超强频率梳激光场驱动下多光子共振谐波辐射的相位突变研究

本文从理论上研究了在双色频率梳激光场驱动下多光子谐波辐射光谱中的相位突变现象。我们利用Floquet理论非微扰地模拟了频率梳激光场与原子分子等量子系统的相互作用过程。谐波辐射信号是多光子偶极跃迁相干叠加的结果,通过调节频率梳激光场间的相对相位,可以相干地控制谐波辐射信号的强度。通过对谐波信号进行傅里叶变换,可以提取不同跃迁路径的相对相位信息。我们通过改变频率梳组激光场的强度和频率组分实现多光子跃迁频率,让其跨越共振跃迁频率时,谐波相位会发生突变。从而可以观测超强激光场驱动下量子系统共振跃迁频率的斯塔克能移。     

Study into mechanisms of the enhancement of multibubble sonoluminescence emission in interacting fields of different frequencies

The main factor of the enhancement of sonoluminescence (SL) emission by the interaction of two fields of highly different frequencies is the generation of new cavitation nuclei upon collapse of bubbles driven by the low-frequency (LF) field. The factors connected with the direct interaction of the two fields play a significant role in the enhancement of SL emission only in the case when intensities of the fields are less or not much higher than the corresponding thresholds of SL emission. The phenomena of afteraction of the LF field on cavitation generated by the high-frequency field is explained also by the generation of new nuclei upon collapse of bubbles driven by the LF fields.     

Intraband dynamics and terahertz emission in biased semiconductor superlattices coupled to double far-infrared pulses

This paper studies both the intraband polarization and terahertz emission of a semiconductor superlattice in combined dc and ac electric fields by using the superposition of two identical time delayed and phase shifted optical pulses. By adjusting the delay between these two optical pulses, our results show that the intraband polarization is sensitive to the time delay. The peak values appear again for the terahertz emission intensity due to the superposition of two optical pulses. The emission lines of terahertz blueshift and redshift in different ac electric fields and dynamic localization appears. The emission lines of THz only appear to blueshift when the biased superlattice is driven by a single optical pulse. Due to excitonic dynamic localization, the terahertz emission intensity decays with time in different dc and ac electric fields. These are features of this superlattice which distinguish it from a superlattice generated by a single optical pulse to drive it.     

Partial ordered homogeneous magnetic moments in the Hubbard-model

In this contribution, we study the behaviour of magnetically disordered electron systems. In a model with localized magnetic fields at the atomic sites, a CPA-like method, which has regard for the vector character of the fields, is used to examine the case where the localized fields, which correspond to atomic magnetic moments, are distributed statistically. In an example for a non-isotropic distribution of the fields, we construct a system state with partial homogeneous order of the localized fields (or moments). The ordering behaviour of the system and the comparison of the new magnetic state with pure magnetic and non-magnetic band states and with the non-magnetic state of (isotropic) stochastic distribution of the localized fields is discussed. With this paper we are able to introduce typical properties of localized models into a band model.Work supported in part by the Deutsche Forschungsgemeinschaft     

Luminescence from hot electrons relaxing by LO phonon emission in p-GaAs and GaAs doping superlattices

Laser excited hot electrons in GaAs relax by LO phonon emission within a few hundred femtoseconds, leading to a series of peaks in the distribution of hot electrons in the conduction band, which we observe in luminescence. We find that the luminescence peaks shift according to the acceptor binding energy for C?, Ge?, Zn?, and Be-p-doped GaAs layers grown by MBE and LPE. Thus we prove that recombination is between hot electrons and neutral acceptors. The series of peaks due to electrons from the heavy hole band agree well with $\text{k}\text{.}\text{p}$ band structure, while peaks due to those from light holes are about 15 meV lower than expected from the band structure. We show that the discrepancy is not due to heating or surface fields. The peak separation in the luminescence ladder is about 6% larger than the LO energy suggesting emission of renormalised LO phonons. We find thermalisation by LO emission also in GaAs nipi doping superlattices. In nipi crystals the emission is shifted to higher energies (by 12 meV for light and by 6 meV for heavy holes) due to a change in band structure caused by the space charge fields.     

Spontaneous emission spectra of a four-level atom in photonic crystals driven by two coherent fields

We investigate the spontaneous emission spectra of a four-level tripod-type atom embedded in a photonic crystal and driven by two coherent fields. It is found that due to the quantum interference caused by two driving fields, the spontaneous emission spectra have different features from the case of only one driving field. The spectra are sensitively dependent on the detuning of the driving fields. A dark line occurs for some particular initial states. By appropriately adjusting the external driving fields, the spectral-line can be narrowed, enhanced or suppressed.     

多目标优化发射层析算法在等离子体场光谱诊断中的应用

提出一种基于多目标优化原理的发射光谱层析(EST)图像重建新算法MCIRT.通过计算机数值 模拟，考察了该算法对非对称发射系数场分布的重建效果.结果表明，与传统层析算法相比 ，MCIRT算法具有收敛快，重建精度高的优势，适合于非完全数据情况下的等离子体发射系 数场重建，并且实时性更好.作为一个应用实例, 运用谱线相对强度法重建了自由电弧等离 子体的三维温度及粒子数密度分布. 关键词： 等离子体诊断 图像重建     

Self-consistent density functional calculation of field emission currents from metals

We have developed a fully self-consistent method which is suitable to examine field emission currents, on the basis of the density functional theory. In our method, the nearby counterelectrode is not necessary. By using this method, we have investigated field emission currents from a biased metallic surface represented by the jellium model. We have found that the energy barrier between the jellium and vacuum becomes lower than the Fermi energy under strong electric fields (e.g., 10 V/nm for r(s) = 4 bohr). In this situation, the slope of the Fowler-Nordheim plot becomes flatter than that under a weaker field.     

两个双能级原子与双模腔场的拉曼相互作用

研究了两个双能级原子与双模辐射腔场的拉曼相互作用，计算了两个原子与腔场具有相同耦合常数但同时考虑原子间偶极一偶极相互作用情形下的辐射谱．讨论了双模腔场处于不同数态时辐射谱的新特点．     

Controlling spontaneous emission in a driven M-type atom by low-frequency coherence

We have studied the spontaneous emission behaviour in a five-level M-type atom driven by two optical fields of high frequencies and a microwave field of low-frequency. In absence of non-orthogonal decaying pathways, due to microwave field induced low-frequency coherence, the present model produces the emission spectrum resembling that of a three-level system controlled by the effect of vacuum induced decay-interference. For particular sets of values of the Rabi frequencies of the resonant coherent fields, the system exhibits quantum interference induced switching effect. By using this model, we have shown that the phenomenon of narrowing can be induced in the emission peaks without any detuning and phase control of the coherent fields. With the increase in the value of the Rabi frequency of the microwave field, this feature will be accompanied by the peak-compression and -repulsion effect. When the coherent fields are far from resonance, the appearance of the single-photon and the two-photon peaks in the emission spectrum can be easily controlled by changing the value of the Rabi frequency of the microwave field. We have shown the appearance of multiple dark regions in the emission line shape for equal as well as unequal decay rates of two emission pathways. Other interesting phenomena like elimination, enhancement and suppression of spectral line are also explored in various resonant and non-resonant cases.     

Anomalous enhancement of negative sputtered ion emission by oxygen

Enhancement of negative sputtered ion yields by oxygen (either O⁺₂ bombardment or O₂ gas with Ar⁺ bombardment) is demonstrated for Si^?, As^?, P^?, Ga^?, Cu^? and Au^?, sputtered from a variety of matrices. Because oxygen also enhances positive ion yields of the same species, this effect cannot be simply explained on the basis of existing sputtered ion emission models. To rationalize these phenomena, a surface polarization model is developed which invokes localized electron emissive or electron retentive sites associated with differently oriented surface dipoles in the oxygenated surface. Such sites are considered to dominate the emission of negative and positive ions respectively. The model is shown to correctly predict that Au⁺ and Au^? ion yields are much more strongly enhanced by oxygen in dilute Au-Al alloys than in pure gold.     

Electron field emission from boron doped microcrystalline diamond

Field emission properties of hot filament chemical vapor deposited boron doped polycrystalline diamond have been studied. Doping level (N_B) of different samples has been varied by the B/C concentration in the gas feed during the growth process and doping saturation has been observed for high B/C ratios. Threshold field (E_th) for electron emission as function of B/C concentration has been measured, and the influences of grain boundaries, doping level and surface morphology on field emission properties have been investigated. Carrier transport through conductive grains and local emission properties of surface sites have been figured out to be two independent limiting effects in respect of field emission. Emitter current densities of 500 nA cm⁻² were obtained using electric fields less than 8 V/μm.     

Non-classical correlation of the two emission fields by a four-level atomic ensemble

The normalized second-order correlation of the emission fields from a driven four-level atomic ensemble is investigated theoretically by using the state vector method. The violation of Cauchy-Schwarz inequality, which indicates the establishment of non-classical correlation between two emission fields, has been found. The effects of various decays and time delay on the correlation are discussed in detail, which are helpful in finding the ways to obtain high non-classical correlation. This technique for the generation of non-classical light is operable based on the current experimental technology and will lead to some potential applications in quantum information science.     

A stochastic theory for clustering of quenched-in vacancies-V. Temperature dependence of cluster density

It is known that the density of vacancy loops in quenched aluminium and stacking fault tetrahedra in quenched gold show a saturation for low ageing temperatures. The physical mechanism leading to this effect is not well understood. In this paper we consider a simple model which allows us to obtain the temperature dependence of total density. The analysis shows that the plateau region arises due to the fact that the number of absorption sites of a cluster is larger than the number of emission sites. The temperature dependence of the average number of vacancies in a cluster and the single vacancy concentration in equilibrium with the clusters are discussed.     

Hyperfine interactions of111Cd in ion-implanted face centered cubic cobalt

The magnetic-dipole and electric-quadrupole hyperfine interactions of¹¹¹Cd probes in fcc cobalt after implantation of radioactive¹¹¹In⁺ ions have been investigated by PAC measurements with fast BaF₂ detectors. Six different sites of the probe atoms could be distinguished and characterized by their hyperfine parameters and annealing behaviour. Besides the substitutional site, three sites are assigned to In-vacancy complexes which are formed athermally in the implantation process or by thermally-activated trapping of lattice defects in annealing stage III. The remaining two sites are attributed to In located in stacking faults or hcp regions of the host. Systematic trends of impurity hyperfine fields in defect sites become evident from a comparison with other impurity-host combinations. The temperature dependence of the magnetic hyperfine fields has been measured between 20 K and 390 K. Large differences found for the various sites are discussed.     

Spontaneous emission from a microwave-driven four-level atom in an anisotropic photonic crystal

The spontaneous emission from a microwave-driven four-level atom embedded in an anisotropic photonic crystal is studied. Due to the modified density of state(DOS) in the anisotropic photonic band gap(PBG) and the coherent control induced by the coupling fields, spontaneous emission can be significantly enhanced when the position of the spontaneous emission peak gets close to the band gap edge. As a result of the closed-loop interaction between the fields and the atom,the spontaneous emission depends on the dynamically induced Autler–Townes splitting and its position relative to the PBG.Interesting phenomena, such as spectral-line suppression, enhancement and narrowing, and fluorescence quenching, appear in the spontaneous emission spectra, which are modulated by amplitudes and phases of the coherently driven fields and the effect of PBG. This theoretical study can provide us with more efficient methods to manipulate the atomic spontaneous emission.     

Local structure and triplet energy migration in p-dichlorobenzene-p-dibromobenzene solid solutions

Studies of the first triplet absorption and emission spectra of p-dichlorobenzene-p-dibromobenzene (DCB-DBB) mixed crystals agree generally with the data, indicating that this system forms solid solutions. However, the spectral properties are found to be very different from that of isotopically mixed crystals of comparable concentrations. The singlet-triplet absorption spectra of the DCB-DBB mixtures are generally broad and not amenable to detailed analysis indicating significant site dependent perturbations of the DCB and DBB triplet energies. Energy migration enhances emission from the lower energy sites and in consequence a red shift in the position of the emission (0,0) is observed, which is a maximum at equimolar concentrations. The emission bands are generally much broader than found for isotopically mixed crystals, indicating that the many types of sites in the DCB-DBB system remained uncoupled. This is a direct consequence of exciton trapping by inhomogeneous energy broadening caused by the site energy disorder being greater than the triplet exciton band width. Long-range triplet energy migration is not observed at DCB concentrations less than 99 per cent. This high limit is only expected for near one-dimension energy migration topologies. New structure observed at low DCB concentrations is tentatively interpreted as being due to the formation of DCB n-mers. The observed splittings indicate that the gas-to-crystal shift of the DCB T ₁ state increases (becomes more negative) by 11 cm^-1 when a neighbouring DBB molecule is replaced by DCB.     

Polarization fields in the positronium atom undergoing emission or absorption of optical photons

This paper solves the problem of the interaction of an electron and positron via the field of soft and hard photons with emission or absorption of a real photon. The interaction is interpreted as a third-order QED effect in the coordinate representation. The role of intermediate states with positive and negative frequencies is studied. A general expression is derived for the matrix elements of the operator of the effective electron-positron interaction energy for different types of quantum transitions. The expression makes it possible to calculate the probabilities of the corresponding transitions in the nonrelativistic approximation. Electric dipole transitions in the positronium atom accompanied by emission (absorption) of an optical photon are investigated. Two-particle wave functions of the positronium atom are used to introduce the concept of polarization fields inside the positronium atom. It is found that the polarization fields depend on the coordinates and time and on the choice of the pair of states between which a quantum transition with emission or absorption of a photon takes place. Zh. éksp. Teor. Fiz. 113, 471–488 (February 1998)     

Modification of the tungsten carbide field emitter surface to localize the electron and ion emission

Using field emission microscopy, the shape modification of the tungsten carbide emitter simultaneously exposed to high electric fields and high temperatures is studied. It is shown that in this case the emitter shape changes observed on the emitter surface are the same as those observed in the pure metal emitters. The possibility to grow a single nanoprotrusion on the emitter surface which can emit charged particles with stability similar to that for the carbon material emitters is demonstrated. The values of the emission current, current density, emission angle, and reduced brightness are comparable to those for the carbon nanotube emitters, and the advantage of this single nanoprotrusion is its complete reproducibility and capability to emit not only electrons but also ions.     

Coupled field induced conversion between destructive and constructive quantum interference

We study the control of quantum interference in a four-level atom driven by three coherent fields forming a closed loop. The spontaneous emission spectrum shows two sets of peaks which are dramatically influenced by the fields. Due to destructive quantum interference, a dark line can be observed in the emission spectrum, and the condition of the dark line is given. We found that the conversion between destructive and constructive quantum interference can be achieved through controlling the Rabi frequency of the external fields.