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1.
The sign of the exchange interactionJ in a series of radical triplet pairs (RTPs), formed by a nitroxide free radical and a triplet excited fullerene, has been determined from the spin polarization of time-resolved electron paramagnetic resonance spectra. Radical and fullerene are linked together by covalent bonds in different geometries. It is shown that the sign ofJ depends on the overlap between the orbital of nitroxide unpaired electron and the LUMO of fullerene, which is singly occupied in the excited triplet state. When the overlap does not vanish, a negative contribution toJ arises from the admixing of a charge transfer structure in the wave function of the excited doublet state D* of the RTP, which does not take place in the excited quartet state Q*. The mixing of D* and Q* states lowers the energy of the former spin state and gives antiferromagnetic coupling.  相似文献   

2.
The screening of an impurity in the quasi-two-dimensional (2D) electron gas in a δ-doped semiconductor structure is investigated. The screened impurity matrix elements are calculated and compared using three different approaches: the 2D random phase approximation (RPA), the corresponding 2D Thomas–Fermi theory and a quasi-three-dimensional (3D) Yukawa-like screening model. It is found that the 2D Thomas–Fermi theory differs from the RPA result, even in the limit of low q vectors, if more than one subband is occupied. This result is explained analytically by closely examining theq  0 limit of the dielectric tensor. The 2D Thomas–Fermi theory is shown to represent a poor approximation to the RPA whereas the quasi-3D screening model agrees well with the RPA results for not too smallqvectors. Furthermore, this model reduces computing times by orders of magnitude in comparison with the RPA. Thus, our 3D screening model considerably simplifies the calculation of impurity scattering rates in the investigation of the electron mobility in a δ-doping layer.  相似文献   

3.
The collective plasma modes in a quasi-two-dimensional (Q2D) electron system located over the free surface of liquid helium are studied theoretically within many-body dielectric formalism. The dispersion of modes is considered both over bulk liquid and over helium film where the essential modification of interelectron interaction occurs due to screening effects in the substrate with a large value of dielectric constant. It is shown that the plasma spectrum consists of longitudinal and transverse branches which dispersion laws depend on the values of the dielectric constant of helium and the film thickness. For the helium film covering metal, the longitudinal mode is acoustic differing of that for the surface electron (SE) system over bulk helium.  相似文献   

4.
The volume (3D), quasi-two-dimentional (Q2D), and two-dimentional (2D) oscillations of degenerated electrons of the Shubnikov-de Haase reluctance reveal common properties. The region of quantum oscillations is bounded (in the magnetic field) from below by the weak field condition (ωcτt≤1) and from above by the quantum limit condition (ξF≥ħωc/2). The monotonic oscillation component is saturated for the occupied main conduction Em-subband and excitation Ep-subband of dimensional quantization for the Q2D and 2D electron systems in strong magnetic fields. The reluctance of the Q2D system in the quantum limit changes according to a law ∼B α with α ≈ 2.6–2.8. The oscillation amplitude is described by an exponential dependence on the magnetic field strength and temperature, similarly to the 3D case. This is caused by the identity of physical conditions and the topology of resonant escape of the Landau levels out of the Fermi surface. __________ Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 3, pp. 33–39, March, 2006.  相似文献   

5.
We use numerical simulations to investigate the spin Hall effect in quantum wires in the presence of both Rashba and Dresselhaus spin-orbit coupling. We find that the intrinsic spin Hall effect is highly anisotropic with respect to the orientation of the wire, and that the nature of this anisotropy depends strongly on the electron density and the relative strengths of the Rashba and Dresselhaus spin-orbit couplings. In particular, at low densities, when only one subband of the quantum wire is occupied, the spin Hall effect is strongest for electron momentum along the [N110] axis, which is the opposite of what is expected for the purely 2D case. In addition, when more than one subband is occupied, the strength and anisotropy of the spin Hall effect can vary greatly over relatively small changes in electron density, which makes it difficult to predict which wire orientation will maximize the strength of the spin Hall effect. These results help to illuminate the role of quantum confinement in spin-orbit-coupled systems, and can serve as a guide for future experimental work on the use of quantum wires for spin-Hall-based spintronic applications.  相似文献   

6.
We compute the corrections from two-photon and gamma-Z exchange in parity-violating elastic electron-proton scattering, used to extract the strange form factors of the proton. We use a hadronic formalism that successfully reconciled the earlier discrepancy in the proton's electron to magnetic form factor ratio, suitably extended to the weak sector. Implementing realistic electroweak form factors, we find effects of the order 2%-3% at Q(2) less, similar0.1 GeV2, which are largest at backward angles and have a strong Q2 dependence at low Q2. Two-boson contributions to the weak axial current are found to be enhanced at low Q2 and for forward angles. We provide corrections at kinematics relevant for recent and upcoming parity-violating experiments.  相似文献   

7.
In this paper we investigate temperature dependence of the electron self-energy in the polar-crystal slab using Green-function method. We introduce Q2D free Green's function for the first time. Numerical calculations of the electron self-energy using GaAs as an example are performed. The results show that the electron self-energy is a decreasing function of temperature. In calculation, we consider the effect of the excited states on the electron self-energy and find the ground-state energy be about 11% lower than that of bulk polaron. The results also imply that the high excited states pay a larger contribution to the electron self-energy with increasing temperature.  相似文献   

8.
We report superconductivity in a new ternary molybdenum pnictide Rb2 Mo3 As3,synthesized via the solid state reaction method.Powder x-ray diffraction analysis reveals a hexagonal crystal structure with space group P6 m2(No.187), and the refined lattice parameters are a=10.431(5) A,c=4.460(4) A.SEM images show rod-like grains with good ductility,confirming a quasi-one-dimensional(Q1 D) structure.Electrical resistivity and dc magnetic susceptibility characterizatio...  相似文献   

9.
We studied the interlayer magnetoresistance of the representative quasi-one-dimensional (Q1D) layered organic conductor, (TMTSF)2PF6, over the full range of magnetic field orientations in three dimensions, and constructed a stereographic conductivity plot. Our results show that the previously reported angular-dependent magnetoresistance phenomena in Q1D conductors are closely related to one another in intermediate field orientations. Based on a comparison with theories, we can conclude that the Lebed resonance is the only fundamental effect and that other effects result from the modulation of the Lebed resonance amplitude. Most of the observed phenomena can be explained within the framework of the conventional Fermi liquid; however, the anomalous enhancement of the interlayer conductivity under a field parallel to the conducting planes suggests the existence of a new electron state.  相似文献   

10.
Song BS  Jeon SW  Noda S 《Optics letters》2011,36(1):91-93
We design and fabricate ultra-high-quality (Q) photonic nanocavities in a symmetrically glass-clad silicon (Si) two-dimensional (2D) photonic crystal (PhC) structure. We theoretically investigate the dependence of the refractive index of the glass on the Q factors for asymmetric and symmetric structures. We show that the index-symmetric distribution of the glass is a critical factor to realize ultrahigh Q factors for glass-clad 2D PhC structures. We fabricate symmetrically glass-clad Si PhC nanocavities and achieve a record Q factor of 1×10(6), comparable with the highest Q factors of nanocavities in air-bridge structures.  相似文献   

11.
An analytic theory has been derived for determining the eigenfrequencies, RF-field distribution and Q of the TEmpq modes of a gyrotron resonator consisting of a circular cylinder joined to a slowly tapered section. Explicit results are obtained for a linear taper. The cavity modes are found to have an RF-field distribution which is useful for prebunching the electron beam and enhancing efficiency. For high Q cavities, the cavity Q depends on axial mode number q as q–2, which is important for mode discrimination. Proper selection of taper length is found to reduce the Q of high q modes, also aiding in mode discrimination. The present approach may be applied to other forms of weakly irregular cavities, such as cavities with nonlinear tapers.Work supported by U.S.D.O.E. Contract DE-AC02-78ET-51013Supported by U.S. Department of Energy  相似文献   

12.
13.
We report on a new measurement of the parity-violating asymmetry in quasielastic electron scattering from the deuteron at backward angles at Q2=0.038 (GeV/c)2. This quantity provides a determination of the neutral weak axial vector form factor of the nucleon, which can potentially receive large electroweak corrections. The measured asymmetry A=-3.51+/-0.57 (stat)+/-0.58 (syst) ppm is consistent with theoretical predictions. We also report on updated results of the previous experiment at Q2=0.091 (GeV/c)2, which are also consistent with theoretical predictions.  相似文献   

14.
The magnetotransport in a nondegenerate quasi-one-dimensional (Q1D) electron system over superfluid helium has been investigated experimentally. The measurements are performed in the presence of a perpendicular magnetic field B up to 2.6 T in the temperature range T=0.48–2.05 K in the system of conducting channels of 100–400 nm width. It is shown that the value of longitudinal magnetoresistance ρxx increases with B. In the electron-gas scattering region (T>0.9 ), the behaviour of ρxx agrees with classical Drude law. In the quantum transport regime, the self-consistent Born approximation (SCBA) theory for a 2D electron system over liquid helium describes the experimental data qualitatively. The deviation due to the difference of the experimentally studied Q1D system of the electrons in a parabolic potential well differs from theoretically analysed one. The experimental data agree with the theoretical calculation for the Q1D electron system at the weak magnetic field and the low temperature.

The negative magnetoresistance of the conducting channels has been observed in both the gas- and the ripplon-scattering region. These effects have been explained by weak carrier localization on the gas atoms at high temperature and by display of the quantum magnetotransport features in a mesoscopic system at low temperature.  相似文献   


15.
A theory for the magnetocapacitance of a partially screened two-dimensional (2D) electron gas is proposed. The model investigated is sensitive to different types of screening in a 2D electron gas with an integer filling factor: the so-called conventional approach and the self-consistent approximation introduced in the present paper. The calculations point to the importance of the self-consistent treatment of the magnetocapacitance of a 2D electron gas under the conditions of an integer filling factor. The final self-consistent results are qualitatively consistent with the available experimental data. Fiz. Tverd. Tela (St. Petersburg) 39, 742–745 (April 1997)  相似文献   

16.
In this paper, we provide a set of sufficient conditions under which a lattice Boltzmann model does not admit an H theorem. By verifying the conditions, we prove that a number of existing lattice Boltzmann models does not admit an H theorem. These models include D2Q6, D2Q9 and D3Q15 athermal models, and D2Q16 and D3Q40 thermal (energy-conserving) models. The proof does not require the equilibria to be polynomials.  相似文献   

17.
Experiment shows that in AlGaAs/GaAs heterostructures the sheet electron concentration remains almost constant up to a certain temperature, while it increases at higher temperatures. We attempt an interpretation of this temperature dependence, taking into account the fact that in the bulk, n-AlGaAs deep and shallow donors exist, which independently and by different mechanisms provide electrons to the different conduction band minima of the bulk n-AlGaAs, and contribute to the formation of the Q2DEG. We calculate the electronic states of this structure, the Q2DEG and the bulk concentrations, and the corresponding mobilities as a function of temperature. Our numerical results are in an excellent agreement with experimental data.PACS:  相似文献   

18.
The polar optical phonon vibrating modes of a quasi-zero-dimensional (Q0D) wurtzite cylindrical quantum dot (QD) are solved exactly based on the dielectric continuum model and Loudon’s uniaxial crystal model. The result shows that there exist four types of polar mixing optical phonon modes in the Q0D wurtzite cylindrical QD systems, which is obviously different from the situation in blende cylindrical QDs. The dispersive equations for the interface-optical-propagating (IO-PR) mixing modes are deduced and discussed. It is found that the dispersive frequency of IO-PR mixing modes in wurtzite QD just take a series of discrete values due to the three-dimensional confined properties. Moreover, once the radius or the height of the QD approach infinity, the dispersive equations of the IO-PR mixing modes in the wurtzite Q0D cylindrical QD can naturally reduce to those of the IO and PR modes in Q2D QWs or Q1D QWWs systems. This has been analyzed reasonably from both physical and mathematical viewpoints. The analytical expressions obtained in the paper are useful for further investigating phonon influence on physical properties of the wurtzite Q0D QD systems.  相似文献   

19.
We fit the reduced cross section for deep-inelastic electron scattering data to a three parameter ln2s fit, A + beta ln2(s/s0), where s = (Q2/x)(1-x) + m2, and Q2 is the virtuality of the exchanged photon. Over a wide range in Q2 (0.11 < or = Q2 < or = 1200 GeV2) all of the fits satisfy the logarithmic energy dependence of the Froissart bound. We can use these results to extrapolate to very large energies and hence to very small values of Bjorken x-well beyond the range accessible experimentally. As Q2-->infinity, the structure function F2(p)(x,Q2) exhibits Bjorken scaling, within experimental errors. We obtain new constraints on the behavior of quark and antiquark distribution functions at small x.  相似文献   

20.
We construct a generalized gradient approximation of the exchange-correlation energy that satisfies the nonuniform scaling in one dimension and is accurate in the whole quasi-two-dimensional (Q2D) regime. Using spatial and energetic analyses of metal (111) surfaces, we show that the Q2D behavior is important at the surface of most transition metals, and that the here proposed Q2D-generalized gradient approximation functional predicts for these metals accurate surface energies as well as bulk properties.  相似文献   

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