具有各向异性的梯度颗粒复合材料的有效介电响应

本文研究了具有梯度壳层椭球颗粒复合体系的有效介电响应，在稀释条件下用准静态近似方法, 推导了颗粒壳层具有任意介电梯度形式的椭球颗粒复合体系的有效介电常数和部分共振条件的一般表达式。并以壳层的介电常数为主轴的幂函数形式为例，得出了通过调节壳层的介电梯度形式、颗粒的结构和形状,可以提高该体系的有效介电常数和实现部分共振的结论。     

ZnO薄膜的光学性质研究

采用直流反应磁控溅射方法在玻璃基底上成功地淀积ｃ轴取向性好的ＺｎＯ薄膜。经过优化计算，获得并分析了不同氧分压下制备的ＺｎＯ薄膜的折射率ｎ和消光系数ｋ的数值；同时得到了吸收光学带隙Ｅｏｐｔ，用能带模型解释了Ｅｏｐｔ的变化规律。     

梯度铝镓氮缓冲层对氮化镓外延层性质的影响

采用金属有机物化学气相沉积系统在硅面碳化硅衬底的(0001)面上生长氮化铝缓冲层,并通过改变3层梯度铝镓氮(Al_xGa_(1-x)N:x=0.8,0.5,0.2)缓冲层的生长温度和氨气流量,制备出了高质量的氮化镓外延层。分别采用X射线衍射、原子力显微镜、光致发光谱和拉曼光谱对氮化镓外延层进行表征。实验结果表明,随着氮化镓外延层中张应力的降低,样品的晶体质量、表面形貌和光学质量都有显著提高。在最优的梯度铝镓氮缓冲层的生长条件下,氮化镓外延层中的应力值最小,氮化镓(0002)和(1012)面的摇摆曲线半峰宽分别为191 arcsec和243 arcsec,薄膜螺位错密度和刃位错密度分别为7×10~7cm~(-2)和3.1×108cm~(-2),样品表面粗糙度为0.381 nm。这说明梯度铝镓氮缓冲层可以改变氮化镓外延层的应力状态,显著提高氮化镓外延层的晶体质量。     

光学复合体系中有效介质理论的适用条件

以纳米晶掺杂复合体系为例,研究该类多组分光学材料的有效介电系数随复合体系结构和组分介电系数的变化,进而分析有效介质理论的适用条件。假定纳米晶被周期性掺杂到背景晶体中,且均为各向同性材料。借助转移矩阵理论研究发现,当纳米晶和背景晶体的介电系数相差较大时,有效介电系数会表现出波长依赖性。此外,发现复合体系在其光学能隙处没有有效介电系数,说明此时基于等效介质思想的有效介质理论均不适合描述复合体系的光学性质,这是因为在物理上均一的光学材料无法形成光学能隙。     

离子型声子晶体的光学性质

提出了离子型声子晶体的概念,发展了相应的理论：在实验上证实了离子型声子晶体中存在超晶格振动与电磁波的强烈耦合,观察到原先存在于离子晶体中的极化激元等长波光波行为;预言了一些可能的物理效应,离子型声子晶体超晶格振动和电磁波的耦合方程与黄昆方程在形式上完全一致,说明了超晶格与实际晶格在物理上的相似性。     

基于折射率梯度门限的气动光学窗口光传输研究

基于流场界面厚度（Interfacial—Fluid—Thickness,IFT）理论,建立了高折射率梯度门限模型来研究气动光学窗口光传输畸变。首先在光学窗口折射率梯度场基础上,提出高折射率梯度门限,忽略绝对值低于该门限的折射率梯度值,重构折射率场,并对其气动光学传输效应进行仿真。结果表明,当58．37％的梯度值被忽略时,得到的重构折射率场与原折射率场仿真光程差（OPD）最大相对误差不超过1．5％,验证了气动光学窗口高折射率梯度区域是产生光传输畸变的主要原因,也证实了该门限模型对气动光学窗口光传输效应进行仿真的可行性,对气动光学失真的机理、预测及校正有一定的指导意义。     

三元合金缺陷层对有限超晶格中局域界面光学声子模的影响

在宏观介电连续近似下，采用转移距阵方法，研究了三元合金缺陷层对有限超晶格中局域界面光学声子模的影响.在这种有限超晶格结构中，可以清楚地看到所有界面模的演化轨迹.结果表明：存在两类局域模，它们的宏观静电势波函数分别局域在缺陷层和表面层附近，且这些模随着超晶格组分层和缺陷层的相对厚度和介电常数的改变，其局域位置和特性发生显著变化.此外，发现虽然能隙中局域模的数目不守恒，但所有界面模的总数守恒.     

四层异质结构的表面和界面光学声子模

用连续介电模型研究了有限厚度四层异质结构的表面和界面光学声子模。精确得到本征失量、色散关系和面电荷密度。前人关于介电平板、双层、三层以及无限四层结构等所有已得结果，都可从此文普遍关系重新推出。另外，还给出了有限阶梯量子阱等有趣而实用结构的色散关系及其数值显示。本研究可视为文献［８］的推广。 关键词：     

Pt/Si界面的椭圆偏振光谱研究

本文应用椭圆偏振光谱法,研究未经热处理的Pt/(n-Si)界面.在350O(?)～650O(?)的光谱范围内,对椭圆偏振光谱的测量数据进行分析计算,以确定界面的光学响应.结果表明,Pt/(n-Si)界面存在着一界面层,其厚度d_2-30±1(?).本工作同时得到了该界面层的表观光学常数谱和介电函数谱.应用有效介质理论对界面层的介电函数谱进行拟合分析,结果指出,界面层存在着富硅的氧化物(其平均效果是SiO_(1.54)),界面区是Pt、Si和富硅氧化物的物理混合和化学混合区.     

铁电半导体碘硫化锑量子点复合材料及其光学性能的研究

用溶胶-凝胶法成功地制备了铁电半导体碘硫化锑(SbSI)微晶掺杂有机改性的TiO_2薄膜及块状凝胶。铁电SbSI晶体在C轴具有非常大的介电常数,非常高的电-光系数,较大的光电导系数,同时又是一种本征半导体材料。将SbSI掺杂到非晶态的基质中,通过热处理及气氛保护的方法控制微晶的生长。通过X射线衍射光谱与高分辨透射电子显微镜观察到微晶的存在以及晶体尺寸和分布情况。使用简并的四波混频的方法测得了薄膜样品的三阶非线性极化率,并在块状样品中发现了复合材料中存在的电控双折射效应,测得样品的有效电光系数为2.42×10~(-3)nm/V。     

梯度圆柱颗粒复合介质的有效非线性响应

应用非线性微分有效偶极近似方法,导出了关于非线性梯度圆柱颗粒的等效线性介电常数和三阶非线性极化率的微分式,研究了稀释极限下,圆柱形梯度颗粒无规置入线性介质中组成的复合介质的有效线性介电常数和三阶非线性极化率.作为应用,数值计算了具有幂指数梯度分布的介电常数的颗粒复合介质的有效非线性响应,及梯度金属电介质颗粒复合介质的表面plasmon共振效应.     

Effect of the effective anisotropy field of soft layer on magnetic properties of soft/hard stacked media

Magnetic properties of soft/hard stacked perpendicular magnetic recording media were investigated using a two-moment model with taking account of demagnetizing energy. Demagnetizing energy of the soft layer may improve the uniformity of magnetic properties of the composite media and also decrease the interlayer thickness, although weaken the thermal stability a little. The application of high saturation magnetization (M_s) soft magnetic material as the soft layer may compensate for the undesirable contribution while maintaining its benefits.     

Controlling electric fields spatially by graded metamaterials: Implication on enhanced nonlinear optical responses

The local electric field of a graded metal-dielectric cylinder, with complex permittivity given by a spatially dependent Drude model, has been derived analytically in terms of hypergeometric functions. Our results show that the electric field inside the cylinder can be confined in desired positions. Thus one can achieve the control of electric fields by fabricating graded metamaterials with specific material parameters. The enhanced nonlinear optical responses are also examined. The results suggest that the gradation-controlled field distribution may be a consequence of a combination of surface plasmon resonance and microgeometry in graded metamaterials.     

绝缘颗粒液体主体基质复合介质的非线性光学性质

利用Maxwell-Garnett近似，并结合谱表示方法，理论研究了具有一般非线性的绝缘颗粒，无规则浸入液体主体基质复合体系的非线性光学性质-在弱非线性条件下，数值研究了体系的有效线性介电函数和光学非线性随体积分数的变化，并发现体系的线性介电函数比光学非线性更依赖于绝缘颗粒组分的体积分数-在一般非线性条件下，研究体系的有效介电函数随入射光强度的依赖关系，还研究了s方向和p方向极化的总反射率的行为- 关键词： 复合介质 谱表示 非线性光学性质     

Effective optical constants and effective optical properties of ultrathin trilayer structures

This work presents an extension of the characteristic effective medium approximation (CEMA) to ultrathin trilayer systems. The extension has been carried out analytically and is supported by corresponding calculations of the effective optical constants of Cu-Au-Cu and Ag-SiO-Ag trilayer systems using the CEMA approximation. This work is in essence a generalization of the characteristic effective medium approximation introduced earlier for ultrathin bilayer structures. This method is used to derive the effective optical constants of a trilayer system, consisting of three thin layers with each constituent layer of thickness much less than the wavelength of the incident radiation. Within this regime a trilayer system is viewed as one effective layer referred to as an effective stack (ES) with well defined effective optical constants, which can be used to calculate the optical properties of the trilayer stack within a specified wavelength range. The CEMA based calculations of the effective optical constants are applied to two trilayer systems with a total of five stacks. Three are Cu-Au-Cu and two are Ag-SiO-Ag stacks. The thicknesses of the parent layers in the Cu-Au-Cu stack range from 3 to 30 nm for Cu and 4 to 40 nm for Au; in the Ag-SiO-Ag stack the constituent layers are 6 nm for Ag, but range from 5 to 10 nm for SiO. This study is for normal or near normal incidence spectroscopy in a wavelength range that extends from visible to near infrared. The agreement between CEMA based ES stack results and those of the standard CMT technique is very satisfactory.     

Effect of Li incorporation on the structural and optical properties of ZnO

This paper presents the structural and optical properties of the as-prepared and lithium-doped ZnO at different percentages of Li incorporation (5%–15%) in ZnO. Effect of doping with various percentages of Li at a particular annealing temperature of 600 C is studied. The samples are characterized by X-ray diffraction, absorption spectroscopy, photoluminescence and Raman spectroscopy. The X-ray diffraction and micro-Raman spectroscopy confirm that the lithium substituted zinc and retains the wurtzitic structure of the lattice. Such substitutional Li in ZnO gives rise to shallow acceptor levels and contributes to the p-type conductivity. From the results of the absorption spectroscopy we observed the evidence of shallow levels upon doping and we also determined the bandgap of the materials which is found to be 3.36 eV. Photoluminescence studies reveal that no deep level is formed. The electrical measurements show that the Li-doped samples are p-type in nature and this is due to substitutional Li.     

光学薄膜界面互相关特性的确定

本文实验测量了光学薄膜的散射波场分布,根据多层光学薄膜的矢量散射理论,确定了膜层界面的互相关特性.当空间频率较低时,对于膜层层数较少的膜系,膜堆内的各界面是完全相关的;若空间频率较高,则逐渐趋于部分相关模型.实验指出,膜层界面的互相关特性亦与所采用的蒸发技术有关.     

Research on the optical properties of collodion film

This paper centers on the deposition process and optical properties of collodion film. Collodion film was prepared on the double side polished silicon and k9 optical glass using the sol–gel method. The studying results have showed four characteristics of collodion film. First of all, the thickness of collodion film decreases with increasing the revolution speed. Secondly, the refractive index of collodion film changes from 1.529306 to 1.500128, which accords with the normal dispersion. Thirdly, the transmittance of collodion film is higher in the visible wavelength range 380–760 nm and its average transmittance is 91.9%. At last, the absorption property is very well in the infrared region. The infrared absorption coefficient is greater than 0.69/μm in range of 3–5 μm, and it is up to 1.433528/μm in 8–14 μm because of its many strong infrared absorption peaks. In addition, the absorption characteristics have been analyzed in detail.     

三苯胺衍生物分子非线性光学性质的理论研究

在密度泛函理论水平上,利用响应函数方法,研究了1-{(1E)-2-[4-(二苯胺基)苯基]乙烯基}-4-[4-N,N-二甲胺]苯(PVMB)和1-[(1E)-2-(4-(1E)-2-{4-[4-N,N-二甲胺]苯基}乙烯基)苯基]苯胺}苯基)乙烯基]-4-[4-N,N-二甲胺]苯(DPVMB)两分子的双光子吸收特性.计算结果表明,这两个化合物都具有较好的双光子吸收特性,且具有两分支结构的DPVMB分子比具有单支结构的PVMB分子有更强的双光子吸收强度.计算数值结果和实验结果符合地较好.