Stable biexcitonic lasing of CuCl quantum dots under two-photon resonant excitation

We have observed ultraviolet lasing of CuCl quantum dots embedded in a NaCl single crystalline matrix. Stable ultraviolet lasing of biexciton (two e–h pairs) luminescence has been achieved below 70 K under the two-photon direct excitation of biexcitons of CuCl quantum dots. Laser action occurs with parallely cleaved surfaces of the NaCl crystalline matrix acting as an optical cavity, which shows a very high efficiency of lasing.     

Dynamics of confined excitons and biexcitons of CuCl quantum dots

We investigated the dynamics of confined excitons and biexcitons in CuCl quantum dots in an NaCl matrix by using subpicosecond pump and probe absorption spectra, and time-resolved luminescence spectra. Then temporal changes of the absorption, optical gain, and luminescence are interpreted in relation to the exciton dynamics. The optical nonlinearity is discussed in terms of the exciton-exciton interaction in the quantum dot.     

Two-photon absorption from single InGaN/GaN quantum dots

We present a study of the time-integrated and time-resolved photoluminescence properties of single-InGaN/GaN quantum dots (QDs) using two-photon spectroscopy. Two samples containing QDs produced by different growth techniques are examined. We find that two-photon excitation results in the suppression of the emission from the underlying quantum well to which the QDs are coupled and yet relatively strong QD emission is observed. This effect is explained in terms of the enhancement of two-photon absorption in QDs due to the full confinement of carriers. Furthermore, evidence of the presence of excited states is revealed from the two-photon photoluminescence excitation spectra presented in the study.     

Two-dimensional probe absorption in coupled quantum dots

We investigate the two-dimensional (2D) probe absorption in coupled quantum dots. It is found that, due to the position-dependent quantum interference effect, the 2D optical absorption spectrum can be easily controlled via adjusting the system parameters. Thus, our scheme may provide some technological applications in solid-state quantum communication.     

Quantum confined Stark effect in single self-assembled GaN/AlN quantum dots

We have experimentally and theoretically investigated quantum confined Stark effect in hexagonal self-assembled GaN/AlN quantum dots. We have observed a blueshift of up to 100 meV for vertical electric field applied against the built-in electric field while we have observed a redshift for the electric field along the built-in field. The experimental result is compared with a charge self-consistent effective mass calculation, taking into account strain, piezoelectric charge, and pyroelectric charge. The tunability of the emission energy and the exciton binding energy is discussed.     

水溶性CdTe:Mn量子点的双光子吸收

采用激发波长800 nm、脉宽50 fs、重复频率1 kHz的Ti:sapphire放大飞秒激光器作为激发光源,利用开孔Z扫描技术研究了不同粒径的CdTe:Mn量子点的非线性吸收性质。理论计算结果表明,同一生长时间CdTe:Mn量子点的双光子吸收系数是CdTe量子点的1.1倍,其双光子吸收系数随量子点尺寸的减小而增大,这是由于CdTe:Mn量子点非线性吸收属于反饱和吸收,掺杂了Mn元素,减小了表面缺陷浓度,表明掺杂量子点具有很好的双光子吸收现象。     

Optical absorptions of a biexciton quantum dot

A investigation of the linear and nonlinear optical properties for intersubband electronic transitions associated with a biexciton in a quantum dot has been performed by using the method of few-body physics. The optical absorption coefficients and the refractive index changes have been examined based on the computed energies and wave functions. It is over two orders of magnitude higher than that obtained in an exciton quantum dot. The results show that the optical absorption saturation intensity can be controlled by the confinement potential frequency and the relaxation time.     

Capacitance fluctuations in quantum dots

We discuss fluctuations of the charging energy E_C and gate voltage spacings between Coulomb oscillation conductance peaks, as computed within spin density functional theory for a realistic GaAs–AlGaAs dot. We explicitly exhibit the fluctuations in the portion of the total free energy which incorporate the interaction between the dot and its surroundings. These variations in the dot capacitance show a dispersion which is typically greater than the dispersion of the total dot charging energy.     

Anomalous quantum Hall effect induced by nearby quantum dots

Transport measurements in high magnetic fields have been performed on two-dimensional electron system (2DES) separated by a thin barrier layer from a layer of InAs self-assembled quantum dots (QDs). Clear feature of quantum Hall effect was observed in spite of presence of QDs nearby 2DES. However, both magnetoresistance, ρ_xx, and Hall resistance, ρ_xy, are suppressed significantly only in the magnetic field range of filling factor in 2DES ν<1 and voltage applied on a front gate . The results indicate that the electron state in QDs induces spin-flip process in 2DES.     

Confined states in two-dimensional flat elliptic quantum dots and elliptic quantum wires

The energy spectrum and corresponding wave functions of a flat quantum dot with elliptic symmetry are obtained exactly. A detailed study is made of the effect of ellipticity on the energy levels and the corresponding wave functions. The analytical behavior of the energy levels in certain limiting cases is obtained.     

Effect of the electron population on intraband absorption in InAs/GaAs self-assembled quantum dots

We present a comprehensive study of the intraband transitions in n-type InAs/GaAs quantum dots (QDs) with a filling varying from 0.5 to 4 electrons per dot, using both polarization-dependent absorption and photocurrent spectroscopy. Applying these complementary mid- and far-infrared spectroscopies over a wide energy range allows us to obtain a detailed picture of the intraband transitions and energy levels in self-assembled QDs.     

Selecting wave function states in open quantum dots

We study how wave function scarring in an open quantum dot is influenced as the strength of its environmental coupling is varied and show evidence for groups of wave function scars that recur periodically with gate voltage. The precise form of these scars is found to evolve with gate voltage, which we discuss in terms of the properties of the semi-classical orbits that give rise to the scars. We also provide convincing experimental evidence for a correlation between the scars and the oscillations observed in the conductance when the gate voltage is varied.     

Auxiliary field quantum Monte-Carlo simulation of interacting electrons in quantum dots

Accurate auxiliary field quantum Monte-Carlo (AFQMC) simulations of interacting electrons in quantum dots are reported. Two different formulations of this approach are presented both of which have been designed specifically for application to quantum dots. A deflation technique for calculation of anti-symmetrized traces is introduced. The auxiliary field is sampled with a hybrid algorithm and the artificial dynamics needed for use with the present formulation of AFQMC is described. The constrained path approximation is used to control the sign problem. Results for the ground state energy of two spin-polarised, interacting electrons are presented and are found to agree well with exact diagonalization results for a wide range of screening lengths. The sign problem does not appear in the regime of small screening length.     

Quantum dots in quantum well structures

Recent progress toward fabricating and characterizing quantum dots in III–V quantum well structures is reviewed. Quantum dots made by use of lithography and etching, including deep-etched, barrier-modulated, strain-induced and interdiffused quantum dots, are described. Quantum dots fabricated by growth, including natural quantum dots, dots on patterned substrates, and self-assembled dots, are discussed. Dot sizes and uniformity, energy-level splittings, and luminescence efficiencies that are now being achieved are discussed. The status of key issues, such as the energy relaxation in quantum dots, is mentioned.     

Eigenstate symmetry probed by biexciton transitions in a single quantum dot

The eigenstate symmetry in CdSe/ZnSe single quantum dots (SQDs) has been studied by low-temperature magnetoluminescence spectroscopy. Regarding both, the fine structure splitting and the polarization properties of the biexciton transition, the influence of exchange and Zeeman interaction on the eigenstate symmetry of the final state of recombination, the ground state of the single exciton, is investigated.     

Insulating state in open quantum dots and quantum dot arrays

We describe the observation of novel localization in mesoscopic quantum dots and quantum dot arrays, which are realized in high mobility GaAs/AlGaAs heterojunctions using the split‐gate technique. With a sufficient gate voltage applied to form the devices, their resistance diverges as the temperature is lowered below a degree Kelvin, behavior which we attribute to localization. Evidence for the localization is found over the entire range of gate voltage for which the dots are defined, persisting to conductances higher than 50e²/h.     

Observation of biexcitonic quantum beat in strain-induced GaAs quantum dots

Four-wave mixing in strain-induced GaAs quantum dots formed in a GaAs quantum well is studied using a highly sensitive heterodyne technique. A clear oscillation with a period of 1 ps is observed, recognized as a biexcitonic quantum beat based on its polarization dependence. The period of the beat is about 1.5 times shorter than that from the quantum well in the same sample. The beat represents direct evidence of an increase in the biexciton binding energy in the dots due to lateral confinement potential originating from the stressors.     

Disappearance of quantum chaos in coupled chaotic quantum dots

Statistical properties of the single electron levels confined in the semiconductor (InAs/GaAs, Si/SiO₂) double quantum dots (DQDs) are considered. We demonstrate that in the electronically coupled chaotic quantum dots the chaos with its level repulsion disappears and the nearest neighbor level statistics becomes Poissonian. This result is discussed in the light of the recently predicted “huge conductance peak” by R.S. Whitney et al. [Phys. Rev. Lett. 102 (2009) 186802] in the mirror symmetric DQDs.     

Optical properties of individual manganese-doped quantum dots

The magnetic state of a single magnetic ion (Mn²⁺) embedded in an individual quantum dot is optically probed using micro-spectroscopy. The fine structure of a confined exciton in the exchange field of a single Mn²⁺ ion (S=) is analyzed in detail. The exciton–Mn²⁺ exchange interaction shifts the energy of the exciton depending on the Mn²⁺ spin component and six emission lines are observed at zero magnetic field. The emission spectra of individual quantum dots containing a single magnetic Mn atom differ strongly from dot to dot. The differences are explained by the influence of the system geometry, specifically the in-plane asymmetry of the quantum dot and the position of the Mn atom. Depending on both these parameters, one has different characteristic emission features which either reveal or hide the spin state of the magnetic atom. The observed behavior in both zero field and under magnetic field can be explained quantitatively by the interplay between the exciton–Mn²⁺ exchange interaction (dependent on the Mn position) and the anisotropic part of the electron–hole exchange interaction (related to the asymmetry of the quantum dot).