Absence of proton weak coupling states in93Nb

The reactions⁹³Nb(p, p)⁹³Nb,⁹³Nb(p, n)⁹³Mo, and⁹³Nb(p, p′) through isobaric analog resonances in⁹⁴Mo have been used to study the structure of low-lying⁹³Nb states, specifically the degree to which these states can be described as single protons coupled to the core states of⁹²Zr. Excitation curves were obtained from 5.8 to 7.6 MeV incident proton energy, for eight states in⁹³Nb. Results of this work are compared to results from Coulomb excitation studies,⁹³Nb(n, n′γ),⁹³Nb(d,p),⁹²Zr(³He,d),⁹⁴Mo(d,³He) and other related work.     

The decay of93g Ru,93m Ru,91g Mo,91m Mo,91g Tc and91m Tc

Decay studies on a number of short-lived odd nuclei in theN=50 region are described. The 59.6-s ⁹³Ru ground state decay was studied in detail for the first time; in these experiments the 10.8-s activity^93m Ru was discovered. The⁹¹Tc activities were also observed for the first time. The ground state and an isomeric state of this nucleus decay with nearby equal half-lives (3.14 and 3.3-min). The activities^91g Mo (16.6-min) and^95m Mo (65.1-s) have been reinvestigated. A number ofγ-rays, previously erroneously assigned to the⁹¹Mo activities, could be eliminated. A strong similarity is noted for the decay schemes of theN=49 isotones^91m Mo and^93m Ru. The energy of the 1/2^? isomeric state in⁹³Ru and theB(M4)-value of the isomeric transition fit well into the systematics of the previously knownN=49 isotones.     

High-spin states in the isotones 89Zr, 91Mo and 93Ru populated in α-particle-induced reactions

The reactions (α, 3nγ) and (α, α′nγ) on ⁸⁸Sr, ⁹⁰Zr and ⁹²Mo were used to populate excited states in ⁸⁹Zr, ⁹¹Mo and ⁹³Ru. The de-excitation of these states was studied by in-beam γ-ray spectroscopy. The short-lived radioactivity of the ⁹²Mo target was measured in order to study the decay of ⁹³Ru. Many new levels were observed, particularly in ⁹¹Mo. They are interpreted as due to the coupling of a $\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$ neutron hole with known excited states in ⁹⁰Zr, ⁹²Mo and ⁹⁴Ru.     

A study of the γ-ray decays from single particle states in 91Zr and 93Mo

Lifetimes have been measured in ⁹¹Zr and ⁹³Mo by the Doppler shift attenuation method through the ⁹⁰Zr(¹³C, ¹²C)⁹¹Zr and the ⁹²Mo(¹³C, ¹²C)⁹³Mo reactions. Gamma rays were observed in coincidence with the back scattered particles and the reactions took place at sub-Coulomb energies. The lifetimes measured in ⁹¹Zr are τ(1205) = 250⁺⁹⁰_?70 fs, τ(1467) = 280⁺¹⁶⁰_?110 fs, τ(2042) < 30 fs, τ(2558) = 180⁺⁹⁰_?60 fs. The lifetimes measured in ⁹³Mo are τ(1361) = 170⁺⁸⁰_?40 fs, τ(1494) = 60 ± 40 fs, τ(1697) = 440⁺²³⁰_?130 fs, τ(2705)=160⁺⁸⁰_?60fs These results are compared with the expectations of the shell model and the $\text{3}\text{s}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{→ 2}\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}\text{E}\text{2}$ transition is shown to be very enhanced.     

The excitation functions and Isomer ratios for neutron-induced reactions on Mo and Zr

Absolute cross sections of the reactions ⁹²Mo(n, 2n)^91m,91gMo, ⁹²Mo(n, p)⁹²Nb and ⁹²Mo(n, α)^{89m, 89g}Zr, relative cross sections of the reaction ⁹⁰Zr(n, 2n) ^89mZr and isomer ratios of the ⁹⁰Zr(n, 2n) reaction have been measured in the neutron energy range 13–15 MeV. The results for the (n, 2n) reactions are in good agreement with those of the previous studies. The present results for the (n, p) and (n, α) reactions are in disagreement with the previous works. The experimental data are analysed by the statistical model to determine the level-density parameter a, the moment of inertia ? and the strength of the γ-ray transition S_l in order to simultaneously reproduce the experimental data on the excitation function and the isomer ratio in the (n, 2n) reaction. The γ-ray competition, the yrast level and the experimental information on the excited levels of the residual nucleus in the (n, 2n) reaction are taken into account. The obtained values of a, ? and S_l are consistent with those deduced from other types of nuclear data.     

The decays of the Tz = 32 β-delayed proton precursors 83Zr, 87Mo and 91mRu

The decays of the nuclides ⁸³Zr,⁸⁷Mo and ^91mRu have been studied with singles proton counting as well as with pX and pγ coincidences. The half-lives for the three nuclides were measured to be 37.8 ± 1.1 s, 13.3 ± 0.4 s and 7.6 ± 0.8 s, respectively. The proton branch in the decay of ⁸³Zr that populates the first excited state in ⁸²Sr was measured to be (6 ± 4) % of the total delayed proton decay. The corresponding branch in the decay of ⁸⁷Mo, populating the first excited state in ⁸⁶Zr was measured to be (15 ± 8) %. Restrictions to the possible spin and parity assignments of ⁸³Zr and ⁸⁷Mo were deduced from comparisons between the experimental excited-state branches, and those predicted from a statistical model of delayed particle decay. Fits to the endpoints of the delayed proton spectra from ⁸³Zr and ⁸⁷Mo yielded values of the energy available for delayed proton decay (Q_e.c.?B_p) of 2.75 ± 0.10 MeV and 3.7 ± 0.3 MeV, respectively. Comparison between calculated and experimental proton spectra was used as an argument that the source of ⁹¹Ru activity is actually a $\text{1}\text{2}{}^{\mathrm{?}}$ isomer.     

The (d, α) reaction viewed as a two-step process

The ^{98, 97, 94}Mo(d, α)^{96, 95, 92}Nb and ⁹³Nb(d, α)⁹¹Zr reactions have been studied at 12 MeV bombarding energy. A DWBA analysis using one- and two-step processes has been carried out. The two-step process is found, in general, to dominate the one-step and together give rise to cross-section predictions within a factor of 10 of experiment. The angular distribution patterns are found to be best reproduced by DWBA predictions based on certain L-transfers (“parity violating”) associated with only the two-step process and which play but a minor role in their contribution to the overall cross section.     

Isomeric ratios of the products of (γ, xnp) reactions on 90,91Zr nuclei for a maximum bremsstrahlung energy of 84 MeV

We present the results from measuring and calculatoffing the isomeric ratios for the ^87m,g Y nucleus produced in the ⁹⁰Zr(γ, 2np)^87g,m Y and ⁹¹Zr(γ, 3np)^87g,m Y reactions, and for the ^86m,g Y nucleus produced in the ⁹⁰Zr(γ, 3np)^86g,m Y and ⁹¹Zr(γ, 4np)^86g,m Y reactions. The method of measuring the induced activity of irradiated samples with a semiconductor spectrometer based on an HPGe detector with a relative efficiency of 20% and an energy resolution of 1.9 keV for the 1332 keV ⁶⁰Co line was used to determine the isomeric ratios. The obtained results are compared to calculations using the TALYS code, employing statistical and preequilibrium model approaches.     

Elastic scattering of 3He and 4He at incident energies near the coulomb barrier

The elastic scattering of ³He and ⁴He from Zr, Mo, Cd, and Te isotopes is studied at incident energies near the Coulomb barrier. Marked differences are observed between the excitation curves of ³He and ⁴He. These differences are shown to be due to a large surface absorption in the ³He scattering. A systematic study of the size parameters deduced from the present and other ⁴He experiments shows deviations from the $\text{A}\text{1}\text{3}$ law for nuclei near closed neutron shells.     

Determination of the Products of Irradiation of Natural Molybenum By Deuterons with Energy up to 13 MeV by Means of Semiconductor Gamma- and X-Ray Spectrometry

Introduction

Among the products of irradiation of natural molýbdenum by deuterons with energies up to 13 MeV, by means γ and X-ray speclrometry were identified these radlonudldes: ⁹⁹Nb, ^92mNb, ^95m+gNb ⁹⁶Nb, ⁹⁹Mo, ¹⁰¹Mo, ⁹²Tc, ^93m+gTc, ^94m+g^>Tc, ^95m+gTc, ⁹⁶Tc, ^97mTc, ^99mTc,¹⁰¹Tc, and ⁸⁹Zr. With the more intensive lines of γ transitions of ⁹⁰Nb, ⁹⁶Nb, ^93m+gTc, ^94m+gTc, ^95m+gTc, ⁹⁹Tc and ^97mTc accurate photon energies have been established and for the lines 1475.7 and 1520.5 keV of ⁹³Tc, 820.2 keV of ^95mTc, and 96.4 keV of ^97mTc also the absolute intensities of the emitted γ were determined. By means of aluminium foils, by which the set of Mo foils had been interlaid, the atomic recoil in forward and backward direction ivas established for the 17.82 mg/cm² Mo foils and deuteron energy up to 12.7 MeV and the ion current of 3.4 μA.     

Scattering and transfer reactions for 6, 7Li + 90, 91Zr

Elastic scattering data have been measured for the ⁷Li + ⁹⁰Zr, ⁶Li + ⁹⁰Zr, and ⁶Li + ⁹¹Zr systems at E(Li) = 34 MeV. Inelastic scattering data for the ⁷Li + ⁹⁰Zr and ⁶Li + ⁹⁰Zr systems were also measured for the 2⁺(2.18 MeV) and 3^?(2.75 MeV) states in ⁹⁰Zr and the $\text{1}\text{2}{}^{\mathrm{?}}\text{(0.48}\text{MeV}\text{)}$ state in ⁷Li. Optical model analyses of the elastic scattering data and DWBA analyses for the states in ⁹⁰Zr were performed. The deduced deformation lengths for the 2⁺ state agreed with those extracted in other studies but the deformation length for the 3^? state was smaller. The ⁹⁰Zr(⁷Li, ⁶Li)⁹¹Zr angular distributions were measured for the 1.21 and 2.03 MeV states and the 2.19 MeV doublet in ⁹¹Zr. Also, ⁹⁰Zr(⁷Li, ⁶He)⁹¹Nb angular distributions were measured for the ground states, 0.10, 3.41 and 4.82 MeV states in ⁹¹Nb. The transitions well matched in angular momentum were described by finite-range DWBA calculations, while other transitions displayed the same phase problems seen with heavier ions. The extracted spectroscopic information was consistent with the results of other reaction studies. At the present energy, it was not possible to determine whether the l = 1 phase problem that occurs for heavy-ion single-nucleon transfer reactions on 2s-1d shell nuclei occurs in ⁹¹Zr also.     

Study of the excited 0+ states through conversion electron spectroscopy of neutron rich Zr and Mo fission products

A windowless Si(Li) electron detector has been used in conjunction with the gas filled fission product separator JOSEF to study totally converted transitions in Zr and Mo isotopes. The existence of twoβ-decay modes in⁹⁶Y,⁹⁸Y and¹⁰⁰Nb is confirmed. The half-lives of theβ-decaying levels feeding O ₂ ⁺ states in⁹⁶Zr and⁹⁸Zr are 6.0 ± 0.4 sec and 0.60±0.05 sec respectively. A search for other first excited O ₂ ⁺ states shows that no such states are apparent in¹⁰⁰Zr and¹⁰⁴Mo.     

Spin distribution factors for formation of metastable states of 90Y and 91Y through (n,p) reactions over neutron energies 5–15 MeV

The variations in the isomer ratio with the spin distribution factor were studied to obtain the cross-sections for formation of metastable states of ⁹⁰Y and ⁹¹Y nuclei formed respectively through ⁹⁰Zr(n,p)⁹¹Y^m and ⁹¹Zr(n,p)⁹¹Y^m reactions over the neutron energy range 5 to 15 MeV. The theoretical values of the cross-sections could be obtained very close to the respective literature experimental values by varying the spin distribution factor from 1.5 to 2.75. The limiting value of the cross-section was derived from the maximum value of the isomer ratio at that neutron energy, and for this the spin distribution factor was found to vary from 2 to 3.5 over the neutron energies 5 to 15 MeV. Using enriched zirconium targets, cross-sections for formation of ⁹⁰Y^m and ⁹¹Y^m nuclei at 14.8 MeV neutron energy were also measured in the laboratory; the values obtained are 17 ± 2 mb and 22 ± 2 mb respectively for ⁹⁰Y^m and ⁹¹Y^m. Both these values are close to the corresponding limiting cross-sections at 14 MeV neutron energy.     

A proton stripping study of92Nb

Levels up to energies of 4 MeV have been studied with the⁹¹Zr(³He,d)⁹²Nb reaction with an incident particle energy of 25.5 MeV. The product deuterons were analyzed by a split-pole spectrometer. Angular distributions were obtained for many of the transitions and compared with DWBA calculations. The assigned transferl values and spectroscopic factors were used to assign shell model structures to these levels.     

Pressure dependence of the distribution of hyperfine fields in ZrFe2 and Zr(Nb)Fe2

The pressure dependence of the hyperfine fields of⁹¹Zr and⁵⁷Fe, and of⁹³Nb as a dilute impurity, has been measured for ZrFe₂ up to 8 kbar at 4.2 K. The results suggest that Nb, like Zr, carries a magnetic moment anti-parallel to the Fe moment.     

Magnetic field dependence of the nuclear spin—lattice relaxation of 93mMo and 94,95Tc in Fe

The nuclear spin—lattice relaxations of ^93mMo$\text{Fe}$ and ^{94, 95}Tc$\text{Fe}$ at T ? 10 mK have been investigated with frequency- modulation-pulsedNMR on oriented nuclei as a function of an external magnetic field B₀. In the range 0?B₀?6kG the relaxation constant varies by a factor >10 and ?6 for ^93mMo$\text{Fe}$ and ^94,95Tc$\text{Fe}$, respectively. The high-field Korringa constants for ^93mMo, ⁹⁴Tc and ⁹⁵Tc in Fe were determined to be 2.5(4), 1.3(4) and 0.55(10) sK.     

Decay scheme of92m Nb

The beta decay of the 2^{+ 92m} Nb was reinvestigated via⁹³Nb(γ, n) reaction. The feeding of the 2⁺ 2,067 keV level of⁹²Zr was determined measuring the intensity of the 1,132 keV gamma-ray transition.     

The Zr(d,n)Nb and Zr(d,n)Nb reactions

The (d, n) reaction on ⁹⁰Zr and ⁹⁶Zr has been studied at 12 MeV deuteron bombarding energy using the neutron time-of-flight technique with an overall neutron time resolution of 1.9 ns. Angular distributions of neutron groups leading to states in ⁹¹Nb and ⁹⁷Nb were measured in the angular range between 15° and 60°. The measured cross sections were analyzed in the framework of the distorted-wave theory of stripping reactions to deduce l-values and proton spectroscopic factors of states in the residual nuclei. The results are compared with the corresponding data available from (³He, d) studies. The fractionation of the single-particle proton states and their centroid energies are determined.     

Untersuchung isobarer Analogresonanzen oberhalb derN=50-Schale mit polarisierten Protonen

In the region of isobaric analog resonances the analyzing power was measured in elastic scattering of polarized protons from the target nuclei⁸⁸Sr,⁹⁰Zr,⁹²Zr and⁹⁴Zr. From the analysis of the energy and angular dependence spin and parity values were determined for 19 pronounced resonances, isobaric analog to states in⁸⁹Sr,⁹¹Zr,⁹³Zr and⁹⁵Zr.