Simultaneous wavelength tuning and amplitude modulation in QPM optical parametric amplifiers

We repot simultaneous optical parametric amplifiers (OPA) and amplitude modulation of signal pulse in a monolithic periodically poled KTP (PPKTP) by electrically controlling the relative phase between the pump, signal and idler waves in a KTP dispersion section sandwiched between two PPKTP gratings, theoretically. The controlling electric field can be arbitrary direction. For an ultrashort pulse group velocity mismatch, group dispersion and diffraction must be regarded, simultaneously. The solutions of the truncated equations, including the above effects in the two PPKTP gratings of simultaneous frequency tuning and amplitude modulation OPA, were analyzed. It is shown that the intensity of output signal pulse of OPA depends on the thickness of the dispersion section, the magnitude and azimuth of controlling electric field and one evidences periodicity. For the certain angular dispersion there exist the largest frequency bandwidths of optical parametric amplifiers. Certain angular dispersion of a signal pulse can increase the frequency bandwidth, and broadband amplification of ultrashort pulse can be performed effectively.     

Investigation of near-collinear degenerated quasi-phase matching optical parametric amplification using PPKTP crystal

The gain properties of near-collinear degenerated phase-matched optical parametric amplification (OPA) using PPKTP crystal are investigated theoretically. The results indicate that the type-0 phase matching of PPKTP has larger accepted angle and better gain spectrum by tuning crystal temperature or rotating crystal angle.     

基于光束偏转的扫描式宽带光参量啁啾脉冲放大

光参量啁啾脉冲放大(OPCPA)是超短激光脉冲领域的重要技术之一,增大增益带宽对提高OPCPA的转换效率、实现宽带光参量放大具有重要的意义.本文将光束偏转和非共线OPCPA有机结合,提出了基于光束偏转的扫描式宽带OPCPA模型.分析了通过光束偏转来时刻改变非共线角,以保证各频率成分的相位匹配,从而增大增益带宽的基本原理.采用提出的扫描式宽带OPCPA,针对800 nm中心波长、带宽约为100 nm信号光的光参量放大进行了数值计算.结果表明:经过扫描式OPCPA后,信号光的带宽与放大之前几乎相同,光谱没有窄化;扫描式OPCPA比固定非共线角方式的放大极大地增加了增益带宽和转换效率,实现了宽带的光参量放大;要满足信号光各频率成分的相位匹配,达到最大的增益带宽和转换效率,需要尽量减小加载到钽铌酸钾(KTa_(1-x) Nb_xO_3, KTN)电光晶体上的电压抖动和电压延时.     

Mid-infrared ZGP OPO pumped by near-degenerate narrowband type-I PPKTP parametric oscillator

The total pulse energy of the signal and idler in a near-degenerate type-I periodically poled KTiOPO₄ (PPKTP) optical parametrical oscillator (OPO) was spectrally confined within a 2 nm spectral bandwidth at 2.13 μm. This was achieved by using a volume Bragg grating as the output coupler. Both the signal and the idler from the PPKTP OPO were then simultaneously used to pump a mid-infrared ZnGeP₂ (ZGP) OPO. The 2 nm bandwidth was narrower than the ZGP crystal acceptance bandwidth and, thus, made efficient conversion in the second OPO possible. A total slope efficiency of 10% from 1.06 μm to the 3.5–5 μm region was demonstrated, generating 250 μJ in the mid-IR with only 3.6 mJ of 1.06 μm pump energy. This corresponds to a Nd:YAG pump to mid-IR conversion efficiency of 7%. PACS 42.65.Yj; 42.72.Ai; 42.40.Eq     

Double quasi phase matching for both optical parametric oscillator and difference frequency generation

We present simultaneous phase matching of optical parametric oscillator (OPO) and difference frequency generation (DFG), using a noncollinear interaction in periodically poled crystal with single grating. Selecting proper grating period Λ and titled angle ξ between the grating vector G and the optical axis of crystal, the noncollinear scheme provides double phase matching solutions over continuous regions of the midwave infrared spectrum. At certain wavelength regions, for DFG process the group velocities between interaction pulses are matching and the phase matching bandwidth reaches maximum. Selecting the different grating period, the broadband midwave tuning and better gain spectrum can be obtained at different wavelength range. For the certain period grating the conversion efficiency is higher. Hence, using the double phase matching configuration, the broadband tunable midwave infrared wave can be produced in single grating. But the configurations have a relatively narrow angular bandwidth.     

Broadband noncollinear optical parametric amplification without angularly dispersed idler

We report a new scheme for direct generation of broadband angular-dispersion-free mid-IR idler pulses via noncollinear optical parametric amplification when group-velocity matched wavelengths cannot be found and the traditional noncollinear geometry fails to increase the phase-matching bandwidth. The scheme does not require any post-amplification idler angular dispersion compensation. We derive and interpret the condition for broadband amplification and absence of idler angular dispersion. A broadband angular-dispersion-free 2.15 μm idler pulse is generated as an experimental demonstration. We identify the potential of the scheme to generate a broadband 3.5 μm idler, with a bandwidth supporting a sub-two-cycle pulse.     

Numerical study on pulse contrast enhancement in a short-pulse-pumped optical parametric amplifier

We investigate pulse cleaning behaviors in short-pulse-pumped optical parametric amplifiers (OPA). We theoretically study the contrast enhancement of amplified signal pulse and generated idler pulse, and reveal their dependence on the parametric gain in both the regimes of small signal and saturated amplifications. The signal contrast enhancement is nearly equal to the parametric gain, while the idler contrast is approximately equal to the product of the contrasts of the pump and signal pulses in a low gain OPA and increases with the gain. The effects of group-velocity mismatch and group-velocity dispersion on the contrast enhancement are also investigated. The results presented in this paper are of value for pulse cleaning.     

飞秒BBO光参量放大中闲频光二次谐波的产生

由于相位匹配条件和非线性晶体透光范围的限制，400nm蓝光抽运的飞秒β-BaB₂O₄（BBO）光参量放大（OPA）输出的参量光调谐范围有限，很难得到波长小于460nm的蓝光和近紫外光.实验采用1kHz钛宝石九通啁啾脉冲放大器的倍频蓝光作抽运光，超连续白光 作种子光，在Ⅰ类非共线相位匹配条件下，利用宽带的飞秒BBO OPA，在一定的实验参数下 获得了530—810nm放大的信号光，以及810nm—17μm波段范围的闲频光.与此同时 ，还获得了410—700nm连续可调的闲频光的二次谐波，其与闲频光层叠分布，单脉冲能量 为26μJ，转换效率大于5%.仅利用单块晶体的飞秒BBO OPA就可以获得410—810nm连 续可调的飞秒脉冲输出，从而为更多研究和应用的需要提供了重要的光源.对飞秒光参量放 大中闲频光二次谐波产生的条件也进行了理论分析. 关键词： 二次谐波 闲频光 非共线相位匹配 飞秒光参量放大     

Ultrabroad gain in an optical parametric generator with periodically poled KTiOPO4

An optical parametric gain bandwidth of 115 THz at full-width half maximum is generated from a picosecond Ti:sapphire pumped degenerate optical parametric generator. This ultrabroad bandwidth could be obtained by first identifying the wavelength where the nonlinear optical material has zero group-velocity dispersion (GVD). By pumping at half this wavelength the degenerate signal–idler pairs can accommodate ultrabroad bandwidths. The explanation for this is that the group velocities of the signal and the idlers are approximately matched and the GVD is small. However, in order to thoroughly investigate the degeneracy region around 1700 nm we fabricated several periodically poled KTiOPO₄ (PPKTP) crystals with different periods, and also one periodically poled RbTiOPO₄ (PPRTP). Both collinear and noncollinear configurations were employed for broadband parametric generation in this region. It was found that the optimum pump wavelength is in the region between 800 nm to 850 nm for PPKTP, and we could also conclude that a similar performance was found for PPRTP. This work will allow the design of optical parametric devices for generating few-cycle pulses in the spectral region between 1.1 μm and 3.8 μm. PACS 42.65.Re; 42.65.Ky; 42.65.-k     

Simultaneous collinear and non-collinear parametric generation in 1D single grating periodically poled lithium tantalate

We report a detailed study of multiple wavelengths optical parametric generation in a single grating one-dimensional periodically poled lithium tantalate crystal. Simultaneous collinear and non-collinear generations are observed around the pump collinear direction. Similar spectra are found in continuous spatial positions symmetrical to the collinear direction, with decreasing signal and increasing idler wavelengths, associated with decreasing powers when the far-field angle increases. A phase matching scheme is proposed to describe these interactions. Numerical simulations emphasize the agreement of our phase matching scheme with the experimental results. Single-pass gain and high pump power density are very likely at the origin of the simultaneous collinear and non-collinear QPM interactions.     

Optical parametric oscillators for high pulse energy and high average power operation based on large aperture periodically poled KTP and RTA

We report on optical parametric oscillators (OPOs) based on large aperture periodically poled KTiOPO₄ (PPKTP) and RbTiOAsO₄ (PPRTA) pumped with high pulse energy and high average power Q-switched solid-state lasers. The OPOs were pumped with 1064-nm pulses of a diode-pumped Nd:YVO₄ laser at 20 kHz repetition rate. The emitted signal wavelengths were 1.72 μm and 1.58 μm and the idler wavelengths were 2.79 μm and 3.26 μm, respectively. Pumping the PPKTP OPO with 7.2 W and the PPRTA OPO with 8 W average power, 2 W and 1.3 W total OPO output powers were generated. Two-dimensional measurements of the total OPO output power, the signal wavelength and the signal bandwidth in dependence on the crystal location indicated a good uniformity of the quasiphasematching structure over the entire 3-mm-thick crystals. This allowed pumping with larger pump beams and therefore with pulse energies of tens of millijoules. Pumping with different flash-lamp-pumped lasers, good OPO performance and high output pulse energies could be achieved for all pump lasers. Maximum input pulse energies of 56 mJ gave output pulse energies of as much as 18 mJ. The temperature tuning behaviors of both OPOs were measured, showing excellent agreement with calculated temperature tuning curves. New equations for temperature dispersion in RTA are presented. These results show that large-aperture PPKTP and PPRTA crystals are well suited for tunable nanosecond OPO operation with multi-watt average pump power and several tens of millijoules pump pulse energies. Received: 7 September 2001 / Published online: 7 November 2001     

板条放大器同步泵浦的宽调谐MgO:PPLN中红外光参量振荡器（英）

搭建了Nd:YVO4/SESAM锁模激光器,采用LDA泵浦的Innoslab对其进行功率放大,最后同步泵浦MgO:PPLN实现了宽调谐皮秒中红外光参量运转。通过改变MgO:PPLN的温度和通道,实现了信号光1415~1557 nm、闲频光3362~4290 nm范围的宽调谐输出,其中最高的光光转换效率为17.5%。同步泵浦功率为16 W,脉冲重复频率为116.9 MHz时,同时获得1.33 W的1518 nm信号光和1.26 W的3558 nm闲频光输出。     

Few‐cycle,broadband, mid‐infrared optical parametric oscillator pumped by a 20‐fs Ti:sapphire laser

A few‐cycle, broadband, singly‐resonant optical parametric oscillator (OPO) for the mid‐infrared based on MgO‐doped periodically‐poled LiNbO₃ (MgO:PPLN), synchronously pumped by a 20‐fs Ti:sapphire laser is reported. By using crystal interaction lengths as short as 250 µm, and careful dispersion management of input pump pulses and the OPO resonator, near‐transform‐limited, few‐cycle idler pulses tunable across the mid‐infrared have been generated, with as few as 3.7 optical cycles at 2682 nm. The OPO can be continuously tuned over 2179‐3732 nm (4589‐2680 cm^‐1) by cavity delay tuning, providing up to 33 mW of output power at 3723 nm. The idler spectra exhibit stable broadband profiles with bandwidths spanning over 422 nm (FWHM) recorded at 3732 nm. The effect of crystal length on spectral bandwidth and pulse duration is investigated at a fixed wavelength, confirming near‐transform‐limited idler pulses for all grating interaction lengths. By locking the repetition frequency of the pump laser to a radio‐frequency reference, and without active stabilization of the OPO cavity length, an idler power stability better than 1.6% rms over >2.75 hours is obtained when operating at maximum output power, in excellent spatial beam quality with TEM₀₀ mode profile. Photograph shows a multigrating MgO:PPLN crystal used as a nonlinear gain medium in the few‐cycle femtosecond mid‐IR OPO. The visible light is the result of non‐phase‐matched sum‐frequency mixing between the interacting beams.     

Investigation of spectral bandwidth of optical parametric amplification

The spectral bandwidth of three-wave-mixing optical parametric amplification has been investigated. A general mathematical model for evaluating the spectral bandwidth of optical parametric amplification is developed with parametric bandwidth and gain bandwidth via three-wave noncollinear interactions. The spectral bandwidth is determined by expanding the wave-vector mismatch in a Taylor series and retaining terms through second order. The model takes into account the effects of crystal length, noncollinear angle, group velocity, group-velocity dispersion and gain coefficient. The relation between parametric bandwidth and gain bandwidth is clearly defined. The model is applied to a BBO OPA, a LBO OPA and a CLBO OPA. PACS 42.65.Yj; 42.65.Lm; 42.65.Ky; 42.60.By     

All-optical control of the carrier-envelope phase with multi-stage optical parametric amplifiers verified with spectral interference

Intense ultrashort laser pulses with stabilized carrier-envelope phase (CEP) are generated at 800 nm by using multi-stage collinear and non-collinear optical parametric amplifiers (OPAs). The first-stage collinear OPA is directly pumped by the fundamental-wave pulses and tuned to generate idler pulses at 1600 nm, which are further amplified by a second-stage collinear OPA, and then frequency-doubled to generate CEP-stabilized pulses at 800 nm. A non-collinear OPA is used to amplify the CEP-stabilized pulses at 800 nm. The combination of different OPAs can generate and amplify CEP-stabilized pulses at 800 nm without any detrimental influence from the fundamental-wave pulses. The CEP stabilization is verified with a simple and robust spectral interference setup. The stable interference pattern is measured for every single pulse and compared with the unstable pattern from pulses of random CEP. PACS 42.65.Re; 42.65.Yj; 42.25.Kb     

周期性极化铌酸锂晶体中半非共线型宽带光学参变放大理论研究

基于周期性极化铌酸锂晶体(PPLN)的准相位匹配光参变放大过程,通过倾斜周期极化铌酸锂晶体中极化域(极化光栅)一定角度,实现了介于共线匹配方式和非共线匹配方式之间的一种半非共线型准相位匹配方式,并以该匹配方式下的各光矢量几何关系得出相位匹配曲线,找到在特定抽运光和信号光波长下能获得宽带增益放大的周期极化长度。并研究其极化倾斜角度与温度特性。模拟计算表明,在合适的角度与温度条件下,该方式可以532 nm抽运光抽运的信号光在800 nm和1064 nm处均获得宽带光参变放大。     

基于MgO:QPLN的多光参量振荡器电场调谐特性理论与实验研究

报道了基于掺氧化镁准周期极化铌酸锂(MgO:QPLN)的多光参量振荡器电场调谐特性理论与实验研究. 通过对电场调谐能力与极化结构参数间关联性的理论分析, 确定了高正负晶畴比MgO:QPLN电场调谐的可行性, 并模拟得到跨周期参量光输出波长与加载电压的关系曲线. 实验中通过对MgO:QPLN有效的电场加载, 实现了3.84 μm波段参量光的电场调谐, 频谱调谐带宽约6 nm, 调谐速率接近1 nm/kV, 进一步结合温度调谐, 实现了参量光宽谱段高精度的连续调谐. 所获得实验结果与理论模拟结果基本符合, 电场调谐在精度控制、快速响应方面相比于传统温度调谐更具技术优势.     

Generation of broadly tunable picosecond mid-infrared laser and sensitive detection of a mid-infrared signal by parametric frequency up-conversion in MgO:LiNbO₃ optical parametric amplifiers

Picosecond optical parametric generation and amplification in the near-infrared region within 1.361-1.656 μm and the mid-infrared region within 2.976-4.875 μm is constructed on the basis of bulk MgO:LiNbO 3 crystals pumped at 1.064 μm.The maximum pulse energy reaches 1.3 mJ at 1.464 μm and 0.47 mJ at 3.894 μm,corresponding to a pumpto-idler photon conversion efficiency of 25%.By seeding the hard-to-measure mid-infrared radiation as the idler in the optical parametric amplification and measuring the amplified and frequency up-converted signal in the near-infrared or even visible region,one can measure very week mid-infrared radiation with ordinary detectors,which are insensitive to mid-infrared radiation,with a very high gain.A maximum gain factor of about 7 × 10 7 is achieved at the mid-infrared wavelength of 3.374 μm and the corresponding energy detection limit is as low as about 390 aJ per pulse.     

Design considerations for a compact grism stretcher for non-collinear optical parametric chirped-pulse amplification

The dispersion management of a non-collinear optical parametric chirped-pulse amplifier is presented. A stretcher based on a combination of a grating and a prism pair (grism) is given and analyzed in detail. This combination can provide up to 300 nm acceptance bandwidth and is suitable for parametric amplification of few-cycle pulses. The amplified pulses can be compressed by the dispersion of optical glasses such as SF57 and the residual high-order dispersion may be compensated by adaptive optical filters and chirped mirrors.     

Wavelength-swept optical parametric oscillator for broadband mid-infrared spectroscopy

In this work we describe a wavelength-swept continuous-wave optical parametric oscillator (OPO) for the rapid acquisition of mid-infrared spectra spanning over hundreds of wavenumbers. Rapid tuning of a ytterbium-doped fibre pump laser resulted in the OPO idler tuning over 900 cm^?1 in 3.36 ms at a resolution of 4.5 cm^?1, within a total accessible range of 2.67 to 4.34 μm (2304–3752 cm^?1). Predictable tuning characteristics allowed simple online calibration of recorded spectra for absolute mid-infrared frequency. The system thus offers a viable approach to broadband spectral acquisition in applications requiring high-radiance illumination.