Surface-Radiative Modes and Longitudinal Excitons in the Spectra of Exciton–Polariton Luminescence

A cascade fiber-optic system that generates pulses of high spectral density by using the effect of nonlinear spectral compression is proposed. It is demonstrated that the shape of the pulse envelope substantially influences the degree of compression of its spectrum. In so doing, maximum compression is achieved for parabolic pulses. The cascade system includes an optical fiber exhibiting normal dispersion that decreases along the fiber length, thereby ensuring that the pulse envelope evolves toward a parabolic shape, along with diffraction gratings and a fiber spectral compressor. Based on computer simulation, we determined parameters of cascade elements leading to maximum spectral density of radiation originating from a subpicosecond laser pulse of medium energy.     

Anderson Localization in a Two-Dimensional Electron–Hole System

JETP Letters - Anderson localization is discovered in a highly disordered two-dimensional electron–hole system in a HgTe quantum well. The behavior of this localization is fundamentally...     

Dynamics of a Spinor Exciton–Polariton System in Laterally Strained GaAs Microcavities under Resonant Photoexcitation

The evolution of the spatial coherence and the polarization has been studied in a freely decaying polariton condensate that is resonantly excited by linearly polarized picosecond laser pulses at the lower and upper sublevels of the lower polariton branch in a high-Q GaAs-based microcavity with a reduced lateral symmetry without excitation of the exciton reservoir. It is found that the condensate inherits the coherence of the exciting laser pulse at both sublevels in a wide range of excitation densities and retains it for several dozen picoseconds. The linear polarization of the photoexcited condensate is retained only in the condensate at the lower sublevel. The linearly polarized condensate excited at the upper sublevel loses its stability at the excitation densities higher a threshold value: it enters a regime of internal Josephson oscillations with strongly oscillating circular and diagonal linear degrees of polarization. The polariton–polariton interaction leads to the nonlinear Josephson effects at high condensate densities. All the effects are well described in terms of the spinor Gross–Pitaevskii equations. The cause of the polarization instability of the condensate is shown to be the spin anisotropy of the polariton–polariton interaction.     

Terahertz Cyclotron Photoconductivity in a Highly Unbalanced Two-Dimensional Electron–Hole System

The magnetic properties of the α-Fe₂O₃ hematite at a high hydrostatic pressure have been studied by synchrotron Mössbauer spectroscopy (nuclear forward scattering (NFS)) on iron nuclei. Time-domain NFS spectra of hematite have been measured in a diamond anvil cell in the pressure range of 0–72 GPa and the temperature range of 36–300 K in order to study the magnetic properties at a phase transition near a critical pressure of ~50 GPa. In addition, Raman spectra at room temperature have been studied in the pressure range of 0–77 GPa. Neon has been used as a pressure-transmitting medium. The appearance of an intermediate electronic state has been revealed at a pressure of ~48 GPa. This state is probably related to the spin crossover in Fe³⁺ ions at their transition from the high-spin state (HS, S = 5/2) to a low-spin one (LS, S = 1/2). It has been found that the transient pressure range of the HS–LS crossover is extended from 48 to 55 GPa and is almost independent of the temperature. This surprising result differs fundamentally from other cases of the spin crossover in Fe³⁺ ions observed in other crystals based on iron oxides. The transition region of spin crossover appears because of thermal fluctuations between HS and LS states in the critical pressure range and is significantly narrowed at cooling because of the suppression of thermal excitations. The magnetic P–T phase diagram of α-Fe₂O₃ at high pressures and low temperatures in the spin crossover region has been constructed according to the results of measurements.     

Nonlinear Dynamics of Parametric Oscillations of Exciton–Polaritons in a Semiconductor Microcavity

Journal of Experimental and Theoretical Physics - The polariton dynamics in a microcavity in the parametric oscillator mode is studied when two pump polaritons turn into polaritons of signal and...     

Effect of Cluster Coulomb Fields on Electron Acceleration in Laser-Cluster Interaction

Single particle simulations are used to investigate electron acceleration in the laser-cluster interaction, taking into account the Coulomb fields around individual clusters. These Coulomb fields are induced from the cluster cores with positive charge when electrons escape from the cluster cores through ponderomotive push from the laser field. These Coulomb fields enable some stripped electrons to be stochastically in phases with the laser fields so that they can gain net energy from the laser efficiently. In this heating mechanism, circularly polarized lasers, larger cluster size and higher cluster densities make the acceleration more efficient.     

Vacuum Rabi Splitting and Kerr Effect of a Hybrid Spin–Magnon–Photon System

The vacuum Rabi splitting and Kerr effect are investigated theoretically in a hybrid spin–magnon–photon system, where the nitrogen-vacancy center in diamond driven by two light fields is coupled to a spherical micromagnet embedded in a superconducting coplanar waveguide resonator. The results indicate that the phenomenon of the Mollow triplet and vacuum Rabi splitting can appear by controlling the spin–magnon coupling and magnon–photon coupling. It is shown that the probe absorption spectrum can be adjusted effectively via the pump frequency detuning. Moreover, it is demonstrated that the optical Kerr effect can be tuned by changing the Rabi frequency. This work may provide a possibility for the applications in quantum information processing and quantum sensing of magnetic signal.     

Double Electron–Electron Resonance Between Trapped Electron and Hole in a Semiconductor

We demonstrate the spin interactions between dispersedly trapped electrons and holes in a semiconductor using the double electron–electron resonance (DEER) method of the pulsed electron paramagnetic resonance (EPR) techniques. An aluminum-doped titanium dioxide crystal is adopted as a spin system, in which optically generated electrons and holes are trapped, to reveal EPR signals that appear close to each other at a selected crystal orientation under an external magnetic field. We used the four-pulse DEER method by applying two microwave frequencies to a microwave cavity for pumping electrons and probing holes at the optimum temperature of 32 K. The dipolar modulation in the probed signal by pumping interacting spins was successfully detected. The observed non-oscillating decay shape indicates that the detected interaction is caused by widely distributed trapped electron and hole spins over long distances. We were able to extract a spin-pair distribution function by the first derivative of a background-corrected curve, referring to a previously reported method.     

Interactions between Surface Impurities and the Electron–Hole System of a Semiconductor Crystal

The effects of creation and annihilation of impurities on the surface of a highly doped semiconductor under changes in the surface concentration n of dopant atoms constituting impurities are predicted theoretically. The effects are determined by electrostatic interactions of charged surface impurity species with charge carriers and semiconductor ions. The effects are observed in a certain range of n, provided the surface impurities exhibit donor (acceptor) properties, and the semiconductor is doped with an acceptor (donor) impurity.     

Spin Chemistry Investigation of Peculiarities of Photoinduced Electron Transfer in Donor–Acceptor Linked System

Photoinduced intramolecular electron transfer in linked systems, (R,S)- and (S,S)-naproxen-N-methylpyrrolidine dyads, has been studied by means of spin chemistry methods [magnetic field effect and chemically induced dynamic nuclear polarization (CIDNP)]. The relative yield of the triplet state of the dyads in different magnetic field has been measured, and dependences of the high-field CIDNP of the N-methylpyrrolidine fragment on solvent polarity have been investigated. However, both (S,S)- and (R,S)-enantiomers demonstrate almost identical CIDNP effects for the entire range of polarity. It has been demonstrated that the main peculiarities of photoprocesses in this linked system are connected with the participation of singlet exciplex alongside with photoinduced intramolecular electron transfer in chromophore excited state quenching.     

Electron–Phonon Renormalization of the Electron Mass in a Metal beyond the Adiabatic Approximation

Journal of Experimental and Theoretical Physics - We analyze the renormalization of the electron mass due to the electron–phonon interaction and interaction constant λ associated with...     

Optical Resonant Saturation of Dipole–Dipole Broadened Transitions in High-Density Atomic Vapor

Journal of Russian Laser Research - We discuss the experimental research of an optical resonant saturation of a dipole–dipole-broadened atomic transition in the high-density rubidium vapor....     

Specific Features of Interatomic Dipole–Dipole Interaction near a Perfectly Conducting Charged Surface

Specific features of dipole–dipole interaction between two motionless point atoms located near a perfectly conducting charged plate are investigated theoretically within a consistent quantum microscopic approach. These features are analyzed on the basis of the dynamics of cooperative spontaneous decay of excited states of a diatomic quasimolecule. The decay rate is investigated as a function of the interatomic distance, the orientation angle of the quasimolecule with respect to the plane of the plate, and the distance between the quasimolecule and the plate. It is shown that the conducting plate significantly modifies the character of dipole–dipole interaction even when the plate is not charged. When the plate is charged, the Stark splitting of atomic levels leads to an additional modification of the interatomic interaction. The features observed are explained on the basis of the analysis of the spectrum of collective states of diatomic molecules.     

Entanglement Dynamics of Two V-type Atoms with Dipole–Dipole Interaction in Dissipative Cavity

In this work, a coupled system of two V-type atoms with dipole–dipole interaction in a dissipative single-mode cavity, which couples with an external environment, is studied. The analytical solution of this model is obtained by solving the time dependent Schrodinger equation after Hamiltonian of dissipative cavity is diagonalized by introducing a set of new creation and annihilation operators according to Fano theorem. It is also discussed in detail how the entanglement dynamics of different initial states are influenced by the cavity-environment coupling, the spontaneously generated interference (SGI) parameter, and the dipole–dipole interaction between two atoms . The results show that the SGI parameter has different effects on entanglement dynamics under different initial states. Namely, the SGI parameter will increase the decay rate of the initially maximal entangled state and reduce that of the initially partial entangled state. For the initially product state, the larger SGI parameter corresponds to the more entanglement generated. The entanglement monotonically decreases under the weak cavity-environment coupling, while the oscillation of entanglement will occur under the strong cavity-environment coupling. The larger the dipole–dipole interaction is, the slower the entanglement decays and the more the entanglement will be generated. So the dipole–dipole interaction can not only protect and generate entanglement very effectively, but also enhance the regulation effect of the SGI parameter on entanglement.     

Hybrid Exciton—Polaritons in a Bad Microcavity Containing the Organic and Inorganic Quantum Wells

We study the hybrid exciton-polaritons in a bad microcavity containing the organic and inorganic quantum wells,The corresponding polariton states are given.The analytical solution and numerical result of the stationary sepctum for the cavity field are finished.     

Effects of Plasmon–Exciton Interaction in the Spectra of Light Absorption by Hybrid Systems Consisting of Two- and Three-Layer Organometallic Nanoparticles

The effects of plasmon-exciton interaction on the spectra of light absorption by hybrid systems of two- and three-layer nanoparticles that consist of a metallic nucleus, the outer shells of ordered molecular dye J-aggregates, and an intermediate passive organic spacer between them is analyzed theoretically. It is established that the type of the absorption spectra and the efficiency of a near-field electromagnetic coupling between the particles in the system depends largely on the distance between the centers of concentric spheres and the direction of light polarization.     

Observation of Phase Transitions in an Electron–Hole System Associated with Dislocation Cores in Cadmium Telluride

Bulletin of the Lebedev Physics Institute - Evolution of the fine structure of dislocation microphotoluminescence lines in cadmium telluride with a decrease in the optical-excitation power density...     

Nonlinear Dynamics of Parametric Oscillations of Exciton–Polaritons in a Semiconductor Microcavity with Allowance for Decay

Optics and Spectroscopy - We have studied the dynamics of polaritons in a microcavity in the parametric oscillator regime, when the pump is carried out by two laser pulses with close frequencies....