46.7MeV/u 12C诱发核反应中的双质子干涉研究

本文讨论了46.7MeV/u ¹²C+⁵⁸Ni,¹¹⁵In,¹⁹⁷An实验中双质子干涉的研究结果,研究了零寿命Koonin模型中核力、库仑力及费米统计对关联函数的影响,并从实验中提取了发射源的半径参数r₀,实验发现r₀随着靶核质量的增加而增加,实验中还研究了发射源的大小与两个关联粒子能量和E₁+M₂的关系,得出的r₀值随着E₁+E₂的增加而减少,反映了高能质子主要来源于反应的早期.     

百兆电子伏特/核子原子核诱发乳胶核反应靶核反冲质子多重数涨落分析(英文)

利用标度阶乘矩方法对290 A MeV $^{12}$C-AgBr, 400 A MeV $^{12}$C-AgBr, 400 A MeV $^{20}$Ne-AgBr及500 A MeV $^{56}$Fe-AgBr 作用靶核反冲质子在二维正常相空间及累积变量空间发射过程中的多重数涨落分别进行了分析。实验结果表明:在正常相空间,对于秩数q较小时标度阶乘矩（$ln$）随相空间的分割数的增加而增加,而对于秩数较大时标度阶乘矩（$ln$）随相空间的分割数的增加表现出先增加后趋于饱和或减小的趋势;在累积变量空间,标度阶乘矩（$ln$）随相空间的分割数的增加而减小,这表明对于我们所研究的核作用体系靶核反冲质子发射过程中不存在非统计涨落。Multiplicity fluctuation of the target recoil protons emitted in $290$\,A MeV $^{12}$C-AgBr, $400$\,A MeV $^{12}$C-AgBr, $400$\,A MeV $^{20}$Ne-AgBr and $500$\,A MeV $^{56}$Fe-AgBr interactions are studied using the scaled factorial moment (SFM) method in two-dimensional normal phase space and cumulative variable space, respectively. It is found that in normal phase space the SFM ($\ln$) increases linearly with the increase of the divided number of phase space ($\ln{M}$) for lower q-values and increases linearly and then becomes saturation or decrease with the increase of $\ln{M}$ for higher q-values, and in cumulative variable space $\ln$ decreases linearly with the increase of $\ln{M}$, which indicates that no evidence of non-statistical multiplicity fluctuation is observed in our data sets.     

质子轰击钨靶表面时的电子发射产额与靶温度的相关性研究

在中国科学院近代物理研究所兰州重离子加速器国家实验室测量了能量为50～250 keV的质子入射不同温度下钨靶表面的电子发射产额。实验结果发现,不同能量的质子引起的电子发射产额均随着靶温度的升高而降低;利用功函数对温度的依赖性定性地解释了该结果。在不同靶温度下,总电子发射产额与电子能损的比值随着质子能量的增加而逐渐变小;利用靶原子不同壳层中电子之间的电离竞争机制来解释实验结果。     

50~250 keV质子入射SiC和Si靶时的电子发射特性研究

在中国科学院近代物理研究所兰州重离子加速器国家实验室测量了能量范围为50~250 keV 的质子入射碳化硅靶和硅靶表面的电子发射产额。实验结果发现,两种半导体靶材的电子发射产额随质子入射能量变化趋势均与作用过程中电子能损随质子入射能量的变化趋势相似。通过分析电子发射的能量来源,发现实验中电子发射产额主要由动能电子发射产额贡献,势能电子发射产额可以忽略不计。两种靶材的电子发射产额均近似地正比于质子入射靶材过程中的电子能损,比例系数B随入射能量略有变化。     

利用质子能损检测气体靶区有效靶原子密度的实验研究

准确测量气态靶区的有效靶原子密度能够提升离子与气体和离子与等离子体靶相互作用实验结果的精度和对物理过程的认识.实验中利用离子加速器引出的100 ke V质子束穿过一定长度的氢气靶,对质子的剩余能量进行了精确测量,获得了在气体靶内的质子能损数据,结合已有的能损研究结果,重新标定了气体靶区内的有效靶原子密度.分别比较了能损、电离型真空计IonIVac ITR 90和薄膜电容型真空计Varian CDG-500的实验测量结果,对比了修正后的电离型真空计有效气压曲线,结果发现质子束能损的测量方式具有原位、高准确性、在线监测等突出优势,为诊断气态靶有效原子密度提供了新的方法.     

进一步指认近质子滴线核129Pm的衰变

2004年曾报道过利用⁴⁰Ca＋⁹²Mo融合蒸发反应产生了近质子滴线新核素Pm,并首次观测到它(EC+b+)衰变产生的能量为99keV的γ射线. 为了进一步确认上述指认，以下提供了三方面的新证据：1)在164－190MeV能量范围内测量了99keV衰变γ射线的激发函数;2)进行了交叉反应 ³⁶Ar＋⁹⁶Ru的实验,观察到了相同的99keV衰变γ射线；3)用Woods-Saxon Strutinsky方法计算了¹²⁹Pm的核势能面，其基态自旋宇称被预言为5/2^－，所以¹²⁹Pm的(EC＋b＋)衰变有利于馈送到子核¹²⁹Nd的5/2_－的低位态，这也与前期报道相符.     

利用改进的Gamow-like模型研究原子核的α衰变和质子放射性

通过引入离心势和静电屏蔽效应对Gamow-like模型进行了改进,并将其用于α衰变和质子放射性研究,发现改进的Gamow-like模型能更好地符合实验数据。另外,还利用改进的Gamow-like模型预言了16个丰质子核的质子放射性的半衰期以及7个$Z=120$超重核素($^{296-308}120$)α衰变链上原子核的α衰变的半衰期,为将来在大科学装置上合成和鉴别这些新核素提供重要的理论参考。     

400~1500 MeV质子轰击铅靶和钨靶的出射中子能谱的FLUKA和Geant4模拟研究

在ADS散裂靶系统的优化设计中,蒙特卡罗方法结合可靠的散裂反应理论模型进行中子学计算具有重要的作用。本工作利用Geant4程序中的INCLXX模型、BIC模型以及BERT模型和FLUKA程序分别模拟了597 MeV和1 500 MeV质子轰击薄铅靶不同出射角度的中子双微分截面,500,1 500 MeV质子轰击厚铅靶不同出射角度的中子双微分产额,以及400,600,800,1 000和1 200 MeV质子轰击厚钨靶在反角方向（175 °）的中子双微分产额,并与实验数据进行比较。研究表明,对于薄铅靶,Geant4程序的INCLXX模型和FLUKA程序模拟结果与实验符合得更好。能量在10～40 MeV范围内,BIC模型模拟结果明显高于实验数据,而BERT模型模拟结果略微低于实验数据。对于厚铅靶,在40 MeV左右所有的模拟结果都低于实验数据。对于厚钨靶,Geant4程序的BIC模型和FLUKA程序与实验数据符合得较好,INCLXX模型在能量高于60 MeV时模拟结果低于实验数据,BERT模型与实验数据差异较大。总体来看,Geant4程序的INCLXX模型和FLUKA程序进行ADS散裂靶相关的中子学的计算是合理和可靠的。The reliable Monte Carlo simulation codes coupled with nuclear reaction models play an important role in the neutronic calculation for the design and optimization of the ADS spallation target. In this work, the double differential cross sections at different angles produced from a thin lead target bombarded with 597 and 1 500 MeV protons, the neutron energy spectra at different angles produced from a thick lead target bombarded with 500 and 1 500 MeV protons, and the neutron energy spectra in the backward direction(175°) produced from a thick tungsten target bombarded with 400, 600, 800, 1 000 and 1 200 MeV protons are calculated with the Geant4 code coupled INCLXX, BIC and BERT models and the FLUKA code. The calculations are compared with the available experimental data. The results show that, for the thin lead target, the calculations with the Geant4 coupled INCLXX model and FLUKA code well reproduce the experimental results. In a energy range from 10 to 40 MeV, BIC model obviously overestimates the experimental results, and BERT model slightly underestimates the experimental results. For the thick lead target, all of the calculations underestimate the experimental results around 40MeV. For the thick tungsten target, the Geant4 coupled BIC model and FLUKA code well reproduce the experimental results. INCLXX model underestimates the experimental results above 60 MeV. BERT model bad reproduces the experimental results. Overall, the neutronic calculations with the Geant4 code coupled INCLXX model and FLUKA code for the ADS spallation target is reasonable and reliable.     

利用GEANT4和FLUKA研究质子诱发散裂反应出射中子双微分截面

在中高能质子诱发散裂反应相关核工程设计中,可靠的蒙特卡罗模拟程序结合核反应理论模型具有较好的理论指导意义。本工作中,利用GEANT4耦合INCL4和ABLA理论模型以及FLUKA耦合PEANUT模型模拟计算了几百MeV至几个GeV质子轰击Be,Al,Fe,W,U等靶后30°,60°,120°,150°出射角产生的散裂中子双微分截面,并与现有实验数据进行了比较。结果发现,FLUKA和GEANT4模拟计算较好地再现了Al,Fe,W,U等靶实验测量数据。然而,模拟结果明显低估了Be靶出射中子能量小于10 MeV能区的实验数据。For the design of nuclear engineering related with medium-high energy proton induced spallation reaction,the reliable Monte Carlo simulation codes coupled with nuclear reaction models have a good theoretical guidance.In this work,the production spallation neutron double differential cross sections at 30°,60°,120°,150°emission angle for Be,Al,Fe,W,U target materials at incident proton energies between several hundred MeV and GeV are theoretically calculated by using the GEANT4 coupled INCL4 and ABLA,and the FLUKA coupled PEANUT.The calculated results were compared with the available experimental data.It is found that the GEANT4 and FLUKA calculations well reproduced the experimental measurement of Al,Fe,W,U target materials.However,calculations obviously underestimated the emission neutrons of Be target for lower than 10 MeV energy range.     

Proximity Approach to Study the Fusion Barriers for Proton and Helium Induced Reactions

By using various proximity potentials, the fusion barrier heights and positions are calculated for proton and helium induced reactions with targets in the mass range 51≤ A ≤130 and 12≤ A ≤233, respectively. The calculated fusion barriers are parameterized by using the relations RB^Par = aX1 ＋ b and VB^Par = cX2, where X1 and X2 are A2^1/3 and Z1Z2/RB^Par, respectively. The values of the constants a, b and c are different for different versions of proximity potentials. We find that the parameterized forms derived by using Proximity 1977 yield values closer to the empirical data in proton as well as helium induced reactions and can be used further to estimate directly the barrier parameters for the fusion reactions of proton and helium with any target.     

利用GEANT4和TALYS研究中子与铁作用的次级中子双微分截面

铁的次级中子双微分截面对核装置的设计、运行与维护具有重要作用。相关实验数据缺乏,且评价数据不完善,需要使用可靠的核理论模型进行计算。本工作利用GEANT4程序结合不同的中子评价数据计算了8.17, 11.5, 14.1和18 MeV等入射能量下中子轰击薄铁靶不同出射角度的次级中子双微分截面;同时利用TALYS程序和GEANT4程序结合BIC、BERT和INCLXX模型计算了25.7, 65, 100和150 MeV等入射能量下中子轰击薄铁靶不同出射角度的次级中子双微分截面,并与实验数据进行对比。研究表明,在20 MeV以下能区,ENDF/B-VIII.0库的计算结果与实验数据符合较好,BROND-3.1、CENDL-3.1、JENDL-4.0u和JEFF-3.3库的计算结果与实验数据存在差异。在20~150 MeV能区,GEANT4程序的BERT模型和TALYS程序的计算结果与实验数据符合较好,INCLXX模型和BIC模型的计算结果与实验数据存在分歧。整体来看,需要对铁的中子评价数据和核反应理论模型做进一步研究。     

中子引起氘核破裂反应的实验研究

对25 MeV中子引起氘核破裂反应的中子-中子准自由散射和17.36 MeV中子引起氘核破裂反应的中子-中子末态相互作用进行了细致的研究。首先,以小于5%的不确定度,精确测量了25MeV中子-中子准自由散射出射的中子三重微分截面。实验数据用基于现实核子-核子势(CD-Bonn,Argonne!18,Nijm I和II)的理论计算配合Monte-Carlo模拟进行了分析。实验结果比基于CD-Bonn势的理论预言高(16.0±4.6)%,进一步证实了目前的理论在中子-中子准自由散射方面还无法准确描述实验数据。其次,通过运动学非完全测量,精确测量了17.36 MeV中子引起氘核破裂反应在0°角附近出射的质子能谱,用基于现实核子-核子势(CD-Bonn、Bonn-B和Nijm I)的理论计算以及Monte-Carlo模拟分析了所测得的质子能谱,确定了中子-中子散射长度ann=(-16.8±0.6)fm。     

Experimental Study of Photon Induced Reactions on 3He and 4He at Low Energies

Data are reported for the photodisintegration cross section of the reaction ³He(??, p)²H at ten energies between 7.0 and 16.0?MeV. Very preliminary data are presented for the reaction ⁴He(??, p)³H between 22.0 and 29.5?MeV in 0.5?MeV energy steps, and for the reaction ⁴He(??, n)³He at three energies around 28.0?MeV. High-pressure He/Xe gas scintillators served as target and detector. Our data are in better agreement with recent theoretical calculations than the majority of the existing data for all three reactions, but differ significantly from recent data taken with a mono-energetic photon beam and a time-projection chamber.     

Analytic Treatment of Proton Induced Electromagnetic Cascades

The electromagnetic cascade induced by the π⁰'s produced by the interaction of a proton and its secondaries (mainly π±'s) is described. Simple considerations indicate that a large part of the energy of the proton is used to produce π⁰'s (see Appendix B). Using the scaling hypothesis of FEYNMAN we derive analytical solutions for the cascade equations. The solution indicate that at the beginning of the cascade the π⁰'s produced by the nucleon are more important for the development of the cascade than those produced by π±'s. The situation changes with increasing atmospheric depth. The average energy of the electrons and photons is nearly the same as indicated by the above mentioned simple considerations. A comparison with a photon induced cascade shows that the proton induced electromagnetic cascade is developing slowly and living longer.     

利用FLUKA研究加速器生产医用放射性同位素的产额

针对目前核医学广泛关注的医用放射性同位素99Mo/99mTc、64,67Cu、68Ge/68Ga、82Sr/82Rb、211At、225Ac等,本文利用FLUKA程序对加速器生产上述同位素的产额及产物分布进行了研究。研究表明,医用放射性同位素的产额随束流能量增加而增加,增加趋势逐渐降低;产额随辐照时间的增长而增加,随辐照后冷却时间的增长而降低,变化情况主要取决于目标医用同位素的半衰期;入射束流在同位素靶的有效射程内产生医用放射性同位素,选取合适的靶厚可以优化目标医用同位素的比活度值等;此外,束流能量越高产生的杂质核素种类及产额也相应增加,合适的辐照能区和辐照时间等,可以降低后续目标医用同位素分离纯化等工作的复杂程度。本文通过FLUKA的计算初步为加速器生产医用同位素提供了重要的依据。     

S-Factor Analysis of Proton Capture Reactions on 112,114,116,119Sn and 113,115In Isotopes

Physics of Atomic Nuclei - The probability of a reaction’s occurrence is known as reaction cross section which provides researchers numerous benefits and details to generate advanced studies....     

质子衰变研究

介绍了质子衰变的基本原理,综述了质子衰变实验研究的现状． The principle of proton radioactivity is introduced. The present status of experimental studies on proton radioactivity is reviewed.      

Study of Cold Fusion Reactions Using Collective Clusterization Approach

Within the framework of the dynamical cluster decay model(DCM), the 1n evaporation cross-sections(σ_(1n)) of cold fusion reactions(Pb and Bi targets) are calculated for ZCN = 104–113 superheavy nuclei. The calculations are carried out in the fixed range of excitation energy E_(CN)~*= 15 ± 1 MeV, so that the comparative analysis of reaction dynamics can be worked out. First of all, the fission barriers(B_f) and neutron separation energies(S_(1n)) are estimated to account the decreasing cross-sections of cold fusion reactions. In addition to this, the importance of hot optimum orientations of β_(2i)-deformed nuclei over cold one is explored at fixed angular momentum and neck-length parameters.The hot optimum orientations support all the target-projectile(t,p) combinations, which are explored experimentally in the cold fusion reactions. Some new target-projectile combinations are also predicted for future exploration. Further,the 1n cross-sections are addressed for Z_(CN) = 104–113 superheavy nuclei at comparable excitation energies which show the decent agrement with experimental data upto Z_(CN) = 109 nuclei. Finally, to understand the dynamics of higher-Z superheavy nuclei, the cross-sections are also calculated at maximum available energies around the Coulomb barrier and the effect of non-sticking moment of inertia(INS) is also investigated at these energies.     

核苷酸和芳香酮的电子转移和质子转移反应研究

利用时间分辨的激光闪光光解方法在1∶1乙腈/水溶液中得到了4种核苷酸和芳香酮的瞬态吸收光谱,通过瞬态吸收光谱的变化研究了鸟苷酸、腺苷酸、胞苷酸、胸腺苷酸猝灭二苯甲酮、呫吨酮激发三重态的反应。由于实验中生成了抽氢自由基和负离子自由基,以及核苷酸正离子在水中的快速抽氢反应,推断出芳香酮和鸟苷酸、腺苷酸的反应机理是先发生电子转移后发生质子转移。而在芳香酮和胞苷酸、胸腺苷酸的反应中没有观察到相应的抽氢自由基和负离子自由基的瞬态吸收峰,由此推断出它们和胞苷酸、胸腺苷酸没有发生电子转移和质子转移反应。对瞬态吸收峰处的时间衰减曲线进行拟合得到了核苷酸猝灭芳香酮的速率常数,可以看到随着反应自由能变ΔG的增大,反应速率常数逐渐减小。