Time-of-flight measurement of resonant molecular formation in muon-catalyzed dt fusion

Preliminary results are reported for an experiment at TRIUMF where a time-of-flight technique was tested for measuring the energy dependence of the rate for muon-catalyzed dt fusion. Muonic tritium atoms were created following transfer of negative muons from muonic protium in a layer of solid hydrogen (protium) containing a small fraction of tritium. The atoms escaped from the solid layer via the Ramsauer-Townsend mechanism, traversed a drift region of 18 mm, and then struck an adjacent layer of deuterium, where the muonic atom could form a molecular system. The time of detection of a fusion product (neutron or alpha) following muon arrival is dependent upon the energy of the muonic tritium atom as it traverses the drift region. By comparison of the time distribution of fusion events with a prediction based on the theoretical energy dependence of the rate, the strength of resonant formation can in principle be determined. The results extracted so far are discussed and the limitations of the method are examined.     

Muonic atoms and muon-catalyzed fusion in inhomogeneous mixtures of hydrogen isotopes

The emission of µd and µt atoms from multilayer solid targets consisting of the mixtures of hydrogen isotopes has been investigated with a kinetics model. The methods to study the elastic scattering of muonic atoms, muon transfer, and molecular formation reactions with µ-atomic beams are discussed.     

Time-of-flight spectroscopy of muonic tritium

Emission of muonic tritium from a solid hydrogen layer has been studied via imaging of the muon-decay electrons and the time-of-flight distributions have been compared with detailed Monte Carlo calculations. Results are consistent at the 10% level with the theoretical prediction of a Ramsauer-Townsend minimum cross-section energy. This revised version was published online in August 2006 with corrections to the Cover Date.     

Dynamics of muonic atom cascade in hydrogen-helium mixtures

The deexcitation of excited muonic protium and deuterium in the mixture of hydrogen and helium isotopes is considered. Methods of experimental determination of the probability of direct atomic muon capture by hydrogen and muon transfer rates from excited muonic hydrogen to helium are proposed. Theoretical results for the population of the muonic atoms in the ground state, , are compared with the existing experimental data. Results obtained for mixtures are of interest for investigation of nuclear fusion in muonic molecules. Received: 6 August 1998 / Revised: 1st October 1998 / Accepted: 2 October 1998     

Experiments with energetic μd and μt emitted from solid hydrogen

A set of experiments is reviewed which makes use of the emission of muonic deuterium from the surface of a layer of solid hydrogen. The behaviour of muons in a solid target system has been studied via detection of muon decay electrons, muonic X-rays, and fusion products (neutrons and charged particles). The emission of muonic deuterium is understood to result from the Ramsauer-Townsend scattering minimum. The energy distribution of the emitted atoms ranges from tenths of eV to about 10 eV, and can be controlled to some extent. A proposal is described to use muonic tritium emission to measure the energy dependence of muonic molecular formation.     

Proposal for X-ray spectroscopy of muonic atoms formed from implanted ions in solid hydrogen films

A new method is proposed to extend muonic atom X-ray spectroscopy to the study of nuclear beams, including radioactive beams, by stopping both muon and nuclear beams in a solid hydrogen film. The muon transfer reaction to higher Z nuclei is used then to form muonic atoms. This method would allow studies of the nuclear charge distribution of unstable atoms. This revised version was published online in August 2006 with corrections to the Cover Date.     

Scattering of muonic hydrogen atoms

Our measurement compares the energy dependence of the scattering cross-sections of muonic deuterium and tritium on hydrogen molecules for collisions in the energy range 0.1–45 eV. A time-of-flight method was used to measure the scattering cross-section as a function of the muonic atom beam energy and shows clearly the Ramsauer–Townsend effect. The results are compared with theoretical calculations by using Monte Carlo simulations. The molecular pdμ and ptμ formation creates background processes. We measure the formation rates in solid hydrogen by detecting the 5.5 MeV (pdμ) and 19.8 MeV (ptμ) γ-rays emitted during the subsequent nuclear fusion processes. This revised version was published online in August 2006 with corrections to the Cover Date.     

Resonant formation measurements of dt\mu via time of flight

Solid hydrogen in the form of an inhomogeneous layered target offers several experimental advantages when compared with liquid or gas. Beams of non-thermalized muonic hydrogen atoms allow us to explore resonant molecular ion formation processes near eV kinetic energies. Isotopically specific layers make it possible to separate competing and confusing interactions and to employ the time of flight for comparison with predictions based on theoretical energy dependences. Unambiguous charged fusion product detection simplifies absolute intensity measurements. The systematic uncertainties encountered in resonant molecular ion formation measurements, using solid hydrogen target layers, are being investigated with simulations which use the many calculated energy-dependent rates and cross-sections which are now available. The importance of the rates for processes such as muon transfer and elastic scattering are discussed, and results of some recent analyses are presented. This revised version was published online in August 2006 with corrections to the Cover Date.     

Thermalization of muonic hydrogen in hydrogen targets

The thermalization of pµ atoms in protium and dµ atoms in deuterium is considered. Monte Carlo calculations are performed for gaseous (300 K) and solid (3 K) protium and deuterium targets. Complete sets of the total and differential cross sections for the scattering of pµ on protium targets and dµ on deuterium targets are used as an input to the Monte Carlo simulations. At 300 K, muonic atom scattering from single molecules of H₂ and D₂ is considered. In the case of solid hydrogen the correlation effects from all molecules of the sample are taken into account. In particular, the Bragg and phonon scattering cross sections are calculated. The spin states and average energy of the muonic atoms are shown as functions of time. It is shown that at energies below about 0.01 eV the solid-state effects influence strongly the calculated cross sections, and therefore the deceleration processes in the solids are much slower than in the gaseous targets. It is shown that the neutron spectrum due to ddµ formation and subsequent dd fusion is significantly affected by slow dµ thermalization in solid deuterium.     

Resonant Scattering of Muonic Hydrogen Atoms and Dynamics of the Muonic Molecular Complex

Resonant scattering of muonic hydrogen atoms via back decay of the molecular complex, a key process in the understanding of epithermal muonic molecular formation, is analyzed. The limitations of the effective rate approximation are discussed and the importance of the explicit treatment of the back decay is stressed. An expression of the energy distribution for the back-decayed atoms is given. This revised version was published online in August 2006 with corrections to the Cover Date.     

Muonic Molecule Formation in Condensed Deuterium

Resonant formation of the muonic molecule ddμ in dμ atom scattering in condensed deuterium is considered. In particular, ddμ formation in D₂ solid targets containing different ortho-D₂ concentration is discussed, and the respective time spectra of the dd fusion products are shown. The results of the first calculation of the resonant ddμ formation rate in liquid deuterium are presented. At large momentum transfers the ddμ formation rate takes the Doppler form, similar to that obtained for a dilute gas target. A condition of validity of this approximation is also discussed. This revised version was published online in August 2006 with corrections to the Cover Date.     

Kinetics of muonic hydrogen drift in axial symmetric geometry

The kinetics of muonic atoms of hydrogen isotopes in an axially symmetric trap is studied. The problem of the determination of the initial kinetic energy distribution of µp and µd atoms from time-of-flight spectra is discussed. The effects of the scattering of muonic atoms from gas and of the stopping distribution are evaluated. When the collision length is much larger than the target radius, the moments of the kinetic energy distribution are shown to be determined by the time-of-flight spectrum in a model-independent way.     

Diffusion radius of muonic hydrogen atoms in H-D gas

The diffusion radius of the 1S muonic hydrogen atoms in gaseous H₂ targets with various deuterium admixtures has been determined for temperatures T=30 and 300 K. The Monte Carlo calculations have been performed using the partial differential cross sections for pμ and dμ atom scattering from the molecules H₂, HD and D₂. These cross sections include hyperfine transitions in the muonic atoms, the muon exchange between the nuclei p and d, and rotational-vibrational transitions in the target molecules. The Monte Carlo results have been used for preparing the time-projection chamber for the high-precision measurement of the nuclear μ^- capture in the ground-state pμ atom, which is now underway at the Paul Scherrer Institute.     

New effects in low energy scattering of pµ atoms

Strong solid state effects in low energy scattering of pμ atoms in solid hydrogen are reported and analyzed. Such effects have been observed in TRIUMF experiment E742 where muons are stopped in thin frozen (3 K) layers of hydrogen. Emission of low energy pμ atoms from the hydrogen layer into adjacent vacuum was much higher than expected, based on calculations which ignored the solid nature of hydrogen. Monte Carlo simulations, performed using the scattering cross-sections with solid state effects taken into account, show the important role of the coherent elastic Bragg scattering in the diffusion of pμ atoms. For pμ energies lower than the Bragg cut-off limit (∼2 meV) the total scattering cross-section falls by several orders of magnitude, the hydrogen target becomes transparent and the emission of cold pμ atoms takes place. This revised version was published online in August 2006 with corrections to the Cover Date.     

Deceleration of muonic hydrogen atoms in solid hydrogens

Results of recent calculations of cross-sections for muonic hydrogen atom scattering in solid hydrogen isotope targets are presented. The coherent parts of these cross-sections, namely, the elastic Bragg scattering and phonon coherent scattering, are calculated accurately for the first time. A fine structure of Bragg peaks is obtained in the case of Bravais fcc structure of hydrogen targets frozen rapidly at 3 K. The one-phonon coherent cross-section is estimated using the Debye approximation. The calculated differential cross-sections are used for Monte Carlo simulations of muonic atom diffusion and slowing down in solid hydrogens. Also is calculated the energy-dependent rate of resonant ddμ molecule formation in 3 K solid deuterium quantum crystal, using the Debye model and Van Hove's formalism of the response function. This rate is very different from that obtained for the 3 K gas model. The influence of dμ atom slowing down on the average ddμ formation rate is considered. It is shown that very slow dμ deceleration below 10 meV is important for explanation of experimental results. This revised version was published online in August 2006 with corrections to the Cover Date.     

Cascade Processes in Muonic Hydrogen Atoms

The QCMC scheme created earlier for cascade calculations in heavy hadronic atoms of hydrogen isotopes has been modified and applied to the study of cascade processes in the μp muonic hydrogen atoms. The distribution of μp atoms over kinetic energies has been obtained and the yields of K-series X-rays per one stopped muon have been calculated. Comparison with experimental data indicated directly that for muonic and pionic atoms new types of non-radiative transitions are essential, while they are negligible for heavy (kaonic, antiprotonic, etc.) atoms. These processes have been considered and their probabilities have been estimated. This revised version was published online in August 2006 with corrections to the Cover Date.     

Muonium/muonic hydrogen formation in atomic hydrogen

The muonium/muonic hydrogen atom formation in μ^±−H collisions is investigated, using a two-state approximation in a time dependent formalism. It is found that muonium cross-section results are similar to the cross-section results obtained for positronium formation in e⁺-H collision. Muonic hydrogen atom formation cross-sections in μ^--H collision are found to be significant in a narrow range of energy (5 eV–25 eV).     

Ramsauer–Townsend Effect in Solid Hydrogen

The TRIUMF E742 experiment has measured the energy dependence of the scattering cross-sections of muonic deuterium and tritium on hydrogen molecules for collisions in the energy range 0.1–45 eV. The experimental setup permits the creation of muonic atom (μd or μt) beams. The multilayered target system gives the possibility to choose the type of interactions to study and to isolate a particular interaction. The scattering of μd or μt beams on H₂ is analyzed via the muon transfer reaction to neon. The time-of-flight method is used to measure the scattering cross section as a function of the energy of the muonic atom beam. The results are compared, using Monte Carlo simulations, with theoretical calculations which have been recently performed with high accuracy. This revised version was published online in August 2006 with corrections to the Cover Date.     

Muon molecular formation and transfer rate in solid hydrogen-deuterium mixtures

In an experiment at TRIUMF to study muon-catalyzed fusion and associated atomic and molecular effects, negative muons were stopped in a solid protium hydrogen layer containing a small amount of deuterium. Most of the resulting µp atoms disappeared by formation of ppµ molecules or by muon transfer to a deuteron. The µd can drift almost freely through the hydrogen layer due to the Ramsauer-Townsend effect and may even leave the layer. If a thin neon layer is frozen atop the hydrogen, the exiting muonic atoms will very rapidly release their muon to a neon atom. The analysis of the time structure of the neon X-rays is used to determine the rates of the slower processes involved in the evolution of the µp. This analysis has been performed with the help of Monte Carlo calculations, which simulate the kinetics of both µp and µd atoms in the hydrogen mixtures.     

Development Towards Muonic Atom Formation with Unstable Nuclei

We report on the latest development of a new method for extending muonic atom X-ray spectroscopy to the use of radioactive isotope beams to form muonic atoms with unstable nuclei. This would allow studies of the nuclear properties and nuclear sizes of unstable atoms by means of the muonic X-ray method at facilities where both negative muon and radioactive nuclear beams would be available. Progress of a feasibility study at RIKEN-RAL muon facility is also reported. This revised version was published online in August 2006 with corrections to the Cover Date.