Absorption of ultrashort laser pulses in strongly overdense targets

Absorption measurements on solid conducting targets have been performed in s and p polarization with ultrashort, high-contrast Ti:sapphire laser pulses at intensities up to 5x10{16}W/cm{2} and pulse duration of 8 fs. The particular relevance of the reported absorption measurements lies in the fact that the extremely short laser pulse interacts with matter close to solid density during the entire pulse duration. A pronounced increase of absorption for p polarization at increasing angles is observed reaching 77% for an incidence angle of 80 degrees . Simulations performed using a 2D particle in cell code show a very good agreement with the experimental data for a plasma profile of L/lambda approximately 0.01.     

Femtosecond X-ray line emission from multilayer targets irradiated by short laser pulses

The invention of high-power, ultra-short-pulse lasers has opened the way to investigations aimed at the creation of a new type of bright X-ray source for various uses including material science applications and time-resolved X-ray diffraction for biology. The efficiency with which laser energy incident on a solid target is converted into an X-ray emission depends on many factors, including the temporal profile of the laser pulse. Here we report the results of our theoretical and experimental investigations of the line X-ray emission from layered solid targets irradiated by ultra-short laser pulses. The laser prepulse parameters and target thickness are optimized to convert the maximum laser energy into an emission in the selected X-ray line. Multilayer foils are proposed to increase the energy of the K-line emission from laser plasma while simultaneously keeping the X-ray pulse duration at a hundred femtoseconds. The emission is studied both experimentally and theoretically by means of an analytical model and numerical simulations. PACS 52.38.Ph; 52.38.Dx; 52.50.Jm     

X-ray production by irradiation of solid targets with sub-picosecond excimer laser pulses

A table-top excimer laser system generating sub-ps pulses was used to irradiate solid targets at intensities of up to 4×10¹⁵ W/cm². Soft X-ray spectra of various materials were measured. The X-ray conversion efficiencies were between 1–5%. Streak camera measurements showed instrument-limited X-ray pulse duration of a few ps.Partially based on the plenary talk X-Ray Generation by Sub-Picosecond UV Laser by F. P. Schäfer, G. Kühnle, S. Szatmári, and M. Steyer, presented at the XVI Int. Quant. Electron. Conf., Tokio, July 18–21, 1988, Technical Digest (The Japan Society of Applied Physics) p. 2     

Generation of harmonics during the interaction of ultrashort superstrong laser pulses with solid targets

Generation of even and odd harmonics in the skin layer formed during the interaction of a short relativistic laser pulse with solid targets is considered. The complex motion of free electrons in the skin layer along the electric field vector and along the direction of propagation of a laser wave is analyzed. The Fourier expansion of the trajectory of this motion is used to obtain the components of the conductivity tensor and of the amplitude of the transverse electromagnetic field of harmonics propagating along the electric field. Even harmonics appear due to relativistic effects. The efficiency of generation of even and odd harmonics at the leading front of a laser pulse is calculated.     

Measurement of the energy penetration depth into solid targets irradiated by ultrashort laser pulses

The energy penetration depth of a short (100 fs) Ti-sapphire laser pulse (0.8 &mgr;m) of intensity 3x10(16) W/cm(2), in solid density materials has been measured. High-Z (BaF2) and low-Z (MgF2) solid layers targets were used. The penetration depth was determined from the measurement of the x-ray emission spectra, as a function of the target thickness. The investigation of these spectra showed that in the low-Z case, solid density material to a depth of 50 nm was heated to a peak electron temperature of approximately 150 eV. For the high-Z material, the penetration depth corresponding to this temperature exceeded 100 nm. This is evidence of a larger heat penetration depth in a high-Z material in comparison to a low-Z material. A model based on electron heat conduction is used to estimate the energy penetration depth. It is suggested that the larger heat penetration in high-Z material is due to heating of the material, caused by the radiation flux, generated by the electron heat conduction.     

Electron acceleration by a short relativistic laser pulse at the front of solid targets

Acceleration of electrons in a low-density plasma in front of a solid target by a propagating short ultraintense laser pulse is studied. When the laser is reflected at the target surface the accelerated electrons, with energy scaling as the laser intensity, continue to move forward inertially and thus escape from the pulse. Electrons accelerated backwards by the reflected light can attain even higher energies due to their longer acceleration length and their high initial momentum from a relativistic return current.     

Floquet theory for short laser pulses

We develop adiabatic perturbation theory for quantum systems responding to short laser pulses, with or without a frequency chirp. Our approach rests on lifting the time-dependent Schr?dinger equation to an extended Hilbert space, then applying standard perturbational techniques to Floquet states in this extended space, and finally projecting back to the physical Hilbert space. The same strategy also allows us to construct superadiabatic bases for monitoring the quantum evolution in the course of a pulse. These bases provide a diagnostic tool for improving the efficiency of pulse-induced population transfer. The formalism is applied to the selective excitation of molecular vibrational states by chirped laser pulses, which exploit either successive single-photon resonances or a multiphoton resonance, and by a STIRAP-like process. Received: 23 June 1998 / Revised: 18 August 1998 / Accepted: 25 August 1998     

Processing of metals by double pulses with short laser pulses

Experimental results related to the influence of time delayed pulses for ablation efficiency with short multi pulses (pulse duration of 5 ps) are reported. A significant improvement of the micro structuring quality at relatively high fluence regime in metals is obtained. Less removed or recast matter is observed and the processed surface appears to be smoother with better roughness. Ablation depths and burr heights are compared for single pulses and double pulses in steel, Al and Cu as a function of scans number. Best results are obtained for weak time delays, typically less than 1 ps. PACS 79.20.Ds; 42.62.Cf; 81.65.Cf     

Plasma heating with very short laser pulses

In experiments with laser produced plasmas there we have obtained d-d neutrons with help of both nanosecond and picosecond laser pulses. The possibility of plasma heating by 10⁻¹²–10⁻¹⁴ sec laser pulses is discussed, considering turbulent heating mechanisms. The expected neutron yield and electromagnetic radiation are evaluated.     

Absorption of subpicosecond ultraviolet laser pulses in high-density plasma

The absorption of 250 fs KrF laser pulses incident on solid targets of aluminum, copper and gold has been measured for normal incidence as a function of laser intensity in the range of 10¹²–10¹⁴ W cm^–2 and as a function of polarization and angle of incidence for the intensity range of 10¹⁴–2.5×10¹⁵ W cm^–2. As the intensity increases from 10¹² W cm^–2 the reflectivity at normal incidence changes from the low-intensity mirror reflectivity value to values in the range of 0.5–0.61 at 10¹⁴ W cm^–2. For this intensity maximum absorption of 63–80% has been observed for p-polarized radiation at angles of incidence in the range of 54°–57°, increasing with atomic number. The results are compared with the expected Fresnel reflectivity from a sharp vacuum-plasma interface with the refractive index given by the Drude model and also to numerical calculations of reflectivity for various scale length density profiles. Qualitative agreement is found with the Fresnel/Drude model and quantitative agreement is noticed with the numerical calculations of absorption on a steep density profile with normalized collision frequencies, v/, in the range of 0.13–0.15 at critical density and normalized density gradient scale lengths, L/₀, in the range of 0.018–0.053 for a laser intensity of 10¹⁴ W cm^–2.At 2.5×10¹⁵ W cm^–2 a small amount of preplasma is present and maximum absorption of 64–76% has been observed for p-polarized radiation at angles of incidence in the range of 45°–50°.Dedicated to Prof. Dr. Rudolf Wienecke on the occasion of his 65^th birthdayOn leave from: Department of Electrical Engineering, University of Alberta, Edmonton, T6G 2G7, Canada     

Reaching the nonlinear regime of Raman amplification of ultrashort laser pulses

The intensity of a subpicosecond laser pulse was amplified by a factor of up to 1000 using the Raman backscatter interaction in a 2 mm long gas jet plasma. The process of Raman amplification reached the nonlinear regime, with the intensity of the amplified pulse exceeding that of the pump pulse by more than an order of magnitude. Features unique to the nonlinear regime such as gain saturation, bandwidth broadening, and pulse shortening were observed. Simulation and theory are in qualitative agreement with the measurements.     

Interaction of short laser pulses with biological structures

Focusing of light pulses emitted by a Q-switched laser, which have a duration of some nanoseconds, into a medium leads to laser-induced breakdown. The shockwaves produced by this propagate through the medium and can interact with inhomogeneities situated within the medium and consequently cause destruction. Because of the increasing interest in these short light pulses in the medical field the interaction of the shockwaves with biological tissue has been investigated. The observed results indicate the influence of two physical quantities of the shockwave: the peak pressure and the duration.     

On the interaction of femtosecond laser pulses with cluster targets

The heating of clusters by femtosecond laser pulses is studied theoretically and experimentally. Both the formation of a cluster target and the results of experimental studies of the cluster plasma by the methods of X-ray emission spectroscopy are considered. A numerical model of cluster formation in a supersonic gas jet is proposed. It is shown that detailed studies of two-phase gas-dynamic processes in a nozzle forming the jet give the spatial distributions of all parameters required for the correct calculation of the cluster heating by short laser pulses. Calculations of nozzles of different configurations show that in a number of cases an almost homogeneous cluster target can be formed, whereas in other cases the distributions of parameters prove to be not only inhomogeneous but also even nonmonotonic. A simple physical model of the plasma production by a femtosecond laser pulse and a picosecond prepulse is proposed. It is shown that a comparison of X-ray spectra with detailed calculations of the ion kinetics makes it possible to determine the main parameters of the plasma being produced.     

Molecular alignment by trains of short laser pulses

We show that a dramatic field-free molecular alignment can be achieved after exciting molecules with proper trains of strong ultrashort laser pulses. Optimal two- and three-pulse excitation schemes are defined, providing an efficient and robust molecular alignment. This opens new prospects for various applications requiring macroscopic ensembles of highly aligned molecules.     

Detuned raman amplification of short laser pulses in plasma

The recently proposed scheme of so-called "fast compression" of laser pulses in plasma can increase peak laser intensities by 10(5) [Phys. Rev. Lett. 82, 4448 (1999)]. The compression mechanism is the transient stimulated Raman backscattering, which outruns the fastest filamentation instabilities of the pumped pulse even at highly overcritical powers. This Letter proposes a novel nonlinear filtering effect that suppresses premature backscattering of the pump in a noisy plasma layer, while the desired amplification of a sufficiently intense seed persists with a high efficiency. The effect is of basic interest and also makes it robust to noise the simplest technologically fast compression scheme.     

Absorption of iodine laser pulses in potassium and cesium vapors

The absorption of ns iodine laser pulses at a wavelength of 1.315 μm in potassium and cesium vapors has been measured. At elevated temperature there is considerable absorption in both vapors. The absorption was not saturable at intensities up to 1 GW/cm², but increased with increasing intensity.     

Photonuclear reactions induced by intense short laser pulses

A measurement of the decay in time of nuclei excited by an intense short laser pulse of energy E₀$E_0$ yields the Fourier transform of the autocorrelation function of the associated scattering matrix. We determine the optimal length (in time) of the pulse and evaluate the time-decay function using random-matrix theory. That function is shown to contain information not otherwise available. We approximate that function in a manner that is useful for the analysis of data. For E₀$E_0$ below the threshold energy En$E_n$ of the first neutron channel, the time-decay function is exponential in time t while it is the product of an exponential and a power in t   for E₀>En$E_0>E_n$. The comparison of the measured decay functions in both energy domains yields an unambiguous and novel test of random-matrix theory in nuclei.