Gamow-Teller beta decay of 105Sn

The β-decay of ¹⁰⁵Sn was re-investigated at the ISOL facility of GSI Darmstadt by using a total absorption spectrometer. The experimental results include the half-life and β-delayed proton branching ratio of 32.7(5)s and 1.1(4) ^. 10^-4, respectively, and the contribution of electron capture to the ¹⁰⁵Sn decay of 0.420(35). The Gamow-Teller strength distribution peaking at 3.6MeV was measured, yielding a summed Gamow-Teller strength of 3.0(4). The latter data are discussed in comparison with shell-model predictions based on an empirical interaction.     

Interplay of direct and spin-flip contributions in Gamow-Teller decay to odd-odd N = Z nuclei

Strengths of Gamow-Teller decays of T_z = ±1 nuclei to T_z = 0 odd-odd nuclei have been calculated by using spherical shell model and deformed Nilsson wave functions. The role and competition of the microscopic direct and spin-flip mechanisms generating Gamow-Teller transitions are analyzed. Analytical expressions derived for the B(GT) values give useful insight into the regularities of B(GT) values along the N = Z line. The crucial role of configuration mixing is discussed.     

Breaking of the SU(4) limit for the Gamow-Teller strength in N ∼ Z nuclei

We have performed large-scale shell model calculations of the Gamow-Teller strength distributions in N ∼ Z pf -shell nuclei. These calculations were motivated by the experimental attempts to measure the low-lying GT strength for the even-even N = Z + 2 or N = Z - 2 nuclei ⁴⁶Ti , ⁵⁰Cr , ⁵⁴Fe and ⁶²Ge , where a sizable low-energy GT strength could be interpreted as reminiscence of SU(4) symmetry; in the limit of exact SU(4) symmetry the GT_- strength would be concentrated in a single transition to the lowest T = 0, J = 1⁺ state in the daughter. We confirm that the SU(4) symmetry is strongly broken by the spin-orbit interaction and by increasing neutron excess.     

On the unusual properties of the 282 keV state in <Superscript>135</Superscript>Sb

Recently the first excited state in ¹³⁵Sb has been observed at the unexpectedly low excitation energy of only 282keV and interpreted as mainly d _5/2 proton coupled to the ¹³⁴Sn core. Based on theoretical considerations it was suggested that its low excitation energy is related to a relative shift of the proton d _5/2 and g _7/2 orbits induced by the neutron excess. We have measured the lifetime of the 282keV state by the advanced time-delayed βγγ(t) method. The measured half-life, T _1/2 = 6.1(4)ns, yields exceptionally low limits of B(M1;5/2₁ ⁺→7/2₁ ⁺)≤3.0×10^-4 μ ² _N and B(E2;5/2₁ ⁺→7/2₁ ⁺)≤54e ² fm ⁴. These strongly hindered M1 and slow E2 transition rates are similar to those for the transition de-populating the first excited state at 405keV in ²¹¹Bi. Results of shell model calculations with realistic interactions are presented. The M1 decay rate was found to be extremely sensistive both to the wave function and to the M1 effective operator.     

Beta decay of the proton-rich nuclei 102Sn and 104Sn

The β decays of ¹⁰²Sn and ¹⁰⁴Sn were studied by using high-resolution germanium detectors as well as a Total Absorption Spectrometer (TAS). For ¹⁰⁴Sn, with three new β-delayed γ-rays identified, the total Gamow-Teller strength (B_GT) value of 2.7(3) was obtained. For ¹⁰²Sn, the γ-γ coincidence data were collected for the first time, allowing us to considerably extend the decay scheme. This scheme was used to unfold the TAS data and to deduce a B_GT value of 4.2(8) for this decay. This result is compared to shell model predictions, yielding a hindrance factor of 3.6(7) in agreement with those obtained previously for ⁹⁸Cd and ¹⁰⁰In. Together with the latter two, ¹⁰²Sn completes the triplet of Z ⩽ 50, N ≥ 50 nuclei with two proton holes, one proton hole and one neutron particle, and two neutron particles with respect to the doubly magic ¹⁰⁰Sn core.     

Precise atomic masses of neutron-rich Br and Rb nuclei close to the r-process path

The Penning trap mass spectrometer JYFLTRAP, coupled to the Ion-Guide Isotope Separator On-Line (IGISOL) facility at Jyv?skyl?, was employed to measure the atomic masses of neutron-rich ^85-92Br and ^94-97Rb isotopes with a typical accuracy less than 10keV. Discrepancies with the older data are discussed. Comparison to different mass models is presented. Details of nuclear structure, shell and subshell closures are investigated by studying the two-neutron separation energy and the shell gap energy.     

β-delayed proton decays of 93Pd and 92Rh

β-delayed proton precursors ⁹³Pd and ⁹²Rh were produced by the irradiation of ⁵⁸Ni with a ⁴⁰Ca beam, and identified using proton-gamma coincidence measurements in combination with a helium-jet fast tape transport system. The half-lives of ⁹³Pd and ⁹²Rh were determined to be 1.3(2), 3.0(8) s, respectively. The measured energy spectrum of β-delayed protons and the estimated relative branching ratios to the final states in the daughter nuclei were fitted by a statistic model calculation, and then the ground-state spin and parity of ⁹³Pd were assigned as 9/2^±. Received: 13 April 2001 / Accepted: 22 August 2001     

Systematics of related high-spin isomers in 144Sm and other N = 82 nuclei

An in-beam experiment with the reaction ¹²²Sn(²⁷Al,4np) at 127 MeV was performed at the Nordball multi-detector array in Roskilde. It provided evidence for a new high-spin isomer in ¹⁴⁴Sm. This isomer with T _1/2= (2.6 ± 0.5) ns at an excitation energy E _x= 9232 keV seems to belong to a family of isomers of similar configuration in neighbouring N= 82 nuclei. Received: 16 November 1997     

Shell-model structure of exotic nuclei beyond <Superscript>132</Superscript>Sn

We report on a study of exotic nuclei around doubly magic ¹³²Sn in terms of the shell model employing a realistic effective interaction derived from the CD-Bonn nucleon-nucleon potential. The short-range repulsion of the bare potential is renormalized by constructing a smooth low-momentum potential, V_low-k, that is used directly as input for the calculation of the effective interaction. In this paper we focus attention on the nuclei ¹³⁴Sn and ¹³⁵Sb which, with an N/Z ratio of 1.68 and 1.65, respectively, are at present the most exotic nuclei beyond ¹³²Sn for which information exists on excited states. Comparison shows that the calculated results for both nuclei are in very good agreement with the experimental data. We present our predictions of the hitherto unknown spectrum of ¹³⁶Sn.     

New states in heavy Cd isotopes and evidence for weakening of the N = 82 shell structure

A chemically selective laser ion source has been used in a β-decay study of heavy Ag isotopes into even-even Cd nuclides. Gamma-spectroscopic techniques in time-resolving event-by-event and multiscaling modes have permitted the identification of the first 2⁺ and 4⁺ levels in ¹²⁶Cd₇₈, ¹²⁸Cd₈₀, and tentatively the 2⁺ state in ¹³⁰Cd₈₂. From a comparison of these new states in ₄₈Cd with the E(2⁺) and E(4⁺)/E(2⁺) level systematics of ₄₆Pd and ₅₂Te isotopes and several recent model predictions, possible evidence for a weakening of the spherical N = 82 neutron-shell below double-magic ¹³²Sn is obtained. Received: 13 July 2000 / Accepted: 12 October 2000     

Beta decay of 101Sn

The β decay of the very neutron-deficient isotope ¹⁰¹Sn was studied at the GSI on-line mass separator using silicon detectors for recording charged particles and germanium detectors for γ-ray spectroscopy. Based on the β-delayed proton data the production cross-section of ¹⁰¹Sn in the ⁵⁰Cr + ⁵⁸Ni fusion-evaporation reaction was determined to be about 60nb. The half-life of ¹⁰¹Sn was measured to be 1.9(3)s. For the first time β-delayed γ-rays of ¹⁰¹Sn were tentatively identified, yielding weak evidence for a cascade of 352 and 1065keV transitions in ¹⁰¹In. The results for the ¹⁰¹Sn decay as well as those from previous work on the ¹⁰³Sn decay are discussed by comparing them to predictions obtained from shell model calculations employing a new interaction in the ⁸⁸Sr to ¹³²Sn model space.     

(EC + β+) decay of 133Sm and 1.1 s isomer of 133Pr

The very neutron-deficient isotope ¹³³Sm was produced by irradiation of an enriched target of ⁹⁶Ru with ⁴⁰Ca and studied by using a helium-jet fast tape transport system in combination with X-γ and γ-γ coincidence measurements. A simple ( EC + β⁺) decay scheme of ¹³³Sm was proposed for the first time. As a by-product ¹³³Pr was produced simultaneously because of the ^98-102Ru content of the ruthenium target. The half-life of a 11/2^- low-lying isomeric state in ¹³³Pr was measured to be 1.1±0.2 s. Received: 22 March 2001 / Accepted: 18 July 2001     

Nonmesonic decay of the Λ-hyperon in hypernuclei produced by p + Au collisions

The β-delayed proton precursor ¹⁴⁹Yb was synthesized in the reaction ¹¹²Sn(⁴⁰Ca, 3n) and identified by using a proton-gamma coincidence measurements in combination with a helium-jet fast tape transport system. Its β-delayed proton spectrum was observed. The half-life of ¹⁴⁹Yb was determined to be 0.7±0.2 s. The 253, 101, and 365 keV γ transitions in ¹⁴⁷Dy, following β-delayed proton emission of ¹⁴⁸Ho decay, were reported for the first time. Received: 14 March 2001 / Accepted: 26 September 2001     

Decay study of neutron-rich zirconium isotopes employing a Penning trap as a spectroscopy tool

A new technique to produce isobarically pure ion beams for decay spectroscopy by using a gas-filled Penning trap was commissioned at the ion guide isotope separator on-line facility, IGISOL. β-decays of neutron-rich ¹⁰⁰Zr, ¹⁰²Zr and ¹⁰⁴Zr isotopes were studied with this technique. In addition, the values of ^100,102,104Zr β-decays were determined from the direct mass measurements of zirconium and niobium isotopes performed with a high-precision Penning trap. The mass of ¹⁰⁴Nb was directly measured for the first time and the obtained mass excess value for the longer-living (1⁺) state is -71823±10 keV. For the ground states of ¹⁰⁰Nb and ¹⁰²Nb the obtained mass excess values were -79802±20 keV and -76309±10 keV, respectively. The observed distribution of the β strength supports a prolate deformation assignment for ^100,102,104Zr isotopes.     

β-decay half-lives of very neutron-rich isotopes of elements from Ti to Ni

The unknown β-decay half-lives of 22 isotopes far off stability (5 < T _Z < 10) in the region from Ti to Ni were measured at GSI, Darmstadt. The nuclei were produced in a fragmentation reaction of 500 A.MeV ⁸⁶Kr-projectile impinging on a thick Be target. The isotopes of interest were separated and identified with the fragment separator, FRS, by a combination of Bρ,Z, and ToF techniques. An additional range separation was performed by a selective implantation into granular detectors. The spatial and time correlations of the implant with the consecutively detected β-particles were used to determine the unknown half-lives. For nuclei far off stability, β-decay chains were measured and analyzed as well, leading to an even more reliable evaluation of the lifetimes. The large discrepancies found between the measured and the theoretical values emphasize that most recent theoretical work is not an improvement over calculations made almost a decade ago. Received: 1 October 1997     

Beta decay of 94Pd and of the 71 s isomer of 94Rh

The β decay of ⁹⁴Pd and of the 71s isomer of ⁹⁴Rh was investigated by using total γ-ray absorption techniques. Several levels in ⁹⁴Rh are established, including a new low-lying isomer characterized by a half-life of 0.48(3)μs and a de-exciting transition of 55keV. E2 multipolarity is determined for this transition by measuring the intensities of its γ-rays and the characteristic X-rays from its electron conversion. On the basis of the measured reduced β-decay transition rates to known ⁹⁴Ru levels and shell model considerations, the spin-parity of the 71s and the 0.48μs isomers of ⁹⁴Rh is assigned to be (4⁺) and (2⁺), respectively. The β-decay strength distributions measured for ⁹⁴Pd and the 71s isomer of ⁹⁴Rh yield Q _EC values of 6700(320) and 9750(320)keV for these decays and give evidence for the population of those states below and above the magic N = 50 gap that belong to both components of the 0g spin-orbit doublet.     

(EC +β+) decay study of 128Ce

The (EC+β⁺) decay of ¹²⁸Ce was reinvestigated in the ¹¹⁶Sn (¹⁶O, 4n) reaction by using a helium-jet tape transport system. The close half-lives of ¹²⁸Ce and ¹²⁹Ce made it difficult to separate the decay γ rays of both nuclei apart. Instead of the excitation-function measurements, both reactions of ¹⁶O+¹¹⁶Sn and ¹⁶O+¹¹⁷Sn were carried out, and from their comparisons, the decay γ rays of ¹²⁸Ce were clearly told from those of ¹²⁹Ce. Based on X-γ and γ-γ coincidence measurements, a detailed (EC +β⁺) decay scheme of ¹²⁸Ce has been proposed, which revises the previous one. Received: 29 September 1999 / Revised version: 5 November 1999     

Selective laser ionization of N≥82 indium isotopes: The new r-process nuclide 135In

Production yields and β-decay half-lives (T _1/2) of very neutron-rich indium isotopes were determined at CERN/ISOLDE using isobaric selectivity of a resonance-ionization laser ion-source. Beta-delayed neutron (βdn) multiscaling measurements have yielded improved T _1/2 for 206(6) ms ¹³²In, 165(3) ms ¹³³In and 141(5) ms ¹³⁴In. With 92(10) ms ¹³⁵In, a new r-process nuclide has been identified which acts as an important “waiting point” in the In isotopic chain for neutron densities in the range n _n≃ 10²⁴-10²⁶ n/cm³, where the r-matter flow has already passed the A≃ 130 abundance peak region. Received: 17 January 2002 / Accepted: 30 January 2002     

Microscopic calculations of weak interaction rates of nuclei in stellar environment for A = 18 to 100

We report here the microscopic calculation of weak interaction rates in stellar matter for 709 nuclei with A = 18 to 100 using a generalized form of proton-neutron quasiparticle RPA model with separable Gamow-Teller forces. This is the first ever extensive microscopic calculation of weak rates calculated over a wide temperature-density grid which includes 10⁷≤ T(K) ≤ 30 × 10⁹ and 10 ≤ρ Y_e (gcm⁻³) ≤ 10¹¹, and over a larger mass range. Particle emission processes from excited states, previously ignored, are taken into account, and are found to significantly affect some β decay rates. The calculated capture and decay rates take into consideration the latest experimental energy levels and ft value compilations. Our calculation of electron capture and β-decay rates, in the fp-shell, show considerable differences with a recently reported shell model diagonalization approach calculation. Received: 16 April 1999