Formation of periodic surface structures by ultrashort laser pulses

The formation of periodic surface structures by ultrashort laser pulses was observed experimentally and explained theoretically. The experiments were performed on graphite with picosecond laser pulses. The spatial period of the structures is of the order of the wavelength of the incident radiation, and the orientation of the structures is correlated with the direction of polarization of the light. The key point of the theoretical model proposed is resonance excitation of surface electromagnetic waves, which under conditions such that the temperature of the electronic subsystem is decoupled from the temperature of the crystal lattice causes a “temperature grating” to be written on the flat solid surface of the sample while the laser pulse is being applied on account of the temperature dependence of the surface impedance. The formation of a periodic surface profile from the temperature grating occurs by the volume expansion of a melted layer near the surface of the material. For typical values of the surface tension and viscosity for metals, there is not enough time for the periodic profile to be resorbed before the liquid layer solidifies. The formation of periodic surface structures is delayed in time relative to the laser pulse. Zh. éksp. Teor. Fiz. 115, 675–688 (February 1999)     

Effects of nanostructure-covered femtosecond laser-induced periodic surface structures on optical absorptance of metals

In this paper, we find, for the first time, that optical absorptance of metals can be significantly enhanced by a new type of surface structures following femtosecond laser ablation, namely nanostructure-covered periodic surface structures. Especially, the effect of the nanostructure-covered periodic structures on optical absorptance of metals has a clear polarization dependence that suggests a more controllable way to modify material optical properties with femtosecond laser processing. PACS 81.40.Wx; 78.20.Ci; 81.07.-b; 61.80.-x     

Propagation of optical pulses in periodic nonlinear fibers

We study the conditions of formation and propagation of soliton pulses in a periodic two-mode nonlinear fiber with allowance for dispersion of the fiber material and intermode dispersion of interacting modes under the condition of their phase synchronism. State University, Ul’yanovsk, Russia. Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Radiofizika, Vol. 41, No. 8, pp. 1032–1042, August, 1998.     

Dynamics of optical pulses in periodic nonlinear fibers

Dynamics of a two-mode wave packet with strong linear and nonlinear (cross-modulation) coupling is investigated. The effect of the initial conditions of the pulse excitation on its further transformation is considered. The possibility to control the dispersion parameters of the wave packet by varying the initial conditions of its input is pointed out. The effective parameters of the dispersion and nonlinearity that govern the dynamics of an optical pulse in a periodic nonlinear fiber light guide are obtained.     

Laser-induced periodic surface structures on different poly-carbonate films

Laser-induced periodic surface structures (LIPSS) were generated on oriented and amorphous thick, as well as on spin-coated thin, poly-carbonate films by polarized ArF excimer laser light. The influence of the film structure and thickness on the LIPSS formation was demonstrated. Below a critical thickness of the spin-coated films the line-shaped structures transformed into droplets. This droplet formation was explained by the laser-induced melting across the whole film thickness and subsequent de-wetting on the substrate. The thickness of the layer melted by laser illumination was computed by a heat-conduction model. Very good agreement with the critical thickness for spin-coated films was found. The original polymer film structure influences the index of refraction of the thin upper layer modified by the laser treatment, as was proven by the dependence of the structure’s period on the angle of incidence both for ‘s’- and ‘p’-polarized beams. The effect of the original surface roughness – grains in thick films or holes in thin films – was studied using atomic force microscopy. It was shown that the oblique incidence of ‘s’-polarized beams results in an intensity confinement in the direction of the forward scattering and in asymmetrical interference pattern formation around these irregularities. A new, two-dimensional grating-like structure was generated on spin-coated films. These gratings might be used as a special kind of mask. Received: 10 July 2001 / Accepted: 23 July 2001 / Published online: 30 August 2001     

Erasable holographic recording in photosensitive polymer optical fibers

We report what is to our best knowledge the first holographic recording in photosensitive polymer optical fibers by guided beams. The fibers are made of poly(methyl methacrylate) doped with Disperse Red 1 dye. We also demonstrate what we believe is the first recording of Fourier-transform images in these fibers.     

Femtosecond laser induced periodic large-scale surface structures on metals

The periodic ripple structures on wolfram and titanium surfaces are induced experimentally by linear polarized femtosecond laser pulses at small incident angles. The structural features show a material difference in the s- and p-polarized laser irradiation. The interspace between the ripples increases significantly for p-polarized laser irradiation when it exceeds a threshold angle, and the ripples' periodicities are larger than the wavelength of the incident p-polarized femtosecond laser; however, no significant change in the period of the ripples is observed with increasing incident angle for s-polarized laser irradiation. To explain these phenomena we propose a resonant absorption mechanism, by which the experimental observations can be interpreted.     

Electrostrictive cross-phase modulation of periodic pulse trains in optical fibers

Electrostriction-induced cross-phase modulation between subsequent bits of a nonreturn-to-zero pulse train in optical fibers leads to nonlinear frequency shifts of opposite sign for the 1's and the 0's. Direct experimental measurements of the electrostrictive and Kerr-induced nonlinear phase shift across the bit profiles agree well with the theoretical modeling.     

Study of optical properties of electrospun light-emitting polymer fibers

We realize light-emitting polymer fibers based on both optically inert polymers doped by molecules exhibiting optical gain and optically active conjugated polymers. Waveguiding properties of the produced polymer structures are demonstrated, with a loss coefficient of around 10³ cm⁻¹. We also find that single polymer fibers doped with gain molecules form Fabry–Pérot cavities, showing photoluminescence spectra with modes equally spaced by 1.7 nm. Coherent emission is demonstrated from fibers made upon increasing the excitation fluence above threshold values of the order of a few tens of μJ/cm².     

The energy of periodic surface structures in ferromagnetism

The periodic domain structures on unfavourably oriented surface layers of ferromagnetic materials were studied both experimentally and theoretically. The connection between the surface structure and the crystallographic orientation of the crystals was confirmed. All the terms contributing to the total energy of the surface layer were calculated. A general solution of the potential problem is given for arbitrary periodic distribution of the charges.

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Femtosecond pulsed laser-induced periodic surface structures on GaN/sapphire

Femtosecond pulsed laser-induced periodic surface structure on GaN/sapphire is reported in this paper. It was found that the period of the laser-induced ripples was much dependent on the incident laser fluence. Through finely adjusting laser fluence and pulse number, uniform ripples could be formed on the sapphire surface. We attributed the formation of such periodic two-dimensional structures to optical interference of the incident laser light with scattered waves from a surface disturbance. Also, it was found that the GaN capping layer played a very important role in forming the periodic structures on the sapphire surface.     

Sensing ammonia with ferrocene-based polymer coated tapered optical fibers

Abstract

The application of ferrocene-based polymers as variable index materials is discussed. The refractive index of thin film of a particular polymer known as poly(methylphenylsilyeneferrocenylene) is examined during exposure to ammonia, nitrous oxide, nitric oxide, nitrogen, carbon dioxide, carbon monoxide, and argon. A maximum of 9% deviation in the refractive index of the polymer upon exposure to ammonia is observed. The theory of operation and fabrication of polymer-coated tapered optical fiber gas sensors are explained. Experimental data is presented showing qualitative response to ammonia and other gases.     

Sensing ammonia with ferrocene-based polymer coated tapered optical fibers

The application of ferrocene-based polymers as variable index materials is discussed. The refractive index of thin film of a particular polymer known as poly(methylphenylsilyeneferrocenylene) is examined during exposure to ammonia, nitrous oxide, nitric oxide, nitrogen, carbon dioxide, carbon monoxide, and argon. A maximum of 9% deviation in the refractive index of the polymer upon exposure to ammonia is observed. The theory of operation and fabrication of polymer-coated tapered optical fiber gas sensors are explained. Experimental data is presented showing qualitative response to ammonia and other gases.     

超短脉冲激光诱导周期性表面结构

激光诱导周期性表面结构（Laser-induced periodic surface structures,LIPSS）具有纳米尺度的特征结构和自重复的微观尺度的排列图案,因此,LIPSS在传感器、太阳能发电、光催化等方面具有广泛的应用前景。本文首先介绍LIPSS形成过程中超快激光与物质相互作用的复杂过程,强调瞬态光学性质和表面结构变化的作用。然后综述几种具有代表性的LIPSS形成机理,并且讨论了各自的优缺点。接着介绍了LIPSS形成过程中材料的变化,主要包括材料化学成分、晶体结构和表面微观结构的变化。最后综述了LIPSS在材料表面处理、光学和机械等方面的应用。     

Dispersion relations for optical waves in amplifying periodic structures

The characteristics of optical waves in amplifying dielectric periodic nanostructures are studied. The formula for the dependence of the wave number on frequency, which comprises a photonic band gap and is valid for structures possessing a complex dielectric function, is obtained. It is shown that the gain is anomalously high at frequencies residing in the photonic band gap.     

Ultrafast time-resolved imaging of femtosecond laser-induced periodic surface structures on GaAs

We report the formation dynamics of periodic ripples on Ga As induced by femtosecond laser pulses（800 nm, 50 fs） via a collinear time-resolved imaging technique with a temporal resolution of 1 ps and a spatial resolution of 440 nm. The onset of periodic ripples emerges in the initial tens of picoseconds in the timescale of material ejection. The periodic ripples appear after irradiation of at least two pump pulses at surface defects produced by the first pulse and the ripple positions kept stable until the formation processes complete. The formation mechanisms of laser-induced periodic ripples are also discussed.     

Classical simulation of relativistic quantum mechanics in periodic optical structures

Spatial and/or temporal propagation of light waves in periodic optical structures offers a unique possibility to realize in a purely classical setting the optical analogues of a wide variety of quantum phenomena rooted in relativistic wave equations. In this work a brief overview of a few optical analogues of relativistic quantum phenomena, based either on spatial light transport in engineered photonic lattices or on temporal pulse propagation in Bragg grating structures, is presented. Examples include spatial and temporal photonic analogues of the Zitterbewegung of a relativistic electron, Klein tunneling, vacuum decay and pair production, the Dirac oscillator, the relativistic Kronig–Penney model, and optical realizations of non-Hermitian extensions of relativistic wave equations.     

Spectral properties of asymmetrical optical directional couplers with periodic structures

A comparison is made of co- and contradirectional couplers with periodic structures, with a view to their suitability as WDM devices for integrated optical systems. Expressions are obtained for the spectral response within the framework of a coupled-mode theory. It is shown that the competition between direct Bragg, Bragg-exchange and codirectional coupling in the contradirectional coupler leads to shifting and constriction of the stop bands. Calculations are made for a codirectional coupler with a new type of meander structure and for the contradirectional coupler.     

Formation of subwavelength periodic structures on tungsten induced by ultrashort laser pulses

The evolution of surface morphology of tungsten irradiated by single-beam femtosecond laser pulses is investigated. Ripplelike periodic structures have been observed. The period of these ripples does not show a simple relation to the wavelength and angle of incidence. The orientation of ripples is aligned perpendicularly to the direction of polarization for linearly polarized light. Surprisingly, we find that the alignment of the ripple structure turned left or right by 45 degrees with respect to the incident plane when using right and left circularly polarized light, respectively. The period of the ripple can be controlled by the pulse energy, the number of pulses, and the incident angle. We find a clear threshold for the formation as a function of pulse energy and number of pulses. The mechanism for the ripple formation is discussed, as well as potential applications in large-area structuring of metals.