Stimulated Raman Scattering in a Weakly Polar Ⅲ-Ⅴ Semiconductor： Effect of dc Magnetic Field and Free Carrier Concentration

Using the hydrodynamic model of semiconductor plasmas, we perform an analytical investigation of stimulated Raman scattering （SITS） of an electromagnetic pump wave in a transversely magnetized weakly polar semicon- ductor arising from electron-density perturbations and molecular vibrations of the medium both produced at the longitudinal optical phonon frequency. Assuming that the origin of SItS lies in the third-order susceptibility of the medium, we investigate the growth rate of Stokes mode. The dependence of stimulated Raman gain on the external dc magnetic field strength and free carrier concentration is reported. The possibility of the occurrence of optical phase conjugation via SItS is also studied. The steady-state Raman gain is found to be greatly enhanced by the presence of the strong external dc magnetic field.     

液芯波导中受激动力学散射与受激拉曼散射的竞争

研究了液芯波导中受激拉曼散射和受激动力学散射的阈值随泵浦激光脉宽的变化，发现受激动力学散射的阈值随泵浦脉冲前沿增长率增大而下降。研究了受激动力学散射和受激拉曼散射的竞争，结果表明受激动力学散射可分解为两种成分，其中与瞬态泵浦功率密度增长率相关的成分在大于阈值的泵浦脉冲前沿处于竞争优势，与瞬态泵浦功率密度相关的成分在高泵浦功率密度处于竞争优势，并讨论了其相应的机制。     

Picosecond stimulated Raman scattering in crystals

The comparative values of the peak and integral cross sections of spontaneous Raman scattering and the optical dephasing time of molecular vibrations were determined for several oxide crystals by spontaneous Raman spectroscopy. The spectral, time, and energy parameters of stimulated Raman scattering (SRS) were measured for ten crystals using picosecond YLF: Nd laser pumping with a radiation wavelength of 1047 nm. An analysis of the experimental dependence of the threshold energy of pumping SRS on the integral and peak cross sections of spontaneous Raman scattering showed that the SRS gain increment explicitly depended on the integral cross section and was independent of the peak cross section of spontaneous Raman scattering as the ratio between the pumping pulse width (11 ps) and the time of optical dephasing of molecular vibrations changed from 0.42 to 9.3. The gain coefficients of steady-state stimulated Raman scattering under threshold stimulated Raman scattering conditions were determined for all the crystals studied on the basis of the measured threshold SRS pumping energies, the duration and width of the spectrum of pulses, the nonlinear interaction length, the intensity of pumping, and the theoretical dependences that relate the steady-state and transient SRS gain increments. The steady-state SRS gain coefficients obtained in this work fitted well a linear dependence on the peak cross sections of spontaneous Raman scattering, which substantiated the correctness of our analysis and measurements.     

Modulational interactions in magnetised piezoelectric semiconductor plasmas

Based on hydrodynamic model of plasmas an analytical investigation of frequency modulational interaction between copropagating high frequency pump and acoustic mode and consequent amplification (steady-state and transient) of the modulated waves is carried out in a magnetised piezoelectric semiconductor medium. The phenomenon of modulational amplification is treated as four wave interaction process involving cubic nonlinearity of the medium. Gain constants, threshold-pump intensities and optimum-pulse duration for the onset of modulational instabilities are estimated. The analysis has been performed in non-dispersive regime of the acoustic mode, which is one of the preconditions for achieving an appreciable initial steady-state growth of the modulated signal wave. It is found that the transient gain constant diminishes very rapidly if one chooses the pump pulse duration beyond the maximum gain point. Moreover, the desired value of the gain can be obtained by adjusting intensity and pulse duration of the pump and doping concentration of the medium concerned. Received 12 August 1999 and Received in final form 17 December 1999     

Transient Raman gain stimulated by a noise pump

We predict a strong transient Raman gain stimulated by a Gaussian noise field in dispersive media. Our theory is based on the method of successive approximations, the first of which is the Markovian approximation. It is shown that the transient behavior will take place near critical pump intensity both for “short” (τ_p > T₂) and “ultrashort” (τ_p < T₂) laser pulses (τ_p is the pump pulse duration, T₂ is the relaxation time of optical phonons). Solutions for average intensities of the Stokes wave and optical phonons are obtained for arbitrary form of the given pump pulse. We show that transient Raman gain allows to form a very steep leading edge of the Stokes pulse.The steady-state increments of the second approximation describe the effects of a strong noise field. We show that after the intensity of the pump has exceeded a value beyond which the framework of validity of the Markovian approximation does not hold anymore, the steady-state Raman gain is saturated.We give a review of experimental results and make estimations for conditions of observing transient scattering in the field of a noise pump. Methods of obtaining the powerful femtosecond pulses based on stimulated Raman scattering of broad-band excimer lasers and supercontinuum emission are suggested.     

Numerical simulations of pulsed and quasi-cw regimes of synchronously pumped Raman oscillators

Synchronously pumped Raman oscillators allow for an efficient frequency conversion of pump pulses whose power is well below the threshold for extracavity stimulated Raman scattering (SRS). Numerical simulations show that the cavity mismatch of pump laser and Raman oscillator is critical for maximum conversion efficiency and minimum pulse duration for transient and stationary SRS. At a certain mismatch the simulations predict a quasi-cw Raman oscillator output even at moderate cavity quality factors. Optimum operation conditions are discussed for pump pulse trains of finite lengths. The results of the numerical calculations are in qualitative agreement with a simple phenomenological model. PACS 42.55.Ye; 42.65.Dr; 42.55.Lt     

Frequency comb expansion in a monolithic self‐mode‐locked laser concurrent with stimulated Raman scattering

The discovery of a novel phase‐locked frequency comb generated from a monolithic laser with the concurrent processes of self‐mode locking (SML) and stimulated Raman scattering (SRS) is reported. It is experimentally shown that the width of the Raman gain can be exploited to considerably expand the frequency comb of a monolithic SML crystal laser via the SRS process. At a pump power of 6.5 W, an output power of 140 mW in the Stokes wave with a pulse width as narrow as 2.9 ps at a pulse repetition rate of 6.615 GHz is obtained. The present finding not only provides useful insights into the monolithic intracavity SRS process but also paves the way for generating mode‐locked pulses based on monolithic self‐Raman crystals.     

Cascaded compression of the first and second Stokes pulses during forward transient stimulated Raman amplification

The results of numerical modelling of cascaded compression of the first and second Stokes pulses during regenerative regime of the forward transient stimulated Raman amplification are presented for the case when the walk-off length of the first Stokes pulse due to group velocity mismatch is shorter than the length of the nonlinear medium. The influence of the initial amplitudes of the seed first Stokes pulses, its durations and its time delay with respect to the pump pulse, the Kerr nonlinearity of the medium on the conversion efficiency, duration and propagation factor M² of the first and second Stokes pulse are studied. It is demonstrated that for the pump pulse duration of 1 ps the duration of the compressed second Stokes pulses in a KGW crystal near the beam axis may be approximately 14 times shorter than the pump pulse duration. It is shown that the propagation factor of the compressed pulses increases significantly because of complex spatial-temporal dynamics of compression and the influence of Kerr nonlinearity of Raman medium.     

高功率纳秒光脉冲在单模光纤中的受激喇曼散射及抑制研究

利用包含喇曼增益、抽运消耗、自相位调制、交叉相位调制和群速度色散效应的耦合非线性薛定谔方程组,对千瓦级高功率纳秒脉冲在单模光纤中的传输特性进行了模拟计算.分析了输入脉冲和斯托克斯脉冲的演化过程,研究了大模面积光纤对受激喇曼散射的抑制作用.研究结果表明,采用模面积为530 μm~2的光子晶体光纤作为惯性约束聚变脉冲整形系统的传输介质,能有效抑制受激拉曼散射,不但信号衰减较小,而且中心凹陷程度较低.     

Threshold and conversion experiments on seeded stimulated Raman scattering

High energy-conversion efficiencies in Stimulated Raman Scattering (SRS) are demonstrated both in experiments and by simulations for pump powers below SRS threshold. The scattering is induced by a short seed pulse at the Stokes frequency, the pulse width of which is much shorter than the pump pulse width and which is comparable with the medium's dephasing time.     

Coherent control of optical precursors in a warm atomic system with Doppler effects

We theoretically study coherent control of optical precursors via active Raman gain (ARG) in an N-type warm atomic system. When a step pulse passes through an ARG window, main fields are advanced due to fast-light effect and constructively interference with optical precursors, then an enhanced transient pulse appears. As the control field decreases, the interference effect is strengthened, and the transient pulse builds up and becomes narrow. Moreover, its peak intensity is inverse to the system temperature and also determined by the input-pulse form. The scheme may be useful in designing optical devices in optical communication.     

Transient gain in photonic crystals

Using the optical response formula for photonic crystals and the Bloch equations, we analyze coherent emission in arbitrary two-dimensional photonic crystals. The transient emission depends not only on the photon density of the states, but also on the intensity and duration of the pump laser pulses. A transient gain exists if the pump pulse area is a certain value and the transition frequency is tuned to the band edge. The sharp structure of the density of states near the band edge leads to a dramatic enhancement of the transient emission intensity and an abrupt change in the oscillation of the emission field. PACS 42.70.Qs; 32.80.-t; 42.25.Bs     

YbVO4晶体的受激拉曼散射

采用腔外单次通过方式,研究了一种新型晶体YbVO₄的受激拉曼散射.当抽运激光为532 nm皮秒脉冲时获得了3级斯托克斯线(558.47 nm, 587.92 nm, 620.67 nm)和1级反斯托克斯线(507.58 nm),测得YbVO₄晶体1级斯托克斯受激拉曼散射的稳态增益系数为17.8±0.2 cm/GW,受激拉曼散射的整体转换效率达到37%.实现了YbVO₄晶体对355 nm皮秒激光的受激拉曼散射,观察到1级斯托克斯线(366.1 关键词： 受激拉曼散射 稳态增益系数 转换效率 4晶体')" href="#">YbVO₄晶体     

三倍频Nd∶YAG激光抽运氧气中的受激拉曼和布里渊散射

报道了三倍频脉冲Nd∶YAG激光(355 nm)在两种不同带宽模式下抽运氧气中受激拉曼散射(SRS)和受激布里渊散射(SBS)的实验研究。在宽带(约1 cm-1)抽运模式下,只测到了前向受激拉曼散射,而没有观察到后向散射,其一级和二级斯托克斯最大能量转换效率可达22%和8%。在窄带(约0.003 cm-1)模式下,前向、后向受激拉曼散射和受激布里渊散射都测量到了,但大部分抽运能量都转换到受激布里渊散射,其转换效率可达67%。测量了两种带宽模式下各散射组分在它们最佳转换时的波形;窄带情况下后向受激拉曼散射和受激布里渊散射的脉宽分别可压窄至1.5 ns和2.3 ns,不到抽运脉宽的三分之一,使得受激布里渊散射峰值功率可大大高于抽运功率。对氧气中前向、后向受激拉曼散射和受激布里渊散射之间的竞争进行了讨论。     

三倍频Nd:YAG激光抽运氧气中的受激拉曼和布里渊散射

报道了三倍频脉冲Nd：YAG激光（355nm）在两种不同带宽模式下抽运氧气中受激拉曼散射（SRS）和受激布里渊散射（SBS）的实验研究。在宽带（约1cm^-1）抽运模式下,只测到了前向受激拉曼散射,而没有观察到后向散射,其一级和二级斯托克斯最大能量转换效率可达22％和8％。在窄带（约0．003cm^-1）模式下,前向、后向受激拉曼散射和受激布里渊散射都测量到了,但大部分抽运能量都转换到受激布里渊散射,其转换效率可达67％。测量了两种带宽模式下各散射组分在它们最佳转换时的波形;窄带情况下后向受激拉曼散射和受激布里渊散射的脉宽分别可压窄至1．5ns和2．3ns,不到抽运脉宽的三分之一,使得受激布里渊散射峰值功率可大大高于抽运功率。对氧气中前向、后向受激拉曼散射和受激布里渊散射之间的竞争进行了讨论。     

水中受激拉曼散射的能量增强及受激布里渊散射的光学抑制

为提高液体介质中受激拉曼散射的输出能量,提出了通过温度调控来抑制受激布里渊散射的方法,设计了532 nm多纵模宽带脉冲激光泵浦的受激拉曼散射发生系统,测量了不同温度下水中前向受激拉曼散射及后向受激布里渊散射的输出能量,分析了水温、泵浦激光线宽及热散焦效应对受激拉曼散射输出能量影响的物理机制.实验结果表明:通过降低水温可实现对受激布里渊散射过程的有效抑制,同时减小热散焦效应带来的光束畸变,从而有效提高受激拉曼散射的输出能量.研究结果对液体介质中的受激拉曼散射多波长转换具有重要意义.     

窄线宽纳秒脉冲光纤拉曼放大器的理论模型和数值分析

窄线宽纳秒脉冲光纤拉曼放大器在非线性频率变换、遥感探测和量子信息等领域有广泛的应用前景.综合考虑受激拉曼散射(stimulated Raman scattering,SRS)、受激布里渊散射(stimulated Brillouin scattering,SBS)、自相位调制(self-phase modulation)和交叉相位调制(cross-phase modulation)等非线性效应,建立了窄线宽纳秒脉冲光纤拉曼放大器的非线性动力学模型.仿真分析了放大器中脉冲激光的时频演化特性,对比研究了抽运脉冲宽度、光纤长度和信号光功率等因素对放大器性能的影响.研究发现,上述因素会影响放大器的SRS阈值、SBS阈值、输出激光线宽、激光转换效率等.例如,当脉冲宽度为800 ns时,SBS随着抽运功率的增加而发生,限制了激光功率的提升;减短抽运脉宽可以抑制SBS,但是输出激光的线宽易于展宽到数百MHz以上;增加光纤长度可以获得更低的SRS阈值和更高的转换效率,但是SBS效应和光谱展宽程度也随之增强.系统搭建中需要平衡各非线性效应,选择合适的系统参数.研究内容可以为窄线宽纳秒脉冲光纤拉曼放大器的设计搭建提供参考.     

Observation of Raman conversion for 70-fs pulses in KGd(WO4)2 crystal in the regime of impulsive stimulated Raman scattering

Raman conversion of femtosecond pulses in a solid-state medium is reported. Stimulated Raman scattering (SRS) was observed in an impulsive SRS regime when the pump pulse's duration was comparable with the period of Raman-active vibration. The generation of super broadband radiation, which is a distinguishing feature of impulsive SRS, is shown.     

斯托克斯束的时空分布

基于在自由空间光束的分丰是已知的条件下，推导出适用于任意束分布的广义化的耦合波方程并得到一种计算受激拉曼散射过程中泵浦束与斯托克斯束的时、空分布的简单方法。所得结果清楚地示明受激拉曼散射过程既能使斯托克斯信号得到放大，又能使脉宽受到压缩。