Paramagnetic relaxation kinetics of the cation radical C 60 + in C60 powder

The kinetics of spin-lattice and phase relaxation of C ₆₀ ⁺ radicals in C₆₀ powder has been studied at room temperature by pulsed EPR. It is found that the kinetics can be described by the relation exp $( - a\sqrt t )$ characteristic of the case in which the paramagnetic centers are distributed over relaxation times. It is concluded that the observed kinetics are due to the presence of oxygen molecules, which act as a fast-relaxing impurity and accelerate the relaxation of the C ₆₀ ⁺ radicals. The results obtained offer an explanation for a number of features of C ₆₀ ⁺ relaxation in fullerites discovered earlier.     

Mixings and CP violations of theB^0 - \bar B^0 system in the four-generation model

We study the mixings and CP violations in the \(B^0 - \bar B^0 \) system together with the \(K^0 - \bar K^0 \) one in the four-generation model, taking into account the ARGUS data for the \(B_d^0 - \bar B_d^0 \) mixing. We take typical six cases of the mixing hierarchy and search for the allowed regions of three phases in the 4×4KM matrix. The CP violating parameter ? _K in the \(K^0 - \bar K^0 \) system gives a severe constraint for the phases, and the smaller mixing than that in the three-generation model is predicted for the \(B_s^0 - \bar B_s^0 \) system. The asymmetry parameters for the two-body non-leptonic decays of theB ⁰ and \(\bar B^0 \) mesons are also predicted.     

Thep - \bar p decays ofP-wave quarkonium and the helicity characteristics of massless QCD

We consider the exclusive \(p - \bar p\) decays of the quarkoniumP-states. Due to the helicity conservation of massless QCD the \(p - \bar p\) mode is forbidden in this limit for the¹ P ₁ and the³ P ₀ states. The angular distributions for the decays of the remaining states in the cascade \(^3 S\prime _1 \to \gamma ^3 P_J \to \gamma p\bar p\) are specific to QCD and can serve as a test of the theory. The same is true of the formation process \(p\bar p \to ^3 P_J \to ^3 S_1 \gamma \) . In lowest order QCD we obtain overall branching ratios for charmonium of the order of 10^?4.     

Calculation ofn^3 S_1 (Q\bar Q) \to \gamma + (pseudo)scalar

The decays of³ S ₁ quarkonia into a photon and a scalar or pseudoscalar Higgs particle are examined, taking into account the bound-state dynamics in the framework of a nonrelativistic potential model. We find that for realistic quark potentials the naive calculation [1] overestimates the scalar rate. Numerical results are obtained for the \(\bar bb\) and \(\bar tt\) quark systems.     

NMR in Magnetic Field of the Earth: Pre-Polarization of Nuclei with Alternating Magnetic Field

The polarization of nuclei in the low static magnetic field \(B_0\) with an alternating magnetic field \(B^{*} (B^{*} \gg B_0)\) at a very low frequency \(f_m\) (but \(f_m\gg 1\) / \({T_1}\) , where \(T_1\) is the spin-lattice relaxation time) has been investigated. The question of the optimization of the energy consumption during the pre-polarization is also considered. The possibilities of the method are illustrated by the observation of nuclear magnetic resonance signals from a few liquids.     

NMR and spin-lattice relaxation rate of89Y,63Cu in radiation disordered YBa2Cu3O6.9

NMR line shifts and spin-lattice relaxation rates of⁸⁹Y and⁶³Cu in YBa₂Cu₃O_6.9 were measured in disordered samples irradiated by fast neutrons with a fluence of: ?=5·10¹⁸ cm^?2 (T _c ^ons =70 K), ?=1.2·10¹⁹ cm^?2 (T _c ^ons =20 K), in order to investigate the evolution of spin susceptibility χ_S under irradiation. According to the data obtained, χ_S decreases markedly as structural disorder accumulates in the samples. The variation of χ_S is related closely to that observed in oxygen-depleted YBa₂Cu₃O_7?δ compounds with nearly the sameT _c value. The data for yttrium display some features that are absent in oxygen-depleted samples. The different temperature dependence of the⁸⁹Y and⁶³Cu Knight shifts and the increase of the⁸⁹Y spin-lattice relaxation rate in irradiated samples are discussed in terms of the electron localization effects arising in the CuO₂ planes due to the radiation-induced structural disorder.     

Pion photoproduction on197Au to ground and isomeric states in197Hg

The lifetime of the 331.3 keV 0 ₂ ⁺ state in¹⁰⁰Zr has been measured at the gas-filled recoil separator for fission products JOSEF. By observing the delayed coincidences between theβ-particles populating the level and theE0 conversion electrons from its decay into the ground state, a half-life of 3.37±0.30 ns has been obtained. From the measured lifetime and the relative intensities of the 0 ₂ ⁺ →0 ₁ ⁺ and 0 ₂ ⁺ →2 ₁ ⁺ transitions, values of 0.493±0.015 for theE0 strength parameterρ, and of 16 single particle units forB(E2,2 ₁ ⁺ → 0 ₂ ⁺ ) have been deduced. The enhanced nature of theE0 transitions suggests mixing of the 0 ₁ ⁺ and 0 ₂ ⁺ states which may be estimated by comparing the experimentalB(E2) values for the 2 ₁ ⁺ →0 ₁ ⁺ and 2 ₁ ⁺ →0 ₂ ⁺ transitions with the predictions of the asymmetric VMI model.     

Investigation of the two quasiparticle rotational band at 1172 keV in172Yb and determination of theg R -factor of the 3+ 3 band head

Investigations of the rotational band based on the 3⁺ 3 two quasiparticle state in¹⁷²Yb have shown that some of its properties can be well described by the collective model of Bohr and Mottelson. As a result of these investigations we have derived the ratio (g _k – g _R )/Q _o =? (0.0136 ± 0.0007). The magneticg-factor of the band head has also been determined by an integral angular correlation measurement perturbed by an external magnetic field. As a result we foundg=0.201 ± 0.030. Using this value and our result of (g _k – g _R )/Q _o we have calculated theg _R -factor of the two quasiparticle state asg _R =0.283 ± 0.018 which is out of the errors smaller than theg _R -factor of the ground state rotational band. An analysis of our angular correlation experiments gave for the mixing parameter δ of theK-forbidden 1094 keV intraband transition: δ=? (3.63 _?0.06 ^+0.14 ) in agreement with the results of other authors.     

Electron paramagnetic resonance and spinlattice relaxation of Cu2+ ions in ZnSeO4·6H2O

In this paper, we present detailed studies of the EPR spectra of Cu²⁺ ions in single crystals of ZnSeO₄·6H₂O. We describe the spectrum with a rhombic spin Hamiltonian with the following parameters: g_z=2.427; g_y=2.095; g_x=2.097; A _z ⁶⁵ =138.4·10^?4 cm^?1; A _x ⁶⁵ =22.3·10^?4 cm^?1. We studied spin-lattice relaxation in the temperature range 4–300 K at the frequency v≈9.3 GHz. The measured spin-lattice relaxation rate for the orientation H∥L₄ is described well at T<5 K by a linear dependence, while at T>5 K it is described by the sum of three exponentials: $$T_1^{ - 1} = 0.27T + 3.3 \cdot 10^{\text{s}} \exp \left( {\frac{{ - 69.5}}{T}} \right) + 2.6 \cdot 10^7 \exp \left( {\frac{{ - 140}}{T}} \right) + 1.36 \cdot 10^{10} \exp \left( {\frac{{ - 735.6}}{T}} \right){\text{ sec}}^{{\text{ - 1}}} $$ .We discuss possible reasons for the exponential dependence of T ₁ ^?1 for the Raman process.     

Some peculiarities of spin-lattice relaxation of impurity rare-earth ions in crystals caused by the structure defects

The spin-lattice relaxation times for Nd³⁺ ions in yttrium-aluminum garnets (YAG) and for Yb³⁺ ions in CaF₂ in the low-temperature range have been measured. For the first system the temperature dependence of the relaxation rate is determined to a great extent by the method of sample preparation. For samples grow by the method of the horizontally oriented crystallization the dependence is described asT ₁ ^?1 =AT ⁿ ,n ? 4.7, which is an evidence of an influence of local structure disordering on the relaxation. The temperature dependence of the relaxation rate in CaF₂:Yb is also “anomalous”:T ₁ ^?1 =AT ^3.3. The results are compared with the previous data on the relaxation in similar systems, and with other cases of observation of “anomalous” temperature dependences. Different manifestations of the local crystal defects in spin-lattice relaxation are discussed.     

Mass spectrum ofP-wave mesons

Mass splittings of mesons withL≧1 are discussed on the basis of a general spin-dependent potential consisting of a vector (V(r)) and a scalar (S(r)) part. For arbitraryV(r) andS(r), the four masses, for the three³ L _J and the one¹ L _J=L levels, are given in terms of only three unknown expectation values 〈(1/r)(dV/dr)〉, 〈d ² V/dr ²〉 and 〈(1/r)(dS/dr)〉. These expectations values are extracted for theP-wave \(u\bar s\) (or \(d\bar s\) ) mesons which are discussed in detail. It is argued that the 0⁺⁺ mass should be around 1150 to 1230 MeV, rather than at 1350 MeV. On comparing the expectation values for the \(u\bar s\) , \(c\bar c\) , \(b\bar b\) and the \(I = 1u\bar u\) systems, we find that they all scale asa+bμ, wherea andb are constants and μ is the reduced mass. Remarkably enough, we also find that theP-wave meson masses for these systems satisfy mass formulae of the formA+B(m₁+m₂), with constantA andB. It is shown that similar linear mass formulae also work forS-wave mesons. These facts seem to reveal a rather general property of \(q\bar q\) states.     

Optical detected ESR in the4 S 3/2 excited state of Er:YCl3

The electron spin resonance in the⁴ S _3/2 excited state of Er³⁺ in yttrium trichloride was studied by optical detection techniques. From angular dependence of the resonance field the principle value of theg-tensor in direction of the twofold crystal axis was deduced to beg∥=3.350±0.004 and the perpendicular valueg⊥ in the crystallographica-b-plane was extrapolated to beg⊥=2.857±0.004. The lifetime of the excited state is found to be temperature independent with τ _r =(1.62±0.02)·10^?3 sec and the spin lattice relaxation timeT ₁ was determined in the temperature region 1.5 to 2.1 °K by observing the recovery of the fluorescent light signal after a microwave saturation pulse was switched off.T ₁ is found to follow a direct process with \(T_1^{ - 1} = k \cdot cth\left( {\frac{{\rlap{--} h\omega }}{{2kT}}} \right)\) .     

Hyperfine interaction of Ce and La in 3-d ferromagnets

NMR/ON measurements on¹⁴¹CeFe show the sign of the hyperfine field of CeFe to be negative. For the¹⁴¹Ce nucleus a g-factor of ¦g_N¦=0.311±0.011 is found. With this g-value a hyperfine field of H_hf=?41±2 T for CeFe is derived. Low temperature nuclear orientation experiments on¹⁴¹CeCo and¹⁴⁰LaFe yield ¦H_hf¦=30±3 T and ¦H_hf¦=46±5 T respectively. The valence of cerium impurities in Fe, Co and Ni is discussed.     

Charm production in fixed target experiments

Prompt lepton production in proton beam dump experiments has been critically analysed within the general frame work of \(A_c \bar D\) and \(D\bar D\) production and their subsequent semileptonic decays. Realistic decay modes based on recent experiments are used. We have investigated the effect of using differentx dependences for the charm particles obtained either from simple quark counting rules or as inferred from strange particle production data. The \(D\bar D\) production is assumed to have a linearA dependence and for the \(A_c \bar D\) process bothA ¹ andA ^2/3 dependence is used. We show that by a simultaneous fit to the energy and angular distributions of prompt leptons in all the experiments the ratio of \(A_c \bar D\) to \(D\bar D\) production cross section can be determined. A comparison of this fit with these experimental distributions indicates that thex dependences based on strange particle data are strongly favoured. AnA ^2/3 dependence for \(A_c \bar D\) production, which corresponds to a quasi-diffractive process, is favoured although within existing errorsA ¹ dependence cannot be ruled out. Putting together the cross section results from our analysis with other results at similar energies (p _1ab ～400GeV/c) the production cross sections ( \(A_c \bar D\) ) and ( \(D\bar D\) ) are estimated to be ～25 and ～20 μb/nucleon respectively leading to a total inclusive charm cross section of ～90 μb/nucleon.     

The(cc) - (\overline {cc} ) (diquark-antidiquark) states ine + e − annihilation

The mass spectrum and decay modes of the \((cc) - (\overline {cc} )\) states are estimated in a quark-gluon model. We argue that the peculiar resonance-like structures ofR(e ⁺ e ^? →hadrons) for \(\sqrt s = 6 - 7\) GeV may be due to production of theP-wave \((cc) - (\overline {cc} )\) states. They are predicted to lie in the range 6.4–6.8 GeV and mainly decay into charmend mesons.     

N\bar N annihilation at rest into πππ andK\bar K\pi in the3 P 0 model and selection rules on the πρ,K\bar K* and\bar KK* production

\(N\bar N\) annihilation into three pseudoscalar mesons especially πππ and \(K\bar K\pi \) are studied in the quark pair creation model or the³ P ₀ model in which two \(q\bar q\) pairs are annihilated and two \(q\bar q\) pairs are created with quantum numbers of the vacuum or³ P ₀. The correlations of two pions to form ?,f ₂ and the resonance AX(1565) which is recently found by the ASTERIX group are taken into account. A proper treatment of the symmetry among the three pions in the final state shows that the \({}^{31}S_0 p\bar p\) annihilation into ?π is suppressed in agreement with the experiment. We calculate the cosθ distribution or the distribution of the Dalitz plot as the function of the angle between the direction of emission of one decay pion in the resonance centre of mass and the line of flight of the resonance. The interferences of π⁺ρ⁺, π^?ρ⁺ and π⁰ρ⁰ in the isospin 0 channels and π^±ρ^? and π⁰ f ₂ in the isospin 1 channel reproduce the peaks. The cos θ distribution for the P-wave \(p\bar p\) annihilation into πAX depends strongly on the size of the pion since the amplitude interfers with the π^±ρ^? amplitude which is sensitive to the size of the pion. The same model qualitatively explains the \(p\bar p\) annihilation into \(K\bar K\pi \) in whichK or \(\bar K\) and π are correlated to formK* \(\bar K\) or \(\bar K\) *K final states. We can qualitatively reproduce different patterns of the cos θ distribution for theK ^*+ andK ^*0.     

Gyromagnetic ratio of the 2+ rotational state of184W and observation of a large hyperfine anomaly with respect to183Wg in iron

Theg-factor of the 2⁺ rotational state of¹⁸⁴W was redetermined by an IPAC measurement in an external magnetic field of 9.45 (5)T as: $$g_{2^ + } (^{184} W) = + 0.289(7).$$ In the evaluation the remeasured half-life of the 2⁺ state: $$T_{{1 \mathord{\left/ {\vphantom {1 2}} \right. \kern-\nulldelimiterspace} 2}} (2^ + ) = 1.251(12)ns$$ was used. TDPAC-measurements with a sample of carrierfree¹⁸⁴Re in high purity iron gave the hyperfine fields: $$B_{300 K}^{hf} (^{184} W_2 + \underline {Fe} ) = 70.1(21)T$$ and $$B_{40 K}^{hf} (^{184} W_{2^ + } \underline {Fe} ) = 71.8(22)T.$$ A comparison with the hyperfine field known from a spin echo experiment with¹⁸³W _g Fe leads to the hyperfine anomaly: $$^{184} W_{2^ + } \Delta ^{183} W_g = + 0.145(36).$$ The hyperfine splitting observed in a Mössbauer source experiment with another sample of carrierfree^184m Re in high purity iron indicates that the smaller splitting, measured previously by a Mössbauer absorber experiment is due to the high tungsten concentration in the absorber. The new value for theg-factor of the 2⁺ state together with the result of the Mössbauer experiment allow an improved calibration for our recent investigation of theg _R -factors of the 4⁺ and 6⁺ rotational states. The recalculated values are: $$g_{4^ + } (^{184} W) = + 0.293(23)$$ and $$g_{6^ + } (^{184} W) = + 0.299(43).$$ The remeasured 792-111 keVγ-γ angular correlation $$W(\Theta ) = 1 - 0.034(4) \cdot P_2 + 0.325(6) \cdot P_4 $$ gives for the mixing ratio of theK-forbidden 792keV transition: $$\delta ({{E2} \mathord{\left/ {\vphantom {{E2} {M1}}} \right. \kern-\nulldelimiterspace} {M1}}) = - \left( {17.6\begin{array}{*{20}c} { + 1.8} \\ { - 1.5} \\ \end{array} } \right).$$ A detailed investigation of the attenuation ofγ-γ angular correlations in liquid sources of¹⁸⁴Re and^184m Re revealed the reason for erroneous results of early measurements of the 2⁺ g _R -factor: The time dependence of the perturbation is not of a simple exponential type. It contains an unresolved strong fast component.     

p¯p Annihilation into two mesons in the quark rearrangement model and the quark annihilation model

The relativistic³ P ₀ model is applied to the \(p\bar p\) annihilation into twoS-wave mesons. We calculate the branching ratios of the \(p\bar p\) annihilation at rest into two mesons in the quark rearrangement model and in the quark annihilation model. In the annihilation model, we project the intermediate \(cq\bar q\) state to eigenstates ofSU (4) with the relative angular momentum of \(cq\bar q\) equals orp. In the rearrangement model, no annihilation occurs from theS-wave \(p\bar p\) and certain branching ratios conflict with the experimental data. Detailed comparison with the experiment needs inclusion ofP-wave mesons in the final state, nevertheless we find that the annihilation model gives qualitatively better results than the rearrangement model. The effect of initial state interaction through \(N\bar \Delta \pm \Delta \bar {\rm N}\) or \(\Delta \bar \Delta \) channels is discussed.     

K-conversion coefficient of the 53.3 keV transition and\frac{K}{{L + M}}-ratio of the 13.34 keV transition in73Ge

TheK-conversion coefficient of the 53.3 keV transition in⁷³Ge was measured by coincidence techniques to be αk ₁=7.1 ± 0.6 indicating very good agreement with heory forM2-radiation. The \(\frac{K}{{L + M}}\) -ratio of the 13.34 keV transition to the ground state was determined using the same techniques. The resulting value \(\left( {\frac{K}{{L + M}}} \right)_2 \) =0.36 ± 0.03 supports theE2-character of this radiation and therefore a spin assignment of \(\frac{5}{2}\) for the 13.34 keV level. The measured lifetime of this transition (T _1,2=(2.95 ± 0.05) μsec) corresponds to a factor of 15 greater than the Weisskopf estimation for a pureE2-transition. A short discussion of a possible transfer of the collectivity of the⁷²Ge-nucleus to the⁷³Ge-nucleus is given.     

Spin-lattice relaxation of protons and deuterons in NH4NO3 and ND4NO3

The spin-lattice relaxation timesT ₁ were measured for protons and deuterons in polycrystalline NH₄NO₃ and ND₄NO₃. The investigation was carried out at temperatures between about 80°K and 430°K using the NMR pulse method. From the measured values ofT ₁ the activation energies for the reorientation motions of NH ₄ ⁺ and ND ₄ ⁺ ions below 200°K were calculated to be 2.07±0.11 kcal/mole and 2.56±0.23 kcal/mole, respectively. The quadrupole coupling constante ² Qq/h of the deuteron in ND ₄ ⁺ ion was found to be 194±30 kc/s.