Gamma-ray competition with neutron emission in the decay of 137I

Gamma-rays with energies above the neutron binding energy in ¹³⁷Xe have been observed at 3907 and 3994 keV in the decay of ¹³⁷I. Their combined intensity amounts to about 25% of the delayed neutron intensity and demonstrates that γ-ray widths are an important factor in defining the magnitude and energy distribution of the delayed neutron spectrum.     

Thermal neutron captureγ-ray spectroscopy of59Ni and61Ni

Theγ-radiation emitted after thermal neutron capture in isotopically enriched⁵⁸Ni and⁶⁰Ni was measured at the ILL high flux reactor by means of Ge/NaI detectors operated in Compton suppression and pair spectrometer mode. The neutron binding energies were determined asB _n (⁵⁹Ni)=8999.15(23) keV and B_n(⁶¹Ni)=7820.07(20) keV; some 95% of the totalγ-ray fluxes through^59,61Ni were assigned. Theγ-ray strength functions of the primary transitions and the level densities are discussed.     

Angular distributions of elastic and quasi elastic heavy-ion collisions. pattern analysis

From classical in-beam spectroscopy on the¹⁰⁶Cd+¹²C reaction, unambiguousγ-ray assignments have been done for¹¹⁶Xe,¹¹⁶I and¹¹⁶Te nuclei. The ground band levels observed in¹¹⁶Xe have been compared to those of heavier even-even xenon isotopes and to the IBA theoretical predictions. In addition, using the newγ-ray assignments, evaporation cross-sections of the¹¹⁸Xe compound nucleus have been estimated and compared to the evaporation model calculations.     

Levels in182W populated in the decay of182Ta

Theγ-rays emitted in theβ-decay of¹⁸²Ta have been reinvestigated with improved statistics in attempting to clarify the reported new levels at 1460.41, 1592.98, 1620.36, 1712.29 and 1762.91 keV in¹⁸²W observed in theβ-decay of¹⁸²Ta. The present study demonstrated that the fifteen newγ-rays, which were used to support the existence of the five new levels, are not relevant to theγ-decay of¹⁸²Ta. Therefore the five new levels are not populated in this decay. Additionally, theγ-ray with an energy of 1035.6 keV (0 ₂ ⁺ →2 ₁ ⁺ ) deexciting theβ-band head in¹⁸²W is observed for the first time in the present decay study and the previous tentative placement of the 351.0 keVγ-ray in the level scheme is confirmed by the present coincidence measurements.     

Decay of the134Cs isomers and the levels of134Xe,134Cs,and134Ba

A precision study of the decay of¹³⁴Cs ^g and¹³⁴Cs ^m has been made, using ordinary Ge(Li) spectrometers and ā Compton-suppression spectrometer. The logft value of the second forbidden nonuniqueβ-decay to¹³⁴Xe has been measured to be 13.0±0.2. TheM4γ-ray transition in¹³⁴Cs^m(8^?) decay has been measured to haveα _K= 73±7 and a hindrance of 7.0 over the Moskowski estimate. This is discussed in terms of the level configurations and the analogous transition in¹³³Xe. A new intensity limit of 2×10^?6 has been set for the zero-phonon transition between the 4⁺ and 2⁺ members of the two-phonon triplet. This leads to an upper limit forB(E2)_4→2′, greater than 905. This and the more preciseγ-ray intensity values are discussed in relation to presently available nuclear models.     

Determination of the neutron binding energy of the delayed neutron emitter137Xe

The neutron binding energy of¹³⁷Xe has been deduced to be 4025.2±0.6 keV from a study of the¹³⁶Xe(n, γ)¹³⁷Xe reaction. The importance of a precise value for this quantity is due to the fact that an accurate determination of binding energies of delayed neutron emitters is possible only for⁸⁷Kr and¹³⁷Xe, neighbouring stable isotopes. Nuclear reaction.¹³⁶Xe(n,γ), enriched target; measurede89-01, deduced neutron binding energy, Ge(Li) detector.     

Theβ-decays of99Y and99Zr and the level schemes of99Zr and99Nb

Theβ-decays of⁹⁹Y and⁹⁹Zr have been investigated with the two recoil fission product separators JOSEF and LOHENGRIN. Half-lives of 1.51±0.08s and 2.1±0.1s respectively, have been determined. Aβ-decaying isomeric state has been observed in⁹⁹Y. The level schemes of ₄₀ ⁹⁹ Zr₅₉ and ₄₁ ⁹⁹ Nb₅₈ have been established fromγ-ray spectroscopy. Absoluteγ-intensities have been obtained by means of two independent techniques. Halflives of 293±10 ns for the 251.9 keV state and 10.2±1.5 ns for the 614.0 or 667.2 keV level in⁹⁹Zr have been measured through delayedβ,γ- andγ,γ-coincidence experiments. Values for the spins and parities of the low lying levels in⁹⁹Zr are proposed in accordance with the systematics of lighter odd Zr isotopes. Spins and partities are assigned to some levels in⁹⁹Nb fromγ,γ-angular correlation measurements. In this nucleus there is evidence for three-particle configurations of some excited states, where the odd proton is coupled to two neutrons which are in different orbits.     

Half-lives of levels in99Nb and99Mo

The half-lives of the 469-keV level in⁹⁹Nb and the 236-keV state in⁹⁹Mo have been determined to (0.21±0.06) ns and (0.87±0.15) ns, respectively, fromβ,γ-delayed coincidences. Values ofB(E2)=(89±28)e ² fm⁴ andB(M1)=(0.017±0.003) μ _n ² are deduced for the 469-keV transition in⁹⁹Nb and the 138-keV transition in99Mo. The result for theE2-transition probability seems to be in accordance with the particle-core coupling interpretation of the low-lying levels in⁹⁸Nb if⁹⁸Zr is used as the core. TheM1 probability for⁹⁹Mo agrees with the systematics for “l-forbidden” 1g_7/2→2d _5/2 neutron transitions.     

Search for an isomer in94Rb

Measurements of theβ-ray half-life,γ-ray and X-ray spectra andγ-ray half-lives have been done with a plastic scintillation detector, a high resolution Ge(HP) detector and a 142 cm³ Ge(Li) detector to search for an isomeric state in⁹⁴Rb. Mass-separated activities of⁹⁴Rb were obtained from the He-jet type on-line mass-separator at the Kyoto University reactor. No isomeric transition was found in theγ-ray and X-ray measurements with the upper limits of 3×10^?4 and 8×10^?5, respectively, as compared with the 836.9 keV transition. Half-lives obtained from theγ-ray decay measurements are discussed in the light of classification given byQ _β -value measurements.     

The decay of115 mIn

The decay of^115m In has been investigated using accurate counting methods. The emission rate of conversion electrons plusβ ^?-particles was determined with a 4π proportional flow counter. The total andK-shell internal conversion coefficients of the 336 keVγ-ray in¹¹⁵In were measured by the electron X-ray coincidence method using combinations of a Si surface barrier with a NaI(Tl) detector and of a magneticβ-spectrometer with a high energy resolution Si(Li) detector, respectively. The conversion ratioR=K/(L+M+...) was deduced from electron spectra recorded with the magneticβ-spectrometer. The 336 keVγ-ray emission rate of all used sources was determined with a calibrated NaI(Tl)γ-ray spectrometer. A Ge(Li) detector has been used to determine the relative intensity of the 497 keVγ-ray in¹¹⁵Sn. As results have been deduced the 336 keVγ-ray emission per decay (N _γ1/N ₀=(45.9 ± 0.1)%), the total internal conversion coefficient (α=1.073 ± 0.014), theK-shell internal conversion coefficient (α _K=0.843±0.012), the conversion ratioR=3.63±0.07, theβ ^?-transition per decay going to the ground state (N _β1/N ₀=(5.0 ± 0.7)%) and to the first excited level in¹¹⁵Sn¹¹⁵Sn(N _β2/N ₀=(0.047 ± 0.002)%), and the 497 keVγ-ray emission (N _γ2/N _γ1=(0.103 ± 0.004)%). From the obtained internal conversion data it follows that the 336 keVγ-ray transition is ofM4 character with anE5 admixture of less than (3.5±1.5)%. The half-life of the isomeric state¹¹⁵ mIn has been determined with four different methods. The result isT _1/2=(4.486±0.004) h.     

Beta-delayed neutron emission from93–100Rb to excited states in the residual Sr isotopes

Beta-delayed neutron emission from the precursors^93–100Rb to excited states in the residual nuclei^92–99Sr has been measured by means ofγ-ray and neutron spectroscopy. In general, considerable neutron feeding of excited final states is observed. The experimental branching ratios (P _n ⁱ ) are compared to predictions from statistical model calculations. It is demonstrated that the main parameter affecting theP _n ⁱ -values is the shape of theβ-strength function (S _β). For several Rb isotopes hindrance, respectively enhancement of neutron branches to specific final states is observed giving evidence for the persistence of intermediate structure of the neutron-emitting states. By the example of⁹⁸Rb it is shown that a few integralβ-delayed neutron properties may be sufficient to derive first estimates on the real shape ofS _β above the neutron binding energy. This result is of importance for exotic nuclei where detailed spectroscopic investigations are precluded.     

High spin level structure in127Ba produced by the118Sn(12C, 3n) reaction

High-spin states in¹²⁷Ba have been produced by the reaction¹²⁸Sn(¹²C,3n)¹²⁷Ba and studied by in-beamγ-ray spectroscopic techniques. The odd-parity states form a level system based upon a 9/2^? state and generated by an odd neutron in theh _11/2 shell coupled to a triaxial core. Theg _7/2 shell is responsible for theΔ I=1, even-parity band.     

Levels in154Eu populated by thermal neutron capture

The level scheme of¹⁵⁴Eu has been investigated by means of thermal neutron captureγ-rays and conversion electrons. The high energyγ-ray spectrum from thermal neutron capture in enriched¹⁵³Eu has been studied in the energy range of 5700 to 6500 keV. Low energyγ radiation has been observed with Ge(Li) and Si(Li) detectors from 5 to 300 keV and conversion electrons have been measured from 15 to 300 keV. Low energy (n, γγ) coincidences and half lives of transitions have been measured. The data, combined with three very recent studies of the 8^? isomer decay in¹⁵⁴Eu has led to the construction of a level scheme with 12 excited levels. Nuclear Reaction¹⁵³Eu(n, γ),E _n =thermal, measuredE _γ ,I _γ ,E _ce ,I _ce ,γγ-coincidence, halflives,¹⁵⁴Eu deduced levels.     

Evidence for neutron capture through doorway states in29Si

Theγ-ray spectra following neutron capture in silicon have teen recorded in the neutron energy range 2.7–6.2 MeV and partial cross sections forγ-rays to the 2s_1/2 ground state and 1d_3/2 first excited states in²⁹Si determined. The results indicate considerable fluctuations with neutron energy with a prominent resonance peak at 4.6 MeV in the (n,γ _o) cross section. The existence of fluctuations is predicted in a recent theoretical calculation based on a model designed to include single-particle resonances in nuclear reaction processes.     

Level structure of 68 149 Er81 and high-spin isomerism in proton-richN=81, 82, 83 nuclei

The level structure of theN=81 nucleus¹⁴⁹Er has been studied by γ-ray spectroscopy following the reaction⁹²Mo+255 MeV⁶⁰Ni. Yrast levels in¹⁴⁹Er are established up to ~3.3 MeV, including 0.61 and 4.8 μs isomeric states. Most of the observed levels are interpreted as seniority-three states arising from the coupling of s_1/2, d_3/2 and h_11/2 neutron holes with πh ₁₁ ^2/n . Isomers identified in the reaction⁹⁶Ru+255 MeV⁵⁸Ni are tentatively assigned to¹⁵¹Yb. TheB (E2) values of high-spin isomers inZ=66?70,N=81?83 nuclei are surveyed.     

Low-lying states and degree of chaoticity of40K in IBFFM

The results of aγ-γ angular correlation and a low energyγ-ray singles measurement using thermal neutron capture in³⁹K are presented. The properties of low-lying levels of⁴⁰K are interpreted in a comparison of the experimental data with the Interacting-Boson-Fermion-Fermion Model (IBFFM). The level fluctuation properties of the IBFFM spectrum are analysed and a sizeable deviation from chaoticity is found.     

The decay of105Tc to levels in105Ru

Theβ ^?-decay of 7.6-min¹⁰⁵Tc has been investigated byβ- andγ-ray singles and coincidence measurements. The activities have been produced by thermal-neutron-induced fission of²³⁵U or²³⁹Pu and subsequent chemical separation of the technetium fraction from the fission product mixture. AQ _β-value of 3.2±0.2 MeV has been determined. In a delayed coincidence experiment the lifetime of the first excited state in¹⁰⁵Ru at 20.55 keV has been measured to be 340±15 nsec. A level scheme of¹⁰⁵Ru is proposed and compared with the results of recent nuclear reaction studies like¹⁰⁴Ru(d, p) and¹⁰⁴Ru(n, γ). From beta branching ratios to levels in¹⁰⁵Ru, ground state spin and parity of 5/2⁺ can be suggested for¹⁰⁵Tc in accordance with the trend observed in neutron rich technetium isotopes.     

Collective and two-particle excitations in78Se

Excited states in⁷⁸Se have been studied up to spin (12)? at about 5.8 MeV in the⁷⁶Ge(α, 2n) reaction using in-beamγ-ray spectroscopy. Mean lifetimes could be determined for 27 of the 33 levels observed by applying Doppler shift and pulsed-beam timing methods. According to theB(E2) values most of the levels have been grouped into collective bands. Irregularities in the level spacings of the yrast band above spin 6? are interpreted to be due to the interaction of the ground state band withg _9/2 two-proton and two-neutron excitations. The mutual mixing of these configurations is reflected by strongM 1 transitions between the mixed states. The interaction strengths between the configurations involved have been estimated from three-band mixing calculations.     

Reliability of the data on the cross sections of the partial photoneutron reaction for <Superscript>63,65</Superscript>Cu and <Superscript>80</Superscript>Se nuclei

The cross sections of partial photoneutron reactions are evaluated for the ^63,65Cu and ⁸⁰Se isotopes. The cross sections are free of systematic uncertainties from shortcomings of the experimental methods for neutron multiplicity sorting based on measurements of neutron energy used in experiments with quasimonoenergetic annihilation photon beams. An experimental-theoretical method is used to evaluate cross sections σ^eval(γ, in)= F_i^theor σ^exp(γ, xn), where ratios F_i^theor = σ^theor(γ, in)/σ^theor(γ, xn) = σ^theor(γ, in)/σ^theor[(γ, 1n) + 2(γ, 2n) + …] are calculated using a combined model of photonuclear reactions, and σ^exp(γ, xn) is the experimental cross section of the neutron yield reaction free from neutron multiplicity sorting problems. The cross sections are evaluated for reactions (γ, 1n) and (γ, 2n) for the ^63,65Cu and ⁸⁰Se isotopes, and for the total photoneutron reaction σ(γ, Sn) = σ[(γ, 1n) + (γ, 2n) + …]. It is shown that noticeable deviations of the experimental cross sections from the evaluated values result from the unreliable sorting of neutrons between the channels with multiplicities 1 and 2.     

Band structure on the low-j orbitals in the nucleus125Xe

In¹²⁵Xe eight lowlying band structures of positive parity were established via the¹²²Te(α, n) reaction by means of in-beamγ-ray spectroscopy using a setup of 6 compton suppressed germanium detectors. The systematics of the related quasi- ′s′_1/2, ′d′_3/2, and ′g′_7/2 bands with the variation of the fermi level in the triaxially deformed region from¹²⁵Xe to¹²⁹Xe is discussed.