光纤中受激拉曼散射连续谱研究

我们在实验中研究了自相位调制效应和受激四光子混频效应对受激拉曼散射光谱的影响。在较强的泵浦光和适当的入射条件下,得到九阶受激拉曼散射的级联 Stokes 连续平滑谱带,带宽3500cm~(-1),其强度可与530nm 泵浦光强相比拟。     

受激旋转拉曼散射对强紫外激光相位的影响

 利用瞬态受激旋转拉曼散射（SRRS）模型及相位畸变模型,对具有空间相位畸变的强紫外激光束在空气中长程传输的SRRS效应进行了研究。详细讨论了低频和中高频空间相位畸变对SRRS阈值条件、斯托克斯光转换效率、剩余泵浦光和斯托克斯光相位的影响。研究结果表明,泵浦光的初始相位畸变对斯托克斯光相位畸变的影响较剩余泵浦光的更为明显;高频相位畸变对转换效率影响较低频相位畸变更大; SRRS效应阈值随低频相位畸变的增大而减小,随高频相位畸变的增大而增大。     

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介绍了在神光Ⅱ装置上开展的长脉冲2ns三倍频激光与黑腔靶相互作用的实验。报道了采用PIN探测器阵列测量大角度受激Raman散射（SRS）角分布和采用激光卡计对背向SRS光能量积分测量的实验结果。相同实验条件下激光辐照缝靶产生的SRS光能量要强于激光与全腔靶作用产生的SRS光，小腔靶的SRS光能量要强于标准腔靶。对比长脉冲2ns及短脉冲1ns激光打靶实验结果可以看出：由于激光功率密度的下降，长脉冲激光打靶时SRS散射光能量要弱于短脉冲激光打靶。长脉冲2ns激光与标准腔靶相互作用时，等离子体堵腔比较严重。     

组合型光纤相位共轭器的数值模拟

 组合光纤是一种结合了小口径光纤SBS阈值低和大口径光纤损伤阈值高的特点而形成的新型光纤相位共轭器。通过建立数学模型，数值计算了组合光纤中SBS形成的过程，并对其特性参数进行了一定的理论分析。结果表明组合光纤不但可以大幅度降低SBS阈值、获得高反射率和扩大动态范围，而且通过优化其几何尺寸可以抑制Stokes波形的波动现象并显著压缩泵浦光脉冲。     

Gigantic stimulated Raman scattering in one-dimensional Mott-Hubbard insulators: A possible THz source

One-dimensional Mott-Hubbard insulators like Sr₂CuO₃, halogen-bridged Nickel chain compounds have orders-of-magnitude nonlinear optical properties compared to other one-dimensional organic or inorganic compounds. We show theoretically, that the stimulated Raman scattering susceptibility for such insulators could be order(s)-of-magnitude larger even compared to other nonlinear optical susceptibilities. The lowest two-photon state is at lower energy than the lowest one-photon state in some of these insulators. This leads to a potential for strong Stokes generation in the THz regime from these compounds. Our results and conclusions are based on exact numerical solution of finite size two-band extended Hubbard model.     

Effect of pulse walk off and data formats on stimulated Raman scattering in fiber optic communication systems

A novel numerical method has been presented here which is capable of taking into account pulse walk off effect and different data formats such as non return to zero (NRZ), return to zero (RZ) and optical Manchester while evaluating the effect of stimulated Raman scattering (SRS) in dense wavelength division multiplexed (DWDM)-based fiber optic communication systems. Power tilt because of SRS effect in the DWDM systems has been calculated at different data rates and data formats.     

Soliton experiments in stimulated Raman scattering

Experimental observations of solitons in stimulated Raman scattering are reported. Soliton formation resulted from the introduction of a phase shift in the incident Stokes beam as predicted by theory. Pulse sharpening and retardation on propagation in the Raman medium have been observed along with amplitude diminution. The first two features were predicted and the third was not. Spontaneous soliton formation has been observed in the absense of any amplitude modulation or apparent phase shift in the optical fields, indicating that additional sets of initial conditions may result in soliton formation.Work performed under the auspices of the U.S. Department of Energy.     

受激旋转拉曼散射效应对基频光光束质量的影响

 采用瞬态受激旋转拉曼散射(SRRS)和空间相位扰动模型,定量分析了泵浦光强度和脉冲宽度对基频光在空气长程传输过程中产生的SRRS效应的阈值距离和转换效率的影响,讨论了泵浦光空间相位畸变对长程传输后的基频光光束质量的影响。研究结果表明：SRRS效应的阈值距离随着泵浦光强度和脉宽的增大而变短;空间相位畸变对斯托克斯光和泵浦光的光强分布存在一定影响,对斯托克斯光相位分布的影响比对泵浦光相位的影响大;SRRS效应的存在将导致基频光光束质量明显变差,对谐波转换效率产生明显影响。     

351nm激光入射大腔靶的受激Raman散射光谱

 报道了“神光 Ⅱ”装置上Au大柱腔靶产生的受激Raman散射光谱。通过分析实验条件和测量结果，排除了散射光谱来自增强非相干Thomson散射的可能性，发现用丝化不稳定性与受激Raman散射的耦合能合理解释观测到的Raman光谱。考虑到丝化不稳定性与SRS的耦合，测量到的散射光谱依然能用于密度诊断，其结果与对流SRS理论的计算值相差不到10%。     

Optimization of a Raman/EDFA hybrid amplifier based on dual-order stimulated Raman scattering using a single-pump

Based on dual-order stimulated Raman scattering (SRS) of a single 1395 nm Raman fiber laser in 75 km single mode fiber and its corresponding dispersion compensation module, a hybrid Raman/Erbium doped fiber amplifier (EDFA) for long wavelength band (L-band) amplification is realized by inserting a segment of EDF within the span. By comparing the performance of gain and noise in four hybrid amplifiers with different span configurations, we find that the distribution of the secondary L-band amplification obtained from the EDF along the link has a great influence on the performance of the hybrid amplifier. Both gain and noise performance of hybrid amplifier can be improved significantly by optimizing the location of the EDF. Moreover, we can extend the flat gain bandwidth from L-band to central wavelength band (C-band) plus L-band by recycling the residual first-order SRS to pump a segment of EDF with proper length.     

水中受激拉曼散射的能量增强及受激布里渊散射的光学抑制

为提高液体介质中受激拉曼散射的输出能量,提出了通过温度调控来抑制受激布里渊散射的方法,设计了532 nm多纵模宽带脉冲激光泵浦的受激拉曼散射发生系统,测量了不同温度下水中前向受激拉曼散射及后向受激布里渊散射的输出能量,分析了水温、泵浦激光线宽及热散焦效应对受激拉曼散射输出能量影响的物理机制.实验结果表明:通过降低水温可实现对受激布里渊散射过程的有效抑制,同时减小热散焦效应带来的光束畸变,从而有效提高受激拉曼散射的输出能量.研究结果对液体介质中的受激拉曼散射多波长转换具有重要意义.     

Electron Raman scattering of a hydrogenic impurity in a disc-shaped quantum dot

We have carried out the theoretical calculation of the differential cross section for the electron Raman scattering process associated with a hydrogenic impurity in a disc-shaped quantum dot (QD). We consider the impurity states confined in a disc-shaped QD with parabolic potential in the presence of an external electric field. Effects of the electric field and the confinement strength on the differential cross section are investigated. We make a comparison about the Raman intensity between with and without the Coulomb interaction. We found that the differential cross section of the hydrogenic impurity in a disc-shaped QD dependent strongly on the confinement strength, the external electric field intensity and the Coulomb interaction.     

Performance of an optical wideband WDM system considering stimulated Raman scattering,fiber attenuation and chromatic dispersion

The performance of an optical wideband wavelength division multiplexed (WDM) communication system is analyzed considering the effects of stimulated Raman scattering, fiber attenuation and chromatic dispersion. Improved models for the Raman gain and the fiber attenuation constant are proposed, which yield better and reliable performance results of the WDM system. Effect of fiber chromatic dispersion is also investigated and it is observed that dispersion can suitably be selected to overcome the limitations imposed by the stimulated Raman scattering phenomenon.     

Electric field effect on the Raman scattering of a hydrogenic impurity in spherical quantum dot

Using the perturbation method and the effective mass approximation, we studied the combined effects of impurity and external electric field on Raman scattering in a spherical quantum dot with a parabolic potential. Based on the computed energies and wave functions, the differential cross-section involved in this process is investigated, and the selection rules are also calculated. Our results suggest that the scattering intensity is strongly affected by the impurity and external electric field considered in this work.     

碰撞对受激Raman散射的影响

从动力学方程出发，引入有效碰撞，讨论了碰撞对受激Raman散射线性增长率的影响.结果表 明，碰撞阻尼和Landau阻尼使得受激Raman散射线性增长率有了实质性的下降，受激Raman散 射只能发生在电子温度和电子密度平面的一个有限区域.现在的理论模型能够解释受激Raman 散射光谱上存在的“缝”(gap)现象. 关键词： 受激Raman散射 碰撞阻尼 线性增长率     

氢和甲烷混合气体的受激喇曼散射

使用调Q Nd~(3+):YAG激光的二次谐波(532nm)作为泵浦源,探讨了氢和甲烷混合气体的受激喇曼散射效应。利用光学光谱分析仪(OSA)监测,在不同比例的混合气体中,观测到氢和甲烷各自的SRS谱线以及两种气体的联合谱线,[m,n,=0,|±1,±2,…];观察到斯托克斯和反斯托克斯的谱线频移。实验表明两种气体的混合使得氢和甲烷的受激喇曼散射过程发生了竞争和耦合。     

金属蒸气受激喇曼散射的原子基态抽空效应

将受激Raman散射原子基态及终态粒子数变化的速率方程与聚焦的泵浦光束及喇曼光束功率变化的微分方程组联立并进行数值求解;研究了金属蒸气受激Raman散射过程中基态粒子数的抽空现象及其对Raman能量转换过程的影响。     

2 ns,351 nm激光黑腔靶受激Raman散射实验研究

 介绍了在神光Ⅱ装置上开展的长脉冲2 ns,351 nm激光与黑腔靶相互作用的实验,报道了受激Raman散射光时间分辨谱图及能量测量的实验结果。长脉冲2 ns激光注入小腔靶（Ø700 mm×1 250 mm）时,激光辐照缝靶产生的SRS光能量是激光与全腔靶作用产生的SRS光能量的1.3倍。在2 ns激光与不同尺寸黑腔靶作用的情况下,激光辐照小腔靶产生的SRS光能量比标准腔靶(Ø800 mm×1 350 mm)产生的SRS光能量高1.6倍。由于激光功率密度下降,2 ns激光打靶SRS散射光要弱于短脉冲1 ns激光打靶,但持续时间稍长。实验结果表明：长脉冲2 ns激光与标准腔靶相互作用时,等离子体“堵腔效应”比较严重,标准腔靶尺寸不再合适。     

Raman scattering from microcrystals

This review discusses the size effects on Raman scattering from microcrystals. For ionic microcrystals, the existence of surface phonon modes is predicted from electromagnetic theories. It is shown that Raman spectroscopy is very effective to detect the surface phonon modes. The size effects on nonpolar phonons in covalent microcrystals can also be studied by Raman spectroscopy. However, the relaxation of the wave-vector selection rule or the phonon confinement explains only some of the experimental data. Development of lattice dynamical theories of Raman scattering from microcrystals including surface effects is highly required. Enhancement of Raman intensities arising from the excitation of electromagnetic normal modes of microcrystals is also discussed.