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分别采用空气、氩气大气压介质阻挡放电(DBD)等离子体对重油进行了处理.对经空气DBD等离子体处理后的重油进行粘温特性分析,发现重油粘度升高,流动性变差.红外光谱和四组分分析结果表明重油的重质组分含量升高,重油胶体体系被破坏,同时生成大量刺激性气味气体.为了便于分析气态产物的成分和含量,采用大气压氩气DBD等离子体处理重油并收集气体产物.气相色谱分析发现生成气中含有大量C1-C5的烃类和一定量氢气,其中氢气和甲烷含量占生成气的70％以上.实验结果表明重油在等离子体作用下既发生裂解又发生聚合反应,既生成低碳烃类,本身的流动性也变差.     

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用火花预电离辅助介质阻挡放电装置在大气压空气中实现了均匀的类辉光放电。通过用光谱模拟法和波尔兹曼图解法对N 2 第一负带系B2Σ→X 2Σ(0,0)带发射谱线的分析,对放电过程中N 2 的转动温度进行了诊断。研究了不同频率和放电模式下转动温度的变化规律,对由两种方法计算所得的温度进行了对比。实验结果表明,转动温度会随着外加频率的增加而缓慢的增加;当放电从类辉光模式变到丝状放电模式时,转动温度会有70K左右的升高。     

介质阻挡放电低温等离子体脱硝性能研究

进行了介质阻挡放电低温等离子体脱除伴有SO₂的烟气中NO的研究,分别进行了直接等离子体脱硫脱硝和间接等离子体脱硫脱硝实验。在直接等离子体脱硫脱硝中,模拟烟气等混合气直接通入等离子体发生器,在反应器中电离分解NO以及和生成的高能电子、离子和自由基等离子体相互反应而进行脱除NO;间接等离子体脱硫脱硝中,模拟烟气连接在等离子体发生器出口与从反应器中产生出的等离子体发生氧化反应而进行脱除NO。结果表明,无论直接形式还是间接形式,脱硝效率都要比脱硫效率高,间接脱硫脱硝能够大大降低功率输入,节省能耗,具有重要的实际应用价值和意义。氨气的加入,有利于脱除效率的提升。     

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Based on ORBIT code of a guiding center motion of single particle, the loss of energetic ions in different radial positions of tokamak plasma is studied by using test particle simulation method. The results show that the local magnetic perturbations can cause loss of many energetic ions near the central region of the plasma, but they have little effect on the ion loss near the plasma boundary, assuming that the local field is mainly located near a magnetic surface and its toroidal field is similar to the ripple field. These energetic ions are trapped ions, and the greater their pitch angle is, the easier they lose. In addition, the radial position of the local field that causes the maximum loss rate of energetic ions is usually offset from the initial radial position of these loss ions, and this shift is closely related to the energy of these ions. When the local field appears in certain locations, the ions of lower energy have some loss, but the ions higher energy does not lose.     

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Thomas-Fermi model can be applied to describe state of electrons for mixtures. A method to solve the mixture Thomas-Fermi equation is proposed. With the proper initial test solution and step length, this method searches the solution in a way that reduces the steps by half, which can get solutions with various densities and temperatures fast.     

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基于感应耦合等离子体(ICP)技术设计了一套用于在硅基片上制作形成超浅结的等离子体浸没注入(PIII)系统。该ICP PIII系统工作腔室为圆柱形,采用射频功率源,注入偏压源为一脉冲直流电压源,系统与Langmiur探针相连。探针诊断结果表明,该系统的等离子体离子密度达到1017m-3,离子密度径向均匀性达到3.53%。硼和磷的超低能注入试验的二次离子质谱测试结果表明：掺杂离子注入深度在10nm左右,最浅的注入深度为8.6nm(在注入离子密度为1018cm-3时);注入离子剂量达到了1015cm-2以上;掺杂离子浓度峰值在表面以下;注入陡峭度达到了2.5nm/decade。     

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利用纳秒脉冲放电在单针、环状、以及单针加环状三种不同电极结构下产生了均匀稳定的等离子体射流;通过光学和电学诊断研究了三种不同结构下等离子体射流的运行特性及相应的物理机制。实验结果表明,以上三种等离子体射流的转动温度均为295K,振动温度分别为1900K,2000K和2100K,都属于非平衡态等离子体;其中,基于单针和环状电极的混合型射流可产生更为均匀稳定的等离子体,且富含较多的活性物种,有望在材料表面处理及消毒灭菌等领域发挥一定作用。     

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利用电流丝模型对SUNIST球形托卡马克等离子体边界重构进行了模拟计算。结果表明,用电流丝模型能够比较好地对等离子体自由边界进行快速识别,与EFIT平衡计算的边界径向平均误差小于6mm。     

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采用射频(RF)等离子体对颗粒形状不规则的钨粉球化,研究了加料速率和钨粉分散方式对球化率的影响。通过用电子扫描显微镜(SEM)观测得到的被球化粉末的百分比评估了球化效率。通过对球化处理的钨粉的X射线衍射谱(XRD)的检测,验证了在球化过程中无氧化发生和其它杂质介入。当钨粉以极短暂时间(约几毫秒)快速穿越等离子体炬时,钨粉颗粒因受热而熔化成液滴,快速冷却后,形成致密的球形固态颗粒。     

Properties of surface dielectric barrier discharge plasma generator for fabrication of nanomaterials

This paper presents surface dielectric barrier discharge plasma generators as an efficient source of low-energy ions. Either positive or negative ions can be extracted from a plasma cloud with an external DC field created by the third electrode. Three different cross-section geometries of DBD generators were analyzed, simulated and fabricated. Currents of ions extracted from the plasma cloud were measured and the results were discussed. It was demonstrated that if the third electrode consists of liquid–gas interface, the presented arrangement can be used as a versatile reactor for nanomaterial synthesis (on the example of the synthesis of silver nanoparticles).     

Differential responses of cancer cell lines to non-thermal plasma from dielectric barrier discharge

The differential responses of six cancer cell lines after treatment of non-thermal plasma from dielectric barrier discharge (DBD) were studied. Two plasma exposure methods including cell suspension exposure and media only exposure were used, and the effects were examined in six cancer cell lines including KB, MCF-7, HeLa, H460, SNU-80 and T98G from different human organs. The result indicates that both methods affected six cell lines similarly in proliferation, mitochondria activity, and apoptosis related gene expression, which implies that the cell culture media have significant role in plasma–cell interaction. H460 showed a significant reduction in cell number after plasma exposure, whereas MCF-7 showed less reduction. Mitochondria activity of all the cancer cell lines reduced following exposure and incubation times except MCF-7. The mRNA expression of Bax, the apoptosis related gene, was highly enhanced in KB, HeLa, MCF-7 and SNU-80, while none was detected in T98G. All six cancer cell lines showed unexpectedly low mRNA expression of tumor suppressor gene p53. These differential responses of six cell lines suggest that non-thermal plasma should activate different pathways in each cancer cell line. Further researches on tissue-specific responses to plasma treatment should be conducted, comparing their responses with normal tissue–cell responses.     

估算线筒式介质阻挡放电场强和电子平均动能的方法

利用静电场模型对线筒式介质阻挡放电电场强度进行了计算,并对电子平均动能进行了估算。通过对单双介质阻挡放电(DBD)的对比,发现在相同的放电条件下,双介质DBD产生的电场强度和电子平均动能比单介质DBD的要大。这就很好地解释了在相同的放电参数下,甲苯的降解效率在双介质DBD中要比单介质DBD中大。     

Agglomeration of sub-micron particles by a non-thermal plasma electrostatic precipitator

Non-thermal Plasma agglomeration is presented as a promising process to reduce the number concentration of sub-micron particles in an acrylic duct, which included a saw-tooth electrode and a wire-plate electrostatic precipitator (ESP). The generated plasma by pulse-energized ESP, the particle agglomerations were controlled under operating conditions such as pulse voltages, pulse frequencies, dust loadings, and gas velocities. When gas velocity increased from 0.5 to 1 m s⁻¹ at 45 kV_p, 20 kHz, it was found that efficiency was increased. At gas velocity of 1 m s⁻¹, the sub-micron particle number reduction efficiency for all particle sizes was over 90% in ESP.     

一种新型大气压毛细管介质阻挡放电冷等离子体射流技术

介绍一种结构设计简单、操作运行方便的新型毫米量级大气压冷等离子体射流发生技术.这种射流可以在大气压条件下，利用多种工作气体(如Ar,He,N₂)，通过毛细管介质阻挡放电(DBD)的方式实现.使用频率为33kHz，峰值电压为1—12kV的双向脉冲电源，利用Ar,He,N₂等工作气体，在毛细管内形成了稳定的冷等离子体射流.放电区域的光辐射空间分布利用商用CCD摄像机记录，从中研究放电形态和空间分布，观察到了在DBD区域的流动气体放电和在毛细管出口处形成的等离子体射流 关键词： 冷等离子体射流 毛细管介质阻挡放电 射流射程 射流激发温度     

Influence of wire mesh electrodes on the volume and surface characteristics of dielectric barrier discharge of atmospheric pressure helium

The dielectric barrier discharge of helium in a 6 mm gap at atmospheric pressure was studied. In this paper, the influence of electric field distribution on the uniformity of DBD is analyzed theoretically and verified by experiments. The experimental results show that the mesh electrode produces a local enhancement effect by affecting the electric field and then produces corona discharge, which provides seed electrons for the subsequent discharge process. The effects of mesh diameter and size on discharge uniformity and stability are analyzed, the electrode structure parameters are optimized, the method of a segmented electrode is proposed, and the discharge process and charge distribution are studied. The electrical diagnosis results of plasma technology show that the segmented mesh electrode reduces the breakdown voltage of DBD and increases the charge deposition.     

电荷电压法测量DBD等离子体的放电参量

在DBD应用研究中，使用电荷电压法能够测量许多重要参量，如放电功率、放电间隙等效电容、电介质层等效电容、着火电压、放电间隙等效电压及放电间隙电场强度等．同时根据电荷电压图形随工作条件及状态变化的情况还可以诊断DBD等离子体的工作稳定性．文章对相关原理、模拟实验结果及实际应用效果进行了介绍．     

Availability of indirect atmospheric plasma from a dielectric barrier discharge device on biofilm-forming bacteria

An investigation of the treatment effect of atmospheric cold plasma (ACP)-generated reactive oxygen species (ROS) against problematic bacteria of chronic wounds is presented. To study ROS effects specifically, a vacuum chamber with a flowmeter to control the background gas composition and a mesh electrode for a dielectric barrier discharge (DBD) device were used. In addition, a numerical modeling was developed to simulate the amount of ROS flux transported from the mesh electrode to determine which of the ROS species was the main factor in the treatment effect. Considering the experimental and computational results and the effective transport distance of each species, ozone could be the main factor in the experimental results.