Conversion electron measurement of isomeric primary transitions in196, 198, 199, 200, 201Pb

The transition energies of nine low energy primary transitions from high spin isomers in^{196, 198, 199, 200, 201}Pb have been measured with conversion electron spectroscopy usinge ^? e ^? ande ^? γ coincidences.B(E2) values as deduced from the measured lifetimes and transition energies are discussed in terms of seniority shell model configurations and of a quasiparticle Tamm-Dancoff approach using the surface delta interaction. A revised discussion of the effectiveE2 charge in neutron deficient Pb isotopes is presented.     

ESR of V3+ in zinc oxide single crystals

Electron spin resonance has been investigated in zinc oxide single crystals containing vanadium. Several groups of ordinary and forbidden transitions can be observed. The experimental results are interpreted with the aid of the spin Hamiltonian, for which the following parameters were determined:g∥=1.945; ⊥=1.937; ¦D¦=750×10^?4 cm^?1, ¦A¦=68 × 10^?4 cm^?1; ¦B ¦=93×10^?4 cm^?1; ¦A?P¦=65×10^?4cm^?1.     

EPR of Spin Transitions in Complexes of Cu(hfac)2 with tert-Butylpyrazolylnitroxides

Polymer chain complexes [Cu(hfac)₂L^R] _n exhibit thermally and light-induced magnetic anomalies in many aspects similar to a spin crossover. These compounds attracted significant attention in the field of molecular magnetism and have been extensively studied by electron paramagnetic resonance (EPR) during the last several years. All compounds studied so far were based on copper(II) ions bridged by pyrazolyl-substituted nitronylnitroxides. The present work reports the first EPR study of complexes of Cu(hfac)₂ with tert-butylpyrazolylnitroxides—a new type of nitroxide ligand expected to modify exchange interaction pathways and physical properties of the crystals. The Q-band EPR spectra of three representative novel compounds are principally different from those studied previously, supporting the assumption that the magnetic motif of the compound has changed. Dominant intercluster exchange interactions are now found along the structural polymer chains. This complicates the EPR detection of phase transitions to some extent; however, theoretical modeling of the observed spectral changes allows for unambiguous assignment of different spin states and transitions between them. The magnitudes of intercluster exchange interaction were estimated to be ca. 0.1–1.5 cm^?1 for the studied compounds.     

Dirac-neutrino magnetic moment and the dynamics of a supernova explosion

The double conversion of neutrino chirality ν_L → ν_R → ν_L has been analyzed for supernova conditions, where the first stage is due to the interaction of the neutrino magnetic moment with plasma electrons and protons in the supernova core, and the second stage, due to the resonance spin flip of the neutrino in the magnetic field of the supernova envelope. It is shown that, in the presence of the neutrino magnetic moment in the range 10^?13 μ_B < μ_ν < 10^?12 μ_B and a magnetic field of ～10¹³ G between the neutrinosphere and the shock-stagnation region, an additional energy of about 10⁵¹ erg, which is sufficient for a supernova explosion, can be injected into this region during a typical shock-stagnation time.     

Spin Echo Spectrometry Using Very Cold Neutrons

Concept of spin echo spectrometer on very cold neutrons (wavelengths λ ~ 10?30 nm) to provide extra high resolution in energy transfer (ΔE ~ 10^–13 eV) has been proposed. Simultaneous measurements of spin echo signals at different wavelengths will be realized using broadband spin flippers in combination with Fourier-analysis of λ-spectrum. The application of very cold neutrons should extend the spin echo time diapason radically, t ~ 10^–12?10^–3 s. This promises to open a set of novel scientific areas including the spectroscopy of chemical reactions and catalytic processes, conformational transitions in polymers and biological molecules, dynamic modes in carbon structures (fullerenes, nanotubes, graphenes) at scales from few nanometers to microns. Presently, the development of NSE-spectrometer on VCN becomes relevant since the project of ultra cold neutron source at WWR-M reactor (PNPI) is in progress.     

A 150 ms 10+ Isomer in146Dy

In the course of systematic studies of very proton rich nuclei in theN≈82 region with Ni induced compound reactions, an unusually long-lived high spin isomer has been found. After in-and off-beamγ and conversion electron measurements, asγ excitation functions,γ andeγ coincidences, pulsed beam techniques and multi spectrum analyses of the residual activities, this isomer has been tentatively assigned to be a 10⁺ state in¹⁴⁶Dy, which decays into two 7^? states byE3 transitions. The half-life of the isomer has been measured to be 150±20ms. The isomer has been found to follow the β decay of the previously unknown 3.9 s isotope¹⁴⁶Ho. The mechanism of the appearance of such an isomer is discussed.     

Gamma rays from resonance neutron capture in 115In

Gamma rays in the range 5.4–6.7 MeV have been studied for 31 s-wave neutron resonances of ¹¹⁵In, selected by time of flight in the range 3–430 eV. In a subsidiary experiment, spin J = 5 has been assigned to 17 and J = 4 to 14 resonances by measuring intensity variations of some strong low-energy transitions. The reduced widths averaged over all initial states of the same spin have been estimated for 41 primary transitions: these values have provided information on the spin and parity of the corresponding ¹¹⁶In final states. Overall mean values of E1 and M1 radiative strength have been calculated. The width distribution has been fitted with a χ² function with ν = 1.10^+0.27_?0.09 degrees of freedom for M1 and ν = 1.42 ^{+ 0.014}_?0.08 for E1 radiation. An estimate of the spin cut-off parameter σ = 3.6_?0.4^{+ 0.8} has been derived. A non-statistical effect already evidenced in previous measurements has been confirmed, consisting of a strong modulation of the radiative strength against resonance energy, correlated also with the local neutron strength function. In addition, it has now been shown that this structure is due to E1 radiation only.     

Time distribution of γ-rays from spontaneous fission of 252Cf at short times

The gross time distribution of γ-rays from spontaneous fission of ²⁵²Cf has been measured in the time range 10^?14?10^?10 s after fission for γ-ray energies greater than 0.15 MeV. The measurements have been made by a new method based upon the solid angle aberration. From the measured correlation between half-lives and γ-ray transition energies it is concluded that the transitions are predominantly E2, single-particle transitions at high energies, and mostly vibrational and rotational transitions at lower energies. Some contribution of E1 transitions and M1-E2 mixtures cannot be excluded, however. It was found that about 30% ofthe γ-rays emitted within 12 ns with energies greater than 0.10 MeV, have half-lives shorter than 1 ps and about 52 % half-lives between 1 and 100 ps. The relative yield of γ -rays and γ-ray energy in the time range 10^?14 to 1.2 × 10^?7 s ater fission is given.     

Nuclear spin induced collapse and revival shape of Rabi oscillations of a single electron spin in diamond

A collapse and revival shape of Rabi oscillations in an electron spin of a single nitrogen-vacancy centre has been observed in diamond at room temperature. Because of hyperfine interaction between the host ¹⁴N nuclear spin and the nitrogen-vacancy centre electron spin, different orientations of the ¹⁴N nuclear spins lead to a triplet splitting of the transition between ground state (m_s =0) and excited state (m_s =1). The manipulation of the single electron spin of nitrogen-vacancy centre is achieved by using a combination of selective microwave excitation and optical pumping at 532 nm. Microwaves can excite three transitions equally to induce three independent nutations and the shape of Rabi oscillations is a combination of the three nutations.     

High-spin spectroscopy of168Hf

The nucleus¹⁶⁸Hf was studied up to spin (38⁺) in the yrast band and to spins (41^?) and (38^?) in the lowest two negative-parity bands. The onset of a proton alignment (h_9/2 or i_13/2 quasiparticles) is observed in these three bands for the highest transitions. A new band with even spins and negative parity was found. The interaction strength between the ground-state band and theAB band is measured.     

Coulomb excitation of230Th with32S,84Kr and142Nd projectiles

The Coulomb excitation measurements for the²³⁰Th nucleus with³²S,⁸⁴Kr and¹⁴²Nd projectiles are presented. The use of different projectiles allowed us to get information in the ground-state band and side bands. The energy spectrum of the ground-state band and of the lowest negative-parity band have been investigated up to the spin valueI=24⁺ andI=19^?(21), respectively. Five side bands (K ^π=0⁺, 2 ₁ ⁺ , 2 ₂ ⁺ , 1^?, 2^?) were observed also. The branching ratios for a large number of transitions in the spin regionI≦10 for π=+1 andI≦9 for π=? 1 are analysed. The full set of experimental data contains information on the mixing of the adiabatic states and on the nuclear response to the electromagnetic field ofγ-radiation. It is shown that the experimental data may be explained taking into account the coupling of the ground-β- and twoγ-bands and also of theK ^π=0^?, 1^? and 2^? negative-parity bands. An enhancement of the transitions from theγ-to theβ-band in respect to the transitions from theγ to the ground band and from theβ- to the ground band is reported. The mixing of the negative-parity bands is found to be typical for the alignment of the octupole-vibrational angular momentum. The strong spin dependence of the intrinsic matrix elements of the electric-dipole operator follows from the branching ratios of inter- and intra-band transitions from theK ^π=0^? states.     

Concentration dependence of the transition temperature in spin glasses

The transition temperature T_f of randomly distributed spins interacting via the RKKY interaction (spin glasses) has been calculated numerically within the spherical approximation. The dependence of T_f on the concentration c of magnetic impurities and on the damping of the interaction due to a finite mean free path of the conduction electrons is investigated for 10^?5 < c < 10^?1.     

Gamma-gamma directional correlations in69Ga

Employing a Ge(Li)-NaI(Tl) detector system, gamma-gamma directional correlations for nine cascades in⁶⁹Ga have been measured. The result of the present measurements combined with other existing data allowed the adoption of a 5/2^? spin and parity for the 1106.4 keV level, and a 7/2^? for the 1 336.1 and 1487.5 keV levels. A tentative 7/2^? spin and parity has been adopted for 1923.1 keV level. Mixing ratios have been determined for six transitions. The data obtained are utilized to extractM1 andE2 reduced transition probabilities. A comparison of the experimental data is made with the predictions of the one particle-core and three particles-core coupling models.     

Decay of 8.0-day131I to levels of131Xe and 11.77-day131mXe

The decay characteristics of¹³¹I have been determined with high accuracy. The total branch from¹³¹I to^131mXe has been measured to be 1.086±0.007%. The half life of^131mXe has been measured as 11.770±0.012 days. Theγ-ray spectrum has been determined and new transitions at 85.92, 232.17, 295.83, 302.44, and 449.57 keV established. The position, spin and parity were established for a 9/2^? level at 341.140 keV and spin and parity of 7/2^? established for a level at 666.921 keV. The log f₁t for the unique firstforbiddenβ transition from 7/2^{+ 131}I to 11/2^{? 131m}Xe has been calculated to be 9.78.     

Vibrational band structure in 184W populated in the decay of 184Re

The decay of ^184mRe has been investigated through γ-ray and conversion electron studies. The band head of the K^π = 2^? octupole band has been established at 1130.0 keV. The E2/M1 mixing ratios of three transitions from the γ-vibrational band to the ground state band have been determined by angular correlation measurements. A mixing of El, M2 and E3 multipolarity has been derived for the 921 keV transition combining angular correlation and conversion electron data. A value B(E3, 0⁺ → 3^? = (25 ± 5) × 10⁴e² · fm⁶ was obtained from the measured E2/M1 mixing of the 91 keV 3^? → → 2^? transition and γ-branchings. The data are discussed in terms of the collective model taking into account band mixing.     

Spinaustauschstreuung von Kalium an Caesium

The differential spin exchange cross sectionI _ex(?, E) for the system K-Cs has been measured as a function of angle for 2°???40° and collision energy for 1.2 · 10^?13 erg ?E?2.1 · 10^?13erg. Confirming previous experiments it exhibits a maximum neargj≈10°. The angular position of maximum changes with collision energy. Increasing the energy lowers the maximum angle. The analysis of the cross section with regard to information about the interaction of the collision partners turns out to be very complicated. A first few model calculations are presented and discussed. The most obvious, qualitative relations between the singlet and triplet interaction potentials,V ₀ andV ₁, and the differential spin exchange cross sectionI _ex(?) appear to be: 1. The average magnitude ofI _ex is markedly different below and above the rainbow angle \(\vartheta _{R_1 }\) of the shallow triplet potential V₁. From the observed intensity drop towards large angles we estimate a lower bound for the triplet potential well depth? ₁?1.4 · 10^?14 erg. 2. The expected relation between the integral spin exchange cross sectionσ _ex and the difference potentialΔV(R)=V ₁-V ₀ at large distances is also borne out by the differential spin exchange cross section I_ex(?) below \(\vartheta _{R_1 }\) . Relative to the intensity beyond \(\vartheta _{R_1 }\) the cross section increases if range and strength ofΔV is increased.     

The decay of65Ge

Energies and relative intensities of γ-rays from the decay of⁶⁵Ge have been measured. The half-life was measured to be (31.2±0.7) sec. From the measured intensity of the annihilition radiation the intensity of the groundstate ß⁺ feeding was determined to be <10%. A total of 31 γ transitions was placed in a level scheme. The spin and parity of the groundstate of⁶⁵Ge was determined to be 3/2^? (5/2^?).     

EPR spectra of gable-type copper(II) porphyrin dimers in fluid solution: extraction of exchange interaction in weakly coupled doublet pairs

A comparison between EPR spectra of rigidly linked dicopper porphyrin dimers and those of the corresponding monocopper dimers (copper porphyrin-free base porphyrin dimers) in fluid solution reveals a very weak exchange interaction between the two copper spins. In these dimers, two porphyrin moieties are linked via an aromatic spacer such as benzene, naphthalene or phenanthrene in a gable-type geometry, with a distance of 10–13 Å. Although essentially all the spectra from the monocopper dimers are the same, exhibiting hyperfine (hf) structure due to the copper and nitrogen nuclei, the EPR spectral patterns of the dicopper dimers depend on the spacer molecule. Differences in hf patterns among the dicopper porphyrin dimers are ascribed to isotropic spin—spin coupling, i.e., exchange coupling between the two copper spins. This is because the anisotropic dipole—dipole interaction is averaged out due to random tumbling of the solute molecules in fluid solution. From the line shape analysis, the absolute value of the exchange interaction (|J|) is found to be 4 × 10^?4 cm^?1 ≦|J| < 3 × 10^?3 cm^?1 for the benzene linked dicopper dimer (Cu—Bz—Cu) whereas |J| ～ 1 × 10^?4cm^?1 for the other two dimers (Cu—Np—Cu and Cu—Pn—Cu). These values are comparable with or much smaller than the dipole—dipole coupling, which is estimated as about 1–3 × 10^?3 cm^?1 from the centre-to-centre distance. Since Cu—Bz—Cu shows a significantly larger |J| than Cu—Pn—Cu, despite a slightly longer centre-to-centre distance, and since no correlation could be obtained between |J| and the separation of the two copper atoms, it is likely that the interaction via spacer molecules is dominant between the two halves.     

Das Konversionselektronenspektrum von Sm150 nach Neutroneneinfang

The spectrum of internal conversion electrons emitted by Sm¹⁵⁰ after neutron capture was measured by means of the beta spectrometer at the research reactor at Garching near Munich. Between 3 keV and 8 MeV, 392 conversion lines corresponding to 337 transitions were found. The multipolarity of most transitions could be determined uniquely, the energy of the conversion electrons was measured within an accuracy of≧2.5 × 10^?4. An extension of the level scheme of Sm¹⁵⁰ is proposed.     

On-line nuclear orientation study of184Au

The¹⁸⁴Au→¹⁸⁴Pt decay, studied on-line with the UNISOR facility at HHIRF, is discussed. Gamma-ray and conversion-electron spectroscopy of¹⁸⁴Pt as well as on-line nuclear orientation measurements of¹⁸⁴Au were done. A new low-lying level scheme of¹⁸⁴Pt is proposed. Two coexisting bands with different deformations and their respective γ-vibrational bands are established. Internal conversion coefficients for interband transitions between states with the same spin are extracted from the spectroscopy measurements. The relative E0 contents of the transitions are determined by combining internal conversion coefficients with E2/M1 mixing ratios deduced from gamma-ray anisotropies measured from oriented nuclei.