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针对一般光纤荧光传感器收集荧光能力不足的缺陷,设计了一种在微结构聚合物光纤的空气孔内填充掺有机染料高折射率液体的荧光传感器.使用可调节边界条件傅里叶分解法计算了这种微结构光纤的模场分布,分析了光纤结构参量和液体折射率对荧光捕获分数的影响,结果表明,使用小纤芯半径和高于纤芯折射率的液体可以增强激发光的吸收效率,增大荧光捕获分数,提高光纤荧光传感器的灵敏度. 相似文献
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针对一般光纤荧光传感器收集荧光能力不足的缺陷,设计了一种在微结构聚合物光纤的空气孔内填充掺有机染料高折射率液体的荧光传感器.使用可调节边界条件傅里叶分解法计算了这种微结构光纤的模场分布,分析了光纤结构参量和液体折射率对荧光捕获分数的影响,结果表明,使用小纤芯半径和高于纤芯折射率的液体可以增强激发光的吸收效率,增大荧光捕... 相似文献
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SO2气体激光诱导色散荧光时间断层扫描研究 总被引:2,自引:0,他引:2
以纳秒Nd:YAG激光器的四倍频(266 nm)为激发源,利用门选通增强光学多通道光谱分析仪 (OMA),研究了SO2分子第一激发带粒子的荧光辐射与碰撞弛豫相结合的复杂退激发过程。通过对SO2分子第一激发带的激发及碰撞弛豫过程的时间断层扫描分析,可以将激光诱导色散荧光谱中以305.6 nm、337.2 nm为中心的荧光包络和以424.7 nm为中心的规则序列分别归属于B1B1、A1A2低振动能级和a3B1基振动能级到基电子态X1A1不同振动能级的荧光跃迁,由此可以确定大气污染气体SO2的诱导荧光的灵敏检测波长为425 nm;由规则序列的实验数据可以计算出SO2分子基电子态X1A1的对称振动和弯曲振动模式的基振动角频率分别为ω1= 1151.8±0.6 cm-1和ω2= 517.8±0.6 cm-1,两振动模式的非谐性常数分别为 = 8±0.6 cm-1和 = 9.2±0.6 cm-1。 相似文献
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针对植物荧光遥感探测中信号易受干扰的问题, 提出了一种用于评估植物生长状况及环境监测的荧光寿命成像技术. 采用凹透镜对355 nm波长的激光扩束, 再照射植物激发叶绿素荧光, 由增强型电荷耦合器件接收荧光信号. 采用时间分辨测量法, 连续用相同激光脉冲照射植物以激发相同的荧光信号, 同时不断改变激光脉冲触发探测器启动的延时时间, 从而能够得到完整的离散荧光信号分布图像. 对植物特定位置点产生的离散荧光信号进行拟合, 再运用一种改进型的迭代解卷积法可反演高精度的荧光寿命; 进而反演图像各点的荧光寿命以生成植物的荧光寿命分布图. 该方法所绘制的荧光寿命图比荧光强度图能更准确地反映植物内部的叶绿素含量, 并对活体植物叶绿素荧光寿命的物理特性进行了初步研究, 证明叶绿素荧光寿命与植物生理状态存在一定关联; 并且叶绿素荧光寿命与活体植物所处环境存在着复杂的关系. 未来将与生物物理学家们合作, 继续探寻叶绿素荧光寿命与植物生存环境的关系. 相似文献
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Sanyalak Niratisairak
yvind Haugen Tom H. Johansen Takayuki Ishibashi 《Physica C: Superconductivity and its Applications》2008,468(6):442-446
Hotspot formation is observed in a structured thin superconducting film of Bi2Sr2CaCu2Ox (BSCCO) using the fluorescent thermal imaging technique. The BSCCO film is deposited on SrTiO3 (STO) and has a superconducting transition at 80 K. A film of rare-earth doped polymer film deposited directly on the superconductor is used as thermal sensor down to 4 K. 相似文献
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X-ray diffraction using a coherent beam involves the mutual interference among all the extremities of small crystals. The continuous diffraction pattern so produced can be phased because it can be oversampled. We have thus obtained three-dimensional images of the interiors of Au nanocrystals that show 50 nm wide bands of contrast with [111] orientation that probably arise from internal twinning by dynamic recrystallization during their formation at high temperature. 相似文献
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Based on the solutions of apparent heat capacity method for phase-change problems, numerical simulations were performed to study the heat-storage and release processes for the multi-cavity-structured phase-change microcapsules in this paper. Moreover, the influence of the cavity structures of the phase-change microcapsules on the heat-storage and release capacity was analyzed. The results show that the rate of heat-storage and release will be accelerated by increasing the number of cavities in microcapsules, and cavity interlayer is the key factor to enhance the heat transfer. 相似文献
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Péter Reischig Lukas Helfen Arie Wallert Tilo Baumbach Joris Dik 《Applied Physics A: Materials Science & Processing》2013,111(4):983-995
The characterisation of the microstructure and micromechanical behaviour of paint is key to a range of problems related to the conservation or technical art history of paintings. Synchrotron-based X-ray laminography is demonstrated in this paper to image the local sub-surface microstructure in paintings in a non-invasive and non-destructive way. Based on absorption and phase contrast, the method can provide high-resolution 3D maps of the paint stratigraphy, including the substrate, and visualise small features, such as pigment particles, voids, cracks, wood cells, canvas fibres etc. Reconstructions may be indicative of local density or chemical composition due to increased attenuation of X-rays by elements of higher atomic number. The paint layers and their interfaces can be distinguished via variations in morphology or composition. Results of feasibility tests on a painting mockup (oak panel, chalk ground, vermilion and lead white paint) are shown, where lateral and depth resolution of up to a few micrometres is demonstrated. The method is well adapted to study the temporal evolution of the stratigraphy in test specimens and offers an alternative to destructive sampling of original works of art. 相似文献
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We show that the position of a fluorescent nanoparticle can be measured in three dimensions with subnanometer precision and 100-ms temporal resolution by use of standard epifluorescence video imaging in off-focus mode. The particle can be tracked without feedback in a volume of at least 40 microm x 60 microm x 3 microm. With the technique presented, the structure-mobility relationship of 216-nm latex particle in a porous polymer network was studied in three dimensions. 相似文献
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Daniil N. Bratashov Admir Masic Alexey M. Yashchenok Matthieu F. Bedard Olga A. Inozemtseva Dmitry A. Gorin Tamara Basova Torsten K. Sievers Gleb B. Sukhorukov Mathias Winterhalter Helmuth Mhwald Andre G. Skirtach 《Journal of Raman spectroscopy : JRS》2011,42(10):1901-1907
We present the results of using Raman molecular imaging and atomic force microscopy (AFM) investigation of the composition, stability, and photodegradation of polyelectrolyte multilayer microcapsules and coated microparticles containing copper–phthalocyanine and iron–phthalocyanine. The influence of laser light on degradation of these phthalocyanine dyes embedded in the walls of polyelectrolyte multilayer capsules and shells of microparticles was studied by both AFM and Raman molecular imaging, but only the latter technique gave information on dynamics of photodegradation. Raman peak assignment was performed according to theoretical calculations. The degradation rate of phthalocyanine dyes is estimated from Raman signal measurements and a model is proposed to account for the degradation rate. Practical applications of our approach are outlined. Copyright © 2011 John Wiley & Sons, Ltd. 相似文献
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Biofunctionalization and manipulating of carbon nanotubes (CNTs) is important for biomedical research and application. Cy5 labeled goat anti-rabbit IgG (anti-IgG-Cy5) is chemically bonded to CNTs via a two-step process of diimide-activated amidation. This process can avoid the intermolecular connection of proteins. Fluorescent imaging of CNTs in aqueous solution has been demonstrated using anti-IgG-Cy5 immobilized CNTs (IgG-CNTs) as the model. The biologically functionalized carbon nanotubes (f-CNTs) in solution have been observed successfully using fluorescence microscopy. The fluorescent image of highly oriented f-CNTs is obtained at first time. The influencing factors on fluorescent imaging including oxidation duration, background noise and reactant concentration are discussed. 相似文献
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High-resolution bone microstructure imaging based on ultrasonic frequency-domain full-waveform inversion 下载免费PDF全文
The main challenge in bone ultrasound imaging is the large acoustic impedance contrast and sound velocity differences between the bone and surrounding soft tissue. It is difficult for conventional pulse-echo modalities to give accurate ultrasound images for irregular bone boundaries and microstructures using uniform sound velocity assumption rather than getting a prior knowledge of sound speed. To overcome these limitations, this paper proposed a frequency-domain fullwaveform inversion(FDFWI) algorithm for bone quantitative imaging utilizing ultrasonic computed tomography(USCT).The forward model was calculated in the frequency domain by solving the full-wave equation. The inverse problem was solved iteratively from low to high discrete frequency components via minimizing a cost function between the modeled and measured data. A quasi-Newton method called the limited-memory Broyden–Fletcher–Goldfarb–Shanno algorithm(L-BFGS) was utilized in the optimization process. Then, bone images were obtained based on the estimation of the velocity and density. The performance of the proposed method was verified by numerical examples, from tubular bone phantom to single distal fibula model, and finally with a distal tibia-fibula pair model. Compared with the high-resolution peripheral quantitative computed tomography(HR-p QCT), the proposed FDFWI can also clearly and accurately presented the wavelength scaled pores and trabeculae in bone images. The results proved that the FDFWI is capable of reconstructing high-resolution ultrasound bone images with sub-millimeter resolution. The parametric bone images may have the potential for the diagnosis of bone disease. 相似文献
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W. Hartig W. Rasmussen R. Schieder H. Walther 《Zeitschrift für Physik A Hadrons and Nuclei》1976,278(3):205-210
The frequency distribution of the fluorescent light induced by monochromatic dye laser radiation was investigated. To exclude the influence of the Doppler width a strongly collimated atomic beam was used. The spectrum was measured by means of a piezoelectrically tunable spherical Fabry Perot. The interaction region between the laser light and the atomic beam was placed into the center of the interferometer. Thus the observed fluorescence spectrum was considerably more intense than in the case where the interferometer is used separately from the beam. The fluorescence spectrum was observed for different directions of polarization of the incident laser beam. In the case of weak excitation the spectrum consists of a sharp component essentially due to elastically scattered light. At high intensities a structure of three components is observed which is in agreement with theoretical predictions when circularly polarized light is used for excitation. 相似文献
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W. Hartig W. Rasmussen R. Schieder H. Walther 《Zeitschrift für Physik A Hadrons and Nuclei》1976,71(6):205-210
The frequency distribution of the fluorescent light induced by monochromatic dye laser radiation was investigated. To exclude the influence of the Doppler width a strongly collimated atomic beam was used. The spectrum was measured by means of a piezoelectrically tunable spherical Fabry Perot. The interaction region between the laser light and the atomic beam was placed into the center of the interferometer. Thus the observed fluorescence spectrum was considerably more intense than in the case where the interferometer is used separately from the beam. The fluorescence spectrum was observed for different directions of polarization of the incident laser beam. In the case of weak excitation the spectrum consists of a sharp component essentially due to elastically scattered light. At high intensities a structure of three components is observed which is in agreement with theoretical predictions when circularly polarized light is used for excitation. 相似文献