Second harmonic stimulated Raman scattering of laser radiation in aplasma

A high-power linearly polarized laser propagating through a plasma produces oscillatory electron velocity at the second harmonic due to-the ν&oarr;×B&oarr; force, This velocity couples a Langmuir wave (ω, k&oarr;) and an electromagnetic wave (ω₁, k&oarr;₁), where ω₁=ω-2ω₀ , k-2k&oarr;₀ and ω₀, k&oarr;₀ are frequency and wavenumber of the laser pump, causing second harmonic Raman scattering. The growth rate is maximum for side scattering. This process can occur above the quarter critical density, unlike the first harmonic stimulated Raman scattering which occurs below the quarter critical density     

Second harmonic imaging of chloroplasts using the two-photon laser scanning microscope

BackgroundSecond harmonic information reveals information about the structure of spatially oriented structures with an asymmetry. We study the second harmonic images of the grana and intergranal parts of chloroplasts in the leaves of the shade moss Plagiomnium affine.ResultsA two-photon microscope with blocking filters to suppress fluorescence generated both forward and backward second harmonic illumination to be captured. In the starch free chloroplasts of the single cell layered laminae strong second harmonic generation (SHG) from the granal regions was emitted. Upon illumination the chloroplasts changed their orientation affecting the SHG signal. Chloroplast is reoriented upon illumination.ConclusionsSHG signals were successfully obtained from the grana without any possible confusion from SHG starch grains due to their absence.     

用于激光等离子体诊断实验的二倍频探针光系统

为了满足基准物理实验的要求,准确地探测出靶面的等离子体的电子温度、密度、电子离子漂移速度等参数,在星光Ⅱ激光装置上发展了一束二倍频激光作为探针光。通过模拟实验已经证实了该探针光的二倍频总能量大于5J,焦斑尺寸小于100μm,可以满足激光与等离子体相互作用的高功率要求。目前,该探针光系统已经用于用于激光等离子体诊断实验的常规运行。     

正态分布随机数发生器及其在模拟光传输软件中的应用

利用计算机高级语言提供的伪随机数发生器,通过“高斯筛选”和“求平均值”两种方法,开发出满足正态分布的随机数发生器。将其应用于分析大型激光装置光路稳定性的模拟软件中,成功地完成了对“神光Ⅲ原型装置四程放大器”的光路稳定性分析。     

Second harmonic generation by femtosecond laser pulses in the Laue scheme

Results of the study of second harmonic generation by femtosecond laser pulses in a lithium niobate crystal with a regular domain structure in the Laue scheme are presented. The angular distribution of the intensity and the polarization properties of the second harmonic radiation are studied. The orders of the corresponding phase-matching conditions and the angular width of the second harmonic maxima are calculated theoretically. The theoretical results are compared with experimental data.     

行波管中二次谐波注入对三阶互调的抑制

利用Christine 1维多信号非线性互作用物理模型,对螺旋线行波管中注入二次谐波后三阶互调的输出进行了模拟。模拟结果表明：在螺旋线大功率行波管中,通过二次谐波注入能有效地抑制三阶互调输出,从而降低了行波管的非线性输出,并存在最佳的注入功率和相位条件,使三阶互调可被抑制到最低。介绍了二次谐波注入抑制三阶互调的实验研究,并与模拟结果进行了比较,两者基本一致。     

Second harmonic generation of a self-focused Hermite-Gaussian laser in plasma

Second harmonic generation (SHG) using intense Hermite-Gaussian laser beam (HGLB) propagating through the plasma for mode-indices m = 0 and m = 1 is reported in the present work. Ponderomotive force induced density perturbation beats with the oscillatory velocity of electrons at incident laser frequency, generate the second harmonic nonlinear current that give rise to SHG. Using paraxial approximations, we have derived the coupled equations for the beam width parameter of HGLB and second harmonic's normalized amplitude. Resonance condition is obtained by considering wiggler magnetic field which providing an extra momentum to the second harmonic photon and this result a significant increase in the amplitude of SHG. Our analysis shows the prominent rise in normalized amplitude of second harmonic on increasing the value of the intensity of fundamental laser pulse, normalized wiggler magnetic field and normalized density of plasma. It is notified that the gain of SHG is more prominent for m = 1. Dependency of laser and plasma parameters on SHG is also reported in the current work.     

高功率半导体激光器倍频实现紫外光输出

采用中心波长780 nm、线宽0.13 nm的体布拉格光栅外腔半导体激光作为基频光,基于Ⅰ类相位匹配的三硼酸锂晶体(LBO),获得了中心波长为390 nm的倍频光输出,输出功率30 μW,转换效率0.01%,为高功率紫外光束的实现提供了新的技术路线。     

Second harmonic generation from thick leaves using the two-photon laser scanning microscope

A laser-scanning microscope using second harmonic generation (SHG) as a probe is shown to produce high-resolution images of duckweed Lemna minuta leaves. These leaves are multi-cell layer thick. Second harmonic light is generated by a tightly focused short pulse laser beam and is collected by two objectives yielding forward and backward second harmonic digital images. This measurement shows that the signal of the second harmonic imaging in the forward and backward directions depends on the thickness of the chloroplast and that the forward-SH image was brighter than the backward-SH image. The image intensity also depended on the orientation of the chloroplast in relation to the illuminating polarization direction. Their light-induced re-orientation which was affected by the intensity of the illumination could be observed during the experiments.The novelty of this work is to establish new compact technique in which one can use the SH imaging to investigate the true architecture of the sensitive samples, the unknown samples and the samples which is not producing auto-fluorescence. Moreover, investigation of new or unknown samples needs a long time for looking at details of the sample. Thereby the sample will be exposed for long time to the laser radiation that will cause photobleaching and photodamage. Since the SHG does not undergo photobleaching and photodamage this will be the promising technique for investigating the sensitive and new unknown samples. Then one can move to acquire fluorescence images after complete investigation of the true architecture of the sample. The other advantage of SHG is that it has the ability to image highly ordered structural proteins without any exogenous labels. The SHG is an intrinsic and a coherent process. Imaging of intrinsic compounds avoids the complications of slicing and labeling, and samples can be investigated under physiological conditions.     

Second harmonic generation in proustite using a HF laser as the fundamental

Second harmonic generation in proustite is reported for the first time using a HF laser as the fundamental. The angular dependence of the S.H. power has been studied. A conversion efficiency of about 3% has been obtained.     

Watt-class green-emitting laser modules using direct second harmonic generation of diode laser radiation

Large-area high-resolution displays, using a flying-spot to create the picture, require light sources in the red, green and blue wavelength range with a high optical output power and nearly diffraction limited beam. In this paper we present experimental results of high-brightness distributed Bragg reflector tapered diode lasers at 106x nm that can be used for single-pass second harmonic generation into the green. Based on these lasers we developed compact (2.5 cm³) green laser modules with an output power of 1W at 53x nm and an electro-optical conversion efficiency of about 5%. The output power stability is better than 2% and the wavelength stability is ±10 pm. The excellent beam quality M _?? ² < 2 of the green light allows operation in flying spot application systems. Furthermore, we estimate that our concept allows power scaling up to 2W by using nonlinear planar waveguide crystals and into the multi-watt level by spectral beam combining.     

Optimum conditions for the generation of the second harmonic of intense laser radiation

A generalized approximation of strong interactions of waves is suggested for the theoretical analysis of second-harmonic generation under conditions of self-action. On the basis of the method suggested, approximate solutions for the efficiency of second-harmonic generation are obtained with regard to the influence of higher nonlinearities, depletion of pumping radiation, and linear phase mismatch. The effects of the phase mismatch and the spatial distribution of the amplitude of the fundamental harmonic on the efficiency of second harmonic generation by intense laser radiation is analyzed. The results obtained with the approximate method developed are shown to be in good agreement with known experimental data and numerical calculations. Optimum conditions for second harmonic generation are determined in a wide range of laser radiation intensity and at different spatial distributions of the fundamental harmonic amplitude.     

Irregular frequency chirp in radiation of an injection laser in high-velocity code modulation

The effect of the shape of the excitation pulses on the magnitude of the frequency chirp in an injection laser is investigated. It is established that as the degree of rectangularity of the pulses becomes higher, the frequency chirp increases. Simultaneous consideration of the effect of residual charge in the active region of the laser, the delay of stimulated radiation, and the frequency chirp indicates that in the case of high-velocity code modulation of an injection laser, in the latter an irregular frequency chirp appears that can exert a noticeable influence on the distortion of code trains of pulses having a super-Gaussian shape, when they propagate in media with a dispersion of 100 p.s./nm/km and above. Belarusian State University, 4, F. Skorina Ave., Minsk, 220050, Belarus. Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 64, No. 1, pp. 45–49, January–February, 1997.     

Third harmonic generation of laser radiation in Fe- and Zn-doped polyvinylpyrrolidone

The results of third-order nonlinear susceptibilities studies of Fe- and Zn-doped polyvinylpyrrolidone (PVP) aqueous solution in processes of third harmonic generation of Nd:YAG laser radiation are presented. Nonlinear susceptibilities of PVP:Fe and PVP:Zn were calculated to be 5×10^-13 esu and 3×10^-13 esu respectively. Third harmonic conversion efficiencies in these metallocomplexes were measured to be 8×10^-7 and 5×10^-7 respectively. The Z-scan method was applied to determine Kerr effect influence on frequency conversion process. The value of nonlinear refractive index of PVP:Fe at the wavelength of λ = 1064 nm was measured to be n ₂ = - 6.7×10^-13 esu. Received 30 November 2001 / Received in final form 27 March 2002 Published online 28 June 2002     

Second harmonic generation as a method for polarizing and analyzing laser light

Second harmonic nonlinear crystals can be successfully used as light polarizers and analyzers. An extinction ratio (ER) of 6×10^–9 for a system consisting of a Glan prism and KDP doubler is demonstrated. This nonlinear optical analyzer was used to test ER of calcite Glan air spaced prisms.     

Second harmonic generation: the solution for an amplitude-modulated initial pulse

We address the initial value problem for one-dimensional second harmonic generation starting from a purely amplitude-modulated fundamental wave. A general method to solve the problem in terms of a Schrödinger equation is presented, in which the initial pulse-shape is taken as a potential. Several examples with the complete solution given in analytical form are discussed. A much broader class of solutions can be found with the help of a single numerical integration. In particular, solutions with incident pulses approximating a sech -shape have been obtained.     

Use of carbon-containing materials for efficient high-order harmonic generation of laser radiation

A systematic study of the high-order harmonic generation (HHG) of laser radiation in various carbon-containing plasma plumes (CCPPs) is presented. The materials studied are: graphite, boron carbide, C₆₀, polytetrafluoroethylene, polyethylene, carbon nanotubes, and soot. These studies show that CCPPs present the best plasma media for efficient lower order (from 9th to 19th) harmonic generation, while the harmonic cutoff restricted to the 29th order. The advantages of CCPPs for the harmonic generation are confirmed by comparison of the HHG conversion efficiency with that in Ag and In plasma plumes, where the highest conversion efficiency was reported. Use of two-color pump scheme allows further enhancement of harmonic yield from the CCPPs.     

Application of VUV laser harmonic radiation to the measurement of porous silicon dielectric function

Vacuum ultra-violet (VUV) laser harmonics have been generated in a noble gas jet, which, combined with a standard spectrophotometer, have allowed measurements of the reflectance of porous silicon over a wide energy spectral range from 1 to 16 eV. Porous silicon dielectric function was, then, deduced from reflectance measurements by Kramers–Kronig analysis. Data are found to be in good agreement with those reported in literature, thus showing that laser harmonics represent a new, alternative, and suitable VUV source for optical characterisation of materials such as semiconductors and thin films.     

Generation of shaped ultraviolet pulses at the third harmonic of titanium-sapphire femtosecond laser radiation

We experimentally demonstrate a method to generate shaped femtosecond laser pulses in the ultraviolet at a central wavelength of 267 nm, the third harmonic of conventional titanium-sapphire femtosecond laser systems. Employing a 128-pixel liquid-crystal spatial light modulator, we impose variable spectral phase modulations upon the near-infrared laser pulses. By this, complex laser pulses can be shaped whose overall spectrum is still conserved. Our experiments show that it is possible to easily transfer these pulses into the ultraviolet at 267 nm via sum-frequency mixing in nonlinear crystals and to predictably generate multistructured ultraviolet femtosecond laser pulses. We analyze the temporal and spectral composition of these pulses after frequency conversion into the ultraviolet using difference-frequency cross-correlation and XFROG (cross-correlation frequency-resolved optical gating) techniques with an unmodulated fundamental laser pulse. The method can be employed to facilitate adaptive quantum control experiments in the ultraviolet wavelength regime, where the major absorption bands of many organic molecular systems are located. PACS 42.65.Re; 42.72.Bj; 32.80.Qk