Soft X-ray resonant magnetic scattering studies on Fe/CoO exchange bias system

We have used soft X-ray resonant magnetic scattering (XRMS) to search for the presence of an effective ferromagnetic moment belonging to the antiferromagnetic (AF) layer which is in close contact with a ferromagnetic (F) layer. Taking advantage of the element specificity of the XRMS technique, we have measured hysteresis loops of both Fe and CoO layers of a CoO(40 Å)/Fe (150 Å) exchange bias bilayer. From these measurements we have concluded that the proximity of the F layer induces a magnetic moment in the AF layer. The F moment of the AF layer has two components: one is frozen and does not follow the applied magnetic field and the other one follows in phase the ferromagnetic magnetization of the F layer. The temperature dependence of the F components belonging to the AF layer is shown and discussed.     

Spin reorientation transition in Fe/CeH2 multilayers probed by soft X-ray resonant magnetic scattering

The magnetic domain configurations of Fe 3d spins in Fe/CeH₂ multilayers were measured by soft X-ray resonant magnetic scattering. The interface region could be probed by setting up X-ray standing waves due to the multilayer periodicity. By resolving first- and second-order magnetic scattering contributions, we show that the latter probe directly the magneto-crystalline anisotropy which is dominated by the Fe interface layers causing a spin reorientation transition when the temperature is lowered. Received: 30 May 2001 / Accepted: 4 July 2001 / Published online: 5 October 2001     

Soft X-ray resonant magnetic scattering of magnetic nanostructures

Soft X-ray resonant magnetic scattering offers a unique element-, site- and valence-specific probe to study magnetic structures on the nanoscopic length scale. This new technique, which combines X-ray scattering with X-ray magnetic circular and linear dichroism, is ideally suited to investigate magnetic superlattices and magnetic domain structures. The theoretical analysis of the polarization dependence to determine the vector magnetization profile is presented. This is illustrated with examples studying the closure domains in self-organising magnetic domain structures, the magnetic order in patterned samples, and the local configuration of magnetic nano-objects using coherent X-rays. To cite this article: G. van der Laan, C. R. Physique 9 (2008).     

Radiofrequency magnetoresistance of Fe/Cr superlattices

The rf magnetoresistance of Fe/Cr superlattices is studied for two orientations of the current: parallel and across the superlattice layers. A mutually single-valued correspondence is established between the relative magnetoresistance measured at dc current and the change in the transmission coefficient of electromagnetic waves in the magnetic field. When rf currents flow across the layers, the relative change in the signal amplitude is proportional to twice the change in the electrical resistance of the superlattice and is of opposite sign. It is shown that the rf losses are determined by the surface resistance which is proportional to the superlattice thickness and inversely proportional to its conductivity. An equation is derived for the rf electric field distribution in the superlattice. It is established that when the thickness of the superlattice is small compared with the skin layer depth, field and current components which penetrate through the entire superlattice exist.     

Element specific magnetism with resonant X-ray magnetic scattering

Beam line X29 of the National Synchrotron Light Source (NSLS) has been operating for a year for macromolecular crystallography (PX) research, employing a mini-gap, in-vacuum undulator as its X-ray source. Development of this facility involved a close collaboration among the groups of Mark Chance (Case Proteomics Center, Case Western Reserve Univ. [CWR]), Erik Johnson [NSLS], and Robert Sweet (Macromolecular Crystallography Research Resource [PXRR] of BNL's Biology Dept.).

There were several joint objectives and complexities to this project. Firstly, we hoped to provide an undulator-based beam line with the attractive features of high collimation and high flux for macromolecular crystallography at the NSLS.     

Magnetization temperature dependence in Fe/Cr superlattices

We report the temperature dependence of the saturation magnetization, M_s(T), of Fe(t)/Cr(40 Å) superlattices grown on MgO(1 0 0) and MgO(1 1 0) and its variation with Fe-layer thickness (5 Å<t<80 Å). The structure was characterized by X-ray diffraction. M_s(t) vs. T, as measured by DC magnetization and ferromagnetic resonance, show a large interface effect. The origins of this effect are discussed.     

Effect of magnetic ordering on optical and magneto-optical properties of Fe/Cr superlattices

Optical reflectance/transmittance and magneto-optical Kerr effect of Fe/Cr superlattices (SL) are studied by using the first principles full-potential linearized augmented plane-wave method. Equilibrium atomic structures are optimized through total energy and atomic force approaches. Pronounced peaks in the ellipticity and optical spectra are obtained around 3000 cm⁻¹ for the ferromagnetic SL due to the inter-band electron excitations. The change in magnetic ordering from ferromagnetic to antiferromagnetic cases alters optical functions, namely, the reflectance, R and transmittance T. The calculated ΔR/R and ΔT/T have a pronounced maximum around 2000 cm⁻¹ and decay almost linearly thereafter toward high photon energies, a result that agrees qualitatively well with experiment.     

Polarized neutron reflectometry of Fe/Cr/Gd superlattices

The magnetic structure of Fe/Cr/Gd superlattices is investigated using complementary methods of SQUID magnetometry and polarized neutron reflectometry. The complex magnetic behavior of the given system is caused by exchange interaction between the 3d (Fe) and 4f (Gd) layers of the ferromagnetic metals through the Cr antiferromagnetic spacer layer. It is found that a nonuniform profile of magnetization forms within the Gd layers under the influence of this interlayer interaction.     

Quantitative interface roughness analysis of Fe/Cr superlattices

The quantitative characterization of the interface roughness of Fe/Cr superlattices is necessary for the understanding of the transport properties of such structures. This must include both vertical and lateral roughness components. The information can be obtained by specular and off-specular X-ray diffraction and conversion electron Mößbauer spectroscopy. We show how models describing specular and diffuse X-ray diffraction can be applied to extract quantitative data. The robustness of such data can be further enhanced using anomalous scattering, leading to an enhanced material contrast for Fe/Cr. Similarity and complementarity of the X-ray diffraction results with the Mößbauer data are discussed.     

Interlayer magnetic coupling in multilayer magnetic Fe/Cr/Fe systems

The interlayer magnetic coupling of iron layers as a function of the chromium spacer thickness and temperature has been studied for three-layer epitaxial Fe/Cr/Fe films by the methods of Kerr magnetometry and Mandelstam-Brillouin scattering. The results obtained indicate that the short-period component of the interlayer exchange is related to the spin density wave in the chromium spacer.     

The coupling of Cr to Fe studied by circular magnetic X-ray dichroism

The coupling of Cr to Fe in stacked Cr/Fe/Cr trilayers is studied by circular magnetic X-ray dichroism using fluorescence yield to monitor the absorption. From the dichroic spectra, we determine the thickness dependent average magnetic coupling of Cr to Fe for Cr layer thicknesses of 1, 2 and 3 ML. We compare our results to new calculated spectra. Additionally, all Cr spectra show significant contributions due to photon scattering processes at theL _{2, 3} absorption edges depending on the degree of circular polarization.     

Soft X-ray resonant magnetic scattering study of magnetization reversal in low dimensional magnetic heterostructures

Soft X-ray resonant magnetic scattering (SXRMS) has been used to investigate the microscopic magnetization reversal behavior of complex magnetic systems. SXRMS is a unique technique, providing chemical, spatial and magnetic sensitivity, which is not affected by external magnetic fields. The study of two selected thin magnetic heterostructures is presented, amorphous rare-earth transition metal alloys and perpendicular exchange coupled antiferromagnetic/ferromagnetic films. In the first system, the internal structure of magnetic stripe domains on nanometer length scales is obtained by measuring bi-dimensional (2D) scattering images. In the second system, the element specificity is exploited to identify the role of the uncompensated spins in the antiferromagnetic layer on the exchange coupling phenomena. Future trends are also discussed.     

Distribution of the magnetic scattering amplitudes in the Fe/Cu multilayer investigated by resonant magnetic diffraction with circularly polarized hard X-rays

Resonant X-ray magnetic diffraction profiles were measured for an epitaxial Fe/Cu multilayer using circularly polarized X-rays near the Fe and Cu K-edges. Diffraction intensities were compared with those obtained from the theoretical and empirical models. It is found that the interface Fe moment is reduced to 70% of the inner-layer moment. Concerning the Cu layer, the observed energy dependence of the magnetic diffraction intensities is consistent with that derived from the first-principle band calculation, indicating that magnetic proximity effect in the Cu layer is confined within a few atomic layers near the interface.     

Local magnetic states and hyperfine interactions in Fe/Ti magnetic superlattices

Multilayer Fe/Ti films are synthesized by deposition in a Penning discharge. Measurements are made of thhe static hysteresis loops and Mössbauer spectra on Fe⁵⁷ nuclei. The hyperfine magnetic field distribution functions are calculated. It is established that the spontaneous magnetization of Fe/Ti magnetic superlattices undergoes very strong oscillations as a function of the Ti layer thickness. Three groups of peaks are noted in the hyperfine field distribution functions, corresponding to three nonequivalent states of the Fe ions, in one of which these ions do not have a characteristic magnetic moment. These results also agree with measurements of the temperature dependence of the magnetization in weak magnetic fields. For some Ti interlayer thicknesses the saturation magnetization scaled to the Fe content is much higher than the saturation magnetization of bulk Fe.     

X-ray magnetic scattering

The magnetic scattering of synchrotron X-rays has been developed to the point where it is now a standard technique for the study of magnetism and magnetic materials, often complementing neutron investigations of magnetic structures. In this article, after a brief historical introduction, examples of experiments on lanthanide and actinide antiferromagnets are presented. X-ray diffraction and Compton scattering studies of ferromagnets are then considered. Finally future prospects and possibilities are discussed.