共查询到18条相似文献,搜索用时 156 毫秒
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利用三维经典系综模型研究了氢分子非次序双电离对核间距的依赖性.在不同分子取向下,氢分子双电离率随核间距的增大而先增大后减小,在核间距为4a.u.时取最大值.氢分子非次序双电离对核间距的依赖性随分子轴与激光偏振方向间夹角φ的增大而减弱.φ=0时,氢分子非次序双电离包含丰富的相关模式,对核间距有强烈的依赖性φ=π/2时,不同核间距下的相关模式相似,重碰撞在双电离过程中发挥更重要的作用.这些结果表明分子结构对双原子分子非次序双电离有重要影响.
关键词:
非次序双电离
核间距
关联动量分布 相似文献
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利用经典系综模型研究了椭圆偏振激光脉冲驱动的氩原子非次序双电离.计算结果表明,非次序双电离产率随着椭偏率的增大而减小;双电离得到的电子对在激光偏振平面长轴方向的末态关联动量谱呈现正关联,在激光偏振平面短轴方向的末态关联动量谱呈现反关联;Ar2+在激光偏振平面短轴方向的末态动量谱呈现单峰结构,并且随着椭偏率增大而变宽.轨迹分析显示,椭圆偏振激光脉冲驱动下,非次序双电离仍然是通过再碰撞而发生;随着椭偏率的增大,有效碰撞和单电离之间的时间延迟增加,这是因为椭偏率较大时第一个电子需要经过多次往返才能与母核离子发生有效碰撞. 相似文献
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利用三维经典系综模型系统地研究了反向旋转双色椭偏场中Ar原子非次序双电离对椭偏率的依赖。数值结果显示双电离发生的概率随800 nm激光场椭偏率增大而增大,随1 600 nm激光场椭偏率增大而减小。这是因为当固定1 600 nm激光场椭偏率时,电子的返回概率和碰撞能量随800 nm激光场椭偏率增大而增大。而当固定800 nm激光场椭偏率时,电子的返回概率和碰撞能量随1 600 nm激光场椭偏率增大而减小。在两椭圆激光场的长轴沿x方向条件下,当1 600 nm激光场椭偏率为0.3时,离子动量分布由x负半轴向x正半轴移动。随着1 600 nm激光场和800 nm激光场椭偏率的增大,离子动量分布逐渐在y方向扩展最终形成一个分布于x轴两侧的两层结构。 相似文献
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采用含时密度泛函理论方法研究线性分子碳化锂(Li2C2)对飞秒激光场响应的电子-离子动力学行为.在典型的近共振和非共振的激光频率作用下,分别对比分析了分子的共振和非共振电离过程.研究发现:分子在共振频率激光场的作用下发生更强的电离过程,并倾向于发生库伦爆炸,键长的振荡断裂与电离相互促进影响,而分子在较弱的激光场作用下发生单光子电离过程;随着双脉冲时间间隔的增加,离化电子数在一定范围内呈振荡上升趋势,随后趋于常数. 相似文献
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通过数值求解二维含时薛定谔方程研究了氢分子离子在圆偏振XUV少周期激光电场中的单光子电离,结果观察到不同核间距的氢分子离子的光电子能谱的能移现象.分析表明,在少周期激光场宽频情况下,分子电离电子的双中心干涉改变了夫兰克-康登因子的单调递减趋势,使不同核间距氢分子离子的光电子能谱出现能量移动. 相似文献
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利用三维经典系综模型,研究空间非均匀激光场驱动的氙原子非次序双电离,并对比了空间均匀激光场的情况.结果显示,波长较短时,空间非均匀激光场与空间均匀激光场的非次序双电离的产率较为相近.随着波长的增大,较高激光强度时空间非均匀激光场下非次序双电离受到越来越明显的抑制.相比于空间均匀激光场,空间非均匀激光场下非次序双电离两电子的末态发射角表现出更强烈的关联特性,特别在较大的激光波长下,两电子的末态发射角几乎全部集中在0°附近,这意味着两电子往往是平行发射到相同方向.此外,波长由近红外增大到中红外时,空间非均匀激光场下非次序双电离的有效再碰撞均由第1个电子的第1次返回主导,而空间均匀激光场下则呈现由第1次返回主导到第2次返回主导的转变.进一步,通过反演分析非次序双电离的经典轨迹,揭示了空间非均匀激光场下关联电子超快动力学过程的更多细节. 相似文献
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Theoretical study on non-sequential double ionization of carbon disulfide with different bond lengths in linearly polarizedlaser fields
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By using a two-dimensional Monte-Carlo classical ensemble method, we investigate the double ionization(DI) process of the CS_2 molecule with different bond lengths in an 800-nm intense laser field. The double ionization probability presents a "knee" structure with equilibrium internuclear distance R = 2.9245 a.u.(a.u. is short for atomic unit). As the bond length of CS increases, the DI probability is enhanced and the "knee" structure becomes less obvious. In addition,the momentum distribution of double ionized electrons is also investigated, which shows the momentum mostly distributed in the first and third quadrants with equilibrium internuclear distance R = 2.9245 a.u. As the bond length of CS increases,the electron momentum becomes evenly distributed in the four quadrants. Furthermore, the energy distributions and the corresponding trajectories of the double-ionized electrons versus time are also demonstrated, which show that the bond length of CS in the CS_2 molecule plays a key role in the DI process. 相似文献
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We investigate the quantum mechanical process of two-electron tunneling in strong external electric fields. Numerical solution of a two-electron s-wave model reveals the existence of collective tunneling ionization in a mode where both electrons stay at equal distance from the nucleus. Otherwise the lagging electron is immediately recaptured. The corresponding double ionization rate fails to explain nonsequential multiple ionization in strong-field laser experiments. However, an empirically modified version of the analytical one-electron tunneling rate of Ammosov, Delone, and Krainov agrees with the experiments to a surprising accuracy. The reason for this agreement is presently unknown. 相似文献
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Litvinyuk IV Légaré F Dooley PW Villeneuve DM Corkum PB Zanghellini J Pegarkov A Fabian C Brabec T 《Physical review letters》2005,94(3):033003
Shakeup of a two-electron system is investigated in the strong infrared laser field limit, both theoretically and experimentally. During tunnel ionization the electron shakes up a second electron to an excited bound state. Theoretically, a complete analytical theory of shakeup in intense laser fields is developed. We predict that shakeup produces one excited sigma(u) D(+)(2) state in approximately 10(5) ionization events. Shakeup is measured experimentally by using the molecular clock provided by the internuclear motion. The number of measured events is found to be in excellent agreement with theory. 相似文献
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在最近的实验和理论研究中,我们探讨了氩原子和氖原子在红外强激光场中低于再碰撞阈值的非序列双电离问题。在研究中,我们发现在非序列双电离过程中,氖原子的电子关联表现为在激光偏振面内肩并肩出射,而对于氩原子的电子关联行为表现为在激光偏振面内的背对背出射,我们采用三维半经典模型(考虑电子隧道电离)很好地解释了实验结果。在阈值附近,我们发现电子在激光场中的多次散射以及电子再碰撞激发后电子隧道电离是氩原子反关联行为的主要原因,而电子在激光场作用下的单次碰撞是电子关联行为的主要原因。通过测量双电离过程中产生电子的横向电子动量分布,观察到了库伦聚焦效应,我们认为这是非经典的关联行为。最后,我们给出了氩原子和氖原子在激光场中阈值的解析模型,并给出了原子的关联和反关联激光强度区域。 相似文献
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在最近的实验和理论研究中,我们探讨了氩原子和氖原子在红外强激光场中低于再碰撞阈值的非序列双电离问题。在研究中,我们发现在非序列双电离过程中,氖原子的电子关联表现为在激光偏振面内肩并肩出射,而对于氩原子的电子关联行为表现为在激光偏振面内的背对背出射,我们采用三维半经典模型(考虑电子隧道电离)很好地解释了实验结果。在阈值附近,我们发现电子在激光场中的多次散射以及电子再碰撞激发后电子隧道电离是氩原子反关联行为的主要原因,而电子在激光场作用下的单次碰撞是电子关联行为的主要原因。通过测量双电离过程中产生电子的横向电子动量分布,观察到了库伦聚焦效应,我们认为这是非经典的关联行为。最后,我们给出了氩原子和氖原子在激光场中阈值的解析模型,并给出了原子的关联和反关联激光强度区域. 相似文献
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The multielectron dissociative ionization dynamics of N2 molecule in intense femtosecond laser fields with arbitrary polarization
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The field-ionization Coulomb explosion model is extended to investigate the multielectron dissociative ionization process of N2 molecule irradiated by an intense femtosecond laser field with an arbitrary polarization. The ionization process of N2 molecule is found to be optimal at the critical internuclear distance Rc=7a.u., which is independent of the laser polarization state, the molecular explosion channel and the angle between the molecular axis and the direction of laser electric field. The kinetic energies of the ion fragments are identical in the cases of linear and circular polarizations at the same incident laser intensity. However,the probability of electron ionization is very sensitive to the above three parameters. At the critical distance Rc=7a.u. the angular dependence of the threshold intensity for the over-the-barrier ionization leads to the geometric alignment of molecules in the case of linear polarization. The threshold intensity in the case of circular polarization is apparently higher than that in the case of linear polarization, which can well explain the significant decrease of ionization in the case of circular polarization. The numerical calculations are compared with the experimental measurements. 相似文献
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The effect of electron initial longitudinal velocity on the non-sequential double ionization process in an elliptically polarized laser field
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The effect of initial longitudinal velocity of the tunnelled electron on the non-sequential double ionization(NSDI) process in an elliptically polarized laser field is studied by a semiclassical model.We find that the non-zero initial longitudinal velocity has a suppressing effect on single-return collision(SRC) events in the double ionization process,more specifically,it results in an obvious reduction in the center part of the correlation momentum distributions in the direction of the major polarization axis(z axis) and makes the distribution of single-return collision in the minor polarization axis(x axis) become narrower. 相似文献
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The effect of electron initial longitudinal velocity on non-sequential double ionization process in elliptically polarized laser field
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The effect of initial longitudinal velocity of the tunnelled electron on the non-sequential double ionization (NSDI) process in elliptically polarized laser field is studied by a semiclassical model. We find that the non-zero initial longitudinal velocity has a suppressing effect on single-return collision (SRC) events in double ionization process, more specifically, it results in an obvious reduction in the center part of the correlation momentum distributions in the direction of the major polarization axis (z axis) and makes the distribution of single-return collision in the minor polarization axis (x axis) become narrow. 相似文献