Collapsing dynamics of a laser-induced cavitation bubble near the edge of a rigid wall

In the present paper, the collapsing dynamics of a laser-induced cavitation bubble near the edge of a rigid wall is experimentally investigated with a high-speed photography system. For a symmetrical setup, the two primary control parameters of the bubble collapsing behavior include the equivalent maximum bubble radius and the distance between the bubble and the edge of the rigid wall. Based on the bubble interface deformation during the collapsing process, three typical cases are identified for the categorization of the phenomenon with the influences of the parameters revealed. Through a quantitative analysis of the obtained high-speed photos, the motions of the bubble interface in different directions are given together with the calculations of the bubble centroid. The primary findings of the present paper could be summarized in terms of the bubble-edge distance as follows. When the bubble is close to the edge, the movement of the bubble interface near the edge will be restricted with a clear neck formation in the middle part of the bubble. For this case, the edge could delay the bubble collapsing time up to 22% of the Rayleigh collapsing time. When the bubble is of the medium distance to the edge, the differences of the expansion or shrinkage of the bubble interface among different directions will be reduced with an olive-shaped bubble formed during the collapsing process. For this range of parameters, the bubble moves rapidly toward the edge especially during the final collapsing stage. When the bubble is far away from the edge, the bubble will be a nearly spherical one.     

Study on the spatial distribution of the liquid temperature near a cavitation bubble wall

A simple new model of the spatial distribution of the liquid temperature near a cavitation bubble wall (T_li) is employed to numerically calculate T_li. The result shows that T_li is almost same with the ambient liquid temperature (T₀) during the bubble oscillations except at strong collapse. At strong collapse, T_li can increase to about 1510 K, the same order of magnitude with that of the maximum temperature inside the bubble, which means that the chemical reactions occur not only in gas-phase inside the collapsing bubble but also in liquid-phase just outside the collapsing bubble. Four factors (ultrasonic vibration amplitude, ultrasonic frequency, the surface tension and the viscosity) are considered to study their effects for the thin liquid layer. The results show that for the thin layer, the thickness and the temperature increase as the ultrasonic vibration amplitude rise; conversely, the thickness and the temperature decrease with the increase of the ultrasonic frequency, the surface tension or the viscosity.     

空化泡液体外围压强的分布

本文从空化泡动力学理论出发,分别讨论了空化泡在压缩和膨胀时液体中的压强分布情况,并作了数值模拟。研究结果表明,空化泡在膨胀和压缩时其外围压强分布明显不同,不能将其一并而论。发现当空化泡的半径增大时液体的压强在不断变化,压强是先变小后变大。而且这个压强的变化还与待测点距空化泡的距离有关。当空化泡的半径在不断变小时外界的压强在不断增大,当空化泡刚开始压缩时液体中的压强变化情况不是很明显,但当空化泡的半径变到1μm时,空化泡外界压强出现明显变化。当空化泡压缩到较小时,此时再增加外界压强空化泡的半径也不会在有很大的变化。     

Theoretical investigation and experimental support for the cavitation bubble dynamics near a spherical particle based on Weiss theorem and Kelvin impulse

In the present paper, the laser-induced cavitation bubble dynamics near a fixed spherical particle is comprehensively investigated based on the Weiss theorem, the Kelvin impulse theory and the high-speed photography experiment. Firstly, the applicability range of the theoretical model in the time and the space is statistically obtained based on sufficient experimental results. Then, the in-depth theoretical analysis is carried out in terms of the liquid flow field and the bubble Kelvin impulse with the corresponding experimental results as the reasonable support. In addition, the theoretical prediction model of the bubble movement is established and experimentally fitted from the analytic expression of the Kelvin impulse. Through our research, it is found that: (1) the applicability range of the Kelvin impulse theory for the bubble near the spherical particle is approximately the dimensionless distance between the bubble and particle (γ) greater than 0.50. (2) The effect of the particle on the liquid velocity between the bubble and the particle is mainly manifested in the form of the image bubble, which always causes the liquid velocity in this region to be significantly lower than other surrounding regions. (3) The average movement velocity of the bubble centroid can be reasonably predicted by establishing a directly proportional function between the Kelvin impulse and the velocity with the relationship constant (α) equal to 3.57×10⁻⁶ ± 1.63×10⁻⁷ kg.     

Spatial-temporal dynamics of cavitation bubble clouds in 1.2 MHz focused ultrasound field

Cavitation bubbles have been recognized as being essential to many applications of ultrasound. Temporal evolution and spatial distribution of cavitation bubble clouds induced by a focused ultrasound transducer of 1.2 MHz center frequency are investigated by high-speed photography. It is revealed that at a total acoustic power of 72 W the cavitation bubble cloud first emerges in the focal region where cavitation bubbles are observed to generate, grow, merge and collapse during the initial 600 μs. The bubble cloud then grows upward to the post-focal region, and finally becomes visible in the pre-focal region. The structure of the final bubble cloud is characterized by regional distribution of cavitation bubbles in the ultrasound field. The cavitation bubble cloud structure remains stable when the acoustic power is increased from 25 W to 107 W, but it changes to a more violent form when the acoustic power is further increased to 175 W.     

Dynamics and measurement of cavitation bubble

Based on the introduction of international progress, our investigations on acoustic cavitation have been reported. Firstly we considered the cavity’s dynamics under the drive of the asymmetrical acoustic pressure. An aspheric dynamical model was proposed and a new stable and aspheric solution was found in numerical simulation of the theoretical framework of the aspheric model. Then, a dual Mie-scattering technique was developed to measure the cavity’s aspheric pulsation. A significant asynchronous pulsation signal between two Mie-scattering channels was caught in the case of large cavity driven by low acoustic pressure. As a direct deduction, we observed an evidence of cavity’s aspheric pulsation. Furthermore, we studied the dependency of the asynchronous pulsation signal on the various parameters, such as the amplitude and frequency of the driving acoustic pressure, and the surface tension, viscosity and gas concentration of the liquid. Finally, we introduced a new numeric imaging technique to measure the shapes of the periodic pulsation cavities. The time-resolution was in the order of 20 ns, one order of magnitude lower than that in the previous work, say, 200 ns.     

Experimental investigation of the collapse of laser-generated cavitation bubbles near a solid boundary

The oscillation of a laser-generated single cavitation bubble near a solid boundary is investigated by a fiber-optic diagnostic technique based on optical beam deflection (OBD). The maximum bubble radii and collapse time for each oscillation cycle are determined from a sequence of bubble oscillations. Furthermore, by combining the revised Rayleigh theory, the prolongation factor κ at different dimensionless parameter γ (γ=L/R_max, where R_max is the maximum bubble radius and L is the distance of a cavity inception point from a boundary) is obtained. In addition, the prolongation factor of the collapse time versus laser energy is also derived, which are valuable in the fields of hydraulic cavitation, laser lithotripsy and laser ophthalmology.     

Optical investigation of cavitation erosion by laser-induced bubble collapse

By means of a new force sensor based on optical beam deflection (OBD), the mechanical effects of laser-matter interaction underwater at different incident laser energy are investigated in detail. The experimental results show that a target underwater is impacted in turn by laser-plasma ablation force and high-speed liquid-jet impulse induced by bubbles collapse in the vicinity of a solid boundary. Furthermore, the amplitudes of the two forces increase monotonously with laser energy. According to the ablation force detected by the experiment and the theoretical relationship between laser intensity and ablation pressure, the value of liquid-jet impact against a solid boundary can be easily obtained. In addition, based on the model of a collapsing bubble, some characteristic parameters, such as the liquid-jet impact velocity, the maximum bubble radius, the bubble energy can also be obtained at different laser energy, which are valuable in the corresponding research fields.     

Insights into numerical simulation of controlled ultrasonic waveforms driving single cavitation bubble activity

A computational study treating cavitation phenomenon within a single bubble undergoing various controlled ultrasonic waveforms is presented in this paper. Numerical simulations using sinusoidal, square, triangular and sawtooth waves crossing an aqueous media, saturated with oxygen, are conducted upon various operational conditions of frequency and amplitude. Bubble radius, temperature and pressure were estimated over time for 64 combined cases. The obtained results show that at relatively low acoustic pressure, i.e. 1.5 and 2 atm, the square wave is proved to generate the highest temperature and pressure inside the bubble, while triangular and sawtooth ones remain the less interesting waveforms for sonochemical application within the same operational conditions. At higher amplitudes above 2.5 atm, this trend is changed, especially at low frequencies, i.e. 200 and 300 kHz, where square wave showed some limitations in attaining the optimal values of the strong collapse within one acoustic cycle.     

声场中水力空化泡的动力学特性

以水为工作介质,考虑了液体黏性、表面张力、可压缩性及湍流作用等情况,对文丘里管反应器中空化泡在声场作用下的动力学行为特性进行了数值研究.分析了超声波频率、声压及喉径比对空化泡运动特性以及空化泡崩溃时所形成泡温以及压力脉冲的影响.结果表明,超声将水力空化泡运动调制成稳态空化,有利于增强空化效果. 关键词： 超声波 水力空化 湍流 气泡动力学     

Physical insights into the sonochemical degradation of recalcitrant organic pollutants with cavitation bubble dynamics

This paper tries to discern the mechanistic features of sonochemical degradation of recalcitrant organic pollutants using five model compounds, viz. phenol (Ph), chlorobenzene (CB), nitrobenzene (NB), p-nitrophenol (PNP) and 2,4-dichlorophenol (2,4-DCP). The sonochemical degradation of the pollutant can occur in three distinct pathways: hydroxylation by OH radicals produced from cavitation bubbles (either in the bubble–bulk interfacial region or in the bulk liquid medium), thermal decomposition in cavitation bubble and thermal decomposition at the bubble–liquid interfacial region. With the methodology of coupling experiments under different conditions (which alter the nature of the cavitation phenomena in the bulk liquid medium) with the simulations of radial motion of cavitation bubbles, we have tried to discern the relative contribution of each of the above pathway to overall degradation of the pollutant. Moreover, we have also tried to correlate the predominant degradation mechanism to the physico-chemical properties of the pollutant. The contribution of secondary factors such as probability of radical–pollutant interaction and extent of radical scavenging (or conservation) in the medium has also been identified. Simultaneous analysis of the trends in degradation with different experimental techniques and simulation results reveals interesting mechanistic features of sonochemical degradation of the model pollutants. The physical properties that determine the predominant degradation pathway are vapor pressure, solubility and hydrophobicity. Degradation of Ph occurs mainly by hydroxylation in bulk medium; degradation of CB occurs via thermal decomposition inside the bubble, degradation of PNP occurs via pyrolytic decomposition at bubble interface, while hydroxylation at bubble interface contributes to degradation of NB and 2,4-DCP.     

Characterization of cavitation in a flow-through exposure chamber by means of a resonant bubble detector

Ultrasonic cavitation at frequencies of 0.514, 0.866, 1.03 and 1.61 MHz in water flowing through tubes was observed by counting bubbles downstream with a resonant bubble detector (RBD) operated at 0.89 or 1.7 MHz. In a 21 mm diameter, thin-walled tube, cavitation thresholds in tap water flowing at 5.3 cm s^?1 ranged from 2.0 – 2.5 bar at 0.514 MHz to 3 – 4 bar at 1.61 MHz. When high speed injections were employed to trigger the ultrasonic cavitation with hydrodynamically-generated bubbles, the thresholds were reduced to about 2 bar and bubble production was enhanced for 1.03 and 1.61 MHz exposures. Ultrasonic radiation forces on the bubbles and bubble coalescence appeared to cause, under some conditions, a reduction in bubble counts during subthreshold exposures when bubbles were injected into the flow. The RBD method is a useful tool for detecting and semi-quantitatively observing cavitation in a flow-through exposure system.     

声场中双空化泡的运动特性

空化泡的运动特性是声场作用下的动力学行为,受空化泡初始半径,声压幅值,驱动声压频率,液体特性等众多因素的影响,是个复杂工程。本文从双空化泡运动方程出发,考虑到液体粘滞系数、空化泡辐射阻尼项的影响,研究了不同初始半径、驱动声压频率、驱动声压幅值、液体粘滞系数下空化泡泡壁的运动情况,研究结果表明不同初始半径、外界驱动声压频率、驱动声压幅值、液体粘滞系数均会对空化泡的膨胀比和空化泡的溃灭时间有一定影响。     

含气量对激光空泡在刚性壁面空蚀的影响

采用强脉冲激光器设计液体环境下刚性壁面空蚀实验平台,改变液体中含气量,利用高速相机观察不同含气量条件下激光空泡在壁面附近的脉动过程,并对刚性壁面造成的空蚀结果进行了观测。实验研究发现,随着液体中相对空气含量的提高,激光空泡脉动的最大尺寸增大,空泡的膨胀运动变剧烈,溃灭运动速度降低,空泡的溃灭强度降低,从而影响到溃灭冲击波和壁面微射流对刚性壁面的冲击速度,减弱了壁面空蚀,而液体中含气量的提高能够降低激光空泡对刚性壁面的空蚀程度。     

Modeling of surface cleaning by cavitation bubble dynamics and collapse

Surface cleaning using cavitation bubble dynamics is investigated numerically through modeling of bubble dynamics, dirt particle motion, and fluid material interaction. Three fluid dynamics models; a potential flow model, a viscous model, and a compressible model, are used to describe the flow field generated by the bubble all showing the strong effects bubble explosive growth and collapse have on a dirt particle and on a layer of material to remove. Bubble deformation and reentrant jet formation are seen to be responsible for generating concentrated pressures, shear, and lift forces on the dirt particle and high impulsive loads on a layer of material to remove. Bubble explosive growth is also an important mechanism for removal of dirt particles, since strong suction forces in addition to shear are generated around the explosively growing bubble and can exert strong forces lifting the particles from the surface to clean and sucking them toward the bubble. To model material failure and removal, a finite element structure code is used and enables simulation of full fluid–structure interaction and investigation of the effects of various parameters. High impulsive pressures are generated during bubble collapse due to the impact of the bubble reentrant jet on the material surface and the subsequent collapse of the resulting toroidal bubble. Pits and material removal develop on the material surface when the impulsive pressure is large enough to result in high equivalent stresses exceeding the material yield stress or its ultimate strain. Cleaning depends on parameters such as the relative size between the bubble at its maximum volume and the particle size, the bubble standoff distance from the particle and from the material wall, and the excitation pressure field driving the bubble dynamics. These effects are discussed in this contribution.     

含气量对黏性液体中空泡脉动特性的影响

采用自行研制的高灵敏度光偏转测试系统,研究黏性液体中激光空泡脉动特性.判定了空泡两次脉动对应的最大和最小泡半径,进而计算了激光空泡在前两次脉动过程中泡内的含气量.研究表明：泡内含气量对泡脉动特性有较大影响.随着脉动次数的增加,空泡泡内含气量增大.空泡最大泡半径随含气量的增加而增大.此外,受液体黏性影响,空泡膨胀和收缩过程明显变缓. 关键词： 含气量 黏性 激光空泡 脉动特性     

Laser-induced cavitation bubbles and shock waves in water near a concave surface

The interplay among the cavitation structures and the shock waves following a nanosecond laser breakdown in water in the vicinity of a concave surface was visualized with high-speed shadowgraphy and schlieren cinematography. Unlike the generation of the main cavitation bubble near a flat or a convex surface, the concave surface refocuses the emitted shock waves and causes secondary cavitation near the acoustic focus which is most pronounced when triggered by the shock wave released during the first main bubble collapse. The shock wave propagation, reflection from the concave surface and its scattering on the dominant cavity is clearly resolvable on the shadowgraphs. The schlieren approach revealed the pressure build up in the last stage of the collapse and the first stage of the rebound. A persistent low-density watermark is left behind the first collapse. The observed effects are important wherever cavities collapse near indented surfaces, such as in cavitation peening, cavitation erosion and ophthalmology.     

超声场下刚性界面附近溃灭空化气泡的速度分析

为了揭示刚性界面附近气泡空化参数与微射流的相互关系, 从两气泡控制方程出发, 利用镜像原理, 建立了考虑刚性壁面作用的空化泡动力学模型. 数值对比了刚性界面与自由界面下气泡的运动特性, 并分析了气泡初始半径、气泡到固壁面的距离、声压幅值和超声频率对气泡溃灭的影响. 在此基础上, 建立了气泡溃灭速度和微射流的相互关系. 结果表明: 刚性界面对气泡振动主要起到抑制作用; 气泡溃灭的剧烈程度随气泡初始半径和超声频率的增加而降低, 随着气泡到固壁面距离的增加而增加; 声压幅值存在最优值, 固壁面附近的气泡在该最优值下气泡溃灭最为剧烈; 通过研究气泡溃灭速度和微射流的关系发现, 调节气泡溃灭速度可以达到间接控制微射流的目的.     

流体控制方程的超声空化泡动力学模拟*

本文基于流体动力学控制方程和VOF模型,在FLUENT 14.5软件环境下对超声空化泡进行数值模拟。首先研究了超声空化泡一个周期内的形态变化,并且利用空化泡形态变化的最大面积、最小面积、膨胀时间、收缩时间等数值结果分析超声参数对空化效果的影响。同时探究了双频超声作用下空化泡运动的变化,计算结果表明:在其他条件相同的情况下,在1~5MPa范围内,超声声压幅值为3MPa时空化效果最好;当超声频率大于20kHz时,空化效果随着超声频率的增大而降低。对于频率相同的双频超声,较声压幅值为其两倍的单频超声有更好的空化效果;对于频率不同的双频超声,空化效果受到频率差的影响。