The Reliability of Cross Sections of Partial Photoneutron Reactions for <Superscript>98</Superscript>Mo

The cross sections of partial photoneutron reactions for ⁹⁸Mo were evaluated. These cross sections are free from the shortcomings of various methods for neutron multiplicity determination used at the beams of quasimonoenergetic annihilation photons and bremsstrahlung radiation. New data on the cross sections of reactions (γ, 1n), (γ, 2n), and (γ, 3n) were obtained using the experimental–theoretical method for evaluation of cross sections of partial reactions satisfying the introduced physical reliability criteria. It is demonstrated that considerable deviations of the experimental cross sections from the evaluated ones result from an inaccurate sorting of neutrons between channels with a multiplicity of 1, 2, and 3.     

New data on (γ, n), (γ, 2n), and (γ, 3n) partial photoneutron reactions

Systematic discrepancies between the results of various experiments devoted to determining cross sections for total and partial photoneutron reactions are analyzed by using objective criteria of reliability of data in terms of the transitional photoneutron-multiplicity function F _i = σ(γ, in)/σ(γ, xn), whose values for i = 1, 2, 3, ... cannot exceed by definition 1.00, 0.50, 0.33, ..., respectively. It was found that the majority of experimental data on the cross sections obtained for (γ, n), (γ, 2n), and (γ, 3n) reactions with the aid of methods of photoneutron multiplicity sorting do not meet objective criteria (in particular, F ₂ > 0.50 for a vast body of data). New data on the cross sections for partial reactions on ¹⁸¹Ta and ²⁰⁸Pb nuclei were obtained within a new experimental-theoretical method that was proposed for the evaluation of cross sections for partial reactions and in which the experimental neutron yield cross section σ ^expt(γ, xn) = σ(γ, n) + 2σ(γ, 2n) + 3σ(γ, 3n) + ..., which is free from problems associated with determining neutron multiplicities, is used simultaneously with the functions F _i ^theor calculated within a combined model of photonuclear reactions.     

14.77 MeV neutron-induced nuclear reaction cross sections for zinc,yttrium, and molybdenum targets

The cross sections for neutron-induced nuclear reactions on natural zinc, yttrium, and molybdenum targets were measured at a neutron energy of 14.77 ± 0.17 MeV using the activation technique, offline gamma-ray spectrometry, and a detailed covariance analysis. The uncertainty in the statistical model calculations of cross sections for the (n, 2n), (n, p), (n, α), and (n, γ) reactions with natural zinc, yttrium, and molybdenum at neutron energies from 13 to 17 MeV was calculated using the TALYS-1.96 nuclear code. The measured cross sections of the present study were compared with the experimental cross sections reported in the EXFOR database, the cross sections were calculated with the TALYS-1.96 and EMPIRE-3.2.3 nuclear codes and the evaluated nuclear data from the TENDL-2019, JENDL-5, and ENDF/B-VIII.0 libraries.     

The (γ,2p) reaction on30Si and the (γ,2p), (γ,2pn), (γ,3p) and (γ,3pn) reactions on31P at intermediate energies

The yields of the (γ,2p) reaction on³⁰Si and of the (γ,2p), (γ,2pn), (γ, 3p) and (γ,3pn) reactions on³¹P have been measured as a function of the maximum bremsstrahlung energy in the range 75–640 MeV. The cross sections have been deduced and are compared to Monte-Carlo calculations. The magnitude of the cross sections in the energy range above the threshold for the photoproduction of mesons is also discussed using a simple analytical approach.     

Evaluated Cross Sections of Photoneutron Reactions on the Isotope <Superscript>116</Superscript>Sn and Spectra of Neutrons Originating from These Reactions

With the aid of the results obtained by evaluating cross sections of partial photoneutron reactions on the isotope ¹¹⁶Sn and the energy spectra of neutrons originating from these reactions, the possible reasons for the well-known discrepancies between the results of different photonuclear experiments were studied on the basis of a combinedmodel of photonuclear reactions. On the basis of physical criteria of data reliability and an experimental–theoretical method for evaluating cross sections of partial reactions, it was found that these discrepancies were due to unreliably redistributing neutrons between (γ, 1n), (γ, 2n), and (γ, 3n) reactions because of nontrivial correlations between the experimentally measured energy of neutrons and their multiplicity.     

Evaluation of Reliable Cross Sections of Partial and Total Photoneutron Reactions for the <Superscript>139</Superscript>La Nucleus

Cross sections of partial photoneutron reactions free of the shortcomings of different ways of determining the multiplicity of neutrons used on beams of quasi-monoenergetic annihilation photons are evaluated for ¹³⁹La. The experimental-theoretical method of evaluation of partial reaction cross sections satisfying proposed data reliability criteria is used to obtain new data on the cross sections of reactions (γ, 1n), (γ, 2n), and (γ, 3n). It is shown that noticeable deviations of experimental cross sections from evaluated values are due to the unreliable sorting of neutrons between channels with multiplicities of 1, 2, and 3.     

Main channels of the decay of the giant dipole resonance in the 20,22Ne nuclei and isospin splitting of the giant dipole resonance in the 22Ne nucleus

Data published in the literature on various photonuclear reactions for the ^20,22Ne isotopes and for their natural mixture are analyzed with the aim of exploring special features of the decay of giant-dipole-resonance states in these two isotopes. With the aid of data on the abundances of the isotopes and on the energy reaction thresholds, the cross sections for the reactions ^20,22Ne[(γ, n)+(γ, np)] and ^20,22Ne[(γ, p)+(γ, np)] are broken down into the contributions from the one-nucleon reactions (γ, n) and (γ, p) and the contributions from the reactions (γ, np). The cross sections for the reactions ^20,22Ne(γ, n)^19,21Ne and ^20,22Ne(γ, p)^19,21F in the energy range E _γ=16.0–28.0 MeV and the cross sections for the reactions ^20,22Ne(γ, np)^18,20F in the energy range E _γ=23.3–28.0 MeV are estimated. The behavior of the cross-section ratio r=σ(γ, p)/σ(γ, n) for the ²²Ne nucleus as a function of energy is analyzed, and the isospin components of the giant dipole resonance in the ²²Ne nucleus are identified. The contributions of the isospin components of the giant dipole resonance in the ²²Ne nucleus to the cross sections for various photonuclear reactions are determined on the basis of an analysis of the diagram of the excitation and decay of pure isospin states in the ²²Ne nucleus and in nuclei neighboring it, which are members of the corresponding isospin multiplets. The isospin splitting of the giant dipole resonance and the ratio of the intensities of the isospin components are determined to be ΔE=4.57±0.69 MeV and R=0.24±0.04, respectively.     

The (γ, p n) and (γ, 3p3n) reactions in40Ca at intermediate energies

The yields of the reactions⁴⁰Ca(γ, p n)^38g K and⁴⁰Ca(γ, 3p 3n)^34m Cl have been measured by the activation method in the energy range 80–800 MeV. From the measured yields the cross sections are deduced. The experimental cross sections are compared to calculations with a cascade-evaporation model for photo-induced reactions.     

Investigation of the isomeric ratio for 44m, g Sc

The isomeric ratios measured for ^{44m, g} Sc in (γ, n), (p, n), (p, αp3n), and (α, p3n) reactions are presented. The values obtained in this way are compared with the results of calculations within the cascade-evaporation model and with data coming from an investigation of reactions like (n, 2n), and (d, t).     

Physical criteria for the reliability of data on the photodisintegration of the <Superscript>89</Superscript>Y nucleus

Experimental photonuclear reaction cross sections obtained in experiments using quasimonoenergetic annihilation, monoenergetic tagged photons, and bremsstrahlung γ-radiation are analyzed using physical criteria for the reliability of data on the ⁸⁹Y nucleus. It is found that the reliability of data on the cross sections of partial reactions (γ, 1n) and (γ, 2n), obtained by means of photoneutron multiplicity sorting, is highly doubtful. Reliable cross sections of reactions (γ, 1n) and (γ, 2n) are obtained using the experimental–theoretical method (ETM) for evaluating using both experimental cross sections of neutron yield reaction σ^exp(γ, xn) that are free of neutron multiplicity problems, and theoretically calculated F _i ^theor ratios of the cross sections of definite (i) partial reactions to cross section σ^theor(γ, xn). It is shown that the evaluated cross sections differ noticeably from the experimental data.     

The (γ, n) reaction on 16O between giant resonance and pion threshold

A new TOF facility has been built for measurements of differential (γ, n) cross sections to discrete final states of light nuclei in the photon energy range between giant resonance and pion threshold. The observed neutron angle θ_n can continuously be varied between 0° and 150°, and additionally measurements at 175° and 180° are possible. Differential cross sections for the reaction ¹⁶O(γ, n₀)¹⁵O are presented for E_γ = 60 MeV (40° ? θ_n ? 149°) and for θ_n = 90° (60 MeV ? E_γ ? 160 MeV). The results, combined with the corresponding (γ, p₀) cross sections, indicate an absorption mechanism of high energy photons by neutron-proton pairs.     

Reliability of the data on the cross sections of the partial photoneutron reaction for <Superscript>63,65</Superscript>Cu and <Superscript>80</Superscript>Se nuclei

The cross sections of partial photoneutron reactions are evaluated for the ^63,65Cu and ⁸⁰Se isotopes. The cross sections are free of systematic uncertainties from shortcomings of the experimental methods for neutron multiplicity sorting based on measurements of neutron energy used in experiments with quasimonoenergetic annihilation photon beams. An experimental-theoretical method is used to evaluate cross sections σ^eval(γ, in)= F_i^theor σ^exp(γ, xn), where ratios F_i^theor = σ^theor(γ, in)/σ^theor(γ, xn) = σ^theor(γ, in)/σ^theor[(γ, 1n) + 2(γ, 2n) + …] are calculated using a combined model of photonuclear reactions, and σ^exp(γ, xn) is the experimental cross section of the neutron yield reaction free from neutron multiplicity sorting problems. The cross sections are evaluated for reactions (γ, 1n) and (γ, 2n) for the ^63,65Cu and ⁸⁰Se isotopes, and for the total photoneutron reaction σ(γ, Sn) = σ[(γ, 1n) + (γ, 2n) + …]. It is shown that noticeable deviations of the experimental cross sections from the evaluated values result from the unreliable sorting of neutrons between the channels with multiplicities 1 and 2.     

Interference of isovector and isoscalar giant quadrupole resonances in Y and Pb

We present the calculations of the fore-aft asymmetry of γ-rays in fast nucleon capture reactions ⁸⁹Y(n, γ)⁹⁰Y, ²⁰⁸Pb(n, γ)²⁰⁹Pb and ²⁰⁸Pb(p, γ)²⁰⁹Bi which are based on a consistent version of the direct-semi-direct (DSD) capture model. The results are in good agreement with observed differential cross sections.     

Bestimmung des Kompoundkern- und Stripping-Anteils der (d,p)- und (d,n)-Reaktionen an Zr94 und Zr96

An experiment has been accomplished which gives information on the reaction mechanism of the (Zr^94,96+d)-reactions. Total cross sections and excitation functions up to 11,8 MeV have been measured for the reactions Zr⁹⁴ (d, p), Zr⁹⁴ (d, n), Zr⁹⁶(d, p), Zr⁹⁶(d, n) and Zr⁹⁶(d, 2n) by the activation method. The results are compared with cross sections calculated according to the statistical theory of nuclear reactions. It is shown that the (d, p) -reactions proceed almost completely by the stripping-mechanism. The (d, n)- and (d, 2n)-excitation functions on the other hand are in good agreement with the predictions of the statistical theory and one can conclude that the compound nucleus mechanism is the dominating process.     

Untersuchung der Kernphotoreaktionen12C(γ,n),12C(γ, 2n),39K(γ,n) und40Ca(γ,np) bis zur Mesonenschwelle

In order to obtain data on the photon absorption process between the giant resonance and the meson threshold the cross sections of the reactions¹²C(γ,n)¹¹C,¹²C(γ, 2n)¹⁰C,³⁹K(γ,n)³⁸K^g, and⁴⁰Ca(γ,np)³⁸K^g have been determined by the analysis of yield curves at the 140 MeV electron synchrotron of the PTB. Though the (γ,n) cross sections grow small with increasing photon energy they are different from zero up to energies of 60 MeV and above. The cross section of the reaction¹²C(γ, 2n) is extremely small; its highest value amounts to 0.15% of the highest value of the¹²C(γ,n) reaction. The measured⁴⁰Ca(γ,np) cross section is of the order predicted by the naive quasi-deuteron model. The integrated cross sections of the above reactions up to 140MeV are 85±7,0.90±0.10, 139±16, and 76±7MeVmb respectively.     

Anregungsfunktionen für die (d,p)-, (d,n)-und (d,2n)-Reaktionen an Ce142 bis 11,8 MeV

Total cross sections and excitation functions up to 11·8 MeV have been measured for the Ce¹⁴²(d,p), -(d,n) and -(d, 2n) reactions by the activation method. The cross sections found forE _d=11·8 MeV are 187mb, 54 mb and 535 mb, respectively. By comparing these results with cross sections calculated from the statistical theory of nuclear reactions it can be shown that the (d,p)-reaction and nearly the whole (d,n) -reaction proceed by stripping mechanism.     

Measurements of the (γ, n0) reaction on 12C and 16O and the investigation of the reaction mechanism

Differential (γ, n₀) cross sections on ¹²C and ¹⁶O have been measured for photon energies 60 MeV ? E_γ ? 160 MeV. These results combined with the corresponding (γ, p₀) cross sections support an absorption mechanism of the photon by neutron-proton pairs.     

Zur (γ,p)- und (γ,np)-Reaktion am Argon 40

Argon gas has been irradiated with 34 MeV bremsstrahlung. The yields of the reactions A⁴⁰(γ, p) Cl³⁹ and A⁴⁰ (γ, np) Cl³³ were determined relative to C¹²(γ, n) by β-counting. The resulting upper limits for the cross sections integrated to 28 MeV are 160 MeVmbarns for (γ, p), and 35 MeV mbarns for (γ, np). This does not confirm the anomalously high A⁴⁰ (γ, p)-cross section reported in the literature.     

Microscopic description of γ-induced4He break-up processes

The theory ofγ break-up processes in the cluster model reaction scheme is developed and applied to the⁴He case. The large difference between (γ, p) and (γ, n) cross sections reported in the literature is not found, but the result of this calculation agrees well with (γ, p) measurements. Furthermore (γ, d) reactions are studied for low energies.     

A comparative study of the electric giant dipole resonance of 24−26Mg

The electric giant dipole resonance of ^24?26Mg has been explored up to 30 MeV excitation energy with bremsstrahlung. ΔE, E spectra of charged photo-particles and spectra of prompt deexcitation γ-rays from excited residual nuclear states were obtained at various bremsstrahlung endpoint energies. The ²⁵Mg(γ, p₀), (γ, d), ^24,25Mg(γ, α) differential cross sections as well as ^24?26Mg(γ, xγ′) integrated cross sections are presented. The results are discussed in terms of one-particle, one-hole excitations and isospin composition of giant resonance states. A comparison with calculations for ²⁴Mg gives poor agreement. Excitations from deeper shells were found in the giant dipole resonance of ²⁴Mg, but do not seem to be concentrated at higher energies. In ²⁵Mg, only weak excitations of this kind were found, and they are completely absent in ²⁶Mg.