共查询到18条相似文献,搜索用时 156 毫秒
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通过激光冷却技术在磁光阱中俘获原子数约107,温度约200 μK,直径约400 μm的超冷铯原子,利用超冷铯原子光缔合方法制备了激发态的超冷铯分子。实验研究了光缔合光不同扫描速率对铯分子振转光谱分辨率的影响,发现光缔合光扫描速率较慢时,铯分子振转光谱分辨率较高。通过高灵敏的雪崩光电探测器探测冷原子荧光,获得了超冷铯分子第一激发态6S1/2+6P3/2离解限0-g长程态高分辨振转光谱。为了实现受控拉曼光缔合制备超冷基态分子,光缔合激光频率需要锁定在原子-分子共振跃迁线,对超冷原子光缔合光谱进行了超低频波长调制,通过改变调制幅度和调制频率获得最优化的一阶微分信号,将该信号反馈回激光器,实现闭合环路稳频,满足了受控拉曼光缔合制备振转能级可控的基态分子的实验要求,该工作对研究受限空间中的超冷原子分子具有很重要的意义。 相似文献
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超冷分子的产生对于量子信息、分子物理和分子化学具有重要的意义。本文通过介绍超冷分子的研究进展,主要分析了光缔合产生超冷分子的特点与物理机制,详细介绍了光缔合产生冷分子过程中的光谱测量方法。 相似文献
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超冷原子光缔合光谱对于研究长程分子势能结构、分子常数和分子相关动力学过程具有重要意义.光缔合光谱的信噪比作为衡量探测技术的重要指标之一,直接影响光谱的分辨能力和探测灵敏度.利用调制荧光光谱技术获得了超冷长程铯分子超精细振转光谱.通过研究解调参数,即积分时间和灵敏度,发现解调参数对光谱信号的信噪比有重要影响,且依赖关系呈非线性.结合相关实验系统,实现了对光谱信噪比的最优化控制,为进一步研究超冷铯分子长程态振转能级结构奠定了重要的实验基础. 相似文献
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建立了超冷V型三能级原子注入的微波激射的腔场光子统计的量子理论,研究了原子相干性对光子统计性质的影响.发现腔内原子的发射概率随腔长变化的曲线中存在着共振峰和非共振平台,原子相干性对这些共振峰和非共振平台的绝对大小和相对比例具有灵活的可调性.原子发射概率的这些特点对腔场光子统计产生了直接的影响.平均光子数随腔长变化的曲线中也存在着共振峰和非共振平台;给定腔长,适当调节原子相干参量,可以使光子数分布向大、小光子数两个方向灵活地移动,平均光子数也相应地增加和减少.研究中还发现,适当选取原子相干参量,光子统计在大
关键词:
微波激射
超冷V型三能级原子
原子相干性
光子统计 相似文献
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Effect of external magnetic field on the shift of resonant frequency in photoassociation of ultracold Cs atoms
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《中国物理 B》2019,(1)
We study the influence of external magnetic field on the shift of the resonant frequency in the photoassociation of ultracold Cs atoms, which are captured in a magnetically levitated optical crossed dipole trap. With the increase of the photoassociation laser intensity, the linear variation of the frequency shift is measured by recording the photoassociation spectra of the long-range 0_u~+ state of Cs molecule below the 6S_(1/2)+ 6P_(1/2) dissociation limit at different magnetic fields.The slope of the frequency shift to the intensity of the photoassociation laser exhibits a strong dependence on the external magnetic field. The experimental data is simulated with an analytic theory model, in which a single channel rectangular potential with the tunable well depth is introduced to acquire the influence of the magnetic field on the atomic behavior in the effective range where photoassociation occurs. 相似文献
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利用光缔合超冷Cs原子形成超冷Cs2分子,采用多光子电离方法对超冷Cs2分子进行探测,对分子扩散过程中分子密度随时间的演化进行测量,获得了超冷Cs2分子的弛豫曲线.基于一个简单的模型即原子、分子样品的初始分布是位置和速度的高斯函数,通过理论模拟获得了超冷原子、分子样品的温度,测得的原子温度与释放-再俘获方法获得的结果相符合,这种方法避免了通过探测微弱分子荧光来获得分子温度的弊端,可广泛应用于超冷原子、分子样品的温度测量. 相似文献
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Suppressing the weakly bound states in the photoassociation dynamics by using a frequency cut-off laser pulse
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The photoassociation dynamics of ultracold lithium atoms controlled by a cut-off pulse has been investigated theoretically by solving numerically the time-dependent Schro¨dinger equation using the mapped Fourier grid method. The frequency components of the laser pulse close to the atomic resonance are partly cut off. Compared with the typical Gauss-type pulses, the cut-off pulse is helpful to suppress efficiently the weakly bound states and prepare the associated molecules in the lower vibrational states. Especially, the dependence of photoassociation probability on the cut-off position of the laser pulse is explored. 相似文献
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Suppressing the weakly bound states in the photoassociation dynamics by a frequency cut-off laser pulse
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The photoassociation dynamics of ultracold lithium atoms controlled by a cut-off pulse has been investigated theoretically by solving numerically the time-dependent Schrödinger equation using the mapped Fourier grid method. The frequency components of the laser pulse close to the atomic resonance are partly cut off. Compared with the typical Gauss-type pulses, the cut-off pulse is helpful to suppress efficiently the weakly bound states and prepare the associated molecules in the lower vibrational states. Especially, the dependence of photoassociation probability on the cut-off position of the laser pulse is explored. 相似文献
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Resonant coupling in the formation of ultracold ground state molecules via photoassociation 总被引:1,自引:0,他引:1
Dion CM Drag C Dulieu O Laburthe Tolra B Masnou-Seeuws F Pillet P 《Physical review letters》2001,86(11):2253-2256
We demonstrate the existence of a new mechanism for the formation of ultracold molecules via photoassociation of cold cesium atoms. The experimental results, interpreted with numerical calculations, suggest that a resonant coupling between vibrational levels of the 0+u (6s+6p1/2) and (6s+6p3/2) states enables formation of ultracold molecules in vibrational levels of the ground state well below the 6s+6s dissociation limit. Such a scheme should be observable with many other electronic states and atomic species. 相似文献
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Léonard J Walhout M Mosk AP Müller T Leduc M Cohen-Tannoudji C 《Physical review letters》2003,91(7):073203
We produce giant, purely long-range helium dimers by photoassociation of metastable helium atoms in a magnetically trapped, ultracold cloud. The photoassociation laser is detuned close to the atomic 2(3)S1-2(3)P0 line and produces strong heating of the sample when resonant with molecular bound states. The temperature of the cloud serves as an indicator of the molecular spectrum. We report good agreement between our spectroscopic measurements and our calculations of the five bound states belonging to a 0(+)(u) purely long-range potential well. These previously unobserved states have classical inner turning points of about 150a(0) and outer turning points as large as 1150a(0). 相似文献
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Salzmann W Mullins T Eng J Albert M Wester R Weidemüller M Merli A Weber SM Sauer F Plewicki M Weise F Wöste L Lindinger A 《Physical review letters》2008,100(23):233003
We demonstrate the photoassociation of ultracold rubidium dimers using coherent femtosecond pulses. Starting from a cloud of ultracold rubidium atoms, electronically excited rubidium molecules are formed with shaped photoassociation pump pulses. The excited state molecules are projected with a time-delayed probe pulse onto molecular ion states which are detected in a mass spectrometer. Coherent transient oscillations of the excited state population are observed in the wings of the pump pulse, in agreement with the time-dependent solution of the Schr?dinger equation of the excitation process. 相似文献