This work proves the feasibility of a novel concept of differential absorption lidar based on the Scheimpflug principle. The range‐resolved atmospheric backscattering signal of a laser beam is retrieved by employing a tilted linear sensor with a Newtonian telescope, satisfying the Scheimpflug condition. Infinite focus depth is achieved despite employing a large optical aperture. The concept is demonstrated by measuring the range‐resolved atmospheric oxygen concentration with a tunable continuous‐wave narrow‐band laser diode emitting around 761 nm over a path of one kilometer during night time. Laser power requirements for daytime operation are also investigated and validated with single‐band atmospheric aerosol measurements by employing a broad‐band 3.2‐W laser diode. The results presented in this work show the potential of employing the continuous‐wave differential absorption lidar (CW‐DIAL) technique for remote profiling of atmospheric gases in daytime if high‐power narrow‐band continuous‐wave light sources were to be employed.
An analytical model is presented describing the temporal intensity contrast determined by amplified spontaneous emission in high‐intensity laser systems which are based on the principle of chirped pulse amplification. The model describes both the generation and the amplification of the amplified spontaneous emission for each type of laser amplifier. This model is applied to different solid state laser materials which can support the amplification of pulse durations . The results are compared to intensity and fluence thresholds, e.g. determined by damage thresholds of a certain target material to be used in high‐intensity applications. This allows determining if additional means for contrast improvement, e.g. plasma mirrors, are required for a certain type of laser system and application. Using this model, the requirements for an optimized high‐contrast front‐end design are derived regarding the necessary contrast improvement and the amplified “clean” output energy for a desired focussed peak intensity. Finally, the model is compared to measurements at three different high‐intensity laser systems based on Ti:Sapphire and Yb:glass. These measurements show an excellent agreement with the model.
In this work, we report optomechanical coupling, resolved sidebands and phonon lasing in a solid‐core microbottle resonator fabricated on a single mode optical fiber. Mechanical modes with quality factors (Qm) as high as 1.57 × 104 and 1.45 × 104 were observed, respectively, at the mechanical frequencies and . The maximum Hz is close to the theoretical lower bound of 6 × 1012 Hz needed to overcome thermal decoherence for resolved‐sideband cooling of mechanical motion at room temperature, suggesting microbottle resonators as a possible platform for this endeavor. In addition to optomechanical effects, scatter‐induced mode splitting and ringing phenomena, which are typical for high‐quality optical resonances, were also observed in a microbottle resonator.
This article presents a novel III‐V on silicon laser. This work exploits the phenomenon that a passive silicon cavity, side‐coupled to a III‐V waveguide, will provide high and narrow‐band reflectivity into the III‐V waveguide: the resonant mirror. This results in an electrically pumped laser with a threshold current of 4 mA and a side‐mode suppression ratio up to 48 dB.
In recent years laser light has been used to control the motion of electron waves. Electrons can now be diffracted by standing waves of light. Laser light in the vicinity of nanostructures is used to affect free electrons, for example, femto‐second and atto‐second laser‐induced electrons are emitted from nanotips delivering coherent fast electron sources. Optical control of dispersion of the emitted electron waves, and optically controlled femto‐second switches for ultrafast electron detection are proposed. The first steps towards electron accelerators and matter optics on‐a‐chip are now being taken. New research fields are driven by these new technologies. One example is the optical generation of electron pulses on‐demand and quantum degenerate pulses. Another is the emerging development of interaction free electron microscopy. This review will focus on the field of free electron quantum optics with technologies at the interplay of lasers, electron matter waves, and nanostructures. Questions that motivate their development will also be addressed.
Monocrystalline titanium dioxide (TiO2) micro‐spheres support two orthogonal magnetic dipole modes at terahertz (THz) frequencies due to strong dielectric anisotropy. For the first time, we experimentally detected the splitting of the first Mie mode in spheres of radii m through near‐field time‐domain THz spectroscopy. By fitting the Fano lineshape model to the experimentally obtained spectra of the electric field detected by the sub‐wavelength aperture probe, we found that the magnetic dipole resonances in TiO2 spheres have narrow linewidths of only tens of gigahertz. Anisotropic TiO2 micro‐resonators can be used to enhance the interplay of magnetic and electric dipole resonances in the emerging THz all‐dielectric metamaterial technology.
Narrow‐linewidth lasers are key elements in optical metrology and spectroscopy. Spectral purity of these lasers determines accuracy of the measurements and quality of collected data. Solid state and fiber lasers are stabilized to relatively large and complex external optical cavities or narrow atomic and molecular transitions to improve their spectral purity. While this stabilization technique is rather generic, its complexity increases tremendously moving to longer wavelenghts, to the infrared (IR) range. Inherent increase of losses of optical materials at longer wavelengths hinders realization of compact, room temperature, high finesse IR cavities suitable for laser stabilization. In this paper, we report on demonstration of quantum cascade lasers stabilized to high‐Q crystalline mid‐IR microcavities. The lasers operating at room temperature in the 4.3‐4.6 μm region have a linewidth approaching 10 kHz and are promising for on‐chip mid‐IR and IR spectrometers.
Optically levitated nanodiamonds with nitrogen‐vacancy centers promise a high‐quality hybrid spin‐optomechanical system. However, the trapped nanodiamond absorbs energy from laser beams and causes thermal damage in vacuum. It is proposed here to solve the problem by trapping a composite particle (a nanodiamond core coated with a less absorptive silica shell) at the center of strongly focused doughnut‐shaped laser beams. Systematical study on the trapping stability, heat absorption, and oscillation frequency concludes that the azimuthally polarized Gaussian beam and the linearly polarized Laguerre‐Gaussian beam LG03 are the optimal choices. With our proposal, particles with strong absorption coefficients can be trapped without obvious heating and, thus, the spin‐optomechanical system based on levitated nanodiamonds are made possible in high vacuum with the present experimental techniques.
We reveal unusually strong polarization sensitivity of electric and magnetic dipole resonances of high‐index dielectric nanoparticles placed on a metallic film. By employing dark‐field spectroscopy, we observe the polarization‐controlled transformation from high‐Q magnetic‐dipole scattering to broadband suppression of scattering associated with the electric dipole mode, and show numerically that it is accompanied by a strong enhancement of the respective fields by the nanoparticle. Our experimental data for silicon nanospheres are in an excellent agreement with both analytical calculations based on Green's function approach and the full‐wave numerical simulations. Our findings further substantiate dielectric nanoparticles as strong candidates for many applications in enhanced sensing, spectroscopy and nonlinear processes at the nanoscale.
In the development of microfluidic chips, conventional 2D processing technologies contribute to the manufacturing of basic microchannel networks. Nevertheless, in the pursuit of versatile microfluidic chips, flexible integration of multifunctional components within a tiny chip is still challenging because a chip containing micro‐channels is a non‐flat substrate. Recently, on‐chip laser processing (OCLP) technology has emerged as an appealing alternative to achieve chip functionalization through in situ fabrication of 3D microstructures. Here, the recent development of OCLP‐enabled multifunctional microfluidic chips, including several accessible photochemical/photophysical schemes, and photosensitive materials permiting OCLP, is reviewed. To demonstrate the capability of OCLP technology, a series of typical micro‐components fabricated using OCLP are introduced. The prospects and current challenges of this field are discussed.
Inspired from butterfly wings that exhibit unique dewetting properties and brilliant structural color synchronously, we reported here the preparation of biomimetic few‐layer graphene films through a template‐directed chemical vapor deposition method using laser‐structured Cu foil as substrates. Hierarchical micronanostructures, including microscale stripes derived from the laser scanning and nanoscale laser‐induced periodic surface structures (LIPSS), formed on Cu foil after a simple femtosecond laser treatment. By tuning the laser power, the surface roughness of the resultant Cu foils can be well controlled. Using the laser structures Cu foil as templates, biomimetic few‐layer graphene films with both iridescence and superhydrophobicity have been successfully prepared. The present work may open up a new way to design and prepare structured graphene film in a biomimetic manner, and we deem that the bioinspired few‐layer graphene films may find broad applications in the near future.
Dewetting of thin metal films is one of the most widespread method for functional plasmonic nanostructures fabrication. However, simple thermal‐induced dewetting does not allow to control degree of nanostructures order without additional lithographic process steps. Here we propose a novel method for lithography‐free and large‐scale fabrication of plasmonic nanostructures via controllable femtosecond laser‐induced dewetting. The method is based on femtosecond laser surface pattering of a thin film followed by a nanoscale hydrodynamical instability, which is found to be very controllable under specific irradiation conditions. We achieve control over degree of nanostructures order by changing laser irradiation parametrs and film thickness. This allowed us to exploit the method for the broad range of applications: resonant light absorbtion and scattering, sensing, and potential improving of thin‐film solar cells.
Transformation optics, a recent geometrical design strategy of light manipulation with both ray trajectories and optical phase controlled simultaneously, promises an invisibility cloaking device that can render a macroscopic object invisible even to a scientific instrument measuring optical phase. Recent “carpet” cloaks have extended their cloaking capability to broadband frequency ranges and macroscopic scales, but they only demonstrated the recovery of ray trajectories after passing through the cloaks, while whether the optical phase would reveal their existence still remains unverified. In this paper, a phase‐preserved macroscopic visible‐light carpet cloak is demonstrated in a geometrical construction beyond two dimensions. As an extension of previous two‐dimensional (2D) macroscopic carpet cloaks, this almost‐three‐dimensional carpet cloak exhibits three‐dimensional (3D) invisibility for illumination near its center (i.e. with a limited field of view), and its ideal wide‐angle invisibility performance is preserved in multiple 2D planes intersecting in the 3D space. Optical path length is measured with a broadband pulsed‐laser interferometer, which provides unique experimental evidence on the geometrical nature of transformation optics.
We report complete spatial shaping (both phase and amplitude) of the second‐harmonic beam generated in a nonlinear photonic crystal. Using a collinear second‐order process in a nonlinear computer generated hologram imprinted on the crystal, the desired beam is generated on‐axis and in the near field. This enables compact and efficient one‐dimensional beam shaping in comparison to previously demonstrated off‐axis Fourier holograms. We experimentally demonstrate the second‐harmonic generation of high‐order Hermite–Gauss, top hats and arbitrary skyline‐shaped beams.
The recent progress in integrated quantum optics has set the stage for the development of an integrated platform for quantum information processing with photons, with potential applications in quantum simulation. Among the different material platforms being investigated, direct‐bandgap semiconductors and particularly gallium arsenide (GaAs) offer the widest range of functionalities, including single‐ and entangled‐photon generation by radiative recombination, low‐loss routing, electro‐optic modulation and single‐photon detection. This paper reviews the recent progress in the development of the key building blocks for GaAs quantum photonics and the perspectives for their full integration in a fully‐functional and densely integrated quantum photonic circuit.
A necessary condition for generation of bright soliton Kerr frequency combs in microresonators is to achieve anomalous group velocity dispersion (GVD) for the resonator modes. This condition is hard to implement in the visible as well as ultraviolet since the majority of optical materials are characterized with large normal GVD in these wavelength regions. We overcome this challenge by borrowing ideas from strongly dispersive coupled systems in solid state physics and optics. We show that photonic compound ring resonators can possess large anomalous GVD at any desirable wavelength, even if each individual resonator is characterized with normal GVD. Based on this concept, we design a mode‐locked frequency comb with thin‐film silicon nitride compound ring resonators in the vicinity of the rubidium D1 line (794.6 nm) and propose to use this optical comb as a flywheel for chip‐scale optical clocks.
Nanoscale lasers are attractive for their potential applications in highly integrated photonic devices and systems. Here, nanolaser arrays are realized based on individual waved CdS nanoribbons (NRs) with periodically modulating thickness along the length direction. Microstructure investigations reveal that such a waved NR is formed with triangular‐prism‐like ridges alternately assembled on both sides of a surface flat nanoribbon. Under the focused laser (488 nm) excitation, the emitted light is guided along the length of the waved ribbons and can be well confined into theses ridges, being reflected and leaked out at their ends along both the lateral sides of the NRs. Polarization measurements further demonstrate the formation of the cavities along the length of the ridges. Under pulse laser excitation, the confined light in all these parallel ridges can resonate and realize lasing, forming a nanolaser array based on these individual waved NRs. These nanolasers arrays have potential applications in highly integrated photonics, signal processing, and high‐throughput sensing.
High efficiency, broad bandwidth, and robust angular tolerance are key considerations in photonic device design. Here, a few‐layer, asymmetric light transmitting metasurface that simultaneously satisfies all the above requirements is reported. The metasurface consists of coupled metallic sheets. It has a measured transmission efficiency of 80%, extinction ratio of 13.8 dB around 1.5 μm, and a full width half maximum bandwidth of 1.7 μm. It is as thin as 290 nm, has good performance tolerance against the angle of incidence and constituent nano‐structure geometry variations. This work demonstrates a practical asymmetric light transmission device with optimal performance for large scale manufacturing.
A novel approach to facilitate excitation and readout processes of isolated negatively charged nitrogen‐vacancy (NV) centers is proposed. The approach is based on the concept of all‐dielectric nanoantennas. It is shown that the all‐dielectric nanoantenna can significantly enhance both the emission rate and emission extraction efficiency of a photoluminescence signal from a single NV center in a diamond nanoparticle on a dielectric substrate. The proposed approach provides high directivity, large Purcell factor, and efficient beam steering, thus allowing an efficient far‐field initialization and readout of several NV centers separated by subwavelength distances.
