基于氧化镁晶体中级联四波混频过程的紫外飞秒光脉冲产生

紫外波段飞秒激光脉冲是研究超快化学和超快物理相关过程的重要工具,实现波长可调谐的宽带紫外飞秒光脉冲将有助于推动超快动力学及相关领域的研究.本文报道了以两束400 nm的飞秒光脉冲作为级联四波混频的抽运源,在氧化镁晶体中产生9阶频率上转换和5阶频率下转换边带信号的实验结果.边带波长范围从350 nm到450 nm连续可调谐,这些边带信号的发散角和波长与级联四波混频理论预测结果吻合.紫外边带相对于入射光的整体转化效率约为1.2%.同时,高阶边带的光谱形状呈现高斯型,其谱宽理论上支持傅里叶转换极限脉宽为20—50 fs.本文展示了一种高效产生波长可连续调谐的紫外飞秒光脉冲的便捷方法,为基于紫外超短脉冲的相关研究提供了有效工具.     

Cascaded four-wave mixing generation in photonic crystal fibers

We investigate the efficient generation of broadband cascaded four-wave mixing products seeded at different wavelengths in photonic crystal fibers, with a high-peak power picosecond pulse pumping in the anomalous dispersion region as well as the normal dispersion regime. Multiple four-wave mixing products with different frequency intervals have been experimentally achieved when pumping in the anomalous dispersion region. Measured results present bandwidths of over 500 nm. We have also experimentally demonstrated that only seeding at the Stokes or anti-Stokes peaks can we get the efficient generation of cascaded four-wave mixing or cascaded stimulated Raman scattering when pumping in the normal dispersion regime.     

高非线性光子晶体光纤中飞秒脉冲的传输特性和超连续谱产生机制的实验研究及模拟分析

用实验和数值模拟两种方法研究了高非线性光子晶体光纤中飞秒激光脉冲的传输特性和超连续谱的产生机理，给出了抽运脉冲在三种不同中心波长情况下输出光谱展宽并形成超连续谱的实际测量及理论模拟结果.研究表明：在零色散波长抽运时，光谱展宽以自相位调制为主，同时三阶色散的影响明显，传输脉冲在时域内出现振荡次峰.而在反常色散区抽运时，光谱展宽的初期以自相位调制为主，随后根据抽运功率的不同孤子自频移、高阶光孤子的裂变和四波混频效应会逐渐增强，进而成为光谱展宽的主要原因.与此相应，在时域中能明显看到孤子的形成和红移，飞秒传输脉 关键词： 光子晶体光纤 高非线性光子晶体光纤 飞秒脉冲激光 超连续谱     

Combined nonlinear effects for UV to visible wavelength generation in a photonic crystal fiber

We experimentally study the combined nonlinear effects,including four-wave mixing,stimulated Raman scattering,soliton dynamics,and cross-phase modulation by coupling femtosecond pulses around 850 nm into the normal dispersion region near the zero-dispersion wavelength in the fundamental mode of a homemade silica photonic crystal fiber. The nonlinear optical dynamics at different stages are demonstrated,and the discrete ultraviolet(UV) to visible wavelengths widely separated from the pump wave are generated by the interaction of several nonlinear effects involved. The UV to visible wavelengths can be used as short pulse sources for multiphoton ionization,fluorescence spectroscopy,and biochemical imaging.     

利用自发四波混频测量光子晶体光纤色散

使用脉宽为1.6ps的脉冲光抽运0.6m长的光子晶体光纤,测量由光纤中自发四波混频过程所产生光子对的频谱,并利用所获得的相位匹配数据确定了待测光纤的色散。当抽运光的中心波长以1nm的步长,在1037～1047nm的范围内变化时,通过可调谐滤波器和单光子探测器测量光子晶体光纤产生的信号和闲频光子对的频谱,从而获得11组四波混频相位匹配数据。然后使用阶跃有效折射率模型对所获得的相位匹配数据进行拟合,得出待测光子晶体光纤的纤芯半径和包层空气比的有效值分别为0.949μm和29.52%,并在此基础上计算了光纤的色散及全频谱范围内的四波混频相位匹配曲线。实验结果显示,曲线预测值与实测值之间误差小于0.1%。     

All-solid-state Cr:forsterite laser generating 14-fs pulses at 1.3 mum

We report the generation of 14-fs pulses at 1.3mum with 80-mW average power at 100-MHz repetition rate by an all-solid-state Kerr-lens mode-locked Cr:forsterite laser. The laser spectrum covers wavelengths of 1230-1580 nm, with a FWHM of 250 nm. Since 1.3-mum wavelengths are close to the zero dispersion wavelength of Cr:forsterite, higher-order dispersion is the main factor limiting pulse durations. We use specially designed and fabricated double-chirped mirrors in combination with high-index PBH71 prisms to compensate for the intracavity dispersion over almost 300 nm.     

Mid-infrared supercontinuum generation in a four-hole As2S5 chalcogenide microstructured optical fiber

We demonstrate the supercontinuum (SC) generation in a four-hole As₂S₅ chalcogenide microstructured optical fiber (MOF) experimentally. The As₂S₅ glass has better property of transmission than As₂S₃ glass in the visible range. The four-hole As₂S₅ MOF is fabricated by a rod-in-tube method. The SCs generated by different pump wavelengths at 2,000, 2,300 and 2,500 nm in the MOF whose length is from 2.3 to 20 cm are demonstrated. Those pump wavelengths correspond to the chromatic dispersion wavelength in the normal chromatic dispersion region, the anomalous chromatic dispersion region close to zero-dispersion wavelength (ZDW) and the anomalous chromatic dispersion region far from ZDW, respectively. Wider SCs can be obtained when pumped at a wavelength in the anomalous dispersion region close to ZDW. The widest SC range of 4,280 nm (from 1,370 to 5,650 nm) covering two octaves was obtained in a 4.8-cm-long fiber pumped at 2,300 nm.     

Anti-Stokes Frequency Shift and Evolution in Polarization-Maintaining Photonic Crystal Fiber with Two-Zero Dispersion Wavelengths

Using the tunable pump pulses with about lOO fs pulse duration and 1064 nm central wavelength; the polarization-, wavelength- and power-dependent anti-Stokes lines are generated and modulated simultaneously in a polarization-maintaining photonie crystal fiber （PM-PCF） with two zero-dispersion wavelengths. By accurately controlling the polarization directions, the wavelength and the power of the pump pulse in the fiber anomalous region close to the second zero-dispersion wavelength of the PM-PCF, the output anti-Stokes pulse spectra can be tuned between 563 nm and 603 nm, which is in good agreement with the theoretical simulation. The color conversion of the mode image from yellow to orange is also observed with the different polarization pump pulses. These results can be attributed to the combined interaction between the fiber birefringence （including linear- and nonlinear- birefringence） and dispersion, and are attributed to phase-matching parametric four-wave mixing.     

Broad and ultra-flattened supercontinuum generation in the visible wavelengths based on the fundamental mode of photonic crystal fibre with central holes

By coupling a train of femtosecond pulses with 100 fs pulse width at a repetition rate of 76 MHz generated by a mode-locked Ti:sapphire laser into the fundamental mode of photonic crystal fibre(PCF) with central holes fabricated through extracting air from the central hole,the broad and ultra-flattened supercontinuum(SC) in the visible wavelengths is generated.When the fundamental mode experiences an anomalous dispersion regime,three phases in the SC generation process are primarily presented.The SC generation(SCG) in the wavelength range from 470 nm to 805 nm does not emerge significant ripples due to a higher pump peak power and the corresponding mode fields at different wavelengths are observed using Bragg gratings.The relative intensity fluctuations of output spectrum in the wavelength ranges of 530 nm to 640 nm and 543 nm to 590 nm are only 0.028 and 0.0071,respectively.     

Wavelength-tunable spectral compression in a dispersion-increasing fiber

We demonstrate, both numerically and experimentally, adiabatic soliton spectral compression in a dispersion-increasing fiber (DIF). We show that a positively chirped pulse provides better spectral compression in a DIF with a large anomalous dispersion ramp. An experimental spectral compression ratio of 15.5 is obtained using 350 fs positively chirped input pulse centered at 1.5 μm. A 30 nm wavelength tuning ability is experimentally achieved.     

Low Timing Jitter and Tunable Dual-Wavelength Picosecond Pulse Generation from a Fabry--Pérot Laser Diode with External Injection

A novel scheme to generate tunable dual-wavelength optical pulses with low timing jitter at arbitrary repetition rates is proposed and demonstrated experimentally. The pulses are generated from a gain-switched Fabry-Pérot laser diode with two external cw beams for injection seeding simultaneously. The cw light is generated by two independent distributed feedback laser diodes, and their wavelengths can be tuned independently by two temperature controllers. The dual-wavelength pulses with the pulse width of 57 ps, the timing jitter of 340 fs, are obtained. The sidemode-suppression ratio of the output pulses is better than 23dB over a 10-nm wavelength tuning range.     

Experimental investigation on gain-dependent chromatic dispersion of the semiconductor optical amplifier

Using a chromatic-dispersion analysis method based on K–K transformation of the gain spectrum, we experimentally investigated the chromatic dispersion of semiconductor optical amplifier in detail within the wavelength range from 1530 nm to 1610 nm. Experimental results demonstrate that there are three typical dispersion regions, which are abnormal dispersion, flatten dispersion and normal dispersion region, and three zero-dispersion points, which exist around 1550 nm, 1580 nm and 1600 nm, over the wide wavelength range of 80 nm. With an increase in bias current on SOA, wavelengths of the three zero dispersion points all had a blue shift and the three near-zero dispersion regions corresponding became wider. However, the three near-zero dispersion regions corresponding became narrower when the input optical power increased. Therefore, the dispersion of SOA can be flexibly adjusted by changing the bias current and input optical power to SOA.     

Optimizing input and output chirps up to the third-order for sub-nanojoule,ultra-short pulse compression in small core area PCF

Compression of sub-nanojoule laser pulses using a commercially available photonic crystal fiber (PCF) with zero dispersion wavelength of 860 nm is discussed. A twofold pulse compression starting from 24 fs transform limited seed pulses around 800 nm is experimentally demonstrated as a verification of our simulations. Theory shows that by the optimization of input and output chirp parameters up to the third order, high quality, 5.7 fs pulses can be generated from a cost efficient experimental setup. Further calculations show that 1 ps pulses with central wavelength of 800 nm can be compressed down to 50 fs in the normal dispersion regime of the fiber with proper dispersion compensation. Calculations also show that dispersion flattened fibers can improve both the quality and the duration of compressed pulses. PACS 42.65.Re     

All-Optical Wavelength Conversion Based on Four-Wave Mixing in Dispersion-Engineered Silicon Nanowaveguides

We demonstrate experimentally all-optical wavelength conversion based on four-wave mixing in dispersion-engineered silicon nanowaveguides with a picosecond pulse pump. We find that the conversion efficiency is significantly limited by nonlinear losses induced by the two-photon absorption and freecarrier absorption. Using a picosecond pulse pump centered at 1,550 nm, we show that the input continuous-wave signals can efficiently be converted into a broadband idler pulse in silicon waveguides with various dimensions. Conversion efficiencies versus signal wavelengths are different for silicon waveguides with different dimensions due to the variation in the phase mismatch; we obtain a conversion efficiency of – 32 dB in silicon nanowaveguides with a length of 5.8 mm. Such on-chip optical wavelength converters can find important potential applications in highly-integrated optical circuits for all-optical ultrafast signal processing.     

含氟聚酰亚胺波导波长分离耦合器优化设计

提出并采用统计优化的设计方法解决含氟聚酰亚胺波导波长交叉分离耦合器的偏振态变动的影响.在实测了含氟聚酰亚胺的色散和双折射特性的基础上,优化设计了40路波长信道、1550 nm中心波长、0.8 nm波长间隔的抗偏振变动的波长交叉分离耦合器.数值模拟显示:波长周期偏移小于0.1 nm,1 dB带宽为0.5 nm,3 dB带宽为0.8 nm,串扰小于－30 dB,偏振变动导致的波长漂移小于0.08 nm.     

宽谱段高分辨扫描光谱定标技术

为了满足原子发射光谱仪在紫外至近红外宽谱段范围内的高光谱分辨率快速检测需求,采用精密角位移平台直接驱动光栅,配合面阵探测器,实现高精度光谱分段快速扫描探测。但在扫描过程中,探测器像元波长增量与光栅转角呈非线性关系,且不同像元的波长增量不同,这对该光谱仪波长定标造成障碍。为校正光栅色散的非线性,基于光栅方程精确计算光栅转角与探测器首尾两端像元波长的映射关系,针对同一光栅转角,探测器其余像元波长利用首尾像元波长按照局部线性色散规律计算得到,从而完成全谱段光谱定标。依据定标所得转角与探测波段对应关系依次驱动光栅转动,实现宽谱段范围内的分段高精度光谱快速扫描探测。利用汞灯光源对该定标方法的波长检测精度进行检验,在200~800 nm的宽谱段范围内,波长准确度优于0.018 nm,波长重复性优于0.001 nm。     

Soliton and rogue wave statistics in supercontinuum generation in photonic crystal fibre with two zero dispersion wavelengths

Stochastic numerical simulations are used to study the statistical properties of supercontinuum spectra generated in photonic crystal fibre with two zero dispersion wavelengths. For picosecond pulse excitation, we examine how the statistical properties of solitons generated on the long wavelength edge of the supercontinuum (``optical rogue waves") are modified by energy transfer to dispersive waves across the second zero dispersion wavelength. The soliton statistics (characterized in terms of peak power, wavelength and pulse duration) are shown to be strongly modified by the mechanism of dispersive wave generation, with the detailed form of the probability distribution depending strongly on input pulse energy.     

Group-velocity-dispersion-compensated femtosecond optical parametric amplifier

A tilted pulse front geometry is known to allow group-velocity-dispersion (GVD) compensated propagation of short pulses of different wavelengths in dispersive media. This scheme is shown to be applicable to an optical parametric amplifier (OPA) pumped at 450nm. A numerical calculation shows that a certain combination of the tilt of the pulse front and the angle between the interacting beams provides optimum GVD compensation for each wavelength. The parameters providing broadband tunability are identified. The tunability of the GVD-compensated OPA pumped with 55fs pulses was experimentally demonstrated between 545nm and 645nm. This revised version was published online in November 2006 with corrections to the Cover Date.     

Dispersion-tuned multiwavelength actively mode-locked fiber laser using a hybrid gain medium

We demonstrate a multiwavelength 10 GHz pulse source using a dispersion-tuned actively mode-locked fiber ring laser incorporated with a semiconductor optical amplifier and an erbium-doped fiber amplifier. Simultaneous seven-wavelength operation of the laser is obtained. The side-mode suppression of all wavelengths is above 30 dB. Smooth wavelength tuning is achieved over more than 12 nm by changing the modulation frequency or the length of the optical delay line. Pulse characteristics are almost constant over the entire tuning span. Wavelength spacing can also be varied from 0.9 to 10 nm by adjusting the dispersion of the cavity. These experimental observations agree well with theoretical analyses.     

Anomalous dispersion in the Belousov-Zhabotinsky reaction: Experiments and modeling

We report results on dispersion relations and instabilities of traveling waves in excitable systems. Experiments employ solutions of the 1,4-cyclohexanedione Belousov-Zhabotinsky reaction confined to thin capillary tubes which create a pseudo-one-dimensional system. Theoretical analyses focus on a three-variable reaction-diffusion model that is known to reproduce qualitatively many of the experimentally observed dynamics. Using continuation methods, we show that the transition from normal, monotonic to anomalous, single-overshoot dispersion curves is due to an orbit flip bifurcation of the solitary pulse homoclinics. In the case of “wave stacking”, this anomaly induces attractive pulse interaction, slow solitary pulses, and faster wave trains. For “wave merging”, wave trains break up in the wake of the slow solitary pulse due to an instability of wave trains at small wavelength. A third case, “wave tracking” is characterized by the non-existence of solitary waves but existence of periodic wave trains. The corresponding dispersion curve is a closed curve covering a finite band of wavelengths.