Generation of acoustic waves by power microwave pulses with the use of thin metal films

We study the features of excitation of acoustic waves by high-power microwave pulses in thin metal films bordering on liquid. Aluminum films with thicknesses 1–10 nm deposited onto a quartz substrate were used in experiments. It is shown theoretically that the absorption coefficient of microwaves is maximum for film thickness from 2 to 3 nm and the value of this maximum is determined by the dielectric permittivity of the bordering liquid. Theoretical calculations and experiments are performed for water and ethyl alcohol. The sound generation in a layered system quartz-aluminum film-liquid is analyzed with the help of the step-by-step approach. At the first step, microwave energy is absorbed in the film and heat is released. Then heat almost instantly diffuses into a liquid whose thermal expansion creates an acoustic signal. Profiles of acoustic signals excited in aluminum films by microwave pulses with a 5-ns duration and an energy of up to 1 mJ are experimentally detected. The most efficient transduction was observed for an aluminum film 3.5 nm thick.     

Space- and time-resolved Brillouin light scattering from nonlinear spin-wave packets

We have constructed a new Brillouin light scattering apparatus, based on the Sandercock multipass tandem interferometer design, for space- and time-resolved investigations of nonlinear wave packets in thin films. We have applied the method to studies of nonlinear spin-wave pulse propagation in yttrium iron garnet (YIG) films. Spatial resolution is achieved by scanning the laser spot across the YIG film surface, and temporal resolution is obtained by measuring the elapsed time between the launch of spin-wave pulses by an applied microwave pulse and the arrival of the respective inelastically scattered photons at the detector. We report the observation of nonlinear self-focusing of wave beams and pulses in one and two dimensions, the formation of one-dimensional envelope solitons, and of strongly localized, two-dimensional wave packets, 'spin-wave bullets', analogous to 'light bullets' predicted in nonlinear optics. By generating two counter-propagating wave pulses, pulse collision experiments were performed. We show that quasi-one-dimensional envelope solitons formed in narrow film stripes ('waveguides') retain their shapes after collision, while two-dimensional spin-wave packets formed in wide YIG films are destroyed in collision.     

Optical parametric oscillator pumped by relaxation oscillation pulses of a mechanically Q-switched Nd:YAG laser

We report the generation of mid-infrared pulsed radiation between 2.2 and 3 μm range using a singly-resonant optical parametric oscillator (SR-OPO) based on a 40-mm-long crystal of periodically-poled LiNbO₃ (PPLN) pumped by mechanically Q-switched pulses from a Nd:YAG laser, obtained by chopping the beam inside the laser resonator over a 1–10 kHz duty cycle. An appreciable reduction in pulse width as well as the number of relaxation oscillation pulses of the Nd:YAG pump laser is observed when the frequency of the Q-switch chopper is increased up to 10 kHz. Sub-nanosecond relaxation oscillation pulses of about 170–210 ns duration are generated under the width of the idler envelope varying from 4.6 to 8.55 μs. The same behavior is observed for the signal wave. A maximum extraction efficiency of 22 % is obtained for the idler, corresponding to 785 mW of output power at 10 kHz. The tuning of the signal and idler beams were performed by temperature variation of the PPLN crystal within 100–200 °C range.     

Oscillating Dependence of the Acoustic Attenuation Coefficient in Thin Metal Layers

Dimensional and frequency dependences of the energy absorption coefficient of a longitudinal sound wave in a plane parallel metal layer are theoretically investigated for arbitrary relationship between the layer thickness d and the electron free path l. Exact and asymptotic (for thick (d >> l) and thin (d << l) metal layers) formulas are derived for the coefficient for an arbitrary angular dependence of the probability of specular reflection of charge carriers from the sample surface q(). A square-root dependence of the acoustic absorption coefficient on the thin film thickness is predicted. If the direction of sound wave propagation is perpendicular to the thin metal layer boundary, the acoustic absorption coefficient becomes an oscillating function of the layer thickness; its amplitude decreases with increasing kd, where k is the acoustic wave number.     

Modification of structure, morphology and physical properties of tin sulfide thin films by pulsed laser irradiation

This paper presents modification of tin sulfide (SnS) thin films by pulsed laser irradiation. Tin sulfide films of 1 μm thickness were prepared using chemical bath deposition (CBD) technique. The chemical bath contained 5 ml acetone, 12 ml of triethanolamine, 8 ml of 1 M thioacetamide, 10 ml of 4 M ammonium hydroxide and 65 ml of distilled water. The chemical bath was kept at a constant temperature of 60 °C for 6 h which resulted in SnS films with 500 nm thickness. By double deposition, the final thickness of SnS thin films obtained was 1 μm. Laser processing was conducted to modify the structure, morphology and physical properties of the SnS thin films. The laser specifications were pulsed Nd:YAG laser with 532 nm wavelength, 300 mJ pulse energy and 10 ns pulse width. Properties of the laser-irradiated SnS thin films were compared with the as-prepared SnS thin films. The changes in structure, morphology, optical and electrical properties of the laser-irradiated SnS thin films were described.     

Self-organization in a chromium thin film under laser irradiation

Self-organization of chromium on glass was observed during laser ablation of the metal film with partially overlapping laser pulses. The beam of a nanosecond pulse laser tightly focused to a line was applied to the back-side ablation of the chromium thin film on a glass substrate. While the line ablated with a single laser pulse had sharp edges on both sides with ridges of the melted metal, the use of partially overlapping pulses formed a complicated structure made of the metal remaining from the ridges. Regular structures of ripples were developed in a certain range of laser fluence and pulse overlap. The ripple period could be controlled from 2.5 to 4 μm by variation of the processing parameters. Various experimental techniques were applied to test the structures, and different models of the ripple formation in the thin metal film were considered. The initial quasi-periodical formation started because of dewetting of thin liquid metal films on the glass substrate after its melting. Similar to the evaporation of liquid films, the small perturbation in the ridge thickness was able to induce instability in evaporation of the thin melted metal film. Freezing of the nonequilibrium state between laser pulses was one of the stabilizing factors in self-organization of the metal.     

Testing a thermoacoustic sensor of high-power microwave pulses

We present the results of testing a new thermoacoustic sensor designed to detect microwave pulses having durations from 3 to 120 ns at wavelengths of 0.8 and 3 cm. Operation of the sensor is based on the effect of generation of acoustic signals during absorption of microwave pulses in a radiotransparent substrate–absorber–liquid layered structure . A thin nanometer-thick film deposited on a substrate is used as an absorber. Microwaves are converted to an acoustic pulse in the film and the adjacent liquid. The pulse is received by a wideband acoustic receiver and then recorded by a digital oscilloscope. It is shown that for a pulse duration of 120 ns, the shape of the signal recorded by the thermoacoustic sensor completely corresponds to the signal of a tube-diode detector of microwave pulses. The response of the thermoacoustic sensor to shorter pulses (3 and 5 ns long) is a pulse with a duration of 18 ns which is determined by a limited frequency band of the acoustic receiver.     

Adaptive pulse compression by two-photon absorption in semiconductors

We investigate the adaptive optimization of broadband laser pulses, using a closed-loop learning algorithm in which the merit function is derived from two-photon absorption in semiconductors. Photoluminescence experiments with CdS thin films and photocurrent measurements of a GaAsP photodiode have been performed. The experimental data demonstrate that reliable and accurate pulse compression to the bandwidth limit can be achieved, unperturbed by nontrivial phase effects. Therefore two-photon absorption proves to be an easy-to-implement alternative to second-harmonic generation for the compression of broadband laser pulses.     

Pulsewidth limitation in the relativistic backward wave oscillator

Spontaneous pulse shortening occurring in a relativistic backward wave oscillator (BWO) at gigawatt power levels is studied in experiment and theory. It is experimentally demonstrated that this phenomenon is accompanied by formation of an explosive-emission plasma at the surface of the corrugated slow-wave structure (SWS). Termination of microwave emission is explained by the increase of the BWO starting current from the absorption of the operating electromagnetic wave by electrons emitted from the plasma, whereas the intensity of the absorption radically increases offing to the presence of positive ions emitted from the plasma. Application of oil-free vacuum and electrochemical polishing of the SWS surface in an X-band BWO allowed generation of 3-GW, 26-ns microwave pulses with an energy of ~80 J, thereby demonstrating pulse lengthening by a factor of four     

Generation of electron nanobunches and short-wavelength radiation upon reflection of a relativistic-intensity laser pulse from a finite-size target

We have proposed an efficient scheme of generation of short dense electron bunches during the interaction at large angles of incidence of a laser pulse with a thin transversally semibounded laser target. Streams of bunches can be used to simultaneously and independently generate pulsed X-ray radiation as fast electrons hit secondary targets. Dependences of bunch parameters (the number of particles in the bunch and the bunch energy and thickness) on the angle of incidence and laser intensity have been obtained. It has been shown that, upon reflection from the target, the relativistic-intensity laser wave is efficiently converted (the energy-conversion factor reaches ～20%) into a sequence of electromagnetic tens-of-nanometer-long atto pulses, which follow one after another in the period of the initial laser wave. We have investigated how the parameters of the atto pulse depend on the angle of incidence and the laser intensity. We have shown that atto pulses are generated most efficiently at large angles of incidence (≥50°) of the laser pulse on the target.     

Microstructure parameters and optical properties of cadmium ferrite thin films of variable thickness

CdFe₂O₄ thin films of different thicknesses were deposited onto glass substrates by the thermal evaporation technique. Their structural characteristics were studied by X-ray diffraction (XRD). The microstructure parameters, crystallite size, and microstrain were calculated. It is observed that both the crystallite size increases and microstrain increase with increasing with the film thickness. The fundamental optical parameters like absorption coefficient and optical band gap are calculated in the strong absorption region of transmittance and reflectance spectrum. The refractive indices have been evaluated in terms of the envelope method, which has been suggested by Swanepoel in the transparent region. The refractive index can be extrapolated by the Cauchy dispersion relationship over the whole spectra range, which extended from 400 to 2500 nm. The refractive index, n, increases on increasing the film thickness up to 733 nm and the variation of n with higher thickness lies within the experimental errors.     

Measurement of sound absorption by underwater acoustic material using pulse-separation method

An alternative pulse-separation method is presented for measuring the sound absorption at normal incidence of an underwater acoustic material in a water-filled impedance tube. A damped sine pulse was generated in the water-filled impedance tube with a regular waveform and a short duration time of approximately 1 ms. During the generation of the pulse, the inverse filter principle was used to compensate for the transducer response. In addition, the effects of the characteristics of the tube termination can be eliminated during the generation of the pulse to obtain a single plane pulse wave in the impedance tube, which is a necessary condition for this technique. Measurements of the sound absorption coefficient of the rubber material and the reflection coefficient from a water/air interface were used to verify the pulse-separation method.     

Generation of a stationary train of chaotic soliton-like microwave pulses in self-oscillating ring systems with a ferromagnetic thin film

The generation of a stationary train of chaotic soliton-like microwave pulses has been observed in an isolated self-oscillating ring system with a ferromagnetic thin-film and a resonator. The pulses have been formed owing to three-wave parametric processes and modulation instability of a surface magnetostatic wave. The soliton-like character of the microwave pulses is indicated by the time dependence of the instantaneous phase of the signal envelope.     

纳米金表面修饰与表面等离子体共振传感器的相互作用研究

为了分析纳米金表面修饰对表面等离子体共振(SPR)的放大作用,以及其对传感器本身的影响,首先,基于色散介质的吸收理论,通过建立波长型SPR生物传感器四层膜结构的数学模型,理论分析了传感器表面所吸附纳米金对传感器的影响:纳米金的表面修饰,改变了表面等离子体传感器中棱镜表面各介质层内电磁场的能量分布,削弱了金属膜在共振吸收中的作用,从而使SPR曲线的半波宽度增加,最小反射系数增大,金膜的最优膜厚度也随之改变.其次,通过不同厚度的金膜外吸附纳米金的对比试验,验证了此理论.金膜厚45nm、表面修饰10nm纳米金颗 关键词： 表面等离子体共振 生物传感器 纳米金 金属膜     

Pulsed heating of thin powder layers by intense microwaves

Thin (0.05 cm) layers of mechanical mixtures of conductive and insulating powders are heated by microwave pulses with an intensity of about 10 kW/cm². For mW-power microwaves, the absorption thickness in the mixtures is found to be on the order of 1 cm. For intensities of 10 kW/cm² and above, pulse durations of 5–8 ms, and the number of pulses in a train of 5 or less, the powder layer melts and the characteristic spatial scale of absorption decreases to ≈0.05 cm. The reflection factor drops during a microwave pulse. Ways of improving the absorption efficiency by initiating surface breakdowns and plasma formation in pores between coarse grains in the bulk of the powders are considered.     

Effect of time profile of laser pulse on the excitation of sound signals in a liquid with a series of laser pulses

We have studied the sound generation with high repetition rate pulsed laser. We have solved the inhomogeneous wave equation for acoustic pressure in a liquid generated by a laser, using Green’s function formalism and convolution technique. To obtain the maximum pressure of the sound waves, we found the conditions on repetition rate and on period of laser pulse of various shapes. Our analysis shows that the sound generated in a liquid with a series of laser pulses is highly affected by the time profile of the pulses besides other parameters, namely laser beam diameter, laser beam optical wavelength, repetition rate and period of laser pulse. This effect is pronounced particularly in frequency domain. We found that the noise of higher harmonics in the generated sound can be greatly removed with the proper choice of the time profile of the laser pulses. It is found that the pressure is generated around the fundamental frequency for the half-sine and rectangular pulses, with the proper choice of repetition rate and period of pulse. The application of the present analysis for underwater communication is pointed out.     

Analysis of material modifications induced during laser damage in SiO2 thin films

The damage mechanisms in silica thin films exposed to high fluence 1064 nm nano-second laser pulses are investigated. The thin films under study are made with different techniques (evaporation and sputtering, with and without ion assistance) and the results are compared. The material morphological, optical and structural modifications are locally analyzed with optical microscopy and profilometry, photoluminescence and absorption microscopies. These observations are made for fluences near and above the laser damage threshold, and also in the case of multiple pulse irradiations. An increase in absorption in and around the damages is observed, as well as the generation of different defects that we spatially resolve with absorption and luminescence mappings.     

The evanescent-wave cavity ring-down spectroscopy technique applied to the investigation of thermally grown oxides on Si(100)

We report about the contribution of thermally grown SiO_x overlayer on the SiO_x/Si interface (with oxidation states Siⁿ⁺, where n = 1, 2, 3, 4) to the optical losses of a resonant spectroscopic cavity. The experiments on Si oxide thin films were performed in evanescent wave for Si samples in contact with a total internal reflection surface of a BK7 prism. The evanescent field can be exploited to investigate properties and processes such as the absorption of thin film or solid/air interface reactions. The results show that the oxide overlayer thickness grows with the thermal exposure time and is limited after more than 7 h of treatment. Transmission electron microscopy has been used for the native oxide thickness measurement and angle-resolved X-ray photoelectron spectroscopy used to determine the thermal oxide thickness. A change of absorption coefficient Δα in the range 100–200 cm^?1 is obtained by evanescent-wave cavity ring-down spectroscopy (EW-CRDS) for thermal silicon oxide overlayer, in agreement with the general trend from literature. The evaluation from the EW-CRDS experiments presents the used setup as a competitive method for measuring the absorption properties of thin overlayer.     

Proton beam generation by ultra-high intensity laser–solid interaction

We report on some recent experimental results on proton production from ultra-intense laser pulse interaction with thin aluminium and plastic foil targets. These results were obtained at Laboratoire d'Optique Appliquée with the 100 TW ‘salle jaune’ laser system, delivering 35 fs laser pulses at 0.8 μm, reaching a maximum intensity on target of a few 10¹⁹ W/cm².

In such extreme interaction conditions, an intense and collimated relativistic electron current is injected from the plasma created on the laser focal spot into the cold interior of the target. Its transport through dense matter, ruled by both collisions and self-induced (electro-magnetic) field effects, is the driving mechanism for proton acceleration from the rear side of thin foils: when reaching and leaving the foil rear-side, the fast electrons create a large charge separation and a huge electrostatic field with a maximum value of few TV/m, capable of accelerating protons.

A parametric study as a function of the laser driver and target parameters indicates an optimal value for target thickness, which strongly depends on the laser prepulse duration. In our experiments, we did irradiate targets of various materials (CH, Al, Au) changing the prepulse duration by using fast Pockels cells in the laser chain. CR-39 nuclear track detectors with Al filters of different thickness and a Thomson parabola were used to detect proton generation. The best results were obtained for 2 μm Al targets, leading to the generation of proton energies with energies up to 12 MeV.     

The effect of different drying methods on band gap energy and femtosecond LIDT of nano-porous anti-reflective silica thin films

In this work, nano-porous anti-reflective silica thin films are deposited on the quartz samples by dip-coating in silica sol–gel. After dip-coating, the samples are divided into three groups and each group is heated in an oven with a different drying method. The effect of the heating methods on the morphology and optical properties of the coated layers are studied by SEM imaging and measuring optical transmission of the samples. Then based on the transmission data and calculation of absorption coefficient of the layers, the band gap energy of the silica thin films is calculated. In addition, laser induced damage threshold (LIDT) of the samples are measured by using 35 fs, 100 mJ femtosecond laser pulses. It can be seen that there is a distinct correlation between band gap energy and LIDT of the samples which both of them have been affected by heating method of the coated samples.