Triple differential cross section measurements for the electron impact ionization of helium: Comparison with a second Born approximation

Triple differential cross sections for the ionization of helium by electrons of 500 eV impact energy have been measured in a coplanar, asymmetric geometry and for energies of the ejected electrons of 2.5, 5, 10 and 20 eV. A comparison is made between experimental data and a second Born treatment of Byron, Joachain and Piraux [1] for atomic hydrogen but for corresponding momenta of the incoming and the two outgoing electrons and for corresponding momentum transfer during the collision. The second Born describes quite well the shifts of the binary peak and the recoil peak to larger angles, the asymmetry of the recoil peak and the ratios of the intensities of binary to recoil peaks for different scattering parameters. — A quantitative estimate is made (for high impact energy) of the contributions to the total cross section of those ionizing collisions, in which the recoil peak intensity represents a considerable quantity. Probably most of these events can not be described by a single collision approximation.     

Coincident fragment detection in strong field photoionization and dissociation of H2

Electron-ion momentum spectroscopy is used to investigate the correlated electronic and nuclear motion in fragmentation of H2 in 4 x 10(14) W/cm(2), 25 fs laser pulses at 795 nm. Reaction channel dependent photoelectron spectra indicate that besides the main, stepwise H2 ionization H2(+) dissociation mechanism resulting in the products H(1s) + H(+) + e(-) a second new mechanism has to be assumed. The momentum distribution of H(+) ions in the dissociation channels H(1s) + H(+) + e(-) and 2H(+) + 2e(-) is found to be independent of the kinetic energy of the photoelectrons.     

Intense-field double ionization of helium: identifying the mechanism

We present quantum mechanical calculations of the electron and ion momentum distributions following double ionization of a one-dimensional helium atom by ultrashort laser pulses (780 nm) at various intensities. The two-electron momentum distributions exhibit a clear transition from nonsequential to sequential double ionization. We provide strong evidence that rescattering is responsible for nonsequential ionization by calculating the momentum spectrum of the He2+ recoil ions-which we find in excellent agreement with recent experiments-and by analyzing the electronic center-of-mass motion via Wigner transforms.     

CFCl3分子2e和4a1轨道的电子动量谱研究

由于工业的迅速发展 ,使得空气质量急剧下降 ,因此对影响大气的分子进行深入研究变得非常必要 .本实验室已经对影响环境的甲烷[1] 、丙烷[2 ] 、CO2 [3] 等分子进行了电子动量谱研究 ,为环保提供了有用的数据 .CFCl3作为工业广泛应用的气雾剂和制冷剂原料 ,它的大量使用导致了大气中臭氧的减少[4 ] .前人已用光电子谱学的方法[5- 8] 研究了CFCl3,我们又用电子动量谱的手段对CFCl3分子进行了进一步的研究 ,即从波函数的层次上详细了解CFCl3的电子结构 .(e ,2e)电子动量谱学在研究分子的电子结构方面有非常独特的优越性[9- 12 ] ,它可以…     

Quantum mechanics: cleaning up metaphysical baggage

The dynamic electronic structure of atoms and molecules can be directly observed by means of the (e, 2e) reaction, which measures the distribution of energies and momenta of two electrons in coincidence after a knockout reaction initiated by an electron beam of known momentum incident on a molecular gas target. The molecular state for each event is identified by the electron separation energy. The recoil momentum for each event is known from the difference of measured initial and final momenta. It has been verified that values of this momentum are equal under suitable conditions to the momentum of the electron in the target immediately before knockout. Thus the spherically-averaged electron momentum distribution for each molecular orbital is measured. This is directly related to molecular orbitals calculated by the methods of quantum chemistry. Properties obtained by this method for different types of molecules are discussed.     

Electron Momentum Spectroscopy of Ethanethiol Complete Valence Shell

利用(e,2e)电子动量谱学手段首次测量了乙硫醇分子全部价轨道的束缚能谱和电子动量分布. 谱仪采用非共面对称的运动学条件,入射电子能量为1.2 keV加束缚能. 实验结果与密度泛函和Hartree-Fock方法的理论计算结果基本相符. 在束缚能谱中,观察到了17.8 eV的可能的伴线,并用电子动量谱进行了研究和标识.     

Binary and recoil collisions in strong field double ionization of helium

We have investigated the correlated momentum distribution of both electrons from nonsequential double ionization of helium in a 800 nm, 4.5 x 10(14 W/cm2 laser field. Using very high resolution coincidence techniques, we find a so-far unobserved fingerlike structure in the correlated electron momentum distribution. The structure can be interpreted as a signature of the microscopic dynamics in the recollision process. We identify features corresponding to the binary and recoil lobe in field-free (e,2e) collisions. This interpretation is supported by analyzing ab initio solutions of a fully correlated three-dimensional helium model.     

苯甲醇分子HOMO和N-HOMO轨道的电子动量谱学研究

利用第三代电子动量谱仪研究了苯甲醇(C_6H_5CH_2OH)分子的最高占据轨道(HOMO)和次最高占据轨道(N-HOMO)电子动量谱,给出了外价轨道的电离能谱信息.实验在非共面对称几何条件下完成,入射电子的能量为2400 eV加结合能.通过密度泛函方法计算得到了苯甲醇分子最高和次最高占据轨道的动量谱,理论与实验结果符合较好.     

Electron momentum spectroscopy of valence satellites of neon

Electron momentum spectroscopy (EMS) study of the neon valence satellites is reported. The experiments were performed at impact energies of 1250, 1450 and 1670 eV using a multichannel spectrometer that features high sensitivity. Binding energy spectra up to 100 eV and momentum profiles for the 2p⁻¹ and 2s⁻¹ primary transitions as well as the satellites are presented. The results are used to examine impact energy dependence of the relative intensities and shapes of the satellite momentum profiles. The results are also used to determine symmetries and spectroscopic factors of the satellites, and are compared with the previous experiments by EMS and photoelectron spectroscopy and sophisticated theoretical calculations. The present study has largely resolved controversies in the previous studies.     

Probing the high momentum component of the deuteron at high Q2

The (2)H(e,e'p)n cross section at a momentum transfer of 3.5 (GeV/c)(2) was measured over a kinematical range that made it possible to study this reaction for a set of fixed missing momenta as a function of the neutron recoil angle θ(nq) and to extract missing momentum distributions for fixed values of θ(nq) up to 0.55 GeV/c. In the region of 35°≤θ(nq)≤45° recent calculations, which predict that final-state interactions are small, agree reasonably well with the experimental data. Therefore, these experimental reduced cross sections provide direct access to the high momentum component of the deuteron momentum distribution in exclusive deuteron electrodisintegration.     

Study on Stiffness of the Symmetry Energy at High Densities by π－/π+ Ratio

using the isospin–and momentum–dependent transport model, for three different symmetry energies, we have calculated the π^–/π⁺ ratio as a function of time and tranverse–momentum in central 132sn+124 sn collision at e_beam/A=400mev. the results show that the π^–/π⁺ ratios is very sensitive to the stiffness of the symmetry energy. thus we can probe the stiffness of the symmetry energy at high densities by using the π–/π+ ratio at different time or transverse momentum more accurately than before. comparing experimental data with the calculations will reveal crucial information about the stiffness of the symmetry energy more accurately.hadronic transport model, symmetry energy, π–/π+ ratio     

Valence shell momentum distributions,binding energies,and calculated wavefunction evaluation for H2S by binary (e,2e) spectroscopy

We report preliminary results on the binding energy spectrum and molecular orbital momentum distributions of H₂S as measured by binary (e,2e) spectroscopy at 400 eV. Extensive final ion state structure associated with ionization from the inner valence molecular orbital of H₂S is observed. Three momentum distribution calculations for H₂S using basis sets of varying complexity show a better fit than in H₂O (J. Electron Spectrosc. $\text{11}$ (1977) 205) for a given quality of basis set.     

On the theory of (e, 2e) reactions in atomic hydrogen and helium

We compare the results of eikonal-Born series calculations which we have performed for the (e, 2e) reaction in atomic hydrogen with recent absolute measurements of triple differential cross sections for that process, carried out in the asymmetric coplanar geometry. We find that second-order effects play a crucial role in understanding both the angular positions and the magnitudes of the binary and recoil peaks. The implications of our analysis for the case of (e, 2e) reactions in helium are also discussed.     

Ne原子(e,2e)反应中反冲离子动量分析

利用冷靶反冲离子动量谱仪,对电子轰击Ne原子的单电离反应(e,2e)进行了研究,实验测量了70—3300eV入射能量情况下,反应过程中产生的一价反冲离子的动量分布,并对反冲离子的总动量进行了还原。介绍了一个简单的碰撞机制,据此着重分析了反冲离子纵向动量和横向动量二维谱形成的原因,该碰撞机制能够较好地解释较高能量入射时的实验结果。最后根据反冲离子的动量,估算了出射电子的能量范围,为下一步进行电子、离子的符合测量奠定了基础。     

质子椭圆流与对称能的密度依赖性

基于同位旋和动量依赖的强子输运IBUU04模型, 研究了¹³²Sn+¹²⁴Sn碰撞系统中的质子椭圆流对对称能的敏感关系. 研究发现入射能量从每核子400MeV到800MeV时质子椭圆流在低横动量端对对称能的敏感性高于高横动量端, 同时发现随着入射能量的增大, 质子椭圆流对对称能的敏感性在降低. 在研究入射能量范围内, 当入射能量为每核子400MeV左右时质子椭圆流对对称能最为敏感.     

二乙酰分子内价轨道4ag+4bu的电子动量谱学研究

在高分辨率(ΔE=115eV, Δp≈01a.u.)电子动量谱仪上获得了二乙酰分子(d iacetyl)最内价轨道4ag_g+4bu_u的电离能谱和动量谱的实验结果， 并用Hartree-Fock和密度泛函理论方法做了理论计算.实验结果与理论计算符合较好. 关键词： 二乙酰 内价轨道 电离能 电子动量谱     

Incomplete fusion reactions: Analysis of excitation functions and recoil range distributions in 16O + 51V

Incomplete fusion reactions were investigated by measuring the excitation functions of nine evaporation residues in ¹⁶O + ⁵¹V reaction in the beam energy 4-6 MeV/amu, using the well-known recoil catcher technique and gamma-ray spectrometry. The experimental data were compared with that obtained from Monte Carlo simulation calculations using the PACE2 code. The results indicate the presence of incomplete fusion process in the production of two alpha emission products. This was further confirmed by the measurement of recoil range distribution of these isotopes at 96 MeV beam energy. Calculations of the average angular momentum associated with these products revealed the peripheral nature of these ICF reactions. Received: 20 June 2001 / Accepted: 11 September 2001     

Average Energy Loss Measured in Single and Double Electron Capture Collisions of He^2＋ on Ar at Low Velocities ＊

Employing the recoil ion momentum spectroscopy we investigate the collision between He^2＋ and argon atoms. By measuring the recoil longitudinal momentum the energy losses of projectile are deduced for capture reaction channels. It is found that in most cases for single- and double-electron capture, the inner electron in the target atom is removed, the recoil ion is in singly or multiply excited states （hollow ion is formed）, which indicates that electron correlation plays an important role in the process. The captured electrons prefer the ground states of the projectile. It is experimentally demonstrated that the average energy losses are directly related to charge transfer and electronic configuration     

Large-angle quasi-free scattering in 6Li(p,pd)4He at 670 MeV

The ⁶Li(p, pd)⁴He reaction was investigated at 670 MeV by a coincidence experiment with a large-angle scattering geometry. The energy sharing and angular correlation of the reaction products were measured and the momentum distribution of the recoil nucleus was determined for transitions leading to residual nuclei in the ground and excited states. Results were analysed in terms of a simplified distorted-wave impulse approximation using cluster-model and three-body wave functions. The observed momentum distribution of the p-n pair in the p-shell of ⁶Li is in agreement with three-body calculations, while the spectroscopic factor is larger than predicted by theory. Transitions to breakup states of the α-particle also have the characteristics of quasi-free scattering on deuteron clusters.