一种利用混合介质测量SBS介质布里渊线宽的方法

提出了一种利用双池受激布里渊散射(SBS)系统选用混合介质,进而测量SBS介质布里渊线宽的方法.在紧凑双池SBS系统的放大池中放入待测介质,在振荡池中放入布里渊频移可调的混合介质,测出放大池待测介质增益系数随布里渊频移偏离的洛伦兹曲线,该曲线半高处的线宽即为待测介质的布里渊线宽.实验上在Nd:YAG调Q激光系统中,选用CCl₄/C₆H₆混合介质,测量了四氯乙烯(C₂Cl₄)、六氯丁二烯(C_{关键词： 受激布里渊散射 混合介质 布里渊线宽}     

利用不同介质进行布里渊放大的研究

研究了受激布里渊散射振_放双池系统中振荡池和放大池选用不同种类介质的情况.理论分析 结果表明，当两种介质的布里渊频移接近，布里渊线宽有交叉时，系统仍具有放大作用.采 用CCl4作为放大池介质，CCl4/CS2的混合介质作为振荡池介质，利用Nd:YAG调Q 激光研究了布里渊频移的偏离对布里渊放大的影响，结果表明，当布里渊频移的偏离较小时 ，其种子光放大率和种子光脉宽压缩率仍然很大.采用CS2作为放大池介质，苯作为振荡池 介质，对振 放双池系统进行了实验研究，其种子光放大率达到44，种子光脉宽压缩率为 72，相位共轭保真度为98%，种子光放大率的稳定度小于3%. 关键词： 受激布里渊散射 布里渊放大 布里渊频移 布里渊线宽     

受激布里渊散射新介质——全氟胺的研究

本文从介质化学结构与受激布里渊散射(SBS)特性的关系入手,寻找出了SBS特性良好的全氟胺系列新介质——FC-131,FC-3283,FC-40,FC-43,FC-70等,并测定或计算出了新介质的SBS参数. 结果表明,新介质的吸收系数均小于10^-3 cm^-1,光学击穿阈值均高于100 GW/cm². 全氟胺系列新介质不仅具有良好的SBS特性,而且还具有无毒、低挥发性和高稳定性等一系列独特的物理化学性质. 新介质的发现不仅增加SBS介质的种类,而且能够有效提高SBS系统的性能,对于SBS相位共轭镜在高功率激光系统中的应用打下了良好的基础. 关键词： 受激布里渊散射(SBS) 全氟胺 吸收系数 光学击穿阈值     

选用混合介质优化介质和控制受激布里渊散射特性的研究

本文提出了选用混合介质优化介质和控制其SBS特性的方案.分析了全氟碳化合物系列液体介质具有良好互溶性的缘故,数值模拟了HT-230/FC-72混合介质的增益系数、声子寿命和布里渊频移随混合比的变化曲线.在Countinuum Nd:YAG种子注入激光系统中测定了HT-230/FC-72混合介质的吸收系数和光学击穿阈值随混合比的变化,并实验研究了混合介质的能量反射率和Stokes光脉冲波形随混合比的变化.通过选用混合介质不仅优化介质,而且在一定范围之内可控制其SBS特性. 关键词： 受激布里渊散射 混合介质 优化介质 控制SBS特性     

混合介质的SBS参数随混合比变化的研究

从混合介质的折射率、黏度、密度和声速等物理量随混合比的变化关系入手,推导出了混合介质的布里渊线宽、声子寿命和增益系数等受激布里渊散射(SBS)参数随混合比的变化关系.数值模拟了HT-70/FC-72混合介质的布里渊线宽、声子寿命和增益系数随FC-72体积分数的变化关系,并测定了该混合介质的吸收系数和光学击穿阈值随FC-72体积分数的变化关系.结果表明,HT-70/FC-72混合介质的SBS参数随FC-72体积分数单调变化,不出现极值现象.混合介质的选用不仅增加了SBS介质的种类,而且能够满足SBS系统对不 关键词： 受激布里渊散射 混合介质 SBS参数     

SBS新介质C4Cl6参数确定及性能研究

 从介质对光的吸收机理出发，研究了吸收系数较小的受激布里渊散射（SBS）新介质六氯-1,3-丁二烯（C4Cl6）。通过基本的物理参数，确定了入射光波长为1 064 nm时C₄Cl₆的SBS参数，其吸收系数约为0.003 cm^-1，声子寿命约为0.25 ns，增益系数约为4.9 cm·GW^-1。分析了入射光波长与介质SBS参数的关系，布里渊频移与入射光波长成反比，声子寿命与入射光波长的平方成正比，增益系数一般与入射光波长无关。在单池SBS系统中，利用Nd:YAG调Q激光器研究了C₄Cl₆的SBS性能。实验结果表明：由于其吸收系数小，与具有相同增益系数的H₂O比较，C₄Cl₆具有较高的能量反射率（饱和能量反射率大于55%）和较宽的SBS脉宽；由于其声子寿命短，与具有相同吸收系数的CS₂比较，C₄Cl₆的SBS波形上升时间较短。吸收系数小和声子寿命短的特点，使C₄Cl₆适合作为放大池介质，这对优化SBS介质选取，提高SBS系统性能具有一定意义。     

不同波长激光激发下C6H12受激拉曼散射模式竞争

发现不同波长激光激发下C₆H₁₂的受激拉曼散射模式竞争现象. 在不同波长的激光激发下，不同拉曼模式的Stokes光占优势. 短波长(404，532nm)激光激发时小频移模式ω₁(802cm^-1)为弱增益模式，大频移模式ω₂(2852—3038cm^-1)为强增益模， 主要产生ω₂模式的Stokes光. 长波长(80 关键词： 模式竞争 6H₁₂')" href="#">C₆H₁₂ 受激拉曼散射     

四氯乙烯的同步辐射光电离研究

利用VUV同步辐射光源和反射式飞行时间质谱仪，在超声冷却条件下对四氯乙烯(C₂Cl₄)进行了光电离研究，通过测量各离子的光电离效率(PIE)曲线，得到了C₂Cl₄的电离势IP(C₂Cl₄) =(9.36±0.05)eV及C₂Cl₄光解离碎片离子C₂Cl₃⁺，C_{关键词： 真空紫外光电离 离子出现势 电离势 四氯乙烯}     

种子场对单池受激布里渊散射脉冲波形保真的影响

受激布里渊散射(SBS)产生池中引入种子光场，在种子场诱导下产生SBS，这不但可以降低SBS阈值，更可以获得最小的SBS脉冲形变，确保与抽运光波形基本一致，获得高波形保真.从理论和实验两方面研究了种子光强弱对脉冲波形保真的影响. 关键词： 受激布里渊散射 脉冲波形保真 注入种子     

受激布里渊散射光脉冲波形的研究

从实验和理论上研究了受激布里渊散射(SBS)光脉冲波形.在Nd∶YAG调Q激光器中实验研究了SBS光脉冲波形随抽运光参数、结构参数和介质参数的变化规律，并利用SBS理论模型进行了数值模拟，实验与数值模拟结果的变化趋势基本一致.结果表明，抽运光能量越小，透镜焦距越短，镜-池间距越长，介质声子寿命越长，SBS光脉冲波形就越不容易出现调制现象.分析和讨论了抽运光参数、结构参数和介质参数对SBS光脉冲波形的影响机理. 关键词： 受激布里渊散射 脉冲波形 抽运光参数 结构参数     

Investigation on improving characteristics of two-cell SBS system with CCl4/C2H5OH liquid mixture

In order to improve the performance of the two-cell stimulated Brillouin scattering （SBS） system, this paper proposes the methods of using mixtures, which require amplifier media to have small absorption rate, and generator media to have high optical breakdown threshold and Brillouin frequency shift equal to that of the amplification media. The characteristics of the two-cell SBS system are studied experimentally by using CCl4 as amplifier medium and CCl4, C2H5OH and CCl4/C2H5OH liquid mixture as generator medium pumped by Nd：YAG Q-switched laser. The obtained results show that liquid mixture in generator cell improves the power load ability, phase conjugation fidelity, energy reflectivity （ER） and ER stability.     

Study on two-cell stimulated Brillouin scattering system with mixture medium

In this paper,a method of choosing mixture medium in two-cell stimulated Brillouinscattering(SBS)system to improve the system performance is proposed.The Brillouin frequency shift(BFS)of mixture medium varies with the mixing ratio andthus the difference of the BFS between the two cells can be eliminated.The two-cellSBS system with acetone(C3H6O)in its generator cell and mixture liquid ofCCl4/C2Cl4 in its amplifier cell is investigated.The C3H6O has a high optical breakdown threshold and the mixture liquid of CCl4/C2Cl4 has a small absorption coeffi-cient and the same BFS as that of C3H6O when the volume fraction of CCl4 is 4%.Compared with two-cell SBS system with the same liquid(C2Cl4)or different liquid(C3H6O and C2Cl4)in generator and amplifier cell,the SBS system with mixture liq-uid(CCl4/C2Cl4)in amplifier cell and C3H6O in generator cell improves thepower-load,energy reflectivity(ER),phase conjugation(PC)fidelity and ER stabil-ity.     

Observations of wavefront reproduction by stimulated Brillouin and Raman scattering as a function of pump power and waveguide dimensions

Experimental investigations have been made of wavefront reproduction (WFR) by backward stimulated Raman scattering (SRS) and backward stimulated Brillouin scattering (SBS) in CS₂ and C₇H₆O using a linearly polarized ruby pump at λ=0.694 μm. The studies were carried out as a function of the length and cross-section of the optical waveguide and the pump power at the input to the nonlinear medium; curves showing the percentage of nonreproduced backscattered radiation versus power into the waveguide are presented. In all of the cases studied the degree of reproduction by SBS was higher than that by SRS and the efficiency of WFR for both SBS and SRS improved as the pump power into the waveguide was increased, the bore diameter of the lightpipe decreased, and the length of active media decreased.     

Intensity studies in Raman effect

The dependence of the relative intensities of Raman lines, having different polarisation characters, on the mode of excitation has been studied using unpolarised, horizontally and vertically polarised incident light. Standard intensities have been obtained in the cases of CCl₄, CHCl₃, C₆H₆, C₂Cl₄, C₂H₂Cl₂, C₂H₄Cl₂, C₆H₅Cl, C₆H₅CH₃ and C₆H₅CH₂OH with the intensity of the 458 cm^?1 line of CCl₄ as standard and from these, the values ofα′, the derived polarisability, have been obtained in the case of total symmetric lines characteristic of particular bonds and certain conclusions regarding the intensity variations of corresponding lines in the different liquids have been arrived at. Values of derived anisotropy have also been obtained in the case of the depolarised lines relative to that of 313 cm^?1 line in CCl₄.     

Experimental study of a broad-band XeCl double-pass amplifier with SBS mirror

An oscillator-amplifier XeCl laser system has been used to experimentally investigate the effectiveness of a liquid stimulated Brillouin scattering (SBS) mirror for correcting the spatial aberrations of broad-band laser radiation in a double-pass amplifier. It has been found that the SBS amplifier performance is strongly dependent on the intensity I _p exciting the Brillouin medium. A good beam reconstruction has been attained at I _p1GW/cm², whereas highly aberrated output beams have been delivered by the SBS amplifier for I _p>1 GW/cm². By comparing the broad-band SBS amplifier performance to that of the same amplifier with a dielectrically coated flat mirror at one end, it has been found that the use of a SBS mirror is advantageous to obtain lower divergence output beams only for low energy pump beams (<1 mJ).     

Temperature dependence of overtone intensity in raman scattering by liquids

The intensities are inversely related to temperature for CCl₄, C₆H₁₂, CS₂, C₆H₆, CH₃OH, and C₂H₄Cl₂, on account of molecular orientation change. The trends are interpreted in terms of rotational Brownian motion.We are indebted to G. L. Novikova and L. M. Sverdlov for assistance, and to M. L. Kats, M. A. Kovner, and A. G. Finkel for discussions.     

Energy absorption buildup factors of some potential bioactive compounds in the energy region 0.015–15 MeV

Kinetic energy released per unit mass relative to air and energy absorption buildup factors has been calculated for some potential bioactive compounds in the energy region of 0.015–15?MeV. The bioactive compounds of 1-aryl-3-dibenzylamino-propane-1-on hydrochloride type Mannich bases were used in this work. Aryl part was changed as C₆H₅ (1), 4-CH₃C₆H₄ (2), C₄H₃S-2-yl (3), 4-FC₆H₄ (4), 4-BrC₆H₄ (5), 4-ClC₆H₄ (6), and 4-NO₂C₆H₄ (7). The energy absorption buildup factors have been calculated for penetration depth of 40 mean free paths. It is observed that kinetic energy released per unit mass relative to air depends on the photon energy and chemical content of compounds. The compounds with least mean atomic number possess the maximum value of energy absorption buildup factors. Also, the energy absorption buildup factors are found the highest in intermediate energy, whereas the lowest in low as well as high energies.     

Effects of reducing agents on the electrochemical properties of the prepared manganese oxide powders

Manganese oxide powders with high specific capacitance were successfully fabricated via a simple redox reaction at room temperature. The reducing agents used for the redox reaction significantly affected the oxidation states and the electrochemical properties of the prepared manganese oxide powders. As C₂H₅OH was used as the reducing agent, high Mn³⁺ content and high amount of hydroxide were observed in the prepared manganese oxide powders. In addition, the molar ratios of KMnO₄ and C₂H₅OH also influenced the electrochemical properties of the prepared manganese oxide powders. When the molar ratio of KMnO₄ and C₂H₅OH was 1:40, the specific capacitance of the prepared manganese oxide was as high as 402 F/g. These results of the electrochemical analysis showed that, adjusting the molar ratios of KMnO₄ and C₂H₅OH demonstrated to be an effective method for controlling the electrochemical characteristics of manganese oxide powders.