Ionization and Harmonic Generation of Diatomic Molecular Ion

l.IntroductionRecentexPerimentshavcdemonstratedthehigh-orderharmonicgenerationinraregasandmoleculargas[1~'j.TherearemanytheoreticalpaPersdealingwithharmonicgen-erationofatom[6~8j,comparativelysPeaking,theoreticalworksabouttheharmonicgen-erationofmolecuIeareless[9j,esPeciallyabouttheevolutionofionizationandharmonicgenerationwiththeinternuclearseparation,andtherelationbetweenionizationandhar-monicgeneration.InthispaPerwegivesomenumericalresultsofdiatomicmolecularionirradiatedbyalinearlyPOlari…     

氩气中高次谐波辐射的研究

报道了在４５ｆｓ－２ＴＷ激光装置上以Ａｒ惰性气体为介质产生高次谐波的实验结果,实验中通过研究气体密度和激光能量对谐波辐射的影响,找到了适当的气体密度和激光能量范围,并在Ａｒ气中观察到８１次（９．７ｎｍ）的皆波辐射,这时迄今为止,人们在Ａｒ气中所能观测到的最短波长的谐波辐射,经分析表明,高于５７次的谐波是由Ａｒ离子产生的。     

强场高次谐波辐射过程中的相位匹配

从实验上定性地研究了强 辐射过程中位相匹配的作用与影响,主要通过改变气体密度、激光强度和光束的共焦参数来研究相位对高闪谐波辐射的影响。从改善高次谐波辐射过程中的相位匹配来考虑,气体攻激光强度都有一最佳值。利用大的共焦参数,可以明显改善相位匹配,提高谐波输出的转换效率。     

Theoretical Study of High-Order Harmonic Generation From a Coherent Superposition State in a Chirp-Free Pulse Combined with a Chirped Control Pulse

In this paper, we theoretically investigate high-order harmonic generation (HHG) from a helium atom prepared in a coherent superposition state in a two-color laser field. Numerical results show that the emission efficiency of the harmonic spectrum in a coherent superposition state is enhanced by approximately eight orders of magnitude compared with the case of the ground state. In addition, the effect of the initial population of the excited state on the HHG is presented to reveal the physical origin of the enhancement of HHG. By adjusting the laser parameters of the driving pulse, such as the chirping parameter, the relative phase, and the intensity of the driving pulse, an ultrabroad continuum with a width of 275 eV can be observed. Finally, an isolated 12-as pulse is generated after phase compensation.     

一维多原子分子离子与超短激光场作用产生的高次谐波

从经典方程出发，采用克兰克-尼科尔森中心差分法对一维多原子分子离子与一维超短强激光场相互作用产生的高次谐波进行了数值模拟计算，发现激光场的初始相位对高次谐波辐射谱有明显影响；通过进一步研究，给出了初步解释。从而，可以通过调节适当的激光初始相位和选取适当的系统来改善高次谐波的相位匹配，产生清晰的高次谐波辐射谱。     

Effects of Pulse Durations on High-order Harmonic Generation

ＥｆｅｃｔｓｏｆＰｕｌｓｅＤｕｒａｔｉｏｎｓｏｎＨｉｇｈｏｒｄｅｒＨａｒｍｏｎｉｃＧｅｎｅｒａｔｉｏｎＬＩＸｕｅｘｉｎＬＩＵＹａｑｉｎｇＺＨＡＩＫａｎＸＵＺｈｉｚｈａｎＨＡＮＳｈｅｎｓｈｅｎｇ（ＳｈａｎｇｈａｉＩｎｓｔｉｔｕｔｅｏｆＯｐｔｉｃｓａｎ...     

强激光与一维多原子分子离子的相互作用及高次谐波的增强

研究强激光脉冲与一维多原子分子离子的相互作用,讨论双色激光场中高次谐波转化效率的提高,并应用经典三步模型说明高次谐波平台展宽的物理机制.     

偶次和半整数次谐波的产生

用数值求解一维含时薛定谔方程的方法计算了由频率分别为ω及１．５ω的激光组成的双色场２作用下的模型原子产生的高次谐波谱。发现由于双色场的相干效应,在其谐波谱中不仅产生了奇次谐波,还产生了偶次谐波和半整数次谐波。分析了各次谐波产生的原因以及对谐波转化效率产生影响的主要因素。     

飞秒激光在氦气中的高次谐波

利用中心波长在795nm的线偏振的钛宝石超短脉冲激光除为抽运源，在拟气中观察到40nm-160nm第5－17次谐波的软X射线激光辐射，着重研究了高次谐波谱线强度随气压的变化规律，发现高次谐波谱线强度随充气气压的增加而增强，实验中考虑到如果充气气压过高，探测仪器可能受到损害，充气气压没有达到最佳值。     

压缩真空中的三能级原子的自发辐射强场高次谐波时间特性的理论分析

对压缩真空与V型三能级原子的相互作用作了理论分析, 探讨了量子干涉效应对压缩真空中原子自发辐射的影响。当原子的上能级简并时强的量子干涉效应影响原子的定态和定态出射光谱, 使它们对原子的初态敏感。这种情况下, 压缩使谱线趋于关于压缩真空中心频率对称, 量子干涉使谱线趋于不对称。通过用单电子近似求解含时薛定谔方程, 用加窗傅里叶分析的方法, 分析了单原子产生的高次谐波的时间特性。理论分析表明, 基态粒子数消耗对不同级次谐波辐射的影响程度不一样; 谐波辐射随着入射激光场强度的增加会出现饱和; 随着谐波级次的增加, 谐波辐射越来越趋向于集中在更短的时间间隔内, 相应的线宽也随着谐波级次的增加而增加。     

采用附加共振高频场提高强场高次谐波的产生效率

提高高次谐波效率一直是强场物理研究中的一个重要课题,对此人们采取了很多方法,如采用双色场,实现相位匹配,附加一个强电场或强磁场等。本文在研究双色场高次谐波的过程中,发现原子的能级结构对于高次谐波的产生效率有极大的影响,据此提出利用附加共振高频场来大幅度提高高次谐波的产生效率。     

超短脉冲谐波截止区量子效应研究

采用Lewenstein路径积分模型和准经典三步模型,计算了不同脉宽的超短脉冲高次谐波波谱。通过比较模型截止频率随载波包络相位的变化关系的差异,对辐射过程中的量子效应进行了研究。结果显示,随脉宽的减小,以上两种模型计算结果出现的偏离增加,谐波辐射中的量子效应愈加明显。当脉宽减小至0.5 T(T为光学周期)时,准经典三步模型已不能用以解释Lewenstein模型的计算结果。     

7 fs超快强激光驱动Ar原子产生支持单个阿秒脉冲的高次谐波连续谱

采用脉冲宽度为7 fs,脉冲能量为0.4 mJ的超快强激光脉冲与气体盒子中Ar原子作用获得了高次谐波截止区连续谱,并发现当驱动激光稳定在不同的载波包络相位时,高次谐波的谱结构、谱调制深度和连续谱的带宽都有很大区别。在某些载波包络相位时获得了平滑的连续谱,调制深度小于17%,连续带宽达10 eV,从而支持时域上获得变换极限500 as的单个阿秒脉冲。     

Probing dynamic interference in high-order harmonic generation from long-range molecular ion:Bohmian trajectory investigation

Using Bohmlan trajectory （151） method, we investigate the dynamic interference in nlgn-orcter narmonlc generauon from diatomic molecular ions. It is demonstrated that the main characteristics of the molecular harmonic spectrum can be well reproduced by only two BTs which are located at the two ions. This haiapens because these two localized trajectories can receive and store the whole collision information coming from all of the other re-collision trajectories. Therefore, the amplitudes and frequencies of these two trajectories represent the intensity and frequency distribution of the harmonic generation. Moreover, the interference between these two trajectories shows a dip in the harmonic spectrum, which reveals the molecular structure information.     

强激光啁啾脉冲中原子的高次谐波辐射

数值计算了强激光啁啾脉冲中原子的谐波辐射。啁啾效应使谐波发生移动和展宽，即相对于无啁啾冲情形，负啁啾脉冲中谐波平台的前半部分发生兰移，而后半部分谐波谱则发生红移。     

二次谐波产生中入射啁啾脉冲对相位的影响

讨论了基波为叔率啁啾脉冲的二次谐波产生过程，结果表明选取合适的啁啾参量可以提高二次谐波的光强，但同时会使其波形和相位发生变化，三次相位的畸变主要取决于入射的基波啁啾脉冲，而与相位匹配的失谐量关系不大。     

Harmonic and attosecond pulse enhancement in the presence of noise

<正>In this paper,we theoretically investigate the effect of noise on the photoionization,the generation of the high-order harmonic and the attosecond pulse irradiated from a model He~+ ion.It shows that by properly adding noise fields,such as Gaussian white noise,random light or colored noise,both the ionization probabilities(IPs) and the harmonic yields can be enhanced by several orders of magnitude.Further,by tuning the noise intensity,a stochastic resonance-like curve is observed,showing the existence of an optimal noise in the ionization enhancement process.Finally,by superposing a properly selected harmonic,an intense attosecond pulse with a duration of 67 as is directly generated.     

Generation of the wavelength-tunable XUV pulse using the two-color and three-color infrared pulses

We present an efficient method to generate an ultrashort wavelength-tunable XUV pulse by using the harmonic selec- tive enhancement scheme. The results show that by properly controlling the delay times of a two-color field or a three-color field, selective enhancement of the harmonics with photon energies between 80 eV and 315 eV can be obtained. Fur- ther, a wavelength-tunable and bandwidth-controllable XUV radiation can be obtained by Fourier transformation of these enhanced harmonics.     

纳米氧化锌中三光子吸收与倍频效应致光辐射特性

为研究强光激励下纳米氧化锌发光机制,以气相传输法制备的冠状样品为对象,室温下以1 100nm与1 150 nm脉冲激光以及350 nm氙灯对其进行激励,观测光致发光谱.根据光强关系和强场与物质作用的三阶微扰理论,认为1 100,1 150 nm激光激励下的样品的紫外与可见光波段的辐射机理分别归因于样品中三光子吸收和二次谐波效应.同时,基于激子非弹性碰撞复合机制,对紫外辐射的红移现象进行了分析.     

Extension of Harmonic Cutoff and Generation of Isolated Sub-30 as Pulse in a Two-Color Chirped Laser Field

We theoretically investigate high-order harmonic and isolated attosecond pulse generation in a two-color chirped laser field,which is synthesized by a 9 fs/800 nm fundamental chirped pulse and a 9 fs/1600 nm controlling chirped pulse.Our numerical results show that,by using this method,not only is the harmonic cutoff significantly extended to the 948th order harmonic,but also the bandwidth of the supercontinuum spectrum is effectively broadened to about 1342 eV.In addition,due to the introduction of the chirp,the long quantum path is suppressed and only the short one is selected,and then an isolated 28 as pulse with a bandwidth of 155 eV is obtained directly.