Magnetic moments of high-spin states above the rotational band of 168Hf and 172Hf

The transient magnetic field IMPAC technique was used to measure the magnetic moments of high-spin states above the rotational band of ¹⁶⁸Hf and ¹⁷²Hf, populated in the reactions ^{156, 160}Gd(¹⁶O, 4n). The average g-factors of these prerotational feeding states were deduced to be 0.07 ± 0.04 and 0.14 ± 0.04 for ¹⁶⁸Hf and ¹⁷²Hf, respectively. These results are in agreement with a reduction of the collective g-factors due to a neutron phase transition.     

Investigation of TmFe4Al8 and DyFe4Al8 by means of 169Tm and 161Dy Mössbauer spectroscopy

We have performed ¹⁶⁹Tm and ¹⁶¹Dy Mössbauer spectroscopy on TmFe₄Al₈ and DyFe₄Al₈. From the temperature dependence of the electric quadrupole splitting of the ¹⁶⁹Tm spectra of TmFe₄Al₈ we have determined the second order crystal field potential V⁰₂ = (100 ± 10) K and the exchange field term g_Jμ_BH_M = (1 ± 1) K. The temperature dependence of the hyperfine field of the ¹⁶¹Dy spectrum of DyFe₄Al₈ gives g_Jμ_BH_M = (15 ± 3) K. With these exchange fields magnetic transition temperatures of the rare earth sublattices were found, which are consistent with experiment. The relaxation behaviour of the Tm sublattice below T_N = 187 K is discussed.     

High spin rotational states in 154Dy, 164Er And 162Yb

High spin rotational states in ¹⁵⁴Dy, ¹⁶⁴Er and ¹⁶²Yb have been investigated with (α, 4nγ) and (α, 6nγ) reactions. The ground state rotational bands have been identified up to spin 14 for ¹⁵⁴Dy and ¹⁶²Yb and spin 16 for ¹⁶⁴Er. Anomalous behaviour of the moment of inertia has been observed in ¹⁶⁴Er.     

Measurement of the parity non-conservation in nuclear forces in 75As, 171Tm,and 175Lu and of the polarized bremsstrahlung from 51Cr, 170Tm, 177Lu,and 198Au

The circular polarization P of γ-rays from unpolarized sources of ⁷⁵Se, ¹⁷¹Er, and ¹⁷⁵Yb of strengths ? 500 Ci has been measured with a Compton polarimeter of the radial transmission type. Eight NaI crystals and a four-fold current integration system were used to simultaneously record the data in four independent channels. The results are: P = ?(1.8 ± 6.0) × 10^?5 for the 401 keV transition in ⁷⁵As (the experimental error is ± 1.5 × 10^?5, the remaining part is due to the uncertainty in the decay scheme of ⁷⁵Se), P = (0.8 ± 1.5) × 10^?4 for the 296 keV and 308 keV transition in ¹⁷¹Tm, and P = (5.7 ± 0.8) × 10^?5 for the 396 keV transition in ¹⁷⁵Lu. The last value confirms the parity non-conservation in nuclear forces. The polarimeter was calibrated with bremsstrahlung from ¹⁷⁰Tm. The correction for polarized bremsstrahlung was given special attention. Correction factors are derived for ⁵¹Cr, ¹⁷⁷Lu, and ¹⁹⁸Au from a comparison of the measured and calculated bremsstrahlung yields.     

The g-factors of the first 2+ states in 50, 54Cr, 54Fe and 70Ge

The gyromagnetic ratios of the first excited J^π = 2⁺ states of ^50,54Cr, ⁵⁴Fe and ⁷⁰Ge have been determined by the ion-implantation perturbed angular correlation technique (IMPAC) with ferromagnetic Gd as stopping material. The g-factors were extracted from the measured precession angles with use of known lifetimes, static hyperfine magnetic fields and transient hyperfine magnetic field data for fast ions traversing ferromagnetic lattices. The deduced values are 0.59 ± 0.10, 0.56 ± 0.10, 1.08±0.19 and 0.38±0.08, respectively. With the exception of ⁵⁴Fe all g-factors are close to the collective value. A re-evaluation of earlier IMPAC data on ^{70, 72, 74, 76}Ge with Fe as stopping material has been performed. The value obtained for ⁷⁰Ge is in good agreement with the one measured in this work.     

Messung der magnetischen Momente der tiefsten 2+-Zustände für einige Dy-, Er- und Yb-Isotope

With the Mössbauer technique, the hyperfine splittings of the lowest 2⁺-states of some Dy-, Er-, and Yb-isotopes were observed at 4.2 °K in the paramagnetic compounds Dy-Al-garnet, ErCl₃·6H₂O, and YbCl₃·6H₂O. Most of the sources were produced by photonuclear reactions. Ratios ofg-factors for neighbouring isotopes could be determined with small systematic errors. The results are:g ¹⁶⁴/g ¹⁶⁶=1.103 (15),g ¹⁶⁶/g ¹⁶⁸=0.960 (13) for Er, andg ¹⁷⁰/g ¹⁷²=1.009 (15),g ¹⁷⁰/g ¹⁷⁴=0.994 (13) for Yb. Using known values for the effective magnetic fields at the nuclei, the followingg-factors were obtained:¹⁶⁴Dy 0.336 (14),¹⁶⁴Er 0.353 (10),¹⁶⁶Er 0.320 (8),¹⁶⁸Er 0.333 (8),¹⁷⁰Yb 0.335 (6),¹⁷²Yb 0.332 (8),¹⁷⁴Yb 0.337 (8).     

Mössbauer study of 170Yb in some metals and metal-like compounds. Isomer shift measurements and intermediate valence states of ytterbium

We present here a Mössbauer effect study of the isomer shift and the magnetic behaviour of ¹⁷⁰Yb in compounds with metallic character where the ytterbium valence state ranges from a practically divalent and diamagnetic state (Yb in Ag, Tm and Yb) to a trivalent magnetic state (Yb in Au). Intermediate valence states, all of them probably non-magnetic, have been observed in YbAl₂, TmAl₂, YbAl₃ and Al as well as in the borides YbB₄, YbB₁₂ and TmB₁₂.In Tm metal, in addition to the quadrupole interaction, a weak magnetic hyperfine interaction is visible on ¹⁷⁰Yb below T_N.     

Neutron scattering lengths of the isotopes of thulium,ytterbium and lutetium

Coherent neutron scattering lengths and total cross sections have been measured on samples of ordinary Tm, Yb and Lu and on isotopically enriched compounds. From the experimental data for 0.57 meV neutron energy the following data were obtained: the coherent scattering lengths (in fm) of the bound atoms¹⁶⁹Tm (7.07+0.03);¹⁷⁰Yb (6.8±0.1);¹⁷¹Yb (9.7±0.1);¹⁷²Yb (9.5±0.1);¹⁷³Yb (9.56±0.10);¹⁷⁴Yb (19.2±0.1);¹⁷⁶Yb (8.7± 0.1); Yb (12.41±0.03);¹⁷⁵Lu (7.28±0.09);¹⁷⁶Lu (6.3±0.2) and Lu (7.21±0.03); the thermal absorption cross sections (in barn) for¹⁶⁹Tm (100±2); Yb (34.8±0.8) and Lu (74±2). In combination with the resonance parameters the measured coherent scattering lengths allowed the determination of potential scattering radii R′ which are of particular interest for the permanently deformed and deformable nuclei in the rare-earth region.     

Levels in 161Tm excited in the decay of 4.2 min 161Yb

The decay of ¹⁶¹Yb ($\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 4.2}\text{min}$) has been investigated with Ge(Li) and Si(Li) detectors and a toroidal β-spectrometer. Isobarically separated samples produced by the YASNAPP facility at Dubna Institute were used. The singles γ-ray spectrum, the conversion electron spectrum, γ-γ-τ and e-γ coincidences have been measured. In all, 67 γ-ray transitions have been observed. A decay scheme for ¹⁶¹Yb is proposed involving 12 excited states in ¹⁶¹Tm. The $\text{7}\text{2}$⁺[404], $\text{7}\text{2}$^?[523] and $\text{5}\text{2}$⁺[402] levels have been identified. The interpretation of the high-lying levels is discussed. The Q-value of ¹⁶¹Yb decay has been determined to be 3850 ± 250 keV. The A-dependence of the energies of the one-quasiparticle states in odd-A Tm isotopes is demonstrated.     

The decay of 174Tm and mixing of the Kπ = 5− two-quasiparticle states in 174Yb

The decay of 5.4 min ¹⁷⁴Tm has been investigated using Ge(Li) spectrometers in singles and coincidence measurements. A total of 43 γ-ray transitions, 26 of them not reported before, have been observed following the decay of ¹⁷⁴Tm. All transitions could be placed in a level scheme comprising 19 excited states of ¹⁷⁴Yb. The Nilsson model has been used to interpret the level structure. The mixing of two-quasineutron and two-quasiproton states is studied and the experimental mixing matrix element is compared with the results of theoretical calculations.     

Magnetic rotation of levels of 53Mn and 54Mn following the 53, 54Cr(p,n) and 51V(α, n) reactions

The low-lying levels of ⁵³Mn and ⁵⁴Mn have been studied using the ^{53, 54}Cr(p, nγ) and ⁵¹V(α, nγ) reactions. Angular distributions of γ-rays have been measured and their integral rotations in iron alloy targets studied. The g-factor of the 377 keV, $\text{5}\text{2}{}^{\mathrm{?}}$ level of ⁵³Mn is g = + 1.15±0.17. Products gτ have been found for the 55, 156, 368, 408 and 1072 keV levels of ⁵⁴Mn to be 124±42, 360±60, 75±25, > 10 and 150±80 ps respectively. Using shell model estimates for the g-factors, the lifetimes of the levels have been deduced. An interpretation of the results in terms of shell model wave functions is given.     

The 24Mg(α, α')24Mg reaction; statistical analysis

The ²⁴Mg(α, α')²⁴Mg reaction to the 1.37 MeV state has been studied over an α-energy range of 9.625–13.825 MeV, in ≈40 keV steps, and over a 25°–160° angular interval. These cross sections have been analysed in terms of statistical theory and a number of deviations from its predictions are found. These deviations point to the importance of non-statistical processes, such as intermediate structure, to the α-scattering. The average compound nuclear width o₁ 62±7 keV is found for ²⁸Si over the 18–22 MeV excitation.     

Electromagnetic transition strengths in 24Na

Mean lifetimes, excitation energies and branching ratios of ²⁴Na states, populated in the ²³Na(d, p)²⁴Na reaction have been measured. Gamma-ray spectra were measured at three angles in coincidence with proton groups at θ_p = 169°. Mean lifetimes obtained from DSA are (excitation energy in keV, lifetime in fs): 563, > 1000; 1341, 95 ± 30; 1344, 38 ± 11; 1346, > 1500; 1512, 38 ± 11; 1846, 260 ± 50; 1885, 36 ± 9; 2513, 15 ± 7; 2563, < 25; 2904, 50 ± 15; 2978, < 25; 3216, 22 ± 8; 3372, 19 ± 5. For higher levels up to 4207 keV upper limits of 30 fs were set. In combination with earlier work the following unique spin(-parity) assignments could be made: J^π(1846) = 2⁺, J(2513) = 3, J^π(3745) = 3^?. A new level at E_x = 3681.7 ± 0.6 keV is reported.     

Transient field measurements of g-factors for 28Si and 30Si

Transient field precession measurements have been performed on the first excited J^π = 2⁺ states of ²⁸Si and ³⁰Si with the IMPAC technique on recoil in magnetized iron. The results were analyzed with empirically adjusted Lindhard-Winther predictions. This yields g-factors of $\text{g = +0.56 ± 0.09}\text{and}\text{g = +0.56 ± 0.16}\text{for}{}^{28}\text{Si and}{}^{30}\text{Si}$, respectively. In the present cases the influence of static hyperfine fields is negligible due to the very short mean lives for ²⁸Si and ³⁰Si of 0.68 and 0.35 ps, respectively. The results are compared with theoretical calculations. Previous results for ²⁶Mg(2₁⁺) were reanalyzed with the more recent lifetime of τ_m = 0.72 ± 0.03 ps. The value of the g-factor becomes g = +0.82 ± 0.16.     

Large transient magnetic fields for rare-earth ions recoiling in gadolinium and g-factors of high-spin states in 156, 158, 160Gd

We have determined the transient magnetic field for Coulomb-excited rare-earth nuclei recoiling with velocities in the range between 0.7ν₀ and 6ν₀ into ferromagnetic gadolinium cooled to a temperature T = 80 K. Measured and calculated g-factors in ¹⁶⁹Tm have been used as calibration standards. The transient field is found at first to increase with increasing recoil velocity, and then to level off, approaching a nearly constant value of 5.5 kT at ν = 6ν₀. At the higher velocities (3ν₀ < ν < 6ν₀) the transient fields for ¹⁶⁹Tm recoils in gadolinium are a factor of 1.42 ± 0.12 larger than those in iron, whereas the densities of polarized electrons are the same in both ferromagnets. This result demonstrates that an explanation of the transient field must take into account the atomic structure of the host (and probably also that of the recoil). The transient field is too large to be described only in a statistical picture in which inner-shell (ns) vancancies are filled by capture of polarized (4f) electrons. Possible mechanisms may involve either polarization transfer from the outer shells by spin-flip interactions, or direct vacancy polarization by diabatic molecular orbitals.The transient field calibration has been corroborated making use of known g-factors of low-spin states in ^{156, 158, 160}Gd populated by Coulomb excitation of thick Gd single crystals. For the high-spin states in these nuclei, the g-factors are found to decrease slightly, with the ratio $\text{g(10}{}^{\mathrm{+}}\text{)}\text{g(2}{}^{\mathrm{+}}$) reduced to 0.89±0.12, 0.83±0.11, and 0.93±0.13, respectively. Similar decreases have been observed previously for other N = 90?96 nuclei.     

12C(7Li,t)16O and stellar helium fusion

The reaction ¹²C(⁷Li, t)¹⁶O has been studied at $\text{E(}{}^7\text{Li}\text{) = 34}\text{MeV}$ with the LASL tandem accelerator and QDDD magnetic spectrometer. Angular distributions to levels with E_x < 11 MeV have been obtained from 0° to 90°, including 0°. The results have been analyzed with finite-range distorted-wave Born approximation theory. The α-particle spectroscopic factors and reduced widths obtained are compared with those calculated with group theory (SU(3)) and other models. The analysis of data for the 7.1 and 9.6 MeV J^π = 1^? levels, which are of great importance in stellar helium buring, yields a ratio, R, of dimensionless reduced α-widths $\text{θ}{}^2{}_{\mathrm{<mtext>a</mtext>}}\text{(7.1}\text{MeV}\text{)}\text{θ}{}^2{}_{\mathrm{<mtext>a</mtext>}}\text{(9.6}\text{MeV}\text{)}\text{= 0.35b ± 0.13}$. The observed line width of the 9.6 MeV level (Γ_c.m. = 390 ± 60 keV) is less than the accepted value (Γ_c.m. = 510 ± 60 keV) and implies θ²_a(9.6 MeV) ≈ 0.6. These results as well as data for the 6.92 MeV J^π = 2⁺ and 10.35 MeV J^π = 4⁺ “α-cluster” states indicate 0.09 < θ²_a(7.1 MeV) < 0.33 with a mean value θ²_a(7.1 MeV) = 0.14 ± 0.04. The implication for stellar helium burning is discussed.     

Average g-factors for high-spin states in 78Kr

Inverse reactions of ^{63, 65}Cu beams on ^{18, 16}O targets have been used to populate states of ⁷⁸Kr by fusion-evaporation reactions. The excited nuclei recoiled at high velocity v/c ≈ 7 % through a polarized iron (⁵⁴Fe) layer and were stopped in a copper layer. During the period in iron, 0.05–0.65 ps, the nuclei were subjected to the intense transient magnetic field (initially ～ 3500 T). The resulting precession of the high-spin nuclear states populated during this time was determined by measuring the time integral rotation angle of the discrete γ-ray transitions at low spin.The average g-factor at low spin 2 ≦ J ≦ 8 compared to that at higher spin 8 ≦ J ≦ 12 in ⁷⁸Kr was found to be identical within the experimental uncertainties of ～ 15 %. This result implies that either there are no rotational alignment effects at the backbend in ⁷⁸Kr or more plausibly, proton (g ≈ 1) and neutron (g ≈ 0) aligned bands are equally competitive and both populated in the reaction. It is then likely that the resulting g-factor represents an average over many populated proton and neutron aligned bands.     

g-factors of high-spin isomeric states in 216Ra

The g-factors of two isomeric states at E_x = 3763 and 5170 keV in ²¹⁶Ra have been measured to be 0.51 ± 0.03 and 0.63 ± 0.06, respectively, with a TDPAD method. Spin and parity assignments of 19^? for the 3763 keV state and 25^? or 24⁺ for the 5170 keV state are consistent with the measured g-factors. Proposed configurations for the 19^? and 25^? assignments are of the same type as those predicted by a deformed independent-particle model for ²¹⁴Rn, which is an isotone of ²¹⁶Ra.     

Magnetic moment measurements of the first-excited 2+ states in even Nd isotopes

The g-factors of the first-excited 2⁺ states of ^{144, 146, 148}Nd were deduced from precession measurements in which the excited nuclei recoil through (TF IMPAC) or stop in (IMPAC) magnetized iron. The transient and static hyperfine fields which are active in these cases have been calibrated. The results for the g-factors, combined with previous data which were reanalyzed in the present work, are: g₁₄₄ = 0.15 ± 0.02, g₁₄₆ = 0.25 ± 0.04, g₁₄₈ = 0.32 ± 0.04. The g-factor for ¹⁴⁴Nd, which is abnormally low for a collective 2⁺ state, cannot be accounted for theoretically.     

Optical pumping of the metastable 53P0 level of ODD isotopes of cadmium

Metastable 5³P₀ atoms of ¹¹¹Cd and ¹¹³Cd are optically pumped in an atomic beam. Their magnetic resonances are observed with Landé factors g(³P₀, ¹¹¹ Cd) = (1.090±0.003) × 10^-3 and g(³P₀, ¹¹³Cd) = (1.143 ± 0.003) × 10^-3 which are 1.7 times larger than the g-factors of the 5¹S₀ ground state. This large difference arises from a slight mixing of the 5³P₀ level with the 5³P₁ and 5¹P₁ levels through the hyperfine interaction.