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当酒精的弱增益拉曼模式处于罗丹明640染料分子的激光增益范围时,在由悬垂液滴构成的圆形谐振腔中,观察到乙醇分子C—H伸缩系列模中多个弱增益拉曼模式的受激拉曼散射(SRS)光谱.随着抽运光的增强,迅速增长的强增益拉曼模式的受激辐射抑制了其他弱增益模式的SRS,并导致染料激光的完全淬灭.通过分析圆形腔腔模的光子速率方程和激光染料分子的三能级粒子数速率方程,解释了观察到的实验现象.
关键词:
受激拉曼散射
悬垂液滴
弱拉曼增益模式
激光增益 相似文献
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详细比较了磷酸二氢钾(KDP)晶体的自发拉曼散射和受激拉曼散射光谱,在受激拉曼散射(SRS)中观察到了自发拉曼散射中最强的振动模的三阶Stokes光(559.43,589.74,623.50nm),由于其他振动模的受激拉曼散射增益系数较小,其SRS光谱未观察到。另外,比较了传统生长的未退火和退火后的KDP晶体及快速生长的锥区和柱区KDP晶体的受激拉曼散射增益系数,结果表明生长方法和热退火对KDP晶体的受激拉曼散射增益系数无明显影响。 相似文献
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为解决传统拉曼放大器增益系数低和增益不平坦的问题,采用级联光子晶体光纤的设计方法设计了一种增益平坦的拉曼光纤放大器.采用受激拉曼散射效应的稳态分析理论,分析了光子晶体光纤的拉曼增益谱,建立了拉曼放大器的理论模型.通过解耦合方程,推导了实现增益平坦的约束条件,发现光纤长度和泵浦功率是影响拉曼光纤放大器增益平坦度的两个参数.仿真结果表明,在1 508~1 544 nm的带宽范围内,实现了一个增益高达21 dB,增益平坦度仅为0.14 dB的光子晶体拉曼光纤放大器,可在光纤通信系统应用中发挥重要作用. 相似文献
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Based on dual-order stimulated Raman scattering (SRS) of a single 1395 nm Raman fiber laser in 75 km single mode fiber and its corresponding dispersion compensation module, a hybrid Raman/Erbium doped fiber amplifier (EDFA) for long wavelength band (L-band) amplification is realized by inserting a segment of EDF within the span. By comparing the performance of gain and noise in four hybrid amplifiers with different span configurations, we find that the distribution of the secondary L-band amplification obtained from the EDF along the link has a great influence on the performance of the hybrid amplifier. Both gain and noise performance of hybrid amplifier can be improved significantly by optimizing the location of the EDF. Moreover, we can extend the flat gain bandwidth from L-band to central wavelength band (C-band) plus L-band by recycling the residual first-order SRS to pump a segment of EDF with proper length. 相似文献
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In this study we report the first observation of spontaneous Raman solitons in stimulated Raman scattering (SRS) by the gas NH3. The scattered radiation is called Stokes radiation. Raman solitons are of considerable interest, because their existence can be explained by quantum-mechanical fluctuations of the electromagnetic field in vacuum. We have observed spontaneous Raman solitons in a forward SRS configuration for two different molecular transitions of NH3, the laser emissions at 58 μm and 72.6 μm wavelength. These are optically pumped by 10 μm CO2-laser pulses with a duration of 100 ns and an energy of 150 mJ. Spontaneous Raman solitons are short spikes in the pump pulse which occur during its depletion. Their origin is the rapid π phase change of the Stokes seed. In contrast to other laboratories we have used single-pass cells. Thus, we have succeeded in observing multiple spontaneous Raman solitons during one pump pulse. Previous experiments with multi-pass cells never showed multiple solitons. Since multiple spontaneous Raman solitons have already been reported in an earlier experiment with a single-pass cell filled with hydrogen at high pressure, we conclude that such multiple Raman solitons can be observed mainly in this type of gas cell. Subsequently, we have performed statistical measurements on the delay time and the height of the spontaneous Raman solitons in the depleted pump pulse for the 58 μm-NH3 emission. We have compared these statistics with theory and equivalent experimental results of other laboratories. They are in good agreement with the assumption that quantum-mechanical fluctuations are the origin of spontaneous Raman solitons. The most recent theories postulate that the origin of the formation of spontaneous Raman solitons can be explained by the rapid π phase change of the Stokes seed as well as that of the laser or polarization wave. Therefore, we have determined the phase of the spontaneous Raman solitons relative to the depleted pump pulse. Although, such changes of sign of the relative phase have already been observed in an earlier SRS experiment with hydrogen at high pressure, we did not detect any in our experiment. Therefore, we conclude that in this experiment the π phase change occurs in the Stokes or polarization wave. 相似文献