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1.
Low-dimensional phases engineering for improving the emission efficiency and stability of quasi-2D perovskite films
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The two-dimensional (2D) Ruddlesden-Popper-type perovskites, possessing tunable bandgap, narrow light emission, strong quantum confinement effect, as well as a simple preparation method, are identified as a new generation of candidate materials for efficient light-emitting diodes. However, the preparation of high-quality quasi-2D perovskite films is still a challenge currently, such as the severe mixing of phases and a high density of defects within the films, impeding the further promotion of device performance. Here, we prepared the quasi-2D PEA2MAn-1PbnBr3n+1 perovskite films by a modified spin-coating method, and the phases with large bandgap were effectively suppressed by the vacuum evaporation treatment. We systematically investigated the optical properties and stability of the optimized films, and the photoluminescence (PL) quantum yield of the treated films was enhanced from 23% to 45%. We also studied the emission mechanisms by temperature-dependent PL spectra. Moreover, the stability of films against moisture, ultraviolet light, and heat was also greatly improved. 相似文献
2.
Kangqiao Cheng 《中国物理 B》2022,31(6):67104-067104
Quantum critical phenomena in the quasi-one-dimensional limit remain an open issue. We report the uniaxial stress effect on the quasi-one-dimensional Kondo lattice CeCo$_2$Ga$_8$ by electric transport and AC heat capacity measurements. CeCo$_2$Ga$_8$ is speculated to sit in close vicinity but on the quantum-disordered side of a quantum critical point. Upon compressing the ${c}$ axis, parallel to the Ce-Ce chain, the onset of coherent Kondo effect is enhanced. In contrast, the electronic specific heat diverges more rapidly at low temperature when the intra-chain distance is elongated by compressions along ${a}$ or ${b}$ axis. These results suggest that a tensile intra-chain strain ($\varepsilon_c >0$) pushes CeCo$_2$Ga$_8$ closer to the quantum critical point, while a compressive intra-chain strain ($\varepsilon_c<0$) likely causes departure. Our work provides a rare paradigm of manipulation near a quantum critical point in a quasi-1D Kondo lattice by uniaxial stress, and paves the way for further investigations on the unique feature of quantum criticality in the quasi-1D limit. 相似文献
3.
Quasi-Two-Dimensional Diffusion in Adherent Cells Revealed by Three-Dimensional Single Quantum Dot Tracking
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Intracellular diffusion is critical for molecule translocation in cytoplasm and mediates many important cellular processes.Meanwhile,the diffusion dynamics is affected by the heterogeneous cytoplasm.Previous studies on intracellular diffusion are mainly based on two-dimensional(2 D) measurements under the assumption that the three-dimensional(3 D) diffusion is isotropic.However,the real behaviors of 3 D diffusion of molecules in cytoplasm are still unclear.Here,we have built a 3 D single-particl... 相似文献
4.
This brief review summarizes recent theoretical and experimental results which predict and establish the existence of quantum droplets (QDs), i.e., robust two- and three-dimensional (2D and 3D) selftrapped states in Bose–Einstein condensates (BECs), which are stabilized by effective self-repulsion induced by quantum fluctuations around the mean-field (MF) states [alias the Lee–Huang–Yang (LHY) effect]. The basic models are presented, taking special care of the dimension crossover, 2D→3D. Recently reported experimental results, which exhibit stable 3D and quasi-2D QDs in binary BECs, with the inter-component attraction slightly exceeding the MF self-repulsion in each component, and in single-component condensates of atoms carrying permanent magnetic moments, are presented in some detail. The summary of theoretical results is focused, chiefly, on 3D and quasi-2D QDs with embedded vorticity, as the possibility to stabilize such states is a remarkable prediction. Stable vortex states are presented both for QDs in free space, and for singular but physically relevant 2D modes pulled to the center by the inverse-square potential, with the quantum collapse suppressed by the LHY effect. 相似文献
5.
Il Nuovo Cimento D - We develop the bipolariton concept for a quasi-2D excitonic molecule (m) in quantum wells (QWLs). The bipolariton wave equation, which includes both the exciton-exciton (x-x)... 相似文献
6.
Dimensionality serves as an indispensable ingredient in any attempt to formulate low-dimensional physics, and studying the dimensional crossover at a fundamental level is challenging. The purpose of this work is to study the hierarchical dimensional crossovers, namely the crossover from three dimensions (3D) to quasi-2D and then to 1D. Our system consists of a 3D Bose–Einstein condensate trapped in an anisotropic 2D optical lattice characterized by the lattice depths V1 along the x direction and V2 along the y direction, respectively, where the hierarchical dimensional crossover is controlled via V1 and V2. We analytically derive the ground-state energy, quantum depletion and the superfluid density of the system. Our results demonstrate the 3D-quasi-2D-1D dimensional crossovers in the behavior of quantum fluctuations. Conditions for possible experimental realization of our scenario are also discussed. 相似文献
7.
《Superlattices and Microstructures》2001,30(4):169-179
Nanoprobe near-field photoluminescence (PL) of InGaAs(P) dots with quasi-zero-dimensional (quasi-0D) confinement with various degrees of 0D/2D has been investigated by studying probe-induced pressure effects and probe-bias effects. Fine PL peaks of 0D confinement are superimposed on quantum well (QW) peaks for quasi-0D structures, which proves the coexistence of 0D and two-dimensional (2D) confinement in the same layer. Large blue shifts of approximately 100 meV were observed to occur with pressure increase for 0D fine PL peaks, but no shift was observed for the QW peak. The fine 0D peaks were eliminated by larger probe-induced pressures, which should be attributed to carrier diffusion rather than to Γ–X crossover in energy levels. The QW peak increased with the positive probe bias, while 0D fine PL peaks showed a smaller increase with red shifts up to 8–9 meV. The results obtained can be explained by the excitation of immobile excitons in 0D potentials to mobile carriers in the 2D (QW) layer. 相似文献
8.
Huang SW Huang DJ Okamoto J Mou CY Wu WB Yeh KW Chen CL Wu MK Hsu HC Chou FC Chen CT 《Physical review letters》2008,101(7):077205
Based on resonant soft x-ray magnetic scattering, we report that LiCu2O2 exhibits a large interchain coupling which suppresses quantum fluctuations along spin chains, and a quasi-2D short-range magnetic order prevails at temperatures above the magnetic transition. These observations unravel the fact that the ground state of LiCu2O2 possesses long-range 2D-like incommensurate magnetic order rather than being a gapped spin liquid as expected from the nature of quantum spin-1/2 chains. In addition, the spin coupling along the c axis is found to be essential for inducing electric polarization. 相似文献
9.
Mao ZQ He T Rosario MM Nelson KD Okuno D Ueland B Deac IG Schiffer P Liu Y Cava RJ 《Physical review letters》2003,90(18):186601
We report the first systematic study of the electrical transport and magnetic properties of BaRu6O12, which has a quasi-one-dimensional (quasi-1D) hollandite structure. We show that BaRu6O12 is quasi-1D electronically as well. Its physical properties were found to be extremely sensitive to disorder. Furthermore, a transition from being metallic with a resistance drop around 2 K to being weakly insulating as the applied magnetic field was increased was also found. We propose that these two features are related to the possible presence of a quantum phase transition in this material system. 相似文献
10.
M.W.C. Dharma-wardana 《Solid State Communications》2005,136(2):76-80
We demonstrate a replacement of the non-uniform sub-band density of quasi-2D electron layers by an effective uniform-slab density. Exchange, correlation and Fermi-liquid properties are determined via a mapping of the electron liquid to a classical fluid, using the hyper-netted-chain equation inclusive of bridge corrections, (i.e. the CHNC), as a function of the density, spin-polarization, layer width and the temperature. Our parameters-free theory is in good accord with quantum simulations, with effective-mass and spin-susceptibility results for 2D layers found in GaAs/AlGaAs structures. 相似文献
11.
Kimura S Takeuchi T Okunishi K Hagiwara M He Z Kindo K Taniyama T Itoh M 《Physical review letters》2008,100(5):057202
High-field specific heat measurements on BaCo(2)V(2)O(8), which is a good realization of an S=1/2 quasi-one-dimensional (1D) Ising-like antifferomagnet, have been performed in magnetic fields up to 12 T along the chain and at temperature down to 200 mK. We have found a new magnetic ordered state in the field-induced phase above H(c) approximately 3.9 T. We suggest that a novel type of the incommensurate order, which is caused by the quantum effect inherent in the S=1/2 quasi-1D Ising-like antiferromagnet, appears in the field-induced phase. 相似文献
12.
S. Wessel S. Haas 《The European Physical Journal B - Condensed Matter and Complex Systems》2000,16(3):393-396
Three-dimensional magnetic ordering transitions are studied theoretically in strongly anisotropic quantum magnets. An external
magnetic field can drive quasi-one-dimensional subsystems with a spin gap into a gapless regime, thus inducing long-range
three-dimensional magnetic ordering due to weak residual magnetic coupling between the subsystems. Compounds with higher spin
degrees of freedom, such as N-leg spin-1/2 ladders, are shown to have cascades of ordering transitions. At high magnetic fields, zero-point fluctuations
within the quasi-1D subsystems are suppressed, causing quantum corrections to the ordering temperature to be reduced.
Received 24 March 2000 相似文献
13.
By comparing the properties of In and Pb quantum wells in a scanning tunneling microscopy subsurface imaging experiment, we found the existence of lateral bound states, a 2D Mott-Hubbard correlation gap, induced by transverse confinement. Its formation is attributed to spin or charge overscreening of quasi-2D excitations. The signature of the 2D confinement-deconfinement transition is also experimentally observed, with the correlation gap being pinned in the middle of the conduction band. A self-organized 2D Anderson lattice is suggested as a new ground state. 相似文献
14.
Bose gases confined in highly elongated harmonic traps are investigated over a wide range of interaction strengths using quantum Monte Carlo techniques. We find that the properties of a Bose gas under tight transverse confinement are well reproduced by a 1D model Hamiltonian with contact interactions. We point out the existence of a unitary regime, where the properties of the quasi-1D Bose gas become independent of the actual value of the 3D scattering length a(3D). In this unitary regime, the energy of the system is well described by a hard-rod equation of state. We investigate the stability of quasi-1D Bose gases with positive and negative a(3D). 相似文献
15.
Z.-Ch. Wang H.-W. Yang S. Yin 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2002,20(1):117-119
Starting from the Gross-Pitaevskii energy functional of the 3D Bose-Einstein Condensate, we derive approximately the energy
functional and the effective coupling constant of the quasi-2D condensate. The evolution of the quasi-2D condensate wave function
is studied by a variational method. Low energy excitation spectra for both positive and negative scattering lengths are analyzed.
The condition of collapse instability of a quasi-2D Bose gas with attractive particle interaction is also proposed.
Received 31 October 2001 / Received in final form 1st March 2002 Published online 28 June 2002 相似文献
16.
We demonstrate that scattering of particles strongly interacting in three dimensions (3D) can be suppressed at low energies in a quasi-one-dimensional (1D) confinement. The underlying mechanism is the interference of the s- and p-wave scattering contributions with large s- and p-wave 3D scattering lengths being a necessary prerequisite. This low-dimensional quantum scattering effect might be useful in "interacting" quasi-1D ultracold atomic gases, guided atom interferometry, and impurity scattering in strongly confined quantum wire-based electronic devices. 相似文献
17.
Rüegg Ch McMorrow DF Normand B Rønnow HM Sebastian SE Fisher IR Batista CD Gvasaliya SN Niedermayer Ch Stahn J 《Physical review letters》2007,98(1):017202
The compound BaCuSi2O6 is a quantum magnet with antiferromagnetic dimers of S=1/2 moments on a quasi-2D square lattice. We have investigated its spin dynamics by inelastic neutron scattering experiments on single crystals with an energy resolution considerably higher than in an earlier study. We observe multiple magnon modes, indicating clearly the presence of magnetically inequivalent dimer sites. The more complex spin Hamiltonian revealed in our study leads to a distinct form of magnon Bose-Einstein condensate phase with a spatially modulated condensate amplitude. 相似文献
18.
Dimensional crossover of a Rabi-coupled two-component Bose–Einstein condensate in an optical lattice
Dimensionality is a central concept in developing the theory of low-dimensional physics.However,previous research on dimensional crossover in the context of a Bose-Einstein condensate(BEC) has focused on the single-component BEC.To our best knowledge,further consideration of the two-component internal degrees of freedom on the effects of dimensional crossover is still lacking.In this work,we are motivated to investigate the dimensional crossover in a three-dimensional(3D) Rabi-coupled two-compon... 相似文献
19.
F. Heidrich-Meisner A. Honecker W. Brenig 《The European physical journal. Special topics》2007,151(1):135-145
We present numerical results for the spin and thermal conductivity of
one-dimensional (1D) quantum spin systems. We contrast the properties of
integrable models such as the spin-1/2 XXZ chain against nonintegrable ones such as
frustrated and dimerized chains. The thermal conductivity of the XXZ chain
is ballistic at finite temperatures, while in the nonintegrable models, this quantity is argued
to vanish. For the case of frustrated and dimerized chains, we discuss
the
frequency dependence of the transport coefficients. Finally, we give an overview over related theoretical
work on intrinsic and extrinsic scattering mechanisms of quasi-1D spin systems. 相似文献
20.
We calculate the superfluid transition temperature for a two-component 3D Fermi gas in a 1D tight optical lattice and discuss a dimensional crossover from the 3D to quasi-2D regime. For the geometry of finite size discs in the 1D lattice, we find that even for a large number of atoms per disc the critical effective tunneling rate for a quantum transition to the Mott insulator state can be large compared to the loss rate caused by three-body recombination. This allows the observation of the Mott transition, in contrast to the case of Bose-condensed gases in the same geometry. 相似文献