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1.
Considering the nonlinearity arising from the interaction between electrons and lattice vibrations, an effective electronic model with a self-interaction cubic term is employed to study the interplay between electron-electron and electron-phonon interactions. Based on numerical solutions of the time-dependent nonlinear Schroedinger equation for an initially localized two-electron singlet state, we show that the magnitude of the electron-phonon coupling χ necessary to promote the self-trapping of the electronic wave packet decreases as a function of the electron-electron interaction U. We show that such dependence is directly linked to the narrowing of the band of bounded two-electron states as U increases. We obtain the transition line in the χ × U parameter space separating the phases of self-trapped and delocalized electronic wave packets. The present results indicates that nonlinear contributions plays a relevant role in the electronic wave packet dynamics, particularly in the regime of strongly correlated electrons.  相似文献   

2.
In linear disordered systems Anderson localization makes any wave packet stay localized for all times. Its fate in nonlinear disordered systems (localization versus propagation) is under intense theoretical debate and experimental study. We resolve this dispute showing that, unlike in the common hypotheses, the answer is probabilistic rather than exclusive. At any small but finite nonlinearity (energy) value there is a finite probability for Anderson localization to break up and propagating nonlinear waves to take over. It increases with nonlinearity (energy) and reaches unity at a certain threshold, determined by the initial wave packet size. Moreover, the spreading probability stays finite also in the limit of infinite packet size at fixed total energy. These results generalize to higher dimensions as well.  相似文献   

3.
In this work, we investigate the competition of disorder, nonlinearity and non-adiabatic process on the wave packet dynamics in 1D. We follow the time evolution of the second moment of the wave packet distribution to characterize its spreading behavior. In order to describe the dynamical behavior of one-electron wave packets, we solve a discrete nonlinear Schr?dinger equation which effectively takes into account a diagonal disorder and a nonlinear contribution. Going beyond the adiabatic regime, we consider that the nonlinearity relaxes in time according to a Debye-like law. In the adiabatic regime, it has been recently demonstrated that the interplay of disorder and nonlinearity leads to a sub-diffusive spread of the wave packet. Here, we numerically demonstrate that no sub-diffusive spreading of the second moment of the wave packet distribution takes place when the finite response time of the nonlinearity is taken into account.  相似文献   

4.
We experimentally investigate the evolution of linear and nonlinear waves in a realization of the Anderson model using disordered one-dimensional waveguide lattices. Two types of localized eigenmodes, flat-phased and staggered, are directly measured. Nonlinear perturbations enhance localization in one type and induce delocalization in the other. In a complementary approach, we study the evolution on short time scales of delta-like wave packets in the presence of disorder. A transition from ballistic wave packet expansion to exponential (Anderson) localization is observed. We also find an intermediate regime in which the ballistic and localized components coexist while diffusive dynamics is absent. Evidence is found for a faster transition into localization under nonlinear conditions.  相似文献   

5.
Considering the nonlinearity arising from the interaction between electrons and latticevibrations, an effective electronic model with a self-interaction cubic term is employedto study the interplay between electron-electron and electron-phonon interactions. Basedon numerical solutions of the time-dependent nonlinear Schroedinger equation for aninitially localized two-electron singlet state, we show that the magnitude of theelectron-phonon coupling χ necessary to promote the self-trapping of theelectronic wave packet decreases as a function of the electron-electron interactionU. We show that such dependence is directly linked to the narrowing ofthe band of bounded two-electron states as U increases. We obtain thetransition line in the χ × U parameter space separatingthe phases of self-trapped and delocalized electronic wave packets. The present resultsindicates that nonlinear contributions plays a relevant role in the electronic wave packetdynamics, particularly in the regime of strongly correlated electrons.  相似文献   

6.
We study numerically the spreading of an initially localized wave packet in a one-dimensional discrete nonlinear Schr?dinger lattice with disorder. We demonstrate that above a certain critical strength of nonlinearity the Anderson localization is destroyed and an unlimited subdiffusive spreading of the field along the lattice occurs. The second moment grows with time proportional, variant t alpha, with the exponent alpha being in the range 0.3-0.4. For small nonlinearities the distribution remains localized in a way similar to the linear case.  相似文献   

7.
The dynamic characteristics of self-action in three-dimensional wave packets described by the nonlinear Schrödinger equation with a hyperbolic space operator were studied analytically and numerically. The class of the initial wave field distributions for which self-focusing effects predominated over dispersion spreading and caused the arising of wave collapses was considered. The collapse of tubular wave packets was shown to be accompanied by packet shape changes during its contraction to the axis of the system. The nonlinear stabilization of collapses resulted in wave field fragmentation in the longitudinal direction followed by the expansion of the bunches thus formed along the axis. The dynamics of collapses was numerically studied taking into account medium nonlinearity saturation and nonlinear dissipation.  相似文献   

8.
Attosecond pulses are produced when an intense infrared laser pulse induces a dipole interaction between a sublaser cycle recollision electron wave packet and the remaining coherently related bound-state population. By solving the time-dependent Schr?dinger equation we show that, if the recollision electron is extracted from one or more electronic states that contribute to the bound-state wave packet, then the spectrum of the attosecond pulse is modulated depending on the relative motion of the continuum and bound wave packets. When the internal electron and recollision electron wave packet counterpropagate, the radiation intensity is lower. We show that we can fully characterize the attosecond bound-state wave packet dynamics. We demonstrate that electron motion from a two-level molecule with an energy difference of 14 eV, corresponding to a period of 290 asec, can be resolved.  相似文献   

9.
We study the dynamics of a few-quantum-particle cloud in the presence of two- and three-body interactions in weakly disordered one-dimensional lattices. The interaction is dramatically enhancing the Anderson localization length ξ 1 of noninteracting particles. We launch compact wave packets and show that few-body interactions lead to transient subdiffusion of wave packets, m 2 ~ t α , α< 1, on length scales beyond ξ 1. The subdiffusion exponent is independent of the number of particles. Two-body interactions yield α ≈ 0.5 for two and three particles, while three-body interactions decrease it to α ≈ 0.2. The tails of expanding wave packets exhibit exponential localization with a slowly decreasing exponent. We relate our results to subdiffusion in nonlinear random lattices, and to results on restricted diffusion in high-dimensional spaces like e.g. on comb lattices.  相似文献   

10.
We investigate theoretically the nature of the states and the localization properties in a one-dimensional Anderson model with long-range correlated disorder and weak nonlinearity. Using the stationary discrete nonlinear Schrödinger equation, we calculate the disorder-averaged logarithm of the transmittance and the localization length in the fixed input case in a numerically exact manner. Unlike in many previous studies, we strictly fix the intensity of the incident wave and calculate the localization length as a function of other parameters. We also calculate the wave functions in a given disorder configuration. In the linear case, flat phased localized states appear near the bottom of the band and staggered localized states appear near the top of the band, while a continuum of extended states appears near the band center. We find that the focusing Kerr-type nonlinearity enhances the Anderson localization of flat phased states and suppresses that of staggered states. We observe that there exists a perfect symmetry relationship for the localization length between focusing and defocusing nonlinearities. Above a critical value of the strength of nonlinearity, delocalization due to the long-range correlations of disorder is destroyed and all states become localized.  相似文献   

11.
We investigate the impact of decoherence and static disorder on the dynamics of quantum particles moving in a periodic lattice. Our experiment relies on the photonic implementation of a one-dimensional quantum walk. The pure quantum evolution is characterized by a ballistic spread of a photon's wave packet along 28 steps. By applying controlled time-dependent operations we simulate three different environmental influences on the system, resulting in a fast ballistic spread, a diffusive classical walk, and the first Anderson localization in a discrete quantum walk architecture.  相似文献   

12.
The self-action of three-dimensional wave packets is analyzed analytically and numerically under the conditions of competing diffraction, cubic nonlinearity, and nonlinear dispersion (dependence of group velocity on wave amplitude). A qualitative analysis of pulse evolution is performed by the moment method to find a sufficient condition for self-focusing. Self-action effects in an electromagnetically induced transparency medium (without cubic nonlinearity) are analyzed numerically. It is shown that the self-focusing of a wave packet is accompanied by self-steepening of the longitudinal profile and envelope shock formation. The possibility of envelope shock formation is also demonstrated for self-focusing wave packets propagating in a normally dispersive medium.  相似文献   

13.
We investigate the dynamics of electrons in the vicinity of the Anderson transition in d = 3 dimensions. Using the exact eigenstates from a numerical diagonalization, a number of quantities related to the critical behavior of the diffusion function are obtained. The relation η = d ? D2 between the correlation dimension D2 of the multifractal eigenstates and the exponent η which enters into correlation functions is verified. Numerically, we have η ≈? 1.3. Implications of critical dynamics for experiments are predicted. We investigate the long-time behavior of the motion of a wave packet. Furthermore, electron-electron and electron-phonon scattering rates are calculated. For the latter, we predict a change of the temperature dependence for low T due to η. The electron-electron scattering rate is found to be linear in T and depends on the dimensionless conductance at the critical point.  相似文献   

14.
We study control of wave packets with a finite accuracy, approaching it as quantum information processing. For a given control resolution, we define the analogs of several quantum bits within the shape of a single wave packet. These bits are based on wave packet symmetries. Analogs of one- and two-bit gates can be implemented using only free wave packet evolution and coordinate-dependent ac Stark shifts applied at the moments of fractional revivals. As in quantum computation, the gates form a logarithmically small set of basis operations which can be used to approximate any unitary transformation desired for quantum control of the wave packet dynamics. Numerical examples show the application of this approach to control vibrational wave packet revivals.  相似文献   

15.
矩形弹子球中的量子波包分析(英文)   总被引:1,自引:0,他引:1  
利用波包分析量子力学体系的动力学行为在研究经典和量子的对应关系方面越来越成为一个非常重要的方法.利用高斯波包分析方法,我们计算了矩形弹子球体系的自关联函数,自关联函数的峰和经典周期轨道的周期符合的很好,这表明经典周期轨道的周期可以通过含时的量子波包方法产生.我们还讨论了矩形弹子球的波包回归和波包的部分回归,计算结果表明在每一个回归时间,波包出现精确的回归.对于动量为零的波包,初始位置在弹子球内部的特殊对称点处,出现一些时间比较短的附加的回归.  相似文献   

16.
A solution to the problem of realizing the collapse of three-dimensional wave packets in nonlinear media with normal group velocity dispersion is proposed. Wave packets with pronounced hyperbolic topology are shown to collapse; i.e., the field increases infinitely near the system axis. In particular, wave collapse of the tubular axisymmetric packets occurs through the concentration of the compressed ring field distribution at the axis. The collapse is shown to stabilize due to the saturation of nonlinearity or nonlinear dissipation, which restrict the field increase and lead to the packet splitting in the transverse direction.  相似文献   

17.
The stationary phase method is frequently adopted for calculating tunneling phase times of analytically-continuous Gaussian or infinite-bandwidth step pulses which collide with a potential barrier. This report deals with the basic concepts on deducing transit times for quantum scattering: the stationary phase method and its relation with delay times for relativistic and non-relativistic tunneling particles. After reexamining the above-barrier diffusion problem, we notice that the applicability of this method is constrained by several subtleties in deriving the phase time that describes the localization of scattered wave packets. Using a recently developed procedure - multiple wave packet decomposition - for some specifical colliding configurations, we demonstrate that the analytical difficulties arising when the stationary phase method is applied for obtaining phase (traversal) times are all overcome. In this case, we also investigate the general relation between phase times and dwell times for quantum tunneling/scattering. Considering a symmetrical collision of two identical wave packets with an one-dimensional barrier, we demonstrate that these two distinct transit time definitions are explicitly connected. The traversal times are obtained for a symmetrized (two identical bosons) and an antisymmetrized (two identical fermions) quantum colliding configuration. Multiple wave packet decomposition shows us that the phase time (group delay) describes the exact position of the scattered particles and, in addition to the exact relation with the dwell time, leads to correct conceptual understanding of both transit time definitions. At last, we extend the non-relativistic formalism to the solutions for the tunneling zone of a one-dimensional electrostatic potential in the relativistic (Dirac to Klein-Gordon) wave equation where the incoming wave packet exhibits the possibility of being almost totally transmitted through the potential barrier. The conditions for the occurrence of accelerated and, eventually, superluminal tunneling transmission probabilities are all quantified and the problematic superluminal interpretation based on the non-relativistic tunneling dynamics is revisited. Lessons concerning the dynamics of relativistic tunneling and the mathematical structure of its solutions suggest revealing insights into mathematically analogous condensed-matter experiments using electrostatic barriers in single- and bi-layer graphene, for which the accelerated tunneling effect deserves a more careful investigation.  相似文献   

18.
The application of femtosecond pump-probe photoelectron spectroscopy to directly observe vibrational wave packets passing through an avoided crossing is investigated using quantum wave packet dynamics calculations. Transfer of the vibrational wave packet between diabatic electronic surfaces, bifurcation of the wave packet, and wave packet construction via nonadiabatic mixing are shown to be observable as time-dependent splittings of peaks in the photoelectron spectra.  相似文献   

19.
The object of the present work is to analyze the effect of nonlinearity on wave packet propagation in a square lattice subject to a magnetic and an electric field in the Hall configuration, by using the Discrete Nonlinear Schrödinger Equation (DNLSE). In previous works we have shown that without the nonlinear term, the presence of the magnetic field induces the formation of vortices that remain stationary, while a wave packet is introduced in the system. As for the effect of an applied electric field, it was shown that the vortices propagate in a direction perpendicular to the electric field, similar behavior as presented in the classical treatment, we provide a quantum mechanics explanation for that. We have performed the calculations considering first the action of the magnetic field as well as the nonlinearity. The results indicate that for low values of the nonlinear parameter U the vortices remain stationary while preserving the form. For greater values of the parameter the picture gets distorted, the more so, the greater the nonlinearity. As for the inclusion of the electric field, we note that for small U, the wave packet propagates perpendicular to the applied field, until for greater values of U the wave gets partially localized in a definite region of the lattice. That is, for strong nonlinearity the wave packet gets partially trapped, while the tail of it can propagate through the lattice. Note that this tail propagation is responsible for the over-diffusion for long times of the wave packet under the action of an electric field. We have produced short films that show clearly the time evolution of the wave packet, which can add to the understanding of the dynamics.  相似文献   

20.
The effect of detuning from phase matching on the dynamics of a wave packet consisting of two unidirectional strongly interacting modes in a fiber with Kerr nonlinearity is considered. The effective parameters of dispersion and nonlinearity are analyzed for a wave packet that can be represented by a single partial pulse.  相似文献   

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