基于DBD 悬浮电极低温等离子体杀菌消毒仪研制

基于介质阻挡放电(DBD)原理,研究设计了一种悬浮电极式的低温等离子体发生设备,产生的等离子体温度较低且对人体安全,可直接接触。用所研制的低温等离子体发生设备对大肠杆菌做了灭活实验,实验结果表明,该设备产生的低温等离子体对大肠杆菌作用10s 以上,在等离子体有效作用区内大肠杆菌杀灭率为100%,表明所研制的低温等离子体发生设备具有很好的杀菌消毒效果。     

同轴式DBD分解NO/N_2混合气的光谱研究

本文建立了大气压介质阻挡放电发射光谱测量系统,测得NO/N_2体系的等离子体发射光谱。利用Q-V Lissajous图形法对反应器电学参量进行测试,研究激励电压峰峰值V_（P-P）对NO、N_2各激发态物种光谱强度的影响。实验结果表明：低温等离子体产生的高能电子可有效作用于NO、N-2分子,产生NO（A~2∑~＋→X~...     

电荷电压法测量DBD等离子体的放电参量

在DBD应用研究中，使用电荷电压法能够测量许多重要参量，如放电功率、放电间隙等效电容、电介质层等效电容、着火电压、放电间隙等效电压及放电间隙电场强度等．同时根据电荷电压图形随工作条件及状态变化的情况还可以诊断DBD等离子体的工作稳定性．文章对相关原理、模拟实验结果及实际应用效果进行了介绍．     

双模式放电中DBD放电参数对甲烷滑动弧火焰光谱及活性粒子的影响分析

对未燃烧的可燃混合气体进行DBD放电,放电后会产生大量的活性粒子,这些活性粒子可以辅助气体燃烧,达到提高燃料燃烧利用率等目的。以DBD激励氩气、甲烷、空气产生的自由基（CH基和OH基）等强化燃烧的关键活性粒子为探索对象,研究DBD放电激励甲烷对滑动弧火焰的影响。为此,采用自主设计的DBD-滑动弧双模式等离子体激励器,利用同轴介质阻挡放电结构对氩气、甲烷、空气混合气进行放电激励,将激励后的氩气、甲烷、空气混合气通入滑动弧端进行点火。固定氩气流量不变,调整空气流量为4.76 L·min-1,并加入甲烷0.5 L·min-1,保证进气通道内氩气与空气-甲烷的气体体积流量比达到Ar∶（CH₄+Air）=1∶30,其中空气、甲烷这两种气体达到了化学燃烧当量比φ=1,氩气、甲烷、甲烷混合气体能实现均匀而稳定的放电并燃烧。DBD段放电电压在15～20 kV范围变化,放电频率在6～10 kHz范围变化,滑动弧段的电压和频率分别保持4 kV与10 kHz恒定,通过改变DBD段放电电压和放电频率,用高速光纤光谱仪检测滑动弧火焰中自由基种类及其光谱强度,分析放电参数激励甲烷对火焰中自由基（CH基和OH基）的影响。结果表明,DBD段放电电压及放电频率的增加可以促进火焰内部的偶联反应发生,可有效提升甲烷滑动弧火焰内部的活性粒子含量,其中OH基团、CH基团在燃烧链式化学反应进程中发挥着较为重要的作用。甲烷经过DBD激励后,随放电电压和频率的增加,火焰中OH基、CH基等主要活性粒子都随之增加。DBD放电后,活性粒子的光谱强度增大,特征谱线比单模式更加明显;甲烷经过DBD激励后,火焰组成发生了变化,滑动弧段出口处甲烷燃烧反应更加充分,火焰温度越高越容易产生OH基。与单模式滑动弧相比,双模式放电可有效促进火焰内部的链式化学反应进程,促进燃料燃烧。     

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分别采用空气、氩气大气压介质阻挡放电(DBD)等离子体对重油进行了处理.对经空气DBD等离子体处理后的重油进行粘温特性分析,发现重油粘度升高,流动性变差.红外光谱和四组分分析结果表明重油的重质组分含量升高,重油胶体体系被破坏,同时生成大量刺激性气味气体.为了便于分析气态产物的成分和含量,采用大气压氩气DBD等离子体处理重油并收集气体产物.气相色谱分析发现生成气中含有大量C1-C5的烃类和一定量氢气,其中氢气和甲烷含量占生成气的70％以上.实验结果表明重油在等离子体作用下既发生裂解又发生聚合反应,既生成低碳烃类,本身的流动性也变差.     

大气压Ar／NH3介质阻挡辉光放电的仿真研究

为了研究火气压下氩气（Ar）中掺杂氨气（NH3）的Ar／NH3介质阻挡辉光放电的放电机理,通过建立一‘个多粒子的自洽耦合流体模型,采用有限元方法进行数值计算,得到了气体间隙压降、介质表面电荷密度、放电电流密度随时间的周期变化波形,以及带电粒子、中性粒子与空间电场强度的时空分布．仿真计算结果表明：气体间隙的周期击穿过程主要由气隙电压控制,并受气隙两侧介质极板上积聚的表面电荷的影响．气隙间带电粒子密度和电场强度的时空分布表明本文的放电过程存在阴极位降区、负辉区、法拉第暗区、等离子体正柱区等辉光放电的典型区域,放电模式为大气压辉光放电．在Ar/NH3等离子体中,主要的正离子为NH＋,其次为Ar2＋,主要的负离子为NHi：NH3分解产生的主要的激发态分子为NH,NH2和N2H3,而最终的稳态产物主要是N2和H2．     

低温等离子体分解N2/O2/NO气氛中NO试验研究

利用自行设计的介质阻挡放电型低温等离子体反应器,研究了NO初始浓度、O₂初始浓度、放电功率、电源频率等因素对NTP转化N₂/O₂/NO气氛中NO的影响规律。研究发现,NO去除率随功率增大而升高,到达一最大值后随功率增大而降低;NO去除率随O₂初始浓度增加而降低,随NO初始浓度增大而减小。相同放电功率下,同一组分中NO去除率随电源频率的增加而降低,因此相同放电功率下降低电源频率可提高NO去除率。O₂初始浓度不高于5%时,NO_x大部分为NO,NO₂和O₃浓度均随放电功率增大而降低,NO₂、O₃生成量随O₂初始浓度升高而增多。     

光谱学方法研究介质阻挡沿面放电辉光模式的电场分布

利用介质阻挡沿面放电装置,在低气压空气中实现了辉光放电模式。利用光电倍增管对放电发光信号进行检测,发现外加电压每半周期出现一个发光脉冲,并且正负半周期的光脉冲是不对称的。利用Photoshop软件处理放电的照片,研究发现平行于高压电极不同位置的发光强度基本相同,然而距离高压电极越远,发光强度减小。放电中总电场由外加电场和电介质积累的壁电荷电场共同决定,确定该电场具有重要意义。通过分析放电的发射光谱中N+₂(B 2Σ+_u→X 2Σ+_g)谱线391.4 nm和N₂的第二正带系(C 3Π_u→B 3Π_g)谱线337.1 nm的比值,可以定性地说明电场的分布。研究发现电场在高压电极附近较大而远离高压电极处较小。这些研究结果对沿面放电的数值模拟和工业应用具有重要的价值。     

常压窄间隙介质阻挡放电等离子体辐射特性

利用带有透明电极与可测向观察的一个介质阻挡放电(DBD)实验装置对它的常压窄间隙等离子体辐射特性进行了实验研究。结果表明：这一DBD装置的辐射特性会受激励电压、激励频率、DBD结构等多种因素影响。在频率为10～20kHz高压电源激励下,采用窄间隙、薄电介质层结构DBD可以大幅度提高放电空间的电场强度,增加放电功率密度,提高了放电装置性能。     

针-板DBD微流注与微辉光交替生成的机理研究

在介质阻挡放电体系中产生辉光放电可以有效的提高放电体系产生高能电子的性能, 为等离子体化学反应提供更加丰富的活性粒子.本文对针-板介质阻挡放电体系下的放电模式进行了研究,实验发现放电正负半周期表现出不同的放电模式, 激励电压为3 kV时放电正负半周期分别为微流注放电和电晕放电(或者Trichel脉冲放电),激励电压为6 kV时放电正负半周期分别为微流注放电和微辉光放电.微辉光放电形貌具有与典型辉光放电相同的分层次放电结构, 分析了激励电压6 kV时的放电过程,认为足够强的阴极电场强度和裸露针状电极形成的有效的二次电子发射过程是形成微辉光放电的主要因素,绝缘介质层的存在避免了微辉光放电向弧光放电过渡.     

Availability of indirect atmospheric plasma from a dielectric barrier discharge device on biofilm-forming bacteria

An investigation of the treatment effect of atmospheric cold plasma (ACP)-generated reactive oxygen species (ROS) against problematic bacteria of chronic wounds is presented. To study ROS effects specifically, a vacuum chamber with a flowmeter to control the background gas composition and a mesh electrode for a dielectric barrier discharge (DBD) device were used. In addition, a numerical modeling was developed to simulate the amount of ROS flux transported from the mesh electrode to determine which of the ROS species was the main factor in the treatment effect. Considering the experimental and computational results and the effective transport distance of each species, ozone could be the main factor in the experimental results.     

Properties of surface dielectric barrier discharge plasma generator for fabrication of nanomaterials

This paper presents surface dielectric barrier discharge plasma generators as an efficient source of low-energy ions. Either positive or negative ions can be extracted from a plasma cloud with an external DC field created by the third electrode. Three different cross-section geometries of DBD generators were analyzed, simulated and fabricated. Currents of ions extracted from the plasma cloud were measured and the results were discussed. It was demonstrated that if the third electrode consists of liquid–gas interface, the presented arrangement can be used as a versatile reactor for nanomaterial synthesis (on the example of the synthesis of silver nanoparticles).     

Neutralization of charged dielectric materials using a dielectric barrier discharge

Safety and efficiency are two characteristics that must be satisfied by an electric charge neutralizer. The dielectric barrier discharge (DBD), which has the advantage of preventing arc transition, is an interesting tool to safely neutralize unwanted charge. This paper is aimed at studying the efficiency of neutralizing charged polyethylene (PE) granules by using a dielectric barrier discharge. During this study, several factors were considered such as the amplitude and the frequency of the AC voltage, the polarity and the charging mode of the samples, as well as the electrode configuration. Two DBD electrode configurations were considered: simple DBD and a DBD with installed metallic grid. The obtained results show that using the DBD can lead to excellent neutralization results when the grid is installed. With the appropriate voltage amplitude and frequency and with grid installed, the elimination of nearly 99% of the initial surface charges can be achieved. The metallic grid placed between the DBD electrode and the target enhances significantly the neutralization efficiency.     

平面激光诱导荧光技术在交错电极介质阻挡放电等离子体研究中的初步应用

利用平面激光诱导荧光技术对交错电极介质阻挡放电过程中产生的痕量组分NO进行了检测. 通过数值模拟对实验结果进行了分析说明,并对介质阻挡放电等离子体流动控制原理进行了简要分析. 此外还通过平面激光诱导荧光技术对等离子体诱导流动进行了直观显示. 关键词： 平面激光诱导荧光 等离子体 介质阻挡放电     

Characteristics of parallel-plate and planar-surface dielectric barrier discharge at atmospheric pressure

Experiments are performed to investigate and compare the characteristics of stable parallel-plate and planar-surface dielectric barrier discharge in helium gas at atmospheric pressure. The evolution of applied electric field profile and the discharge initiation processes are found quite different for both electrode geometries. Further discharge voltage, discharge current, power densities etc. are compared. The differences of basic plasma properties are presented for both the electrode configurations.     

Study on the transition from filamentary discharge to diffuse discharge by using a dielectric barrier surface discharge device

Discharge characteristics have been investigated in different gases under different pressures using a dielectric barrier surface discharge device. Electrical measurements and optical emission spectroscopy are used to study the discharge, and the results obtained show that the discharges in atmospheric pressure helium and in low-pressure air are diffuse, while that in high-pressure air is filamentary. With decreasing pressure, the discharge in air can transit from filamentary to diffuse one. The results also indicate that corona discharge around the stripe electrode is important for the diffuse discharge. The spectral intensity of N电介质 表面放电 扩散放电 发射光谱学dielectric barrier surface discharge, diffuse discharge, optical emission spectroscopyProject supported by the National Natural Science Foundation of China (Grant Nos 10575027 and 10647123), the National Science Foundation of Hebei Province, China (Grant No A2007000134), the Education Department of Hebei Province, China (Grant No 2006106),2006-10-24Discharge characteristics have been investigated in different gases under different pressures using a dielectric barrier surface discharge device. Electrical measurements and optical emission spectroscopy are used to study the discharge, and the results obtained show that the discharges in atmospheric pressure helium and in low-pressure air are diffuse, while that in high-pressure air is filamentary. With decreasing pressure, the discharge in air can transit from filamentary to diffuse one. The results also indicate that corona discharge around the stripe electrode is important for the diffuse discharge. The spectral intensity of N＋ （391.4nm） relative to N2 （337.1 nm） is measured during the transition from diffuse to filamentary discharge. It is shown that relative spectral intensity increases during the discharge transition. This phenomenon implies that the averaged electron energy in diffuse discharge is higher than that in the filamentary discharge.