奇A核Pd同位素中h_(11/2)入侵轨道的形状驱动效应研究

过渡区原子核的形变与准粒子占据的轨道密切相关。采用推转壳模型首次系统性地研究了奇A核~(99)Pd,~(101)Pd和~(103)Pd原子核中h_(11/2)轨道对核芯的形状驱动效应,基于Total-Routhian-Surface(TRS)方法的计算结果表明,当过渡区原子核~(99)Pd,~(101)Pd和~(103)Pd中的准粒子开始占据h_(11/2)入侵轨道时将会使原子核产生稳定的四极形变。另外,对A≈210质量区近滴线核的高自旋态研究现状及今后进一步的工作也进行了概述。     

Phase transition in odd-N Pd-isotopes

Phase transition in odd-N isotopes99,101,103 Pd are investigated via the E-GOS(E-Gamma Over Spin)curves, which strongly suggest a structure evolution from vibration to rotation along the yrast lines with increasing spin. Theoretical calculations have been performed for the ground state bands of99,101,103 Pd in the framework of the cranked shell model(CSM) and the alignment properties observed experimentally are analyzed employing this model. The results show that the phase transition in the ground state bands of99,101,103 Pd can be interpreted as the valence nucleons start to occupy the g9/2proton orbitals with increasing spin which would polarize the core to a small, but rigid quadrupole deformation.     

High-j proton alignments in 101Pd

High-spin states in ¹⁰¹Pd have been investigated by means of in-beam γ-ray spectroscopic techniques via the ⁷⁶Ge(²⁸Si, 3n) reaction at beam energies of 85 and 95 MeV. The previously known d _5/2 and 1/2^?[550] bands were extended to higher spins, and the unfavored signature branch of the 1/2^?[550] band was built. The band crossings observed experimentally are explained by the alignment of g _9/2 protons. The band properties in ¹⁰¹Pd are compared with those in the neighboring nuclei and are discussed within the framework of the cranked shell model (CSM).     

125Cs的能级结构

通过116Cd(14N,5n),Ebeam=65MeV的核反应布居了125Cs的高自旋态.利用在束γ谱学实验方法,进行了γ-γ符合测量,使已知的125Cs核能级纲图得到了扩展,并且修正了某些组态的带头激发能.High-spin states in odd-A nucleus~(125)Cs have been studied via the~(116)Cd(~(14)N, 5n) reaction at 65 MeV bombarding energy. γ-γ coincidences were recorded with the NORDBALL detector array at Niels Bohr Institute in Denmark. After careful data analysis, most of the previously-known bands have been confirmed and 5 new rotational sequences have been identified. Spin/parity and configuration assignments are tentatively proposed for all of the observed bands. In addition, the bandheads of the 9/2~(+)and (1/2~...     

A resonant photoemission study of the Ce and Ce-oxide/Pd(1 1 1) interfaces

We have investigated the Ce 4f electronic states in the Ce/Pd(1 1 1) and Ce-oxide/Pd(1 1 1) systems, using resonant photoemission (Ce 4d → 4f transitions), and XPS to understand Pd-Ce interactions in ultra thin layers of cerium and ceria deposited on Pd(1 1 1). Cerium deposited on Pd(1 1 1) at room temperature forms surface Ce-Pd alloys with Ce rich character, while a Pd rich Ce-Pd alloy is formed by heating to 700 °C. A modification of the chemical state of Ce can also be seen after oxygen exposure. RPES provides evidence that Ce-oxide layers deposited on Pd(1 1 1) have a CeO₂ (Ce⁴⁺) character, however a net contribution of the Ce³⁺ states is also revealed. The Ce³⁺ states have surface character and are accompanied by oxygen vacancies. Heating to 600 °C causes Ce-oxide reduction. A significant shift of Pd 4d-derived states, induced by Pd 4d and Ce 4f hybridization, was observed. The resonant features in the valence band corresponding to Ce⁴⁺, Ce³⁺ and Ce⁰ states have been investigated for various Pd−Ce(CeO_x) coverages.     

Projected shell model study of yrast bands in even-even 100–118Pd isotopes

The projected shell model (PSM) study of ^100?C118Pd nuclei is carried out. The reliability of the ground-state wave functions is checked by reproducing yrast spectra and electromagnetic properties. The results of calculations indicate that the observed deformation systematics in ^100?C118Pd isotopes depends on the increase of occupation probability of (1h _{11/2 ??} ) orbit and the deformation producing tendency of n-p interaction operating between Spin Orbit Partner (SOP) orbits (d _5/2)_???(d _3/2) _?? and (g _9/2)_???(g _7/2) _?? . Beside this, the results on band diagrams show that the yrast spectra in Pd isotopes do not arise from a single intrinsic state only but also from multi-quasiparticle states.     

Observation of signature inversion in the πh9/2(×)νi13/2 oblate band

High-spin states in 190Tl have been studied via the 160Gd(35Cl, 5nγ) reaction. The level scheme, consisting of the πh9/2(×)νi13/2 oblate band and a cascade with character of single particle excitations, has been established. Spin values have been firmly assigned to the oblate band in 190Tl, resulting in low-spin signature inversion in the πh9/2(×)νi13/2 oblate band for the first time. Based on the similarity of the level structure in doubly odd Tl nuclei, spin values for the oblate bands in 192―200Tl should be re-assigned, and a consistent low-spin signature inversion has occurred in these oblate deformed nuclei. The low-spin signature inversion phenomena can be interpreted qualitatively by using the 2-quasiparticle plus rotor model including p-n residual interactions.     

The electronic structure of polymeric complex Co(thiazole)2Cl2 studied by first-principle calculation

One-dimensional dihalide-bridged polymer Co(thiazole)₂Cl₂ has been studied with the self-consistent full-potential linearized augmented plane wave method (FP_LAPW) based on the density functional theory (DFT). Spin distributions in ferromagnetic and antiferromagnetic states of it have been obtained by the calculation. The electronic structure and magnetic coupling between tow cobalt (II) ions along chain are discussed.     

奇A核101Pd和101Ru的负宇称带能谱研究

将具有正宇称的gds组态空间扩大到包含具有负宇称的1h11/2轨道,采用修正的表面δ相互作用(MSDI)对101Pd和101Ru两个奇A核进行了形变HF计算,得到了基态和一些激发态的解.同时,还用近似角动量投影形变Hartree Fock(PDHF)方法对101Pd和101Ru进行了能谱计算,得到其正、负宇称带的解,计算结果与实验谱基本一致. Using modified delta interaction, enlarging the gds configuration space to include the 1h_11/2 orbital with negative parity, the deformed Hartree Fock calculations for both nuclei: 101Pd and 101Ru are performed. Their ground state and some excited configurations are obtained. The approximate angular momentum projected deform Hartree Fock (PDHF) method is also applied to nuclei 101Pd and 101Ru, and both of their positive and negative parity bands are obtained...     

Angular distribution measurements of gamma-rays from the22Ne(p, γ)23Na reaction

Angular distribution measurements of gamma-rays from the²²Ne(p, γ)²³Na reaction on theE _p =897, 1006, 1091 and 1278 keV resonances have been made. Spin and parity assignments for several bound states are presented together with multipole mixing ratios for transitions from resonance and bound states. The level at 6617 keV (7/2⁺) is proposed to be a member of the rotational band based on the Nilsson orbit 5(K ^π=5/2⁺).     

Optical orientation of donor-bound excitons in nanosized InP/InGaP islands

Spin splitting of optically active and inactive excitons in nanosized n-InP/InGaP islands has been revealed. Optically inactive states become manifest in polarized-luminescence spectra as a result of excitons being bound to neutral donors (or of the formation of the trion, a negatively charged exciton) in InP islands. The exchange-splitting energies of the optically active and inactive states have been determined. Fiz. Tverd. Tela (St. Petersburg) 40, 1745–1752 (September 1998)     

Specific features of the formation of phase states in a non-Heisenberg magnet with S = 2

Spin states of a non-Heisenberg magnet with a magnetic ion spin of 2 have been determined. It has been shown that the inclusion of the higher-order spin invariants leads to realization of specific phases with the tensor order parameters whose realization is impossible in magnets with S = 1. The free energy of the system in different spin states has been studied. The geometric images of the tensor phases in the spin space have been determined.     

The temperature dependence of the interaction of oxygen with Pd(111); A study by photoemission and auger spectroscopy

The temperature dependence of the different binding states of oxygen on Pd(111) has been studied using photoemission spectroscopy and Auger spectroscopy. By examining the oxygen 2s binding energies, three distinct states are observed, which are identified as surface chemisorbed oxygen, oxygen incorporated into the first Pd layer, and subsurface oxygen. Changes in the relative oxygen Auger peak heights for 1000 K exposure temperature are explained if the oxygen is assumed to become more negatively charged as it penetrates the Pd surface. A model for the interaction of oxygen with the Pd(111) surface is proposed.     

Angle-resolved photoemission study of Pd(111) and Co/Pd(111)

Electronic structure of epitaxial Co films on Pd(111) has been investigated as a function of the Co overlayer thickness, by using angle-resolved photoemission spectroscopy (ARPES). It is found that experimental band structures for Pd(111) and work functions for Co/Pd(111) agree reasonably well with the results of band structure calculations. Compared to Pd(111), valence band ARPES spectra of Co/Pd(111) support the existence of the induced magnetic polarization of Pd atoms near the interface, suggesting large hybridization between Co 3d and Pd 4d states near the interface.     

One-dimensional spin-polarized quantum-wire states in Au on Ni(110)

Au chain structures have been prepared on Ni(110). Au6 s,p-derived features in photoemission spectra are identified as quantum-wire states due to their strong dispersion along the chains and absence of dispersion perpendicular to the chains in agreement with our ab initio calculation of the electronic structure. Spin analysis reveals that the states have minority-spin character showing that the confinement of electrons in the chain structure depends on the electron spin.     

States in 53Mn from the 52Cr(p, γ)53Mn reaction

Eight resonances have been observed in the ⁵²Cr(p, γ)⁵³Mn reaction between E_p = 0.90 and 1.03 MeV. Gamma-ray spectra have been accumulated at four of the resonances. Spin assignments have been made to the resonant states on the basis of the measured angular distributions of primary γ-rays. Excitation energies and γ-ray branching ratios have been determined for 36 levels between 2.0 and 5.6 MeV. Mean lives for nine of the states have been extracted by the Doppler shift attenuation method.     

Influence of a heterogeneous Al2O3 surface on the electronic properties of single Pd atoms

Electronic properties of single Pd atoms, deposited on Al(2)O(3)/NiAl(110), have been characterized by scanning tunneling spectroscopy at 12 K. The spectra reveal distinct conductivity resonances, assigned to discrete electronic levels in the atom. The energy position of the resonances reflects adsorption properties of Pd atoms on different sites of the oxide support. Mapping the spatial extent of conductivity channels in the Pd atoms yields the symmetry of the underlying electronic states. The results demonstrate the effect of a heterogeneous oxide surface on the electronic structure of adsorbed metal atoms.     

Ab initio study of palladium and silicon carbide

Ab initio methods have been used to investigate the properties of Pd as impurity in bulk SiC at five charged states within the framework of density functional theory using the local spin density approximation. It was found that Pd interstitials and substitutionals have similar energy to their intrinsic counterparts. In addition, Pd substitutes for a vacancy, di-vacancy, and tri-vacancy with similar energies. Pd diffuses through SiC via an interstitial mechanism employing the tetrahedral sites and Pd can substitute for Si and C at positive charged states. Removing electrons (p-type doping) from SiC lowers the formation and migration energies of Pd defects in SiC for most configurations.     

126Cs的高自旋态能级结构

利用融合蒸发反应¹¹⁶Cd(¹⁴N,4n)¹²⁶Cs布居了¹²⁶Cs的高自旋态.观测到了100多条新的γ跃迁和相应的能级,建立了双奇核¹²⁶Cs由9个转动带构成的能级纲图.尝试性地指定了大部分能级的自旋和宇称以及各转动带的Nilsson单粒子组态.极大地丰富了已有的实验结果.     

New excited states of the nucleus129Xe

Excited states of¹²⁹Xe have been investigated through the¹²⁶Te(α,n)¹²⁹Xe reaction at the incident energy E=16MeV by means of in-beam gamma ray spectroscopy. Numerous levels below the excitation energy of 2.5MeV were found. Spin assignments were made from side feeding excitation functions. A new level at 274.2keV, which is suggested as spin 9/2 negtive parity bandhead, was observed for the first time.