made it possible to continuously record and retrieve holograms. In the combined multiplexing, holograms were stored at different peristrophic positions and thus their angular selectivity could be much improved in comparison to that of only angle-multiplexed holograms. The theoretical angular selectivity was derived, along with its dependence on the sample rotation. The experimentally measured selectivity was in agreement with the theoretical one. The angular selectivity of angle-multiplexed holograms was measured to be 0.03° in the absence of sample rotation and it became less than 0.0075° with a sample rotation by 5.4°.     

Anisotropic diffraction of stratified volume holographic grating in photorefractive media

We have studied the anisotropic diffraction properties of the stratified volume holographic gratings recorded in photorefractive media using the anisotropic coupled wave theory. It is shown that the diffraction efficiency of such system exhibit the uniform periodic Bragg selectivity properties. In addition the dependence of the stratified volume holographic optical elements (SVHOEs) diffraction properties on the buffer-layer thickness, grating-layer thickness, number of modulation layers, and total thickness of system are discussed in detail.     

Hyper-Raman scattering in the LiNbO3 crystal

The hyper-Raman spectra in non-centrosvmmetric LiNbO₃ crystal were obtained using the multichannel recording technique. The hyper-Raman cross-section and non-linear susceptibility for the 151 cm^-1 band were measured.     

New experimental evidence of the structural modification in single crystal Bi2Sr2CaCu2Oy by X-ray diffraction observation

The variations of the high angle 00 peak-shape by means of X-ray l scans of the 00l fundamental reflections were investigated in detail for a highly oriented Bi₂Sr₂CaCu₂O_y (Bi2212) crystal with sufficiently small intrinsic mosaicity and the same crystal annealed in air at 250, 300, 400, 600, and 750°C for 20 h in consequence. For the first time, we observed a new additional reflection almost overlapped original 00l fundamental reflection at annealing temperature below 400°C by X-ray diffraction measurement, which shows that there coexisted two sets of lattice periodicity in the c-direction of the annealed crystal. The new additional reflection appeared at 250°C and disappeared at 400°C. Its intensity was increased at 300°C. The measurements of the AC susceptibility, c-axis parameter and full width at half maximum (FWHM) of the 00 peaks showed that the new additional reflection was associated with the oxygen diffusion in CuO₂ planes and the changes of strain field. The results provide the new experimental evidence that the structural distortion is more sensitive to the oxygen diffusion in CuO₂ planes than to that in Bi–O layers.     

Lateral-field-excitation properties of LiNbO3 single crystal

LiNbO 3 has been found attractive for lateral field excitation (LFE) applications due to its high piezoelectric coupling. In this paper, bulk acoustic wave propagation properties for LiNbO 3 single crystal excited by a lateral electric field have been investigated using the extended Christoffel-Bechmann method. It is found that the LFE piezoelectric coupling factor for c mode reaches its maximum value of 95.46% when ψ = 0 for both (yxl)-58 and (yxwl)±60 /58 LiNbO 3 . The acoustic wave phase velocity of c mode TSM (thickness shear mode) changes from 3456 m/s to 3983 m/s as a function of ψ. Here ψ represents the angle between the lateral electric field and the crystallographic X-axis in the substrate major surface. A 5 MHz LFE device of (yxl)-58 LiNbO 3 with ψ = 0 was designed and tested in air. A major resonance peak was observed with the motional resistance as low as 17 and the Q-factor value up to 10353. The test result is well in agreement with the theoretical analysis, and suggests that the LFE LiNbO 3 device can be a good platform for high performance resonator or sensor applications.     

Actively Q-switched intracavity second-harmonic generation of 1.06 μm in BiB3O6 crystal

We have investigated the acousto-optically Q-switched intracavity second-harmonic generation of 1.06 μm in a 1.9-mm-long BiB₃O₆ crystal, cut for type-I phase-matching direction of (θ,)=(168.9°,90°), performed in a diode-end-pumped Nd:YVO₄ laser. When the incident pump power was 4.3 W at 30 kHz of pulse repetition frequency, a maximum average green output power of 480 mW, the shortest pulse with FWHM width of 72 ns, the highest single pulse energy of 16 μJ and the maximum peak power of 222 W were obtained, giving the corresponding optical conversion efficiency of 11.2%. The effect of varying temperature in BIBO crystal on the average green output power was also investigated.     

Optical waveguide engraving in a LiNbO3 crystal fiber

This paper reports the engraving of an optical waveguide inside a LiNbO₃ crystal fiber via the photorefractive effect and an optical vortex. Afterwards this waveguide was successfully tested and its properties evidenced.     

二维LiNbO3非线性光子晶体

制备了周期为13.64 μm方形格子二维周期性极化的LiNbO₃，利用二阶准相位匹 配实现了波长为1.064μm二倍频，二次谐波的内部转换效率高达42％. 测量了二次谐波输出功率随晶体温度及入射光入射方向的变化，实验值与模拟计算一致. 制备二阶准相位匹配掩模板，解决了在制备一阶准相位匹配掩模板中遇到周期尺寸太小、数据量大的难题，同时还降低了因周期太小造成的极化难度. 关键词： 二维 准相位匹配 二次谐波     

Out-of-plane low field anisotropic magnetoresistance in Nd0.51Sr0.49MnO3 thin films

A comparative study of the out-of-plane anisotropic magnetoresistance (AMR) in single crystalline and polycrystalline thin films of phase separated manganite Nd_0.51Sr_0.49MnO₃ has been carried out. On-axis DC magnetron sputtering was used to deposit the single crystalline films (30 and 100 nm in thickness) on single crystal (0 0 1) LaAlO₃ (LAO) and polycrystalline films (100 nm) on (1 0 0) Yttrium-stabilized ZrO₂ (YSZ) substrates. The in-plane and out-of-plane magnetotransport properties of these films differ significantly. A large low field AMR is observed in all the films. AMR shows a peak below the insulator-metal transition temperature in the single crystalline films, while the same increases monotonically in the polycrystalline film. Relatively larger low field AMR (∼20% at T=78 K and H=1.7 kOe) in the polycrystalline films suggests the dominance of the shape anisotropy.     

The diamagnetic susceptibilities of donors in quantum wells with anisotropic effective mass

The diamagnetic susceptibility of a hydrogenic donor placed in Si, Ge and GaAs quantum wells with infinite confinement potential which have different effective mass anisotropy parameters (γ=_m⊥/_m∥$\gamma =m_{\perp }/m_{\parallel }$) has been investigated as a function of the well sizes. The binding energies of the donor have also been computed using a trial wave function with two parameters in the framework of the effective mass approximation. It has been observed that the diamagnetic susceptibility of the donor in the anisotropic materials converges rapidly to the bulk limit as the well size increases.     

双掺杂LiNbO3:Fe:Mn体全息光栅的时空衍射特性

通过联立求解两中心带输运物质方程和双光束耦合波方程，建立了研究双掺杂LiNbO_{3< /sub>:Fe:Mn晶体采用双色光记录光折变体全息的时空特性的动力学模型.数值计算表明，该动态体全息光栅的时空衍射特性与晶体中的折射率光栅相对于干涉场的空间相移有关，该空间相移的取值范围为(-π，π)，当空间相移的符号发生变化时，双光束之间的能量耦合方向也相应地发生反转.给出了晶体内的等相位线和光强的重新分布.}     

Spectroscopic analysis of Er transition in Mg/Er-codoped LiNbO3 crystal

We present a Judd-Ofelt spectroscopic analysis on the Mg/Er-codoped congruent lithium niobate (LiNbO₃) crystals. The Judd-Ofelt model is applied to the room temperature unpolarized absorption intensities of Er³⁺ ions on eleven transition bands to determine their intensity parameters: Ω₂=2.36×10⁻²⁰ cm², Ω₄=0.76×10⁻²⁰ cm², Ω₆=0.30×10⁻²⁰ cm² in Er:LiNbO₃ crystal heavily codoped with MgO. The radiative lifetime of ²H_9/2 becomes longer when MgO is added into Er:LiNbO₃ crystal. The experimental lifetimes are obtained using microsecond time-resolved spectra at 400 nm femtosecond pulse excitation to predict radiative quantum efficiency. Combining higher radiative quantum efficiency with longer radiative lifetime, we conclude that Mg/Er-codoped LiNbO₃ crystals are more suitable than Er: LiNbO₃ ones in laser materials.     

Nonvolatile photorefractive holographic recording in Sc:Ce:Cu:LiNbO3

In this paper experimental studies of nonvolatile photorefractive holographic recording in Ce:Cu:LiNbO₃ crystals doped with Sc(0,1,2,3 mol%) were carried out. The Sc:Ce:Cu:LiNbO₃ crystals were grown by the Czochralski method and oxidized in Nb₂O₅ powders. The nonvolatile holographic recording in Sc:Ce:Cu:LiNbO₃ crystals was realized by the two-photon fixed method. We found that the recording time of Sc:Ce:Cu:LiNbO₃ crystal became shorter with the increase of Sc doping concentration, especially doping with Sc(3 mol%), which exceeds the so-called threshold, and there was little loss of nonvolatile diffraction efficiencies between Sc(3 mol%):Ce:Cu:LiNbO₃ and Ce:Cu:LiNbO₃ crystals.     

Anisotropic Bragg diffraction of finite-sized volume holographic grating in photorefractive crystals

Anisotropic diffraction of uniform plane wave by finite-sized volume holographic grating in photorefractive crystals is considered. It is found that the anisotropic diffraction can take place when some special conditions are satisfied. The diffracted image is obtained in experiment for the anisotropic Bragg diffraction in Fe:LiNbO₃ crystals. A coupled wave analysis is presented to study the properties of anisotropic diffraction. An analytical integral solution for the amplitudes of the diffracted beams is submitted. A trade off between high diffraction efficiency and the deterioration of reconstruction fidelity is analyzed. Numerical evaluations also show that the finite-sized anisotropic volume grating exhibits strong angular and wavelength selectivity. All the results are useful for the optimizing design of VHOE based on finite-sized volume grating structures.     

Neutron and X-ray diffraction studies on the Tb2Ni3Si5 single crystal

Neutron and X-ray diffraction studies on the Tb₂Ni₃Si₅ single crystal have been done to investigate its crystal modulation and magnetic properties. The modulated single crystal is constructed by the TbNiSi₂ (CeNiSi₂-type Cmcm) and the Tb₂Ni₃Si₅ (U₂Co₃Si₅-type Ibam) lattices. The relationship between the two lattices is described as direction of the b₁₁₂-axis coincides with the a₂₃₅-axis. The crystal modulation gives significant effects on magnetism. Each of the two lattices takes complex antiferromagnetism with multiplex propagation vectors.     

Direct comparison of anisotropic magnetoresistance and planar Hall effect in epitaxial Fe3O4 thin films

The angular dependence of anisotropic magnetoresistance (AMR) and planar Hall effect (PHE) were studied as a function of temperatures from the same epitaxial Fe₃O₄ film on MgO(001) substrates. The PHE contains only a twofold angular dependence, but the AMR below 200 K is constituted with both twofold and fourfold symmetric terms. Our results also prove that the origin of the fourfold symmetry of AMR is related to the lattice symmetry rather than the spin scattering near the antiphase boundaries.     

Widely phase-matched tunable difference-frequency generation in periodically poled LiNbO3 crystal

We report on the development of a laser source in the mid-infrared spectral region based on difference-frequency generation (DFG) in a periodically poled LiNbO₃ (PPLN) crystal. Continuously tunable coherent radiation from 2.75 to 4.78 μm was produced by optical parametric interaction between a diode-pumped monolithic continuous-wave (CW) Nd:YAG laser operating at 1.064 μm and a CW Ti:Sapphire laser tunable from 767 to 871 nm. Temperature-dependent quasi-phase-matched DFG wavelength acceptance bandwidth was studied and characterized. An empiric formula is given to estimate the phase-matched wavelength acceptance bandwidth as a function of the crystal temperature at Λ = 22.5 μm. A large frequency scan of 128 cm⁻¹ (about 78 cm⁻¹ above 1 μW) near 4.2 μm was achieved. The whole absorption spectrum of the P and R branches of the ν₃ band of atmospheric carbon dioxide has been recorded with a single phase-matched frequency scan.